Experimentelle Untersuchungen am Elektroneneinfang des Mangan 54 und Zink 65

The electron capture decay of Mn 54 and Zn 65 was investigated using Na I(Tl)-detectors. Spectroscopic-coincidence techniques were employed to examine theK-electron capture rates of Mn 54 and Zn 65, the branching ratio and positron rate of Zn 65. The experimental results are:P _k ω _k (Mn)=0.2492±0.0017,P _k ω _k (Zn)=0.3927±0.0026,EC ^* /EC ⁰(Zn)=53.2±1.0/46.8±1.0,γ/β ⁺=35.1±1.7,K ⁰/β ⁺=27.7±1.5. Thus electron capture to the excited state of Cu 65 occurs to the extent of 52.4±1.0% while electron capture and positron decay to the ground state were found to be associated with 46.1±1.0% and 1.49±0.05% of the disintegrations. These data partly disagree significantly from measurements of other authors. Using the fluorescence yieldsω _k (Cr)=0.279 andω _k (Cu)=0.4425, deduced from other measurements, values ofL+M/K of electron capture to the excited state could be derived:L+M/K(Mn 54)=0.120±0.015 andL+M/K(Zn 65)=0.127±0.015. These ratios agree with the calculations ofBahcall. The half-lives of Mn 54 and Zn 65 have been determined to beT _1/2(Mn 54)=312±5d,T _1/2(Zn 65)=243±4d The energy of the Zn 65-γ-rays was measured with a Ge(Li)-counter:E ^γ=1115.5±0.5 keV.     

Experimentelle Untersuchungen am Elektroneneinfang des85Strontium und88Yttrium

The electron capture decay of⁸⁵Sr and⁵⁵Y has been investigated using NaI(Tl)-detectors. Spectroscopic-coincidence techniques have been employed to examine theK-electron capture rates. The experimental results areP _K ω _K (Sr)=.5959 ± 0.0035 andP _K ω _K (Y)=0.6340± 0.0032. Using theK-capture probabilities, derived from the capture ratios ofBrysk andRose with the exchange correction ofBahcall:P _K (Sr)=0.880± 0.008 andP _K (Y)=0.883 ± 0.008, one can derive from these results the fluorescence yieldsω _K (Rb)=0.677± 0.009 andω _K (Sr)=0.712± 0.010. Functions ofω _K (Z) were fitted to recent experimental data and tabulated forZ=5–90. In addition to these results the half life of the 514 keV state of⁸⁵Rb and the branching ratios and the positron rate of the⁸⁸Y-decay have been measured with the same techniques. The data obtained partly disagree from measurements of other authors.     

K-capture probabilities in the electron capture decay of159Dy

TheK-electron capture probabilities (P _k) for the 58 keV state and the ground state of¹⁵⁹Tb in the decay of¹⁵⁹Dy have been determined. The measured values,P _k ⁵⁸ =0.81±0.05 andP _k ⁰ =0.79±0.06 are found to be in excellent agreement with theoretical results.     

DieK-Fluoreszenzausbeute von Titan und der Zerfall des48Vanadium

TheK-fluorescence yieldΩ _K of Titanium has been measured using the coincidence method and investigating the electron capture decay of⁴⁸V. The detectors used have been a Si(Li)- and a Ge(Li)-detector for the X- andγ-rays. The experimental results areP _K Ω _K =0.2005 ±0.0030 andΩ _K (Ti)=0.224±0.003 usingP _K =0.896. For the branching ratios of the decay of⁴⁸V we obtainedEC (3.239) 7.9±0.6%EC (3.224) 2.9±0.4%EC (2.295) 35.6±2.0% Β⁺ (2.295) 52±1.0% all others 1.6%. Additionally someγ-ray-energies of the decay of⁴⁸V and the half-life,T _{1 2}=(16.23 ±0.03)d, have been measured.     

Anomalous conversion of 127 keV (E3) transition in134Cs

The total conversion coefficient of the 127.49 keV E3 isomeric transition in the decay of^134mCs was measured using the gamma intensity balance method with the help of a high resolution low energy photon detector. Theα _Tvalue was found to be 5.84±0.47 as against the theoretical value of 6.96, thus showing an anomaly of (16.1±6.7)%. TheK-conversion coefficient,α _kwas also measured using the X-ray peak to gamma ray intensity method and found to be 2.24±0.04 as against the theoretical value of 2.72, which shows an anomaly of (17.6±1.4)% consistent with the experimental anomaly inα _T. TheE3 hindrance factor of the isomeric transition was estimated to be (3.44±0.23) ·10⁴.     

The determination by an independent method ofP k electron capture probabilities in133Ba and139Ce decays gamma decay of133Ba

The electron capture decays of¹³³Ba (10.4 y) and¹³⁹Ce (140 d) were investigated with high resolution Ge(Li) detectors. By x-ray — γ-ray coincidences values of the quantityP _k ω _k ? _k for various transitions in the decay of¹³³Ba and¹³⁹Ce are obtained. The factor ω _k ? _k was measured independently by means ofK-conversion electron-K x-ray coincidences and was then used to determineP _k , theK-capture probability. The independent measurement of the product ω _k ? _k , together with recent accurate values of ω _k , provides a new method for the accurate calibration of semiconductor x-ray detectors. In the decay of¹³⁹Ce, a value ofP _k =0.78±0.03 is found (where the error represents twice the standard deviation) from whichQ _ec =326 _?30 ⁺⁷⁰ keV to the¹³⁹La ground-state is found by use of theory. In¹³³Ba decay, values are found ofP _k 1=0.72±0.04 for theEC transition to the 437 keV level in¹³³Cs,P _k 2=0.80±0.07 to the 384 keV level, and from an independent measurement, the ratioP _k 1/P _k 2=0.87±0.07. From these results the ground-state value ofQ _ec =522 _?10 ⁺²⁰ keV is derived from theory for¹³³Ba decay. The gamma spectrum of¹³³Ba also was remeasured. From the present gamma intensities and previous conversion electron intensities, new values forK-shell conversion coefficients are obtained. Previously reported γ-rays at 35 and 391 keV are not confirmed.     

The electron capture decay of125I and145Pm

The productP _K ω _K of theK-capture probability and theK-fluorescence yieldω _K was measured in the EC decay of 17.7 y¹⁴⁵Pm and 60.14d¹²⁵I by means ofK x-ray-γ-ray coincidences with semiconductor detectors. Accepting a best value ofω _K =0.920 forZ=60 from the literature, values ofP _K =0.606±0.025 and 0.554±0.025 for decay of¹⁴⁵Pm to the 67.2 and 72.4 keV levels in¹⁴⁵Nd, respectively, were determined, from which the application of EC theory givesQ _EC=153±4 keV to the ground state. TheP _K ω _K ratio to the 67.2 and 72.4 keV levels also was determined independently to be 1.11±0.01, which serves as a good check on theγ-ray-gatedP _K values. Theγ-ray energies were determined more accurately to be 72.4±0.1 and 67.2±0.1 keV, together with a ratio of their relative intensities,I _72.4/I _67.2=3.35±0.09. In the decay of¹²⁵I, a value ofP _K ω _K =0.699±0.030 was measured, and by using an independent determination ofQ _EC=178±2 keV to the ground-state from the literature, a value ofP _K=0.801 is calculated from allowed EC theory, from whichω _K =0.873±0.017 atZ=52 is obtained. This value is in good agreement with theoretical values and with a value of 0.875±0.028 predicted by the best fit curve of Bambyneket al.     

Revision of the109Cd decay data

Combining measurement with the use of a Si(Li) detector and a windowless 4π NaI(T1) detector a new value ofω _K(Ag) equal to 0.84±0.02 has been determined. From the measured ratio of the KX-ray and conversion electron emission rates the relative K-capture probabilityP _K=0.77±0.015 was calculated. Through analysis of data reported in literature and taking into account the new value ofP _K andω _K and the results of the international comparison of absolute activity measurements of¹⁰⁹Cd, the following decay data were chosen for the calculation of yields:ω _K=0.836±0.007;α _T=26.4±0.3; α_K=11.4±0.3; P_K=0.78±0.015. The number of gamma photons per disintegration (gamma-yield) was then determined equal to 0.0365±0.0004; the KX-yield equal to 0.997±0.008; the conversion electrons yield equal to 0.9635±0.0005 and the KX/γ ratio equal to 27.3±0.6.     

K-Ionization probability across the 460-keV12C(p,p 0) resonance

We have remeasured theK-shell vacancy production probabilityP _K across the 460-keV¹²C(p, p ₀) resonance, previously investigated by Duinker et al. We are unable to confirm the large (～70 %) variation ofP _K across the resonance, found by Duinker et al. for protons elastically scattered at 125°. Our values for the ratioP _K (142°)/P _K (16°) are independent (within±20%) of the proton bombarding energy over the resonance region, in agreement with theoretical predictions by Blair and Anholt, Feagin and Kocbach, McVoy and Weidenmüller. Our average value for this ratio, equal to 0.88 ±0.06, agrees with the value 0.88 calculated by Amundsen and Aashamar.     

Disparity in transient field characteristics for Au ions traversing Fe and Gd hosts through measurements ofg-factors in197Au

Transient field precessions were measured for levels in the nuclides of^182,184,186W and¹⁹⁷Au as their ions simultaneously traversed polarized Fe and Gd hosts. Consistent sets of gyromagnetic ratios were inferred for the lowest 5/2⁺ and 7/2⁺ states in¹⁹⁷Au using these two ferromagnetic host media, provided that (i) the transient field for Au ions in Gd is calibrated using the W in Gd precessions (simultaneously measured) and, (ii) the transient field for Au in Fe is calibrated using the field strength and velocity dependence for Pt in Fe (previously measured). The presentg-factor results are: g(5/2 ₁ ⁺ ;¹⁹⁷Au)=0.296±0.023, g(7/2 ₁ ⁺ ;¹⁹⁷Au)=0.241±0.021, and g(5/2 ₁ ⁺ ;¹⁹⁷Au)=1.2±0.2.     

Verzweigungsverhältnisse und Konversionskoeffizienten von angeregten Zuständen des208Tl

The branching ratios of theγ rays of the second and fourth excited states of²⁰⁸Tl have been investigated by coincidence measurements between the α rays of²¹²Bi and subsequent 40keVγ ray. The detectors employed were a silicon surface barrier counter for α particles, and a 1.5 in ×2 mm NaJ (Tl) crystal forγ rays. It has been found that (75.6±3.7)% of all transitions of the 328 keV state and (94±7)% of all transitions of the (492 keV+473 keV) states populate the first excited state of²⁰⁸Tl. The 40 keV state is excited to (3.4±0.3)% by transitions of higher excited states relative to the direct excitation by α particles. The number of α particles with energyE _α = 6.047 MeV and the number of subsequent 40keVγ rays resulted in a conversion coefficient α(40keV)=22.55± 0.46. Similarly coincidence measurements between Tl-x rays and α particles have been used to determine theK- conversion coefficients α_K(328 keV)=0.31±0.03 and α_K(492 keV+ 473keV)=0.100±0.015. The experimental results are in good agreement with the theoretical values ofSliv.     

Electron capture intensities in the decay of133Ba

The ground state decay of¹³³Ba was investigated using NaI(Tl) scintillation crystals.P _L/P_K electron capture ratios were measured for the transitions to the 437 keV and to the 384 keV level of¹³³Cs. The results are: (P _L/P_K)₄₃₇=0.371±0.007 and (PP _L/P_K)₃₈₄=0.221±0.005. From these data a mass difference between the ground states of the¹³³Ba- and the¹³³Cs-atom of (515±3) keV was derived. Besides, these capture ratios yield an exchange correction of 1.03±0.03. Furthermore, the intensity of the transition to the 161 keV level was determined to be smaller than 0.5% of all decays.     

X-ray spectroscopy in the EC nucleus

The probabilities P_KK of double K-shell vacancy production per K electron capture decay and per K internal conversion of ¹⁰⁹Cd and ²⁰⁷Bi have been determined by means of the double- and triple-coincidence experiments using Kα X-ray and K internal conversion. For ¹⁰⁹Cd we find P_KK(EC) = (4.2 ± 0.5) × 10⁻⁵ and P_KK(IC) = (4.32 ± 0.46) × 10⁻⁵, and for ²⁰⁷Bi, P_KK(EC) = (2.54 ± 0.50) × 10⁻⁵. The observed X-ray energy shifts of the hypersatellite Ag (Kα₁^H) X-ray and the hypersatellite Pb (Kα₁^H) X-ray lines are 545±15 eV and 1238±45 eV, respectively.     

DieK-ElektroneneinfangwahrscheinlichkeitP K beim Zerfall von139Ce

TheK-Shell Electron-Capture ProbabilityP _K for the Electron Capture of¹³⁹Ce has been measured using the coincidence method. The detectors used have been a NaJ(Tl)-detector with Be-window for the Lanthan-X-ray, a Ge(Li)- and a 76.2 mm Ø×76.2 mm-NaJ(Tl)-detector for the 166 keV-γ-ray. The escape-effect of the Lanthan-X-ray in the NaJ(Tl)-detector was investigated. The experimental results areP _K Ω_K= 0.726±0.010 andP _K =0.801±0.034 using Ω_K=0.906±0.026.     

Internal conversion coefficients and penetration effect for the 279 keV transition in203Tl

The internal conversion process of theM1+E 2 mixed 279 keVγ-ray transition in the decay of²⁰³Hg has been reinvestigated. The emission rate of theK-shell internal conversion electrons was determined with an electron X-ray coincidence measurement using a magneticΒ-spectrometer and a Si(Li) detector of high energy resolution. Conversion electron ratios were obtained from electron spectra recorded as a function of momentum. The disintegration rate has been taken from measurements with a calibrated NaI(Tl)γ-ray spectrometer. Following results have been deduced: α=0.2279±0.0024, α _K =0.1653±0.0017, α _L =0.0475±0.0013,K/(L+M+?)=2.64±0.03,K/L=3.48±0.12,L/(M+N+ ?)=3.14±0.12. On the basis of the experimental results on theK-shell internal conversion coefficient,α _k , and the conversion ratioK/(L+M+?) the penetration effect on the internal conversion of theM1 part and the mixing ratio,δ ², of the 279 keVγ-ray transition in²⁰³Tl have been studied. Calculations were made using Hager and Seltzer's formalism and their theoretical internal conversion coefficients. The results are consistent with a mixing ratio ofδ ²=1.32±0.11 and a penetration parameter ofλ=6.8 ±0.8.     

DasL/K-Einfangverhältnis von48Vanadium

We measured theL/K-capture ratio of⁴⁸V for all transitions simultaneously and foundP _L /P _K =0.104±0.004. Coincidence measurements with the γ-rays by scintillation counters led toP _L /P _K =0.115 ± 0.015. This latter value is not very exact, but the comparison of the number ofK-pulses in the two sets of measurements allows the statement that the⁴⁹V-impurity in the⁴⁸V was less than 1.1% at the time of delivery and less than 10% during the measurements. So a possible⁴⁹V-impurity did not disturb the results.     

Precise measurement of theX K emission rate following the electron capture-decay of54Mn-fluorescence yield ω K of Cr

This determination was made using the electron capture decay of⁵⁴Mn. Two methods were employed to measure theK X-ray emission rate: by means of a pressurized 4π proportional counter with the gas at 1.5 MPa, and by means of a medium geometry-defined solid angle counter. The final result wasω _k=0.2901±0.003. Special care was taken in determining the corrections, some of which do not appear to have been allowed for so far. It is noteworthy that additional corrections, each about +3 %, had to be applied to the results obtained with each of the two methods. Thus there remains complete agreement between them, but at a higher value ofω _k than those appearing in recent publications.     

Plasmon dispersion in Beryllium

We have measured the plasmon dispersion in polycrystalline Beryllium at wave vectors up tok=1.29 Å^?1 with electron energy loss spectroscopy. The plasmon energy is 18.8±0.1 eV, the fitted quadratic dispersion coefficient is α=0.36±0.03 for 0<k<1.29 Å^?1 and α _L =0.52+0.04 fork<0.55 Å^?1. We compare our results with the plasmon dispersion in other simple metals and point out discrepancies with the theories of the homogeneous electron gas.     

Experimental natural lifetime determination of the Ar(II) lower laser levels

The natural lifetimes of the (³P)4s²P_3/2,1/2 levels of the Ar(II) spectrum have been determined from the natural broadening of argon lines, measured with a Fabry—Pérot interferometer. The natural broadening was determined from the lines with wavelengths of 4880 and 4965 Å by comparing them with the lines at 4806 and 5009 Å having negligible natural broadening. The natural lifetime of the 4s²P_3/2 level appeared to be τ = 0.19 (±6%) ns and of the 4s²P_1/2 level τ = 0.18 (±15%) ns. These values are about 1.5 to 2 times as small as those determined by other authors either experimentally by using a Fabry—Pérot interferometer by the method of Ballik, or calculated using intermediate coupling.The differences between the two experimental methods are discussed.     

Nuclearg-factors of the 328 keV state in194Pt,the 240 keV state in195Pt,and the 356 keV state in196Pt determined by recoil-implantation into iron and cobalt hosts

The iron-implantation-perturbed-angular-correlation technique (IMPACT) has been used to measure the Larmor precessions of the 328, 240, and 356 keV states of¹⁹⁴Pt,¹⁹⁵Pt, and¹⁹⁶Pt nuclei, respectively, in ferromagnetic iron and cobalt hosts. The observed angular precessions in iron, corrected for the transient field effect, wereω τ ₁₉₄(328)=0.103±0.006 rad,ω τ ₁₉₅ (240)=0.142±0.012, andω τ ₁₉₆(356)=0.084±0.010. For cobalt hosts, the observed Larmor precessions were ω τ₁₉₄(328)=0.068±0.006, ω τ₁₉₅(240)=0.096±0.012, andω τ ₁₉₆(356)=0.057±0.013. Agreement between theg-factors obtained from the measurements in iron hosts and the measurements in cobalt hosts is very good, and a weighted average of the two measurements givesg ₁₉₄(328)=0.349±0.031,g ₁₉₅ (240)=0.136±0.013, andg ₁₉₆(356)=0.329±0.039.