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E. Hulpke 《Surface science》1975,52(3):615-640
Energy and angular distributions of Li+ ions scattered from W(110) and Si(111) surfaces have been measured for a wide range of scattering angles and for beam energies between 2 and 20 eV. The collision process can be explained in terms of binary collisions with single surface atoms, if the influence of the attractive part of the interaction potential is taken into account. A square well approximation for the potential makes it possible to predict the form of the energy spectrum as well as the behaviour of the angular distribution of the scattered particles for both systems. The influence of adsorbed atoms and molecules on the scattering behaviour has been investigated. Exposure of the W surface to H2, O2 and CO shows that surface coverages exceeding 10% of a monolayer very drastically influence the scattering. The results from the clean surfaces indicate that sufficiently precise measurements of the energy spectra of the scattered particles can yield very detailed information about the form of the interaction potential. The form of the energy spectra also contains information as to the extent of vibrational excitation of the surface atoms.  相似文献   

3.
The excitation and loss of an electron by ions in relativistic collisions with atoms are studied in first-order perturbation theory. General expressions are obtained for the cross sections for the excitation and loss of an electron. In the limit of nonrelativistic collision velocities these expressions pass into the well-known nonrelativistic results. It is shown that, in contradistinction to the nonrelativistic collisions, in ultrarelativistic collisions the screening of the nucleus of the target atom by the atomic electrons is very important for excitation and loss of an electron by ions even for collisions of heavy ions with light atoms. Our computational results for the cross section for electron loss are in good agreement with existing experimental data.  相似文献   

4.
The two coupled channel formalism for high energy elastic scattering [1] is extended to include spin and isospin effects. For a spin and isospin zero nucleus these manifest themselves by additional spin-orbit terms in the potentials. Explicit formulas for these potentials are obtained in terms of the fully spin and isospin dependent nucleon-nucleon scattering amplitude, the ground state nuclear form factor and the state dependent correlation functions. The coupling potential except for a small term arising from double spin and isospin flip process involving nuclear excitation depends only upon the pair correlations.Numerical calculations are performed for the elastic scattering of 1 GeV protons incident on 4He. Various phenomenological dynamical two-body correlations as well as correlations generated from the Reid soft-core and Tabakin potentials in an approximate Brueckner-Hartree-Fock calculation are considered. The angular distribution beyond its first diffraction minimum as well as the polarization in the same angular range are shown to be sensitive to these correlations. However, the present accuracy of the experimental data and the lack of knowledge of the nucleon-nucleon scattering amplitude prevent any definitive conclusion about their nature.  相似文献   

5.
The anomalous electron-positron coincidences observed in heavy-ion collisions have been interpreted as signal for the pair decay of hitherto unknown neutral objects with masses around 1.8 MeV. We discuss the decay modes of such extended composite particles when they are bound to a nucleus. In particular we investigate the angular correlation of the emitted pair and the competing single-photon decay channel. We confront the particle hypothesis with recent negative results from experiments searching for resonances in Bhabha scattering. The induced pair decay of a metastable 1++ state in secondary collisions with target atoms is discussed as a possible explanation.  相似文献   

6.
We report the results of analysis of correlations of the product protons from inelastic eA collisions at smallQ 2. The experimental data were measured by the ARGUS detector. The correlation effect at small relative momentaq (interference and final state interaction) is closely associated with the angular correlations due to momentum conservation. The examined correlations in eA collisions also show features similar to correlations in hA collisions.  相似文献   

7.
Murrell-Sorbie势下He-HCl碰撞体系微分散射截面的研究   总被引:7,自引:3,他引:4       下载免费PDF全文
根据在CCSD(T)/aug-cc-pVQZ理论水平下计算的He-HCl相互作用能数据,作者采用Murrell-Sorbie势函数形式拟合了He原子与HCl分子相互作用的各向异性势,并与其它势模型进行了比较;然后采用公认的精确度较高的CC近似方法计算了He-HCl碰撞体系的微分散射截面,总结了非弹性微分散射截面的变化规律.研究表明:采用拟合的各向异性势计算的微分散射截面与实验结果符合得很好.拟合势不但表达形式简洁,而且较好地描述了He-HCl系统相互作用的各向异性特征;利用碰撞体系分子间势的量子化学从头计算结果,可解决势能参数难以确定的问题.对进一步研究原子与分子相互作用的机制有一定的参考价值.  相似文献   

8.
Measurements of angular distributions for the scattering of well-defined incident beams of CO and N(2) molecules from a graphite surface are presented. The measurements were carried out over a range of graphite surface temperatures from 150 to 400?K and a range of incident translational energies from 275 to over 600?meV. The behavior of the widths, positions and relative intensities of the angular distributions for both CO and N(2) were found to be quite similar. The experimental measurements are discussed in comparison with calculations using a classical mechanical model that describes single collisions with a surface. Based on the behavior of the angular distributions as functions of temperature and incident translational energy, and the agreement between measured data and calculations of the single-collision model, it is concluded that the scattering process is predominantly a single collision with a collective surface for which the effective mass is significantly larger than that of a single carbon atom. This conclusion is consistent with that of earlier experiments for molecular beams of O(2) molecules and Xe atoms scattering from graphite. Further calculations are carried out with the theoretical molecular scattering model in order to predict translational and rotational energy transfers to and from the molecule during scattering events under similar initial conditions.  相似文献   

9.
简要评述了重离子弹性散射角分散研究的内容、 方法及物理意义。通过前角区重离子弹性散射产物微分截面的角分布测量,作出角分散图ln(dσ/dθ)\|θ2。 分析经典偏转函数, 从而在实验上确定了反应系统的核虹角。 在低能、 重靶的重离子反应系统中, 核虹角远小于擦边角。 晕核及弱束缚核比稳定核具有更小的核虹角和更大的核相互作用范围。 经典偏转函数的计算有助于提供一套光学势参数, 以便于拟合弹性散射产物的微分截面。 In terms of the angular dispersion plot of ln(dσ/dθ) versus θ2, which can be obtained from the angular distribution of the elastic scattering differential cross sections in heavy ion collisions, systematic analysis on the angular dispersions is made by using classical deflection function for the available experimental data on the target of 208Pb. Our systematic analyses bring about some important results. Firstly, there is an angular dispersion turning angle at forward angular range beyond the grazing angle. Secondly, the nuclear rainbow angle for such reaction systems can be determined by measuring differential cross sections of elastic scattering at forward angular range and analyzing the angular dispersion. Thirdly, analysis of angular dispersion may provide a way to determine a set of optical potential parameters by means of fitting the experimental data of elastic scattering differential cross sections. Finally, for the halo nuclei as the projectiles, there is an exotic behaviour, i. e., smaller angular dispersion turning angle.  相似文献   

10.
原子分子相互作用在许多物理过程中都十分重要.原子分子碰撞过程中转动激发截面的研究是确定原子与分子间相互作用的理想方法,许多理论和实验工作者在这方面做了大量工作,并得到理论和实验数据.本文用密耦近似计算了惰性气体He、Ne、Kr与h2、D2、T2碰撞的弹性和转动激发截面,原子入射能量分别为0.05 eV、0.15eV、0.20eV和0.25eV.  相似文献   

11.
The quantum dynamics of colliding Bose-Einstein condensates with 150,000 atoms are simulated directly from the Hamiltonian using the stochastic positive-P method. Two-body correlations between the scattered atoms and their velocity distribution are found for experimentally accessible parameters. Hanbury Brown-Twiss or thermal-like correlations are seen for copropagating atoms, while number correlations for counterpropagating atoms are even stronger than thermal correlations at short times. The coherent phase grains grow in size as the collision progresses with the onset of growth coinciding with the beginning of stimulated scattering. The method is versatile and usable for a range of cold atom systems.  相似文献   

12.
A fluctuation X‐ray scattering experiment has been carried out on platinum‐coated gold nanoparticles randomly oriented on a substrate. A complete algorithm for determining the electron density of an individual particle from diffraction patterns of many particles randomly oriented about a single axis is demonstrated. This algorithm operates on angular correlations among the measured intensity distributions and recovers the angular correlation functions of a single particle from measured diffraction patterns. Taking advantage of the cylindrical symmetry of the nanoparticles, a cylindrical slice model is proposed to reconstruct the structure of the nanoparticles by fitting the experimental ring angular auto‐correlation and small‐angle scattering data obtained from many scattering patterns. The physical meaning of the refined structure is discussed in terms of their statistical distributions of the shape and electron density profile.  相似文献   

13.
An experimental study is reported about the quenching of electronic excitation of Cs atoms caused by their collisions with a glass surface. The energy with which they are scattered from the surface after quenching has been measured to be 0.5 eV, which is about one-third of the excitation energy. A discussion is given of the mechanisms by which the excitation energy is partitioned between the atom and the surface in two different cases, namely, in the excitation of the atom adsorbed on the surface and in the collision of the preexcited atom with the surface.  相似文献   

14.
The energy spectra and the angular distributions of noble gas ions, reflected from a metal surface, yield information about a number of important properties of this surface. A large number of investigations have been carried out in the past decades, not only to get insight into the interaction mechanism but also to develop methods for applying of the knowledge gained. To obtain information about the outermost surface layer, it appears necessary to use noble gas ions as primary particles, and to detect the scattered particles in the charged state only; the fraction of noble gas ions reaching the detector, after reflection from target atoms in the second layer, is very small because of the high probability of neutralization. However, this is only valid if the initial energy of the incoming ions is relatively low, namely ? 10 KeV. Under certain experimental circumstances it appears justifiable, down to a lower limit of about 20 eV, to conceive the interaction of these ions with the target atoms as single collisions. The relation between the initial energy and the post-collision energy is then very simple if the collision is an elastic one; it depends upon the scattering angle and upon the ratio of the two given masses only and not upon the interaction potential. The shift of the peaks in an energy spectrum is caused by inelastic collisions and is relatively small in the considered energy region. The causes of this shift will be discussed. As opposed to single collisions, the post-collision energies after a multiple collision depend largely upon the interaction potential. Attention will be paid to the search for these potentials. Utilization of the multiple collision phenomenon in the study of surface geometry is hampered by the vibrational motion of the surface atoms. As a result, the energy spectra are blurred and a shift of the so-called quasi-single and quasi-double peaks can occur. Under certain conditions a third peak emerges which can give additional information about the surface vibrations. The intensity of the scattered ions depends upon the cross section for scattering. Recently it has been shown that the relation between this cross section and the initial energy has an oscillating character for certain combinations of incident ions and target atoms. This phenomenon has very important consequences, e.g. in the use of single ion scattering as an analytical tool. To investigate surface structures it appears that single and multiple ion scattering, combined with LEED and AES, can provide valuable information.  相似文献   

15.
The scattering of electrons by hydrogen atoms is studied for an incident energy of 15 eV, by means of a close coupling calculation using a pseudostate basis. Results are presented for elastic scattering and n = 2 excitation, including angular correlation parameters. The ionization cross section is extracted by an improved projection technique.  相似文献   

16.
Multiplicities of charged particles produced in the forward and backward hemispheres are investigated for proton-nucleus and proton-nucleon collisions in the range from 20 to 400 GeV/c. Weak, but growing with incident beam momentum, forward-backward multiplicity correlations are observed which cannot be reduced to the inelastic diffraction. These correlations are more pronounced in proton-nucleus than proton-nucleon interactions. The experimental data are discussed in the frameworks of current cluster and multiple scattering models. It is shown that multiple scattering models describe well the forward-backward multiplicity correlations in nuclear production.  相似文献   

17.
We have calculated the electron excitation cross sections of hydrogen atom by the impact of protons, alpha particles and He+ ions using the boundary corrected continuum intermediate state approximation in the intermediate and high energies. The calculated results are compared with other theoretical and experimental results. The angular influence of excitation to the H atom at the intermediate energy is also discussed. The distortion effects due to the projectile charges in reactions of electron excitation to bound states of the target H atom are shown in the intermediate and high collision energy.  相似文献   

18.
Azimuthal angular correlations and the alignment of photons are studied in gamma families recorded by the Pamir Collaboration in a carbon x-ray emulsion chamber. The present interpretation of these experimental data is based on a model of semihard parton scattering in nucleon-nucleus collisions and on arguments favoring the production of exotic beam strings and heavy leading resonances undergoing quasicoplanar decays.  相似文献   

19.
A new type of weak localization of electrons emerging during electron emission is considered. It is manifested in singularities of the angular spectra of particles reflected inelastically from a solid and causing Auger ionization of the atoms. The orientational dependences in this case appear as a result of interference of two types of processes. In one case, an electron from the primary beam penetrates the solid, undergoes inelastic scattering, ionizes an atom, and is then scattered elastically through a large angle, after which it leaves the solid. In the other case, elastic scattering of an electron precedes its inelastic scattering due to the Auger ionization of an atom. The azimuthal angular dependences of currents created by inelastically reflected electrons contain information on new processes of weak localization of particles.  相似文献   

20.
We show how entanglement may be quantified in spin and cold atom many-body systems using standard experimental techniques only. The scheme requires no assumptions on the state in the laboratory, and a lower bound to the entanglement can be read off directly from the scattering cross section of neutrons deflected from solid state samples or the time-of-flight distribution of cold atoms in optical lattices, respectively. This removes a major obstacle which so far has prevented the direct and quantitative experimental study of genuine quantum correlations in many-body systems: The need for a full characterization of the state to quantify the entanglement contained in it. Instead, the scheme presented here relies solely on global measurements that are routinely performed and is versatile enough to accommodate systems and measurements different from the ones we exemplify in this work.  相似文献   

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