Surface modification of polycrystalline oxides (V<Subscript>2</Subscript>O<Subscript>5</Subscript>, MoO<Subscript>3</Subscript>, and WO<Subscript>3</Subscript>) irradiated with high-power ion beams

The influence of a high-power ion beam on polycrystalline oxides (V₂O₅, MoO₃, and WO₃) is investigated. Oxide irradiation with ion beams with current densities of greater than ～30 A/cm² is established to initiate changes in the color of irradiated layers and lead to surface-layer particle melting. It is demonstrated that a distinctive feature of the interaction between a high-power ion beam and V₂O₅ is the formation of surface nanosheets and nanowires whose characteristic cross-sectional size and thickness are ～1 μm and up to ～40 nm, respectively. The nanosheets are generated near emerging surface cracks if the beam current density is ～100 A/cm². Possible mechanisms of surface nanostructures formation under the action of pulsed ion beams are discussed.     

Laser Accelerated, High Quality Ion Beams

Intense beams of protons and heavy ions have been observed in ultra-intense laser-solid interaction experiments. Thereby, a considerable fraction of the laser energy is transferred to collimated beams of energetic ions (e.g. up to 50 MeV protons; 100 MeV fluorine), which makes these beams highly interesting for various applications. Experimental results indicate very short pulse duration and an excellent beam quality, leading to beam intensities in the TW range. To characterize the beam quality and its dependence on laser parameters and target conditions, we performed experiments at several high-power laser systems. We found a strong dependence on the target rear surface conditions allowing to tailor the ion beam by an appropriate target design. We also succeeded in the generation of heavy ion beams by suppressing the proton amount at the target surface. We will present recent experimental results demonstrating a transverse beam emittance far superior to accelerator-based ion beams. Finally, we will discuss the prospect of laser-accelerated ion beams as new diagnostics in laser-solid interaction experiements. Special fields of interest are proton radiography, electric field imaging, and relativistic electron transport inside the target.     

Mössbauer study of Fe3+/Fe2+ ratio in amphiboles to search correlation with hydrogen isotope fractionation

New intense muon beams with flux several orders of magnitude higher than at present muon facilities would allow many novel experimental studies that were until now statistically not feasible. The investigation of the nuclear properties of short-lived nuclei using muonic atom spectroscopy would become possible. A feasibility study at RIKEN-RAL muon facility using the cold hydrogen film method to produce radioactive muonic atoms is in progress. A new surface ionization type ion source was recently installed to expand the variety of available ions. Encouraging experimental results were obtained with stable alkaline-earth and rare-earth isotope ions implanted in solid deuterium films. The latest results are reported in this paper.     

Microstructure of metals and alloys in the heat-affected zone produced by a high-power ion beam

The microstructure of heat-affected zones produced by high-power ion beams in Al, Cu, Ni, and AD1 and Monel alloys are investigated by optical and scanning electron microscopy and X-ray diffraction analysis. It is ascertained that the microstructure is divided into characteristic layers differing in terms of grain sizes and phase components. It is shown that the formation of the structural-phase states of each layer occurs in both solid and liquid phases under pulsed ion-beam treatment and depends on the irradiation parameters and the thermophysical characteristics of a target.     

The effect of working pressure on the chemical bond structure and hydrophobic properties of PET surface treated by N ion beams bombardment

Polyethylene terephthalate (PET) surface was bombarded by N ion beams at room temperature. Varying the working pressure of the ion beams, PET surfaces with different composition and properties were obtained. Characterization by X-ray photoelectron spectrometry showed that only on film surface, ester bonds, especially C-O bonds, were broken and N element chemical bonded with C. The influence depth was less than 5 nm because of the lower ion energy (about 10³ eV). Contact angle results revealed that with increasing the working pressure of ion beams, the contact angle of PET surface to pure water increased from 51° to 130°. With these results, one conclusion could be deduced that the hydrophilic and hydrophobic properties of PET surface could be influenced by N atom chemical bond with C, which in turn is controlled by the working pressure of N ion beams.     

Thermal erosion of metal surfaces under the action of fine-focused scanning electron beams

A model of thermal erosion of a metal surface under the action of low-energy fine-focused scanning electron beams is developed. Peculiarities of thermal erosion of a metal surface irradiated by these beams with a power of 1…10 kW are considered. The influence of the irradiation parameters on the intensity of carrying the substance from the surface is analyzed. It is shown that due to such beams, the coefficients of metal erosion reach values of 10³ atom/electron and even greater. This is characteristic of powerful submicrosecond electron and ion beams, but the efficiency of using their energy turns out to be much higher.     

高功率脉冲离子束的产生

 分析了高功率二极管中的双向流以及提高离子流产生效率的反射三极管、磁绝缘二极管和箍缩二极管工作原理,概述了高功率脉冲离子束研究进展及发展方向。     

Influence of the high-power ion-beam irradiation of a hydroxyapatite target on the properties of formed calcium phosphate coatings

The physical-mechanical of properties of biocompatible calcium phosphate coatings deposited onto titanium and silicon substrates from erosion materials, which are generated by irradiating hydroxyapatite (synthetic and natural) targets by means of the high-power pulsed ion beam of a Temp-4 accelerator, are investigated. A calculation technique for predicting the rate and energy efficiency of deposition using pulsed ion beams is proposed. Their characteristics are analyzed as applied to the formation of calcium phosphate coatings.     

M~2-factor of high-power laser beams through a multi-apertured ABCD optical system

Based on the generalized truncated second-order moments, an approximate analytical formula of the beam propagation factor M~2 of high-power laser beams passing through the optical system with multiple hard-edged apertures is deduced. Numerical examples of the beams passing through an aperture-spatial filter are enclosed, and the influences of amplitude modulations(AMs) and phase fluctuations(PFs) on the beam propagation quality of high-power laser beams passing through the multi-apertured ABCD optical system are considered and discussed. It is shown that PFs are able to degrade the beam propagation quality of laser beams more than AMs when the high-power laser beams passing through the aperture-spatial filter, furthermore, one or two aperture-lens optical systems configured appropriate aperture parameters are both able to upgrade the beam propagation quality of high-power laser beams. The M~2 factor of Gaussian beam passing through the multi-aperture optical system is a special case in this paper.     

Time-division-multiplexing laser seeded amplification in a tapered amplifier

We demonstrate time-division-multiplexing(TDM) laser seeded optical amplification in a diode laser amplifier. With an acousto-optic modulator we combine two seeding beams of different frequencies and inject them alternately in the time domain into the tapered amplifier(TA) chip at a switching speed of 200 ns. The output high-power dual frequency components from the TA are time separated. The TDM seeded TA works safely and efficiently, which is useful for compact precision measurement instruments such as optical clocks and atom interferometers.     

The geometry of CO on Ru(001): Evidence for bending vibrations in adsorbed molecules

As a test of the utility of the ESDIAD method (Electron Stimulated Desorption Ion Angular Distributions) in studies of the geometry of adsorbed molecules, the chemisorption of CO on Ru(001) has been examined. Data previously reported using UPS (ultraviolet photoemission spectroscopy) and EELS (electron energy loss spectroscopy) have indicated that CO is terminally bonded to the Ru surface through the C atom, with the CO axis perpendicular to the surface. The ESDIAD results for CO confirm this orientation; for all CO coverages in the temperature range 90 K to ~ 350 K, the angular distributions of O⁺ and CO⁺ ESD ions are centered about the surface normal. The widths of the ion beams are temperature dependent; for both O⁺ and CO⁺, the half widths at half maximum, α, of the ion cones are ~16° at 300 K, and ~12° at 90 K. This temperature dependence, coupled with a simple model calculation, indicates that the dominant factors contributing to the width of the ESD ion beams are the CO surface bending vibrations, i.e., initial state effects. Thus, the data suggest that both the directions and widths of ESDIAD beams are determined largely by the structure and dynamics of the initial adsorbed state.     

Defect-deformational surface layer instability as a universal mechanism for forming lattices and nanodot ensembles under the effect of ion and laser beams on solid bodies

The defect-deformational (DD) model of surface nanostructure formation under the effect of ion and laser beams is extended to an anisotropic case. The DD theory describes from a unified point of view simultaneous bifurcations in the dependences of grating orientation and period on the ion beam incidence angle, grating rotation, and transition to the formation of a nanodot structure, all of which have been recently observed during ion sputtering of Si. A nonlinear two-dimensional Kuramoto-Sivashinsky DD-equation (DDKS) that describes the formation of lamella-like structures and ordered hexagonal ensembles of nanodots upon normal incidence of ion and laser beams on solid bodies is obtained.     

Properties of calcium phosphate coatings deposited by high-power ion beam ablation plasma

Biocompatible hydroxyapatite coatings (Ca₁₀(PO₄)₆(OH)₂) are used in stomatology and orthopedic surgery as an original structure for production of medical materials. These coatings have been deposited on Si, Ti and VT15-alloy substrates from ablation plasma formed under the impact of pulsed high-power ion beams on a calcium phosphate ceramic target. The nanohardness, Young’s modulus, elastic recovery, adhesion of coatings to substrates, friction constant, and surface roughness were measured.     

Computer Simulation of High Power Ion Beams Interaction with Matter

When high-power ion beams (HPIB) collides with matter, it generates plasma with parameters of a wide range, staring with those well mastered in physics and gas discharge technologies and ending with those appropriate to such natural systems as star nucleus and thermonuclear systems in feasible power projects based on the controlled inertial thermonuclear synthesis. We are interested in a fairly wide range of beam power densities (from 1 GW/cm² to 10 TW/cm²). This paper describes one mathematical model in one dimension (a plane geometry is assumed) and one model in two dimensions (r- and z-coordinates). The models are completed by wide- range equations of state for real matter (construction materials) and supplemented with additional equations describing rheological, thermophysical, and optical properties of solid media under consideration (in various phase states from solid to plasma, including states of a strongly nonideal plasma). On the base of the continual approach, mechanical destruction of materials due to tensile strain generated by rarefaction waves is taken into account. In modeling the action of ion beams of moderate intensity (I < 10 GW/cm²) on metal targets, elastoplastic properties are taken into account, and in describing the action of ion beams with intensities I > 10 GW/cm² (in the two- dimensional model based on the large-particle technique) heat transfer, including radiational processes, is considered. Opportunities offered by contemporary computer simulation techniques in the field of interaction between HPIB and matter are demonstrated, in particular, a possibility of simulating hypervelocity impact with the help of HPIB has been shown and the necessary conditions have been determined. The results of our computer simulation may be interesting from the viewpoint of some technological applications of HPIB, for example, pulsed destruction and strengthening of construction materials, pulsed ion implantation and etc. [1].     

Effects of irradiation parameters on metal surface erosion by pulsed ion beams

Potential application of high-power ion beams of submicrosecond and microsecond durations with the initial particle energy from 50 to 1000 keV and power density 10⁷–10⁹ W/cm² to ensure metal surface erosion are investigated. Evaporation is treated as a major erosion mechanism and the erosion coefficient is taken as an efficiency indicator. Dependences of the erosion coefficients of several metals on beam parameters obtained via calculations using a technique based on the solution of thermal conductivity equation with phase transitions are presented. The ion species, their initial energy, current pulse duration and power density are used as the beam parameters controlling the result of irradiation. __________ Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 8, pp. 49–54, August, 2007.     

Technological sources of charged particles with plasma emitters

At present, ion and electron beams, extensively used in industry, usually have a small cross section. Presented are generators of ion and electron flows with a large cross section using plasma emitters. These devices have a wide range of currents and voltages and are designed for metallurgical treatment and microelectronics. The author discusses a technological source of ions based on the vacuum-arc excited by a constricted discharge electron-beam installation with a large cross-section beam for microelectronics technology, a high-power electron-energy complex for heat treatment of manufactured articles and a generator of a low-energy, high-current electron beam with a plasma anode     

Theory of ion reflection from amorphous surface at low glancing angles

A new theory of ion reflection from a smooth amorphous solid surface is developed. A continuous potential is introduced for describing the ion reflection from amorphous surfaces at low glancing angles. It is shown that the difference, between a true surface potential and a continuous one could be taken into account in terms of a correction factor, thus yielding a Fokker-Planck-type equation for a particle distribution in angle and transverse coordinate. Diffusion coefficients included in this equation are calculated with allowance for atom discrete positions and ion-electron collision effect. On the basis of the derived kinetic equation the angular and energy ion distributions in a reflected beam are analyzed. The presented theory, somewhat modified, can be used for describing ion reflection from a crystal surface as well.     

Propagation of high-power partially coherent fibre laser beams in a real environment

The propagation performance of high-power partially coherent fibre laser beams in a real environment is investigated and the theoretical model of a high-power fibre laser propagating in a real environment is established. The influence of a collimating system and thermal blooming is considered together with atmospheric turbulence and mechanical jitter. The laser energy concentration of partially coherent beams in the far field is calculated and analysed based on the theoretical model. It is shown that the propagation performance of partially coherent beams depends on the collimating system, atmospheric turbulence, mechanical jitter and thermal blooming. The propagation performance of partially coherent beams and fully coherent beams is studied and the results show that partially coherent beams are less sensitive to the influence of thermal blooming, which results in that the energy degeneration for partially coherent beams is only 50% of that for fully coherent beams. Both partially coherent beams and fully coherent beams become less sensitive to thermal blooming when the average structural constant of the refraction index fluctuations increases to 1.7 × 10^-14 m^-2/3. The investigation presents a reference for applications of a high-power fibre laser system.     

三束同步混合注入装置的研制,调试与初步应用

本文扼要地介绍了三束同步混合注入装置,给出离子束源、原子束源和电子束源的设计和调试结果,还给出三束动态混合调试结果及初步开展的动态混合离子注入工艺开发与应用情况。三束同步处理和电子束的活化作用是该装置的主要特点。     

Hydrogen depth profiling using18O ions

Nuclear resonant reaction analysis techniques for hydrogen depth profiling in solid materials typically have used¹⁵N ion beams at 6.40 MeV and¹⁹F ion beams at 6.42 MeV, which require a tandem accelerator. We report a new technique using an¹⁸O ion beam at a resonance energy of 2.70 MeV, which requires only a single stage accelerator. Improved values of the nuclear parameters for the 2.70 MeV (¹⁸O) and 6.40 MeV (¹⁵N) resonances are reported. The beam energy spread was investigated for different ions and ion charge states and found to scale with the charge state. Data obtained using atomic and molecular gas targets reveal the research potential of Doppler spectroscopy. Examples of hydrogen depth profiling in solid materials using¹⁵N and¹⁸O ion beams are presented.