Doublet structure of the first excited state of 71As

The possible multiplet structure of the first-excited state of ⁷¹As has been investigated by the high resolution ⁷⁰Ge(³He, dγ) reaction and the γ-rays emitted in the decay of ⁷¹Se. Both studies reveal a doublet at 143.2 keV and 147.3 keV excitation energies. The existence of this doublet in ⁷¹As brings the low-lying level structure in better resemblance to the heavier odd-A arsenic isotopes.     

Precise atomic mass difference determinations between some stable isotopes of Ge,As and Se

The 1 m radius, high-resolution mass spectrometer at the University of Manitoba (“Manitoba II”) has been used to determine 11 atomic mass differences between some stable isotopes of Ge, As and Se. These values are of greater accuracy and precision than existing data. Their consistency has been checked by a major least-squares adjustment involving relevant data in the region. Results include improved S_2n values for several nuclides and the energies available for the ββ decays of ⁷⁶Ge and ⁷⁴Se, respectively.     

79Se investigated by the reaction76Ge(α, nγ)

⁷⁹Se has been investigated by the reaction⁷⁶Ge(α, nγ). Gamma excitation functions (E _{α=10?15 MeV)}, gamma angular distributions and gamma-gamma coincidences (both at (E _{α=12 MeV)}, have been taken. A level scheme has been established, spins and partities have been assigned. The results are compared with rotational bands in neighbouring odd Se isotopes. Nuclear reaction⁷⁶Ge(α, nγ)E _α =12 MeV; measuredE _γ,I _γ,γ-γ coincidences,γ-angular distribution,γ-excitation function.⁷⁹Se deduced levels,J, π. Enriched target, Ge(Li).     

Single-neutron transfer reactions 76, 78, 80, 82Se(p,d)75, 77, 79, 81Se at EP = 33MeV

Single-neutron transfer reactions on even-even Se nuclei have been studied using 33 MeV incident proton energy from the ANU cyclograaff facility. A total of 120 levels have been seen below 4 MeV excitation energy in ^{75, 77, 79, 81}Se isotopes. Angular distributions for 88 states were extracted and analysed with DWBA theory yielding a number of new l_n assignments. Coriolis coupling calculations have been carried out for low-level spin states in all four isotopes.     

Calculation of nucleon densities in calcium,nickel, and molybdenum isotopes on the basis of the dispersive optical model

The radial distributions of proton and neutron densities in the even–even isotopes ^40?70Cа and ^48?78Ni and the analogous distributions of neutron densities in the even–even isotopes ^92?138Mo were calculated on the basis of the mean-fieldmodel involving a dispersive optical potential. The respective root-mean-square radii and neutron-skin thicknesses were determined for the nuclei under study. In N > 40 calcium isotopes, the calculated neutron root-mean-square radius exhibits a fast growth with increasing N, and this is consistent with the prediction of the neutron-halo structure in calcium isotopes near the neutron drip line.     

Cross sections of fast neutron induced reactions on selenium isotopes

Cross sections for^{74, 76, 77, 78}Se(n, p)^{74, 76, 77, 78}As,⁷⁶,Se(n,2n)⁷⁵Se and⁸⁰Se(n, α)⁷⁷,Ge reactions have been measured in the energy range from 13.0 to 16.6 MeV by the activation technique using Ge(Li) detectorγ-ray spectroscopy. Samples of selenium of natural isotopic composition were used as targets. The measurements provide information on the evolution of the (n, p) excitation functions with the increasing target neutron number (isotopic effect). The reaction model combining the compound nucleus and the preequilibrium emission processes is used to interpret these three types of reactions. The isotopic trend for the (n, p) reactions due to the neutron-proton competition in the compound nucleus is satisfactorily reproduced. However, a further experimental and theoretical work is needed for a better understanding of the origins of discrepancies which are suggested to be related to the precompound aspects of the assumed reaction model.     

First excited 0+ states in the germanium isotopes via the Se(d, 6Li) reaction

A systematic study of the even-A germanium isotopes with mass 70 ≦ A ≦ 78 via the Se(d, ⁶Li) reaction has been performed at E_d = 45 MeV. The reaction products were momentum analysed and mass identified with a QMG/2 magnetic spectrograph and the accompanying focal-plane detector system. The main emphasis of this investigation was on the nature of the first excited 0⁺ states. The striking variation in strength from one isotope to the other already observed in the (p, t) reactions to the same final nuclei is also seen for the α-pickup reaction. Previously derived wave functions that assume the excited 0⁺₂ states to be pure proton configuration states can also account for the present results.     

Investigation of special features of the neutron and proton shell structure of the isotopes 90,92,94,96Zr

The neutron and proton single-particle energies and the occupation probabilities for the valence states of the even-even isotopes ^90,92,94,96Zr are determined by matching data on nucleon-stripping and nucleon-pickup reactions on the same nucleus. The data obtained in this way suggest the magicity of the number N = 56 for Z = 40. The single-particle energies of all bound neutron and proton states in the ^90,92,94,96Zr nuclei are described within the experimental errors on the basis of the dispersive optical model.     

Isomere Wirkungsquerschnittsverhältnisse beim thermischen Neutroneneinfang im Bereich der 2p 1/2 und 1g 9/2 Schalenmodellzustände

Thermal capture cross sections and isomeric cross section ratios in thermal neutron capture were determined for even-even nuclei in the region of the 2p _1/2-1g _9/2 neutron shell. Capture cross sections for formation of Zn 69 ^m , Zn 71 ^m , Zn 71, Ge 71, Ge 75 ^m , Ge 77 ^m , Se 77 ^m , Se 79 ^m , Se 83 ^m , Se 83, Sr 85 ^m and Sr 87 ^m were measured by the activation method. From these data and additional measurements of cross section ratios the isomeric ratios for thermal capture in Zn 68, Zn 70, Ge 70, Ge 74, Ge 76, Se 76, Se 78, Se 80, Se 82 and Sr 84 were determined. In addition epithermal capture isomer ratios were determined for Zn 68, Ge 74, Ge 76, Se 80 and Sr 84. The isomer ratios are compared with calculations based on the statistical model ofHuizenga andVandenbosch. With the exception of Se 80 the measured ratios can be explained theoretically with reasonable values of the spin-cutoff-factorσ and gamma-ray multiplicityN, however there seems to be unexplained difference in eitherσ orN between the two groups of nuclei leading to either 1/2–7/2 or 1/2–9/2 isomers.     

On the structure of71As and 73As

The structure of the nuclei ⁷¹As and ⁷³As has been investigated by studying the decay of ⁷¹Se, ^73gSe and ^73mSe, the ⁷²Ge(p, 2nγ)⁷¹As reaction, the ⁷³Ge(p, nγ)⁷³As reaction and the ⁷²Ge(³He, d) ⁷³As reaction. Level schemes of ⁷¹As and ⁷³As are constructed on basis of the energies and intensities of the gamma transitions and their coincidence relations. Spins and parities are deduced from log ft values, l-values and the decay properties of the excited states. The measured half-life of the lowest excited state in ⁷¹As is $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 59 ± 10}\text{ns}$. The experimental level-schemes are compared with the predictions of the cluster-vibrational coupling model.     

Measurement of the cross sections for the production of the isotopes <Superscript>74</Superscript>As, <Superscript>68</Superscript>Ge, <Superscript>65</Superscript>Zn,and <Superscript>60</Superscript>Co from natural and enriched germanium irradiated with 100-MeV protons

The cross sections for the production of the radioactive isotopes ⁷⁴As, ⁶⁸Ge, ⁶⁵Zn, and ⁶⁰Co in metallic germanium irradiated with 100-MeV protons were measured, the experiments being performed both with germanium of natural isotopic composition and germanium enriched in the isotope ⁷⁶Ge. The targets were irradiated with a proton beam at the facility for the production of radionuclides at the accelerator of the Institute for Nuclear Research (INR, Moscow). The data obtained will further be used to calculate the background of radioactive isotopes formed by nuclear cascades of cosmic-ray muons in new-generation experiments devoted to searches for the neutrinoless double-beta decay of ⁷⁶Ge at underground laboratories.     

High spin states in75Se populated by the72Ge(α,n) and73Ge(α, 2n) reaction

The⁷²Ge(α, n)⁷⁵Se and⁷³Ge(α, 2n)⁷⁵Se reactions have been studied at bombarding energies of 15 MeV and 22.5 MeV respectively using Ge(Li)-detectors.γ-singles spectra,γ-γ-coincidences,γ-angular distributions and excitation functions have been taken. A level scheme has been constructed, which contains a stretched spin and a normal rotational band. Nuclear reactions⁷²Ge(α, n)⁷⁵Se,⁷³Ge(α, 2n)⁷⁵Se; measuredE _γ ,I _γ ,γ-γ-coincidences,γ-angular distribution,γ-excitation function.⁷⁵Se deduced levels,J, π, γ-multipolarity. Enriched target, Ge(Li).     

Study of 71, 73, 75, 77As with Ge(3He,d) reactions

Studies of ^{71, 73, 75, 77}As isotopes using Ge(³He, d) reactions have enabled the identification of many previously unreported levels together with new spin-parity assignments. A comparison of the results with the predictions of the model of Scholz and Malik shows good agreement for both positive- and negative-parity states.     

70Ge(α, γ)74Se cross section measurements at energies of astrophysical interest

The cross section of the reaction⁷⁰Ge(α, γ)⁷⁴Se has been measured over the bombarding energy range of 5.05 MeV <E _α < 7.80 MeV using single and coincidence gamma spectroscopy techniques. The experimental S-factor values are in agreement with theoretical statistical-model calculations. Reaction rates for the⁷⁰Ge(α, γ)⁷⁴Se and the inverse (γ, α) reactions have been determined for appropriate temperatures.     

Single-particle properties of <Emphasis Type="Italic">N</Emphasis> = 12 to <Emphasis Type="Italic">N</Emphasis> = 20 silicon isotopes within the dispersive optical model

Experimental neutron and proton single-particle energies in N = 12 to N = 20 silicon isotopes and data on neutron and proton scattering by nuclei of the isotope ²⁸Si are analyzed on the basis of the dispersive optical model. Good agreement with available experimental data was attained. The occupation probabilities calculated for the single-particle states in question suggest a parallel-type filling of the 1d and 2s _1/2 neutron states in the isotopes ^{26,28,30,32,34}Si. The single-particle spectra being considered are indicative of the closure of the Z = 14 proton subshell in the isotopes ^30,32,34Si and the N = 20 neutron shell.     

A systematic study of (n,d), (n,n' p) and (n,pn) reactions at 14.7 MeV

Cross sections for [(n, d) + (n, n′p) + (n, pn)] reactions induced by 14.7 ± 0.3 MeV neutrons on ⁴⁴Ca, ⁴⁹Ti, ⁵⁰Cr, ^{67, 68}Zn, ⁹²Zr and ^{97, 98}Mo have been measured by the activation technique using enriched isotopes as target materials, modern radiochemical separations and high-resolution counting methods. A brief summary of the literature data and our own earlier measurements is given. Our activation data are generally in agreement with those deduced from emitted charged particle characterisation. Some systematic trends in the activation cross-section data were analysed. Similar to other (n, charged particle) reactions, the [(n, d) + (n, n′p) + (n, pn)] reaction cross section decreases as a function of (N?Z)/A; the data, however, fall on two curves, one for nuclei with neutron separation energies (S_n higher than the proton separation energies (S_p) and the other for nuclei with S_n < S_p. For nuclei with S_n ? S_p the (n, n′p) process is very important. Detailed Hauser-Feshbach calculations show that in general contributions of statistical processes to the (n, d) reaction cross section are very small.     

Neutron-deficient and neutron-rich Fe and Ni isotopes near the drip line

Positions of the proton and neutron drip lines and characteristics of the neutron-deficient and neutron-rich Fe and Ni isotopes have been studied by the Hartree-Fock method with the Skyrme forces (Ska, SkM*, Sly4) with allowance for deformation. Pairing was taken into account on the basis of the BCS approximation with the pairing constant G = (19.5/2)[1 ± 0.51(N ? Z)/A]. Manifestation of magic numbers for the nickel isotopes ⁴⁸Ni, ⁵⁶Ni, and ⁷⁸Ni and for the nucleon-stable isotope ¹¹⁰Ni which is beyond the drip line is discussed.     

Evidence for deformed states in 75Br

The excited states in ⁷⁵Br have been studied via the reactions ⁷⁴Se(p, γ), ⁷⁴Se(d, n), ⁷⁴Se(³He, pn) and ⁷⁴Se(α, p2n) by using in-beam γ-ray spectroscopy. In addition to measurements of γ-γ coincidences, excitation functions and angular distributions of γ-rays, ns lifetime measurements have also been carried out. As a result 19 levels have been identified up to spin ($\text{17}\text{2}$) and excitation energies up to 2.6 MeV. The B(E2) value of 88 W.u. derived for the 88.4 keV γ-ray indicates strong collectivity within a positive-parity band. A comparison of the excitation energies of the unique-parity states in ⁷⁵Br and ⁷⁷Br with those in ¹⁵³Tb and ¹⁵⁵Tb reveals that the average deformation increases when going from ⁷⁷Br (N = 42) to ⁷⁵Br (N = 40).     

Shell structure of <Superscript>107,109</Superscript>Ag nuclei and spin–parities nuclei in which the 1<Subscript><Emphasis Type="Italic">g</Emphasis>9/2</Subscript> orbit is being filled

Occupation numbers and energies of proton and neutron orbits in the isotopes ¹⁰⁷Ag and ¹⁰⁹Ag were obtained on the basis of data on nucleon-stripping and nucleon-pickup reactions. A special data-analysis method reducing systematic and statistical uncertainties was applied in relevant calculations. It is shown that, in this region, the spin–parity of nuclei is determined by shells, pairing, and polarization. The schemes of proton and neutron (sub)orbits were constructed. These schemes explain the ground-state spin–parities of N, Z = 39–49 nuclei.     

Alpha decay of new neutron deficient gold,mercury, and thallium isotopes

In fusion evaporation reactions of a⁹²Mo beam with targets of neutron deficient Rb — Mo isotopes very neutron deficient isotopes of elements between Au and Po have been produced. The new isotopes^{173, 174}Au,^{175, 176}Hg, and¹⁷⁹Tl were identified by alpha spectroscopy. The mass excess value of¹⁷⁶Hg could be linked to known values of theN?Z=16 chain. The location of the new isotopes with respect to the proton drip line is discussed. A new high energyα transition of (7.20±0.02) MeV andT _1/2=(1.4±0.5) ms has been found in the reaction⁹²Mo+⁸⁹Y→¹⁸¹Tl^* at an excitation energy of 37 MeV. It is tentatively assigned to isotopes produced in 2-particle evaporation channels.