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1.
We study the photodissociation of trapped $\mathrm{H}_{2}^{+}$ ions by 248?nm light from an excimer laser. Our results are in good agreement with calculated populations and photodissociation cross sections of the involved vibrational levels and yield a determination of the ion cloud radius. These data are used to obtain a reliable estimate of the efficiency of the resonance-enhanced multiphoton dissociation (REMPD) scheme in our $\mathrm{H}_{2}^{+}$ vibrational spectroscopy experiment. We go on to estimate the expected signal-to-noise ratio and discuss future improvements of the experimental setup.  相似文献   

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In general, clusters are unstable and in many cases several metastable isomers exist even at low temperature. Therefore, a cluster may react with a dramatic geometry change to a small disturbance such as a weak field or to the absorption of a low-energy photon. Here, we study the response of Al3O3-\mathrm{Al}_{3}\mathrm{O}_{3}^{-} to photoexcitation using time-resolved photoelectron spectroscopy. Earlier experimental and theoretical studies suggested that this cluster anion undergoes a geometry change after photoexcitation. In contrast, our time-resolved spectra indicate that photoexcitation triggers ultra-fast fragmentation. This example demonstrates that ultra-fast processes in clusters are not well understood and that it is still difficult to gain reliable experimental data about such processes.  相似文献   

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The non-diagonal correlators of vector and scalar currents are considered at three-loop order in QCD. The full mass dependence is computed in the case where one of the quarks is massless and the other one carries mass M. We exploit the decoupling relations between the full theory and the heavy quark effective theory (HQET) in order to obtain the logarithmic parts of the leading threshold terms. With the help of conformal mapping and Padé approximation numerical estimates for the non-logarithmic terms are extracted which in turn lead to a prediction of the correlator in HQET at order . As applications of the vector and scalar correlator we consider the single-top-quark production via the process and the decay rate of a charged Higgs boson into hadrons, respectively. In both cases the computed NLO corrections are shown to be numerically much less important than the leading ones. On the contrary, the NLO order QCD corrections to the HQET sum rule for the leptonic decay rate of a heavy-light meson proves to be comparable to the leading one. Received: 19 June 2001 / Published online: 10 August 2001  相似文献   

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Femtosecond (fs) laser pulses at variable delay times allowed us to track the fast non-radiative transitions between the manifold of highly excited $\mathrm{M}_{\mathrm{Na}}^{**}$ states to the lower lying fluorescent $\mathrm{M}_{\mathrm{Na}}^{*}$ state in CaF2. Two distinct $\mathrm{M}_{\mathrm{Na}}^{**}$ states of the manifold at 3.16?eV ( $\mathrm{M}_{\mathrm{Na}2}^{**}$ ) and 4.73?eV ( $\mathrm{M}_{\mathrm{Na}3}^{**}$ ) were populated using the second (SH) and third harmonics (TH) of fs laser light at 785?nm. The population kinetics of the fluorescent $\mathrm{M}_{\mathrm{Na}}^{*}$ state in the 2?eV excitation energy range was revealed by depleting its fluorescence centered at 740?nm using fundamental near infrared (NIR) fs laser pulses. The related time constants for $\mathrm{M}_{\mathrm{Na}2,3}^{**}{\sim}{>} \mathrm{M}_{\mathrm{Na}}^{*}$ relaxation amounted to 1.0±0.14?ps and 3.0±0.3?ps upon SH and TH excitation, respectively.  相似文献   

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A semi-empirical potential according to the embedded atom, has been applied to investigate the diffusion of trimers by computing the energy barriers for different mechanisms. Our attention was more focused on the leapfrog process which is likely to occur on missing row surfaces. The activation barriers of this mechanism are calculated using drag method at 0K. These barriers are found to be 0.64 and 0.68 eV for hopping out the channel for $\mathrm{Cu }_{3}/\mathrm{Ag }(110) \mathrm{and Ag }_{3}/\mathrm{Cu }$ (110) respectively. While for hopping down at the other side they are about 0.42 and 0.32 eV. Moreover, a deep metastable position is observed during leapfrog diffusion leading to some spectacular trimer motion. At high temperature and essentially for $\mathrm{Cu }_{3}/\mathrm{Ag }$ (110), we also observed a competition between leapfrog process and concerted jump mechanism with a deformation of trimer geometry. Implications of these findings are briefly discussed.  相似文献   

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The process p $ \bar{{p}}$ $ \rightarrow$ $ \Lambda_{c}^{+}$ $ \bar{{\Lambda}}_{c}^{-}$ is investigated within the handbag approach. It is shown to lowest order of perturbative QCD that, under the assumption of restricted parton virtualities and transverse momenta, the dominant dynamical mechanism, characterized by the partonic subprocess u $ \bar{{u}}$ $ \rightarrow$ c $ \bar{{c}}$ , factorizes in the sense that only the subprocess contains highly virtual partons, namely a gluon, while the hadronic matrix elements embody only soft scales and can be parameterized in terms of helicity flip and non-flip generalized parton distributions. Modelling the latter functions by overlaps of light-cone wave functions for the involved baryons we are able to predict cross-sections and spin correlation parameters for the process of interest.  相似文献   

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An improved search for B s 0 oscillations is performed in the ALEPH data sample collected during the first phase of LEP, and reprocessed in 1998. Three analyses based on complementary event selections are presented. First, decays of B s 0 mesons into hadronic flavour eigenstates are fully reconstructed. This selection yields a small sample of candidates with excellent decay length and momentum resolution and hi gh average B s 0 purity. Semileptonic decays with a reconstructed D s - meson provide a second sample with larger statistics, high average B s 0 purity, but a poorer momentum and decay length resolution due to the partial decay reconstruction. Finally, semileptonic b-hadron decays are inclusively selected and yield the data sample with the highest sensitivity to B s 0 oscillations, as the much higher statistics compensate for the low average B s 0 purity and poorer time resolution. A lower limit is set atps-1 at 95% C.L., significantly lower than the expected limit of 15.2 ps-1. Received: 21 February 2003 / Published online: 11 June 2003  相似文献   

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The kinetics of growth, composition and electronic structure of thin oxide films formed by reactive ion beam mixing (IBM) of Ni/Al interfaces bombarded with low-energy (3-keV) O2+\mathrm{O}_{2}^{+} ions have been studied at room temperature using X-ray photoelectron spectroscopy, ultraviolet photoelectron spectroscopy and factor analysis. Initially, NiO species are formed but, later, with increasing ion dose, Ni–Al mixed oxide species appear due to Al incorporation in the near-surface region. These changes are accompanied by a slight increase of the oxygen concentration and a decrease of the Ni/Al ratio in the thin oxide films formed. Angle-resolved X-ray photoelectron spectroscopy shows that Ni–Al mixed oxide species are located nearer the surface than NiO species. Experimental results have been compared with Monte Carlo TRIDYN simulations, suggesting that processes driven by residual defects or the reaction with oxygen predominate over pure ballistic mechanisms during reactive IBM of Ni/Al interfaces.  相似文献   

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Using the method of laser-induced fluorescence in an atomic beam we have measured the hyperfine splitting constants, A and B, of the ground and excited states of the optical transition 4f 76s 2 8S $_{1/2}\to 4f^{7}$ 6s6p 6P5/2 (564.58 nm) for 151???155Eu isotopes. For all isotopes, the magnetic dipole constants of the 6P5/2 atomic level are determined to a precision better than 0.04%. The A and B constants for the ground state 8S7/2 of the radioactive 152,154,155Eu were obtained for the first time with a precision better than 0.5%. Our data along with previous ground state hyperfine structure measurements for the stable europium isotopes allow us to determine the hyperfine anomaly for mentioned Eu isotopes.  相似文献   

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We construct geometric representatives for the fractional branes in terms of branes wrapping certain exceptional cycles of the resolution. In the process we use large radius and conifold-type monodromies, and also check some of the orbifold quantum symmetries. We find the explicit Seiberg-duality which connects our fractional branes to the ones given by the McKay correspondence. We also comment on the Harvey-Moore BPS algebras.  相似文献   

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A three-body calculation for the \({^4_{\Lambda} \rm{He}}\) and \({^6_{\Lambda}{\rm H}}\) hypernuclei has been undertaken. The respective cores are \({^4_{\Lambda}{\rm H}}\) . The interactions in the \({^6_{\Lambda}{\rm He}}\) system, modeled as \({^4_{\Lambda} {\rm H+p+n}}\) , are reasonably well known. For example, the p n interaction is well determined by the p n scattering data, the \({^4_{\Lambda}{\rm H}}\) p interaction can be fitted to the \({^5_{\Lambda}{\rm He}}\) binding energy. The \({^4_{\Lambda}{\rm He}}\) n interaction can be fitted to α–n scattering data. For the 4He–n system the s-wave can be modeled alternatively as a repulsive potential or as an attractive potential with a forbidden bound state. We explore these alternatives in 6He, because the interaction comes into play in modeling \({^6_{\Lambda}{\rm He}}\) as well as in our \({^4_{\Lambda}{\rm H}}\) + n + n model of \({^6_{\Lambda}{\rm H}}\) , where the valence neutrons are Pauli blocked from the s-shell of the core nucleus.  相似文献   

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