Gammaübergänge und Energieniveaus in Dy 165

220 neutron capture Gamma rays of Dy 165 were measured with the Risø curved crystal spectrometer. The intense transitions permitted the construction of a level scheme for this oddN nucleus. The rotational bandsK=7/2⁺[633],K=1/2^?[521] andK=5/2^?[512] were precisely localized, including the spin 11/2 states. Gammavibrational bands built on these Nilsson orbits were observed with their band heads at 538.6, 573.5 and 570.2 keV. TheI=5/2 term at 533 keV can be considered as the 5/2^?[523] Nilsson state. The branching ratios allowed the determination of (g _K?g^R)²-factors for the [633], [521] and [512] bands and yieldedE 1-hindrance factors.     

In-beamγ-ray spectroscopy of the neutron deficient100Ag

The neutron deficient nucleus¹⁰⁰Ag, three proton holes below and three neutron particles above the N=Z=50 shell closure at¹⁰⁰Sn, has been identified and studied by in-beam spectroscopy. The reactions⁴⁶Ti(⁵⁸Ni,3pn) at 231 MeV and⁶⁴Zn(⁴⁰Ca,3pn) at 167 MeV of the respective⁵⁸Ni and⁴⁰Ca beams were used, and states up to 8.7 MeV excitation energy and spin I?20 were found in two mainγ-ray cascades forming band-like structures of even and odd parity. Large scale shell model calculations suggest predominantπg ₉ ^2/?3 ν(d_5/2,g_7/2)³ andπg ₉ ^2/?3 ν(d_5/2,g_7/2)²h_11/2 structures with maximum spins I ^π = 19⁺ and I ^π =22^?, respectively, for the two level sequences. The influence ofπp_1/2 vs.νh_11/2 excitations is discussed for low lying odd-parity levels.     

EPR study of Fe3+ and Mn2+ in CeO2 and ThO2

Attempts were made to grow CeO₂ and ThO₂ single crystals doped with transition metal ions. Only Fe³⁺ and Mn²⁺ could be detected by the EPR technique. The EPR spectrum of Fe³⁺ in CeO₂ exhibits the well-known fine structure in cubic fields. The parameters areg=2.0044(1) anda=15.6(1)·10^?4 cm^?1. The hyperfine constantA for⁵⁷Fe in hexahedral coordination was found to be 8.9(1)·10^?4 cm^?1. The EPR spectrum of Mn²⁺ in CeO₂ reveals two cubic Mn²⁺ centers. The parameters for center 1 areg=1.9999(1) andA=86.9(1)·10^?4 cm^?1 and for center 2g=1.9984(1) andA=87.0(1)·10^?4 cm^?1. Heating the Mn doped CeO₂ samples in hydrogen, the Mn²⁺ centers transform from cubic into trigonal centers with approximate values ofg=1.9988(2),A=84.5(6)·10^?4 cm^?1 andD=203(1)·10^?4 cm^?1. The two observed Mn²⁺ centers in ThO₂ exhibita priori axial symmetry with approximate values ofg=2.0006(2),A=88.9(4)·10^?4 cm^?1 andD=33(3)·10^?4 cm^?1.     

Magnetic moment of the 5/2−1/2[541] ground state of 14h 185Ir

The magnetic and electric hyperfine splitting frequencies ¦gμ _N B _HF/h¦ ande ² qQ/h of the 5/2^?1/2[541] ground state of 14h ¹⁸⁵Ir in Ni were measured with nuclear magnetic resonance on oriented nuclei to be 360.8(7) MHz and +6.7(2.0) MHz, respectively. The ground state magnetic dipole moment and electric quadrupole moment of¹⁸⁵Ir are deduced to be ¦μ¦=2.601 (14)μ _N andQ=?1.9(5)b, taking values for the hyperfine field and electric field gradient of B_HF=?454.9 (2.3) kG and eq=?0.151(4) × 10¹⁷ V/cm², respectively. The negative quadrupole moment is in agreement with nuclear-orientation data and proves again theI ^π K=5/2^? 1/2 ground state configuration.     

High-spin levels in138Ce and140Nd Observed in the (α, 4n γ) reactions

Levels of¹³⁸Ce and¹⁴⁰Nd have been studied using the¹³⁸Ba(α,4nγ)¹³⁸Ce and¹⁴⁰Ce(α, 4nγ)¹⁴⁰Nd reactions. Singleγ-ray spectra,γ-γ coincidence spectra, angular and time distributions with respect to the beam bursts have been measured. A number of higher excited states with excitation energies up to about 5 MeV and with spin value up to 12 are populated in both nuclei. The lower states with spins and parities 7^?, 5^?, 6^? and 10⁺ can be explained by two-quasiparticle neutron configurations of the types (h _11/2 ^?1 ,d _3/2 ^?1 ) 7^? , (h _11/2 ^?1 ,S _1/2 ^?1 ) 5^?, 6^? and (h _11/2 ^?2 ) 10⁺. Several high-spin states observed in¹³⁸Ce and¹⁴⁰Nd can be explained qualitatively as four-quasiparticle states with two-proton-two-neutron configurations. The 3^? state at an energy of 2,137.4 keV is observed in¹³⁸Ce. The evidence for the existence of the low-lying 3^? states in¹⁴⁰Nd at 2,124.0 keV is discussed. Beside the known 9.6 ms (7^?) isomeric state in¹³⁸Ce another state at 3,538.5keV (10⁺) with a half life of about 200 ns has been observed. The observed levels in the¹³⁸Ce and¹⁴⁰Nd nuclei are compared with theoretical predictions using delta force interaction.     

Gamma spectroscopic study of105Ru

Theγ radiation following thermal neutron capture in¹⁰⁴Ru has been investigated through singles, coincidence, and angular correlation measurements in order to solve existing discrepancies and to complete the knowledge about the transitional odd-N nucleus ₄₄ ¹⁰⁵ Ru₆₁. The resulting level andγ-decay scheme is found to be very similar to that of the odd-Z transitional nucleus ₆₁ ¹⁴⁹ Pm₈₈. Between the 11/2^?, 15/2^?, and 19/2^? states which are interpreted as members of the decoupled band, built on the unique parity 11/2^? single particle state, low spin states of negative parity are found at surprisingly low excitation energies above the 11/2^? state. In the frame of the particleplus-rotor model their positions would require a sharp decrease of the rotational parameter with increasing collective angular momentum of the soft core.     

High-resolution optogalvanic study of the c4(0)1Πu, c′5(0)1Σu+, and a″(0)1Σg+ Rydberg states of N2

A new optogalvanic technique with an rf discharge was applied to a high-resolution study of the Rydberg states of N₂. The Ledbetter band, c₄(0)¹Π_u ← a″(0)¹Σ_g⁺, and a new visible band, c′₅(0)¹Σ_u⁺ ← a″(0)¹Σ_g⁺, were studied at a Doppler-limited resolution of 0.05 cm^?1. A Doppler-free method was also applied to resolve overlapped lines. Precise wavenumbers were determined for the rotational transitions of the two Rydberg bands. The rotational and the centrifugal constants for the lowest Rydberg state, a″(0)¹Σ_g⁺, were determined to be B₀ = 1.913748(42) cm^?1 and D₀ = 6.088(99) × 10^?6 cm^?1, where the numbers in parentheses are the standard deviation and apply to the last digits.     

The gyromagnetic ratio of the 589 keV 3/2− state of117In

Theg-factor of the 589 keV state of¹¹⁷In has been determined by a measurement of the rotation of the 1,303–273 keVγ —γ directional correlation in an external magnetic field of 9.55(1) T. The result,g _3/2(589 keV)=+0.068(39), contradicts the usual interpretation of the state as the 2p _3/2 single proton hole configuration for which the Schmidt value isg _3/2-(Schmidt)=+2.53. It favours the interpretation as the first rotational state built up on the single proton [301] 1/2^? Nilsson orbit in a strongly deformed core of prolate shape.     

The low-lying states and configurations in138La

Tritons from the reaction¹³⁹La(d, t)¹³⁸La atE _d=16 MeV were analyzed at eleven reaction angles from 22 ° to 90 ° with a broad-range magnetic spectrograph. TheQ-value of the reaction is ?2522±5 keV. The nine lowest-lying states in¹³⁸La are interpreted in terms of the shell model configurations (πg _7/2)^?1 (vd _3/2)^?1, (πg _7/2)^?1 (vs _1/2)^?1 and (πg _7/2)^?2 (πd _5/2)^?1(vd _3/2)^?1. Seven levels in the energy range of 700–1300 keV are populated byl=5 transitions and are interpreted as coming from the (πg _7/2)^?1(vh _11/2)^?1 configuration. The ground state of¹³⁸La is shown to haveJ ^π=5⁺. Therefore, beta decay by unique second-forbidden transitions to the 2⁺ one-phonon states of¹³⁸Ce and¹³⁸Ba must be inferred in spite of unusually high logft values of 19.2 and 18.5, respectively.     

Spectroscopy of molecular ions: Laser induced predissociation of O 2 +

The technique of laser induced predissociation and laser induced fluorescence is applied to study spectra of gas-phase molecular ions. The main feature of the experiment is a beam of mass selected molecular ions illuminated by a pulsed dye laser. Over an extended range of excitation energies spectroscopic information can be obtained about positive and negative ions including transient species. As a first result we present predissociation spectra of O ₂ ⁺ ,b ⁴ bE _g ^? ?a ⁴ π _u Δv=3 andgDv=2 which can well be simulated by calculated spectra assuming a rotational ion temperature of 300δK.     

Non-collective oblate states in119Te

High spin states of¹¹⁹Te, populated in¹¹⁰Pd(¹³C, 4n) and¹¹⁰Pd(¹²C, 3n) reactions, have been studied throughγ-ray spectroscopy. The level scheme has been established up to j^π=(55/2^?). Three-quasiparticle states, based onπg ₇ ^2/2 ?vh _11/2 andπg _7/2 d _5/2?vh _11/2 configurations, have been identified. A particularly favoured 39/2^? state is suggested to be the fully aligned [πg ₇ ^2/2 ]₆₊?[vh ₁₁ ^2/3 ]_27/2? yrast non-collective oblate configuration. This assignment is supported by Total Routhian Surface (TRS) calculations which also suggest a similar oblate assignment to states at 21/2^?, 23/2^? and 37/2^?.     

A new high-spin isomer in 39 97 Y58

An isomeric state at 3,523 keV excitation energy in⁹⁷Y with a half-life of 144(10) ms has been discovered with the fission-product separator JOSEF. This isomer is depopulated through aγ transition of 162 keV. AnE3 multipolarity for this transition is consistent with the measured conversion coefficients ofα _K =0.98(20) andα _T =1.00(19). Subsequent electromagnetic transitions populate several new⁹⁷Y levels which have high spins. For the isomer the three-quasiparticle configuration [πg _9/2?ν(h _11/2,g _7/2)]27/2^? is proposed. TheE3 transition with a strength about 2 single-particle units is supposed to be of the typeh ₁₁ ^2/+1 →d ₅ ^2/?1 . These findings provide evidence for the rapid shape transition atA?100 since they indicate shell-model character of ₃₉ ⁹⁷ Y₅₈ even at high excitation energies while the immediate neighbour ₃₉ ⁹⁸ Y₅₉ contains a rotational band based on a level at 495 keV.     

Fragmented 2d 5/2, 1g 7/2 and 1g 9/2 deep proton-hole states of207TI

The three proton-hole states ?2d_5/2, 1g_7/2 and 1g_9/2 are found to be fragmented as a result of coupling of these states with the 3^?, 5^?, 2⁺, 4⁺ and 6⁺ collective states of²⁰⁸Pb. The excited states in²⁰⁸Pb (t,α) reaction can be quantitatively explained in terms of altered 2d_5/2, 1g_7/2 and 1g_9/2 states with the hole-core coupling model.     

Electron-lattice interaction of Ag− and Cu− centers in alkali halides

Absorption, emission, and excitation spectra of Ag^? centers in KCl, RbCl, CsCl, and CsBr are measured at low temperatures. The positions of theA emission bands are slightly different afterC andA band excitation, respectively. This is believed to be due to the existence of two different types of minima in the adiabatic potential energy surface of the³ T _1u state. The symmetry of the energy minima in the¹ T _1u state is trigonal for KCl∶Ag^? and Cu^?, but tetragonal for CsBr∶Ag^?. This becomes evident from the polarization properties of the emission. The energy and temperature dependence of the polarization is discussed. Uniaxial stress causes polarized emission of Ag^? and Cu^? centers measured from LHeT to 100 K. This is due to a splitting and mixing of the relaxed excited states by the stress. The effects are used to calculate the coupling constants between thep electron and theE _g andT _2g lattice modes. They are compared with predictions from the point-charge model for different lattice structures. A new assignment of the absorption bands of KCl∶Cu^? to the excited states of Cu^? is established on measurements of emission spectra and lifetimes.     

Measurements of hyperon semileptonic decays at the CERN Super Proton Synchrotron

The charged hyperon beam at the CERN Super Proton Synchrotron (SPS) has been used to collect data on semileptonic decays ofΣ ^?,Ξ ^? andΛ. A magnetic channel selects 100 GeV/c negatively charged particles produced in the forward direction by interaction of the 200 GeV/c SPS proton beam on a BeO target. TheΣ ^? andΞ ^? hyperons are concurrently identified in a DISC ?erenkov counter, and their decay products are analysed by a magnetic spectrometer. Electron-hadron discrimination is achieved by the combined use of lead-glass and lead/scintillator counters, transition radiation detectors, and a ?erenkov counter. In this article we report results on the \(\Sigma ^ - \to \Lambda e^ - \bar v\) decay mode. Measurements of the Λ polarization and of the centre-of-mass distributions (baryon kinetic energy, electron-neutrino correlation, and Dalitz plot distributions) yield the vector to axialvector form factor ratiof ₁/g ₁=+0.034±0.080, in agreement with the value expected from the conserved vector current hypothesis (f ₁/g ₁=0). TheΣ ^?→Λe ^? v→ branching ratio measurement gives a value of (5.41±0.30)×10^?5. The effects of radiative corrections are not included in these results. They are discussed in the text. Results on the otherΞ ^?,Σ ^?, andΛ semileptonic decays are reported in separate articles.     

g-Faktoren und Multipol-Mischungsverhältnisse in156Gd

By integral perturbedγ-γ-angular correlation the gyromagnetic ratios of a 2-quasi-particle state at 1,513 keV and the 4⁺ state of the ground state rotational band in¹⁵⁶Gd were measured, using sources prepared by¹⁵⁹Tb(γ, 3n) and¹⁵⁶Gd(d, 2n) reactions:g _{1;513 keV} ⁴⁺ =0.78±0.05;g _R ⁴⁺ =0.37±0.05. In addition we obtain the multipole mixing ratiosδ _{535 keV}(M2/E1)=?0.09±0.01;δ _{1,225 keV}(E2/M1)=+1.83±0.10 for the 535 keV and 1,225 keVγ-rays. The classification of the 1,513 keV state is discussed. The internal field of Gd in Tb metal at 77 °K was found to beH=(?192±16)kOe.     

Excited-state photoelectron spectra of the one-photon forbidden C3IIg rydberg state of molecular oxygen

The Rydberg C³II_g, state of molecular oxygen, which is one-photon forbidden from the ground electronic state, has been studied by means of (2 + 1) multiphoton ionization (MPI) ion-current and photoelectron spectroscopic techniques in the laser wavelength region 287–289 nm. Excitedstate photoelectron spectra have been observed at different rotational levels of the C³Π_gv' = 2 state of O₂, and show marked deviation from the Franck-Condon distribution generally expected in ionization of Rydberg electrons. Namely, in addition to main photoelectron peaks due to Δv = 0 transitions, other vibrational peaks are also observed with considerable intensities. The v⁺= 2 photoelectron peak shows different angular dependence from the other vibrational peaks. The rotational structure in the MPI ion-current spectrum of O₂ is well interpreted in terms of the rotational constants of the X²Π_g ground electronic state of O₂⁺.     

The magnetic moment of the lowest 3/2− state in57Co

The reaction⁵⁴Fe(α, n)⁵⁷Ni has been used to implant⁵⁷Co isotopes in ferromagnetic iron. Theg-factor of the lowest 3/2^? state is determined using the internal field in a constant angle reversed field method. The angular correlation of the 127–1,378 keV cascade is also measured. The result of the angular correlation measurement together with reaction data is consistent withp _3/2 andp _1/2 single particle assignments to the lowest 3/2^? resp. 1/2^? state. In view of this statement the quenching of the magnetic moment is discussed.     

Particle × phonon multiplets in 65 147 Tb82

High-spin states of¹¹⁵Sb were studied by inbeamγ-ray spectroscopy using the⁸⁹Y (²⁹Si, 2pn) fusionevaporation reaction at a beam energy of 108 MeV. The experiments includedγ-γ coincidence and directional correlation of oriented nuclei (DCO) ratio measurements using six BGO Compton suppressed Ge detectors. An intruderΔJ=2 rotational band has been identified for the first time and it is interpreted as the h_11/2 proton coupled to a two particle-two hole (2p ? 2h) deformed state of the¹¹⁴Sn core. A ΔJ=1 rotational band based on the 2p ? 1h, π{g ₇ ^2/2 ?g ₉ ^2/?1 }, configuration has been extended to the 29/2⁺ state at an excitation energy of 5241 keV.     

The magnetic moments and halflives of the 5/2− states in199Hg and197Hg and the discrepancies in the experimental hyperfine fields at Hg in Fe

The Larmor-precession frequencies for¹⁹⁷Hg in Fe have been determined to beω _L = 1291 ±25 MHz at 293 K andω _L = 1334±25 MHz at 105 K. For¹⁹⁹Hg in Feω _L =1372±50 MHz has been measured at 293 K. The half-lives of the 5/2^? states in¹⁹⁷Hg and¹⁹⁹Hg have been remeasured asT _1/2(¹⁹⁷Hg)=8.1±0.16 nsec andT _1/2(¹⁹⁹Hg)=2.45±0.05 ns, respectively. The magnetic moment of the 5/2^? 158keV state in¹⁹⁹Hg was redetermined by the integral perturbed angular correlation method in an external magnetic field of 47kG asμ(5/2 ^? ) = 0.905±0.091 nm. With this new value consistency for the magnetic hyperfine fields at Hg in Fe measured with the TDPAC-method and with the NMR/ON-method is obtained. This fact is used to determine theg-factors of the 5/2^? states in¹⁹⁷Hg and¹⁹⁹Hg more precisely fromω _L -values given above:g(¹⁹⁷Hg)=0.342(6);g(¹⁹⁹Hg)=0.352(13). The magnetic moments of the first excited 2⁺ states in^198–204Hg isotopes which rely on calibrations with the¹⁹⁹Hg-g-factor, are revised.