Slow-light optical bullets in arrays of nonlinear Bragg-grating waveguides

We demonstrate that propagation direction and velocity of optical pulses can be controlled independently in the structures with multiscale modulation of the refractive index in transverse and longitudinal directions. We reveal that, in arrays of waveguides with phase-shifted Bragg gratings, the refraction angle does not depend on the speed of light, allowing for efficient spatial steering of slow light. In this system, both spatial diffraction and temporal dispersion can be designed independently, and we identify the possibility for self-collimation of slow light when spatial diffraction is suppressed for certain propagation directions. We also show that broadening of pulses in space and time can be eliminated in nonlinear media, supporting the formation of slow-light optical bullets that remain localized irrespective of propagation direction.     

Elliptic X-shaped light bullets

Elliptic X-shaped light bullets, which are generated as nondiffraction elliptic Bessel-like beams with central humps of elliptical shape during the propagation of asymmetric input ultrashort pulses in normal dispersive quadratic media, are demonstrated to be quite stable against wave-packet breakup due to asymmetric input or anisotropic diffraction. Walking elliptic X-shaped light bullets can be observed without spatial wave-packet breakup for strongly coupled fundamental-wave and second-harmonic ultrashort pulses with nonvanishing group-velocity mismatch.     

Nearly diffraction-limited laser focal spot obtained by use of an optically addressed light valve in an adaptive-optics loop

We demonstrate correction of laser wave-front distortions by use of an adaptive-optical technique based on a light valve. The setup consists of an achromatic and adjustable-sensitivity wave-front sensor and a wave-front corrector relying on an optically addressed liquid-crystal spatial light modulator. Experimental results with strongly aberrated beams focused close to the diffraction limit are presented for the cw regime. Additional experiments with pulses and measurement of damage thresholds show that this approach is relevant for spatial phase correction of ultraintense laser pulses.     

Independent control over the amplitude,phase, and polarization of femtosecond pulses

We introduce a shaper setup which takes advantage of laser pulses passing through a spatial light modulator twice, thereby effectively utilizing a four-liquid crystal mask configuration. This approach grants control not only over the phase and polarization but also the amplitude. The Jones vector of the light wave after passing through the setup is considered in detail including polarization sensitive grating efficiency. A new method of counteracting the polarization dependent grating transmission is described and a comparison between the desired and recorded pulses is presented. PACS 42.25.Ja; 42.15.Eq; 42.65.Re     

Self-broadening of space-time spectra of few-cycle pulses in dielectric media

The nonparaxial dynamics of spectra of pulses comprising a few cycles of a light field is analyzed in transparent nonlinear media with dispersion. It is shown that the inhomogeneous self-broadening of the time spectrum of a pulse proceeds more effectively into the blue region at all spatial frequencies. A decrease in the energy in the central part of the time spectrum is realized mainly at high spatial frequencies.     

Holography of wave packets

We describe the principles of holographic storage and reconstruction of ultrashort light pulses using spectrally nonselective media. This can be achieved by the application of a 3-D recording medium and by the holography of waves produced by spatial spectral decomposition of light pulses. We also describe various transformations of optical temporal signals based on holographic spectral filtering and nonlinear interaction of spectral decomposition waves.     

Frequency doubling and Fourier domain shaping the output of a femtosecond optical parametric amplifier: easy access to tuneable femtosecond pulse shapes in the deep ultraviolet

Tuneable, shaped, ultraviolet (UV) femtosecond laser pulses are produced by shaping and frequency doubling the output of a commercial optical parametric amplifier (OPA). A reflective mode, folded, pulse shaping assembly employing a spatial light modulator (SLM) shapes femtosecond pulses in the visible region of the spectrum. The shaped visible light pulses are frequency doubled to generate phase- and amplitude-shaped, ultrashort light pulses in the deep ultraviolet. This approach benefits from a simple experimental setup and the potential for tuning the central frequency of the shaped ultraviolet waveform. A number of pulse shapes have been synthesised and characterised using cross-correlation frequency resolved optical gating (XFROG). This pulse shaping method can be employed for coherent control experiments in the ultraviolet region of the spectrum where many organic molecules have strong absorption bands. D.S.N. Parker and A.D.G. Nunn contributed equally to this work.     

All‐Optical Transmission Modulation Due to Inelastic Interactions of Ultrashort Pulses in a Disordered Resonant Medium

Random resonant media being one of the possible realizations of disordered metamaterials open a room of opportunities for achieving new fundamental effects and designing advanced nanophotonic devices. Strongly nonlinear optical properties of such media attract ever increasing attention nowadays from both theoretical and experimental points of view. Hereinafter, the case of the photonic‐crystal‐like structure with a randomly varying light–matter coupling provided by the random density of quantum particles is considered. Using numerical solution of the Maxwell–Bloch equations, the effects of the pulse collisions in the medium are studied. It is shown that disorder enables the qualitative changes of the system's response for co‐propagating pulses, whereas this is not the case for the counter‐propagating ones. The scheme for an all‐optical transmission modulation due to the disorder‐induced inelasticity of collisions of co‐propagating pulses is proposed. The ability of precise tuning the modulation via the inter‐pulse distance and background refractive index adjustment is revealed. This novel approach for light control can be utilized for some high demand applications, such as modulation and switching of a pulsed radiation.     

Shaping quantum pulses of light via coherent atomic memory

We describe proof-of-principle experiments demonstrating a novel approach for generating pulses of light with controllable photon numbers, propagation direction, timing, and pulse shapes. The approach is based on preparation of an atomic ensemble in a state with a desired number of atomic spin excitations, which is later converted into a photon pulse. Spatiotemporal control over the pulses is obtained by exploiting long-lived coherent memory for photon states and Electromagnetically Induced Transparency in an optically dense atomic medium. Using photon counting experiments, we observe Electromagnetically Induced Transparency based generation and shaping of few-photon sub-Poissonian light pulses.     

Electromagnetically induced transparency‐based slow and stored light in warm atoms

This paper reviews recent efforts to realize a high‐efficiency memory for optical pulses using slow and stored light based on electromagnetically induced transparency (EIT) in ensembles of warm atoms in vapor cells. After a brief summary of basic continuous‐wave and dynamic EIT properties, studies using weak classical signal pulses in optically dense coherent media are discussed, including optimization strategies for stored light efficiency and pulse‐shape control, and modification of EIT and slow/stored light spectral properties due to atomic motion. Quantum memory demonstrations using both single photons and pulses of squeezed light are then reviewed. Finally a brief comparison with other approaches is presented.     

Pulse propagation analysis based on the temporal Radon-Wigner transform

Based on the space-time duality and the temporal imaging theory, an optical implementation of the Radon-Wigner transform in the time domain is proposed for analyzing the propagation of ultrashort light pulses in guided dispersive media. As an application of this approach, we discuss the temporal selfimaging or Talbot effect originated by a periodic pulse train. The frequency chirp of the pulses is also considered in order to evaluate its effect on both the integer and the fractional selfimages.     

Spatial optimization of filaments

We demonstrate the spatial homogenization of intense laser pulses by adaptive minimization of spatial chirp of the spectrally broadened output pulses of a filament. A liquid-crystal-based two-dimensional spatial light modulator is used to control the spatial phase of the driver pulse. An evolutionary algorithm finds the optimal spatial laser phase distribution that introduces minimal distortions during filamentation and enhances the beam quality of the output pulse. A homogeneous intensity distribution favours efficient temporal compression close to the bandwidth limit without the need for spatial filtering after the filament. PACS 42.65.-k; 42.65.Re; 41.85.Ct     

19 fs shaped ultraviolet pulses

We report the generation of shaped tunable ultrashort ultraviolet pulses with full control over the spectral phase and amplitude. The output of a noncollinearly phase-matched optical parametric amplifier is shaped in phase and amplitude by a liquid-crystal spatial light modulator. The resulting structured visible pulses are transferred into the ultraviolet by sum-frequency mixing with strongly chirped 775 nm pulses. Single, double, and triple pulses at 344 nm with subpulses as short as 19 fs are explicitly demonstrated. The method can easily be adapted to arbitrarily shaped pulses throughout the 295-370 nm range.     

Pulse shaping control of alignment dynamics in N2

Control on the alignment transients of impulsively aligned ensembles of N₂ molecules has been demonstrated by the use of laser pulses shaped by a spatial light modulator. An alignment experiment has been inserted in the feedback loop of an evolutionary algorithm that found optimum pulse shapes for a set of criteria. Optimum pulse shapes for the maximization of total alignment and for the control of certain aspects of the revival structures are given. The physical mechanisms responsible for the control are analysed with the help of single‐parameter control schemes and numerical simulations, which allowed us to explore the low‐temperature region. This approach sheds light on the role played by different control mechanisms for the alignment dynamics of a molecular ensemble. Copyright © 2006 John Wiley & Sons, Ltd.     

Systematic study of highly efficient white light generation in transparent materials using intense femtosecond laser pulses

We report the results of a systematic study of white light generation in different high band-gap optical media (BaF₂, acrylic, water and BK-7 glass) using ultrashort (45 fs) laser pulses. We have investigated the influence of different parameters, such as focal position of the incident laser light within the medium, the polarization state of the incident laser radiation and the pulse duration of the incident laser beam on the white light generation. Our results indicate that for intense, ultrashort pulses, the position of physical focus inside the media is crucial in the generation, with high efficiency, of white light spectra over the wavelength range 400–1100 nm. Linearly polarized incident laser light generates white light with higher intensity in the blue region than circularly polarized light. Ultrashort (45 fs) pulses generate a flatter spectrum with higher white light conversion efficiency than longer (300 fs) pulses of the same laser power. We believe that a flat response over a wide range of wavelengths in the continuum may be efficiently compressed for generation of sub-10 fs pulses. PACS 52.38.Hb; 42.65.Jx; 42.65.Tg; 33.80.Wz; 52.35.Mw     

Controlling single-photon Fock-state propagation through opaque scattering media

The control of light scattering is essential in many quantum optical experiments. Wavefront shaping is a technique used for ultimate control over wave propagation through multiple-scattering media by adaptive manipulation of incident waves. We control the propagation of single-photon Fock states through opaque scattering media by spatial phase modulation of the incident wavefront. We enhance the probability that a single photon arrives in a target output mode with a factor 30. Our proof-of-principle experiment shows that the propagation of quantum light through multiple-scattering media can be controlled, with prospective applications in quantum communication and quantum cryptography.     

Breathing and beating dynamics of Gaussian beam in planar graded-index absorbing nonlinear waveguides

The spatial dynamics of laser beams in absorbing planar waveguides with a parabolic index profile in a saturable or cubic-quintic medium are calculated using the “collective variable approach” technique. In the absence of losses, we construct diagrams which define regions of self-focusing and self-diffractive beam propagation for both types of media. It is found that propagating pulses exhibit an oscillatory pattern, similar to breathing behavior in homogeneous media. If the incident pulse spatial profile and the center of the index profile are not aligned, the pulse oscillates around the index origin with a “beat” frequency that depends on the graded index. Both the breathing and the beat frequencies are also calculated for other graded-index profiles, such as those with additional higher-power terms, and are found to be extremely sensitive to the index profile. In media with linear and nonlinear absorption, we demonstrate the difference between the breathing behavior in graded-index and homogeneous waveguides.     

Generation of single dispersion precompensated 1-fs pulses by shaped-pulse optimized high-order stimulated Raman scattering

We propose and theoretically analyze a new approach for generating and shaping 1-fs pulses. It combines the ideas of strong-field molecular optics and optimal control to manipulate light generation in a pump-probe Raman regime. Flexible phase control over the generated spectrum of about 3 eV width is achieved by controlling the input pulses and maximizing the coherence of medium excitation by adiabatically aligning molecules in the medium with a specially shaped pump pulse. The generated pulse is optimized for an output window, precompensating for its dispersion to all orders.     

Hyperbolic shock waves of the optical self-focusing with normal group-velocity dispersion

The theory of focusing light pulses in Kerr media with normal group-velocity dispersion in (2+1) and (3+1) dimensions is revisited. It is shown that pulse splitting introduced by this dispersion follows from shock fronts that develop along hyperbolas separating the region of transverse self-focusing from the domain of temporal dispersion. Justified by a self-similar approach, this property is confirmed by numerical simulations using an adaptive-mesh refinement code.     

Few-cycle light bullets created by femtosecond filaments

We report a generic mechanism of light bullet formation during the filamentation of femtosecond pulses. This mechanism is tested for gaseous and dense media. It allows the production of robust, sub-10 fs structures of light with no post-compression stage. By coupling an infrared pump with a seed beam, tunable pulses with durations down to a few femtoseconds can be generated by parametric processes.