放射性核束的库仑激发

综述了利用中、高能放射性核束的库仑激发方法研究位于N＝20和28主壳隙附近的丰中子核结构所取得的进展．系统的实验结果清晰地表明,在离开β稳定线区域时N＝20兰壳隙突然消失和N＝28主壳隙的减弱过程．提出了利用兰州放射性束流线开展双幻核Ni50附近核素的低位能级核结构研究的构想． The study of coulomb excitation of the neutron-rich nuclei around N=20 and 28 shell closure with radioactive ion beam at intermediate energy is reviewed. The systematics of the measured energy of the 2+1 state shows that the N=20 shell closure in neutron-rich isotopes with Z≤12 disappears suddenly and N=28 shell elosure appears to be weak for 44S.The coulomb excitation studies of the exotic nuclei around the double magic 7828Ni50 at RIBLL are proposed.     

超重核合成中的靶核形变效应

利用额外推力模型研究了48Ca+238U超重核合成过程中的靶核形变效应.计算表明,在近垒和垒下能区,靶核形变使超重核合成截面明显增强.对于48Ca+238U反应,由于靶核形变蒸发残余截面增大了几倍.同时与球形靶核相比,形变靶核时蒸发残余激发函数的峰位移向较低能量.Effects of target deformation on the synthesis of superheavy nucleus~(283)112 are investigated in the framework of extra-push model. Our results show that the cross sections of the 3n evaporation residue in the~(48)Ca+~(238)U reaction for the case of β_2=0.275 are several times larger than those of β_2=0. Meanwhile, the peak position of ER excitation function in the case of deformed target is shifted to the lower energy as compared to the one of spherical target.     

偶-偶超重核基态性质的理论研究

在形变的相对论平均场模型下采用NL Z2,TMA两套参数对一些偶 偶核基态性质进行了系统的计算,并将理论计算的结合能、α衰变能与已知的实验数据进行了对比分析.结果发现两方面的数据能够比较好地吻合,从而验证了相对论平均场模型对超重核研究是可行的.同时在计算中给出了未知核素基态性质的计算结果,可供以后在理论或实验上研究超重核时参考. The ground state properties of the even even nuclei with proton number Z=94-104 have been systematically calculated in the deformed relativistic mean field (RMF) theory with two sets of force parameters, TMA and NL Z2. Comparing the calculated binding energies and alpha decay energys with the experimental ones, it is found that theoretical results are in good agreement with experimental data. The reliability of the RMF model for even even superheavy nuclei has been tested by this comparison...     

超重核的基态性质

用Skyrme Hartree Fock+BCS方法计算了超重核的基态性质,讨论了结合能、α衰变、形变、壳结构和自发裂变等问题.计算得到的结合能较好地反映了实验测量值,α衰变能与实验值符合很好.发现基本上有两种类型的超重核形变:在270108核附近的β2≈0.2的长椭球形变和在298114核附近的近球形形变.单粒子能级分布计算表明:在质子Z=108和中子N=162存在变形壳,在质子Z=114和中子N=184存在球形壳.用得到的α衰变能和Viola Seaborg公式估算了α衰变半寿命,能合理地符合实验测量值. The ground state properties of superheavy nuclei are investigated using the Skyrme Hartree Fock model. The pairing correlation is treated by the BCS method with the pairing δ force. Binding energies, α decays, spontaneous fissions, shell structures and deformations are discussed. Our calculations reproduce experimential binding energies and α decay energies.It is found that superheavy nuclei can be grouped with two kinds of deformations: i) well deformed prolate shapes (β2≈0.2) around 270108...     

RMF理论对N=60同中子核素形状演化的研究

利用形变约束的相对论平均场理论系统研究了N=60同中子核素的形状演化, 给出了这些核的基态结合能、 形变、 单粒子能级以及形变激发的位能曲线。 通过比较和分析发现, 随着质子数的增加, N=60同中子核的基态形变向轴对称形变方向演化, 114Xe和116Ba位于球形U（5）和轴对称SU（3）的过渡区, 存在形状相变的临界点结构, 这些结果与实验观测一致。 The shape phase transition between spherical U（5）and axially SU（3）deformed nuclei is investigated systemically for N=60 isotonic chain by the constrained relativistic mean|field theory with the interactions NL3 and PK1. The values of bind energy and quadruple deformation β2 are calculated and a good agreement is obtained as compared with the experiments. By examining the potential energy curve and single particle spectra obtained with this microscopic approach, the possible critical point nuclei with the structure of shape phase transition are suggested to be 114Xe and 116Ba, which is favored by the experiments.     

对超重核基态性质的系统性研究

对有限力程小液滴模型计算的质子数z=101—130超重核同位素链核的基态性质进行了系统的分析，通过对这些同位素链中处于裂变稳定线上核的平均结合能、四极形变、单质子分离能、双质子分离能和a衰变能等性质的系统研究，显示了质子数Z=108，114，126和中子数N=162，180，196时壳幻数的存在，同时可以看到Z=127之后超重核的基态性质还需要进一步研究。The calculated data by the Finite Range Droplet Model (FRDM) for the ground state properties of super-heavy nuclear isotope chains from Z=101 to Z=130 are analyzed in a global systematic way. Some quantities of the super-heavy nuclei which lie on the line of stability agains fission, such as the mean binding energy, deformation, single and double proton separation energy, as well as the α decay energy indicate the existence of the shell closure positions at Z=108, 114 and 126 and N=162...     

基于相对论平均场理论对超重核冷熔合反应截面的研究

在形变约束的相对论平均场理论框架下计算了合成Z=102—118元素的(可能)冷熔合反应中复合核及蒸发一或两个中子剩余核的位能曲面,得到了复合核和剩余核平衡点和鞍点的性质、静态裂变垒高度和冷熔合反应的最佳入射能;利用壳修正和对修正方法计算了平衡点和鞍点的壳修正能、对修正能和微观能.利用由此得到的壳结构信息,用简单的熔合蒸发唯象模型计算了相应反应的冷熔合截面.结果发现,TM1参数提供的结构性质给出了与实验接近的反应截面.     

超重核的生成和衰变

简单介绍了近年来在超重核研究方面所取得的成就和理论方面所面临的挑战.着重介绍推广的液滴模型和准分子形状机制,它们的优点是考虑了精确的核半经、质量和电荷的不对称性、形变、亲和力和温度等.推广的液滴模型和准分子形状机制能很好地描述重核和超重核的裂变、衰变及完全熔合反应.The progress and challenge on studies of superheavy elements both experiments and theories has been briefly introduced. It is emphasis to introduce a generalized liquid drop model, including the proximity effects, the asymmetry, an accurate nuclear radius, and quasi molecular shapes. The α decay half lives of 373 nuclei and superheavy elements have been calculated in the generalized liquid drop model and compared with the available experimental data. The deformed energies have also been obtained ...     

基于双核模型对Z = 116~ 121 超重核产生截面的研究(英文)

在双核模型的理论框架下系统研究了超重元素Z = 116 ~121 的蒸发剩余截面,计算过程中核子扩散由主方程描述,同时考虑了全熔合与准裂变的竞争。计算基本再现了利用热熔合反应48Ca+245Cm,48Ca+249Cf 和48Ca+249Bk 产生116~118 号同位素的合成截面。同样,分别以249Bk,249Cf 和243Am 为靶,以48Ca,50Ti 和58Fe 为炮弹,计算了Z = 119~ 121 号同位素的生成截面。结果表明,这些超重核的生成截面随着质子数的增大进一步变小。例如,利用58Fe+243Am 反应合成121 号同位素的最大蒸发剩余截面仅在fb 量级。基于对选择的几个反应系统的系统分析,发现双核系统在熔合蒸发过程中偶Z 奇N 和奇Z 偶N 复合核分别有强的3n 和4n 蒸发道。The production cross sections of superheavy elements with Z = 116~121 have been investigated systematically within the dinuclear system (DNS) concept, where the master equation is solved numerically to obtain the fusion probability. The competition between complete fusion and quasifission, which can strongly affect the cross section of the compound nucleus formation, is taken into account. The evaporation residue cross sections ER calculated for the hot fusion actinide-based reactions (48Ca+245Cm, 48Ca+249Cf and 48Ca+249Bk) are basically in agreement with the known experimental data within one order of magnitude. Similar calculations for the synthesis of superheavy elements up to Z = 121 are performed using the available 249Bk, 249Cf and 243Am as targets and 48Ca, 50Ti and 58Fe as projectiles. Their production cross sections are relatively small,especially for the 58Fe+243Am→301121 reaction. A systematic analysis indicates that the 3n and 4n channelsare respectively the most favorable fusion-evaporation channels in the synthesis of even- and odd-Z superheavy elements.     

Measurement of the linear electro-optic tensor of cubic boron nitride single crystals

The transverse electro-optic(EO)modulation system is built based on cubic boron nitride(cBN)single crystals unintentionally doped and synthesized at a high pressure and high temperature.The photoelectric output of the system includes two parts that can be measured respectively and the value of elements in the linear EO tensor of the cBN crystal can be obtained.This method does not need to measure the absolute light intensity.All of the surfaces of the tiny cBN crystals whose hardness is next to the hardest diamonds are{111}planes.The rectangular parallelepiped cBN samples are obtained by cleaving along{110}planes and subsequently grinding and polishing{112}planes of the tiny octahedral cBN flakes.Three identical non-zero elements of the EO tensor of the cBN crystal are measured via two sample configurations,and the measured results are very close,about 3.68 and 3.95 pm/V,respectively,which are larger than the linear EO coefficients of the general III-V compounds.     

Systematic Study on Alpha Decay Half-Lives of Superheavy Nuclei

The α-decay half-lives of a set of superheavy nuclear isotope chain from Z = 105 to 120 have been analyzed systematically within the WKB method, and some nuclear structure features are found. The decay barriers have been determined in the quasi-molecular shape path within the Generalized Liquid Drop Model （GLDM） including the proximity effects between nucleons in a neck and the mass and charge asymmetry. The results are in reasonable agreement with the published experimental data for the alpha decay half-llves of isotopes of charge 112, 114, and 116, of the element 294118 and of some decay products. A comparison of present calculations with the results by the DDM3Y effective interaction and by the Viola-Seaborg-Sobiczewski （VSS） formulae is also made. The experimental a decay half lives all stand in between the GLDM calculations and VSS formula results. This demonstrates the possibility of these models to provide reasonable estimates for the half-lives of nuclear decays by a emissions for the domain of SHN. The half-lives of these new nuclei are thus well tested from the reasonable consistence of the macroscopic, the microscopic, the empirical formulae and the experimental data. This also shows that the present data of SHN themselves are consistent. It could suggest that the present experimental claims on the existence of new elements Z =110 - 118 are reliable. It is expected that greater deviations of a few SHN between the data and the model may be eliminated by further improvements on the precision of the measurements.     

Precompound charged particle emission (PCE) — a mechanism beyond element production by complete fusion

Complete fusion reactions (xn-channels) using actinide targets are observed for values of the effective fissilities x _eff ∼ 0.80 in the sub-pb range of production cross sections. The elements produced at this limit are Z = 108–112. Beyond complete fusion, heavier elements might still be produced by reaction mechanisms releasing part of the nuclear charge before an equilibrated compound system might have been reached. Precompound Charged particle Emission (PCE) is proposed as a possible mechanism following complete fusion. A scheme delivering isotopes of elements Z = 110–115 is discussed, and experimental evidence for such a process is presented. Compound systems, the atomic numbers of which are smaller than in complete fusion reactions, might be produced in ⁴⁸Ca induced reactions on actinides with larger cross sections than those at the limits of complete fusion. Besides complete fusion, the PCE-mechanism should be considered as an alternative to interpret the ⁴⁸Ca-induced reactions on actinides.     

Doubly magic properties in superheavy nuclei

A systematic study of global properties of superheavy nuclei in the framework of the Liquid Drop Model and the Strutinsky shell correction method is performed. The evolution equilibrium deformations, TRS graphs and α-decay energies are calculated using the TRS model. The analysis covers a wide range of even-even superheavy nuclei from Z =102 to 122. Magic numbers and their observable influence occurring in this region have been investigated. Shell closures appear at proton number Z =114 and at neutron number N =184.     

类镍X光激光研究中的原子参数讨论

 对可能作为X光激光工作介质的47≤Z≤75及Z=41、79各元素的类镍离子, 系统计算了能级结构及各种过程参数。通过对已有部分实验数据的比较、拟合, 给出了对电子关联校正过的激光波长数据。分析了长波长与短波长激光线振子强度随电荷数的变化规律及其相互竞争关系。以类镍钕离子为例, 分析了粒子数反转及谱线放大对各种过程参数的条件要求并讨论了其它几条重要谱线不能产生增益的原因。     

Importance of Relativistic Effects for Intermediate-Z Elements： Photoionization Process of Excited Na

Using a modified R-matrix code, the fine-structure-resolved partial photoionization cross sections of excited Na （Z = 11） are calculated within the Breit-Pauli approximation. Our calculated energy levels of Na＋ and Na are in good agreement with the experimental values within 1% and the branching ratios of the J-resolved partial cross sections are consistent with the recent measurements within the experimental uncertainties. The agreements are impossible to be obtained without adequately taking into account the relativistic effects and the electron correlations together. Therefore, even for the intermediate-Z elements （e.g. Na with Z = 11）, the relativistic effects （mainly the spin-orbit interactions） should not be neglected.     

Correlation of calculated and measured 2p spin-orbit splitting by electron spectroscopy using monochromatic x-radiation

In the past, measurements have been made of the spin-orbit splitting (2p3/₂ -2p1/₂) of medium to large atomic number elements. The present work is concerned with the 2p splitting in elements of low atomic number (e.g. Si,P, S, Cl). We have measured the splitting in such elements by X-ray photoelectron spectroscopy (XPS or ESCA) with the aid of an X-ray monochromator attachment which is described. The results are in good agreement with data obtained by X-ray spectroscopic techniques, and with a theoretical prediction based on the Sommerfeld formula, with a screening constant of S = 3.40. Moreover, the modified formula holds for elements up to Z = 30 as well as for the lower atomic numbers if allowances are made for deviations in the first period of transition elements which may be accounted for by the assumption of interactions between the 2p electrons and unpaired electrons in the 3d level.     

Nuclear shape effect on the g factor of hydrogenlike ions

The nuclear shape correction to the g factor of a bound electron in the 1S state is calculated for a number of nuclei in the range of charge numbers from Z=6 up to Z=92. The leading relativistic deformation correction has been derived analytically, and also its influence on one-loop quantum electrodynamic terms has been evaluated. We show the leading corrections to become significant for mid-Z ions and for very heavy elements to even reach the 10(-6) level.     

Total Routhian Surface Calculations on Hf Isotopes

The two-dimensional total routhian surface calculations have been carried out to study the triaxial superdeformed structure of a neutron-rich nucleus ¹⁷³Hf firstly. In particular the effects of the rotational frequency ω and pairing-energy gap parameter Δ are discussed in detail in the course of shaping its triaxial superdeformation; additionally the neutron-shell correction energy is analyzed with emphasis in the confirmed triaxial superdeformed nucleus ¹⁷³Hf. Finally, more systematical results have been investigated for some confirmed superdeformed nuclei experimentally and a few predicted triaxial superdeformed nuclei theoretically with quadropole deformation ε₂≈0.4 and triaxial deformation γ≈20^º or 30^º in the Z=72 region.