双轴晶体中二次谐波产生的最佳相位匹配条件

从二次谐波产生的理论出发，讨论了双轴晶体中二次谐波产生的相位匹配条件，推导了有效非线性光学系数的精确计算公式，以有机非线性光学晶体二苯甲酮为例，给出了对两种基波(1064μm和0808μm)二次谐波产生的相位匹配条件的数值模拟及相应的有效非线性光学系数的精确计算结果，并确定出相应的最佳相位匹配条件. 关键词： 二次谐波产生 最佳相位匹配 有效非线性光学系数 二苯甲酮晶体     

参变过程中的群速延迟对晶体匹配长度的影响

基于能量守恒和三波耦合波方程,建立了超短脉冲在参变过程中二次谐波产生时的I类和II类相位匹配条件、基波与谐波之间的群速延迟时间、以及群速失配对晶体长度限制的理论基础。以负单轴非线性光学晶体CsLiB6O10为例,分析和数值计算了超短脉冲宽度为100fs时,谐波的群速匹配长度随基波波长变化的规律。研究结果表明在I类相位匹配条件下,基波波长为642nm时,群速延迟最小,相应的群速匹配晶体长度最长为19.1mm;在II类相位匹配条件下,基波波长为767nm,群速延迟最小,群速匹配长度最长为0.89mm。     

非线性晶体中的非共线谐波

根据在非线性晶体中非共线谐波有效产生的相位匹配条件,导出了基波共线和非共线时可能产生的谐波环的解析表达式,给出了谐波环的大小与基波在晶体中传播方向的关系.对KDP和LiNbO_3晶体中的谐波环的变化进行了观测,实验结果与理论计算相符.     

相位畸变光束二次谐波的相位变化

研究了基波相位畸变对二次谐波相位分布的影响。针对具有不同像差、而光强分布为高斯型光束，以KDP晶体I类匹配为例，数值计算得到其二次谐波光束的光强分布和相位分布，分析了基波的像差、离散效率以及衍射效应的影响效果。研究表明不同的像差对于谐波的影响是不同的，主要取决于由其引起的全口径上相位失配的情况；离散效应主要带来的是倾斜像差，其高阶像差的影响随着离散效应的加剧而增大；而衍射效应的影响在一般情况下都是可忽略的。最后给出了在离散效应和衍射效应的影响可以忽略的情况下，基波相位畸变对二次谐波影响的近似估算式。     

二次谐波产生中入射啁啾脉冲对相位的影响

讨论了基波为叔率啁啾脉冲的二次谐波产生过程，结果表明选取合适的啁啾参量可以提高二次谐波的光强，但同时会使其波形和相位发生变化，三次相位的畸变主要取决于入射的基波啁啾脉冲，而与相位匹配的失谐量关系不大。     

二次谐波中大相位失谐下入射啁啾脉冲对相位的影响

讨论了在大相位失谐下,基波为频率啁啾脉冲的二次谐波产生过程,结果表明选取合适的啁啾参量可以使二次谐波的光强提高,但同时会使其波形和相位发生变化.三波相位的畸变主要取决于入射的基波啁啾脉冲,而与相位匹配的失谐量关系不大.     

基于反相位脉冲技术的生物组织谐波成像研究

理论及实验研究了反相位脉冲技术在生物组织二次谐波成像中的应用。结合有限振幅声波的非线性传播理论,从理论上证明了反相位脉冲技术可有效抑制基波信号,同时二次谐波信号增强两倍,轴向及径向声场的实验测量结果基波被抑制30～50dB,二次谐波提高6dB,与理论相符。建立了相应的成像系统,对若干生物离体组织进行了基于反相位脉冲相位技术的二次谐波成像,并与常规的基波及二次谐波图像对比,进一步证明了该技术能有效提高图像的对比度和清晰度。     

生物组织成像中用反相位脉冲技术提高二次谐波信噪比的研究

本文基于有限振幅声波在介质中的非线性传播理论,分析了反相位脉冲技术对生物组织中二次谐波增强的原理.实验中利用反相位脉冲激发超声换能器,对生物组织中传播的非线性信号相加分析.结果表明反相位脉冲技术可有效抑制基波及奇次谐波信号,而可增强偶次谐波信号6dB.与滤波器滤波法相比,反相位脉冲技术在抑制基波信号的同时,可有效地提高二次谐波的信噪比,因而在生物组织的二次谐波成像中具有广阔的应用前景.     

掺杂晶体Cd0.35Hg0.65Ga2S4的光学特性

研究了掺杂非线性晶体Cd0.35Hg0.65Ga2S4的线性和非线性光学特性以及相位匹配.在相同的实验条件下，与已知的中红外晶体相比较，测定了该晶体的损伤阈值.实现了CO2激光二次谐波产生实验，与理论预测相一致. 关键词： 掺杂非线性晶体 Cd0.35Hg0.65Ga2S4 二次谐波产生 CO2激光     

材料非线性衰减系数的二次谐波测量方法研究

采用有限幅值法测量材料在基波和非线性引起的二次谐波作用下的衰减系数:利用准线性下的KZK方程推导基波和二次谐波的声压分布,并提取波束修正系数;采用短纯音信号进行非线性实验,对检测得到的基波和二次谐波声压进行衍射修正处理,有效抑制衍射对衰减系数测量的不利影响,继而通过线性拟合的方法计算得到更精确的基波和二次谐波的衰减系数。以水为例进行实验,研究了实验测量所得衰减系数的频率依赖关系,结果表明在非线性条件下水的衰减系数与频率间存在较强的线性关系,而线性条件下衰减系数随频率呈现二次方增长的特性则不适用于非线性条件。该研究提出了准确测量非线性声波衰减系数的方法,为更有效地应用非线性超声检测提供理论依据。      

Controlling the second harmonic in a phase-matched negative-index metamaterial

Nonlinear metamaterials have been predicted to support new and exciting domains in the manipulation of light, including novel phase-matching schemes for wave mixing. Most notable is the so-called nonlinear-optical mirror, in which a nonlinear negative-index medium emits the generated frequency towards the source of the pump. In this Letter, we experimentally demonstrate the nonlinear-optical mirror effect in a bulk negative-index nonlinear metamaterial, along with two other novel phase-matching configurations, utilizing periodic poling to switch between the three phase-matching domains.     

利用各向同性半导体晶体差频产生可调谐THz辐射的理论研究

理论研究了利用剩余射线带色散补偿相位匹配原理，在Ⅲ-Ⅴ族和Ⅱ-Ⅳ族光学各向同性的半导体非线性晶体中差频产生可调谐THz波的可行性问题.根据这些半导体材料的色散特性，并以近简并点双共振KTP-OPO的可调谐相干双波长输出作为差频抽运源，对它们的相位匹配能力、差频增益特性、品质因数以及差频过程中的相干长度进行了理论分析和计算，确定了ZnTe晶体是在共线相位匹配情况下较为理想的THz波差频晶体，而InP晶体则更适合用于非共线相位匹配情况. 关键词： 非线性光学 THz辐射 差频 各向同性半导体晶体     

一种结构简单的二维左手材料设计及仿真研究

基于产生负介电常数的周期性金属线单元结构,讨论了金属线长度和宽度的变化对负介电常数的影响.在入射波的波矢k方向上放置两个单元结构,使两单元中的金属线响应入射波的磁场产生负磁导率,就可得到一维左手材料.若保持电边界条件的位置不变而调换波端口和磁边界条件位置,即入射波的波矢k转过90°角,两单元结构同样具有左手特性,从而可实现二维左手材料.     

Nonlinear magnetoinductive waves and domain walls in composite metamaterials

We describe novel physics of nonlinear magnetoinductive waves in left-handed composite metamaterials. We derive the coupled equations for describing the propagation of magnetoinductive waves, and show that in the nonlinear regime the magnetic response of a metamaterial may become bistable. We analyze modulational instability of different nonlinear states, and also demonstrate that nonlinear metamaterials may support the propagation of domain walls (kinks) connecting the regions with the positive and negative magnetization.     

Second harmonic generation of propagating collective excitations in Bose－Einstein condensates

We consider a possible second harmonic generation (SHG) of propagating collective excitations in a two-component Bose－Einstein condensate (BEC) with repulsive atom－atom interactions. We show that the phase-matching condition for the SHG can be fulfilled if the wave vectors and frequencies of the excitations are chosen adequately from different dispersion branches. We solve the nonlinear amplitude equations for the SHG derived using a method of multiple-scales and provide SHG solutions similar to those obtained for a SHG in nonlinear optical media. A possible experimental realization of the SHG for the propagating collective modes in a cigar-shaped two-component BEC is also discussed.     

Nonlinear phenomena of left-handed nonlinear split-ring resonators

We theoretically analyze a two-dimensional periodic structure consisting of period nonlinear split-ring resonators (SRRs) with varactor diode. The diode is loaded into the slit of the SRRs. Then, we demonstrate nonlinear phenomena of left-handed nonlinear SRRs. This paper introduces nonlinear SRRs based on left-handed (LH) media and simulates self-tuning mechanisms, bistable effects in the microwave frequency range. In addition, with the increase of input power, the nonlinear response of the SRRs becomes multi-valued, paving a way for creating bistable tunable metamaterials.     

基于双环开口谐振环对的平面周期结构左手超材料

通过理论分析和实验仿真,研究了用双环开口谐振环对（double split-ring resonator pairs,DSRRP）实现平面左手超材料的原理,用等效电路理论解释并描述了其负介电常数和负磁导率的产生机理,并对DSRRP在3维左手超材料设计的应用进行了探索性研究.结果表明,DSRRP可以实现小尺寸的平面左手超材料,此外,DSRRP还可以作为用以实现3维左手超材料负磁导率的3维各向异性磁超材料. 关键词： 双环开口谐振环对 平面左手超材料 3维磁超材料     

Optical second-harmonic generation in a thin-film waveguide without control of film thickness

An optical second-harmonic wave can be generated in a three-layered optical waveguide of arbitrary film thickness under phase-matching condition. Phase-matching is achieved by utilizing mode dispersion in an optical waveguide with a two-dimensional configuration. A numerical analysis of the matching condition is given and the results of the observation of the optical second-harmonic wave of a guided Nd : YAG laser in a Ti-indiffused LiNbO₃ nonlinear film are described.     

Negative-index metamaterials: second-harmonic generation, Manley–Rowe relations and parametric amplification

Second harmonic generation and optical parametric amplification in negative-index metamaterials (NIMs) are studied. The opposite directions of the wave vector and the Poynting vector in NIMs results in a “backward” phase-matching condition, causing significant changes in the Manley–Rowe relations and spatial distributions of the coupled field intensities. It is shown that absorption in NIMs can be compensated by backward optical parametric amplification. The possibility of distributed-feedback parametric oscillation with no cavity has been demonstrated. The feasibility of the generation of entangled pairs of left- and right-handed counter-propagating photons is discussed. PACS 78.67.-n; 42.65.Ky; 42.65.Lm     

Compensation for the thermal effect in the second-harmonic generation of a Q-switched nanosecond-kilohertz Nd:YVO4 laser

We report the quantitative relationship between the phase-matching condition and the surrounding temperature in a critical phase-matching second-harmonic generation of a Q-switched Nd:YVO₄ laser with a high repetition rate. The thermal effect can be effectively compensated for by appropriately changing the phase-matching angle with respect to the surrounding temperature of a nonlinear optical crystal. A stable wavelength conversion from the 1064 nm fundamental to the 532 nm second harmonic in a type-I critical phase-matching lithium triborate crystal is experimentally achieved and the corresponding conversion efficiency up to 70% is obtained.