自发参量下转换双光子场应用研究进展

文章介绍了自发能量下转换双光子场的概念,重点总结了自发参量下转换双光子场应用研究的进展状况,并对该研究领域的发展进行了展望。     

红外光谱辐射的绝对测量方法研究

本文探讨自发参量下转换双光子场的产生机理，研究了基于自发参量下转换相关双光子绝对测量红外光源辐射功率的原理和方法。     

Two-photon interference from separate pulses

Two-photon or biphoton interference has been studied extensively for CW and single pulse pumped spontaneous parametric downconversion (SPDC). In this paper we examine biphoton interference between amplitudes originating in different pump pulses. This novel effect arises from the coherence of the pump pulses. The interference has a natural interpretation in terms of indistinguishability of various Feynman alternatives.     

通信波长频率一致纠缠光源的频谱测量

本文利用光栅单色仪实现了对超短脉冲抽运周期极化磷酸氧钛钾晶体产生的通信波长频率一致纠缠光子源的频谱特性分析.测量到双光子的联合频谱呈正关联分布,为频率一致纠缠光源.信号光、闲置光中心波长分别为1574.4 nm和1574.9 nm,频谱宽度分别为35.3 nm和37.6 nm,双光子符合包络宽度约为3 nm.根据单光子频谱宽度与双光子符合包络宽度的比值可以得到双光子的频率纠缠参量R约为12,表征了信号光子与闲置光子之间具有较高的频率纠缠度.     

超短脉冲抽运下频率一致纠缠光源量子特性实验研究

利用自发参量下转换过程产生的频率纠缠光源在量子信息处理及相关领域中 具有十分重要的应用. 本文利用中心波长为792 nm, 脉冲宽度小于20 fs的脉冲激光源抽运满足II类准相位 匹配条件的周期极化磷酸氧钛钾晶体, 实验产生了偏振相互正交的频率一致纠缠光子对. 基于Hong-Ou-Mandel干涉仪的二阶量子符合干涉装置, 测量到该纠缠双光子对的干涉可见度约为42%, 表明其频率不可分特性较理想频率一致纠缠光源大大降低. 通过理论分析给出, 由于超短脉冲光源对应的宽频谱带宽影响, 相位匹配函数中的高阶色散项不再忽略, 从而导致纠缠光子对的频率不可分性减弱. 进一步利用实验参数给出的数值模拟结果与实验结果符合, 证实了脉冲抽运源带宽对频率一致纠缠光源的量子不可分特性的影响. 关键词： 频率一致纠缠 Hong-Ou-Mandel干涉测量 符合计数     

Biphotons,squeezing, and new states of light in polarization quantum optics

The concept of squeezing is discussed for multimode quantum light beams with consideration of polarization using the polarization gaugeSU (2) invariance of free electromagnetic fields. We separate the polarization and biphoton degrees of freedom from other ones, and consider uncertainty relations characterizing polarization and biphoton observables. As a consequence, we obtain a new classification of polarization states of light within quantum optics. We also discuss briefly some interrelations of our analysis with experiments related to some fundamental problems of physics.     

Evaluation of polarization entanglement generated by spontaneous parametric downconversion using photon number counting

Spontaneous parametric downconversion (SPDC) is widely used to generate entangled photon pairs; however, multi-pair emissions degrade the quality of the entanglement. We numerically evaluate polarization-entangled photon pairs created by SPDC. The effects of multi-pair emission events on the visibility of two-photon interference and on the fidelity (the probability overlap for ideal and real states) are analyzed using single-photon detectors that can count the number of incoming photons and discard multiphoton events. Compared with conventional threshold single-photon detectors, photon-number resolving single-photon detectors have higher fidelity for the same or lower visibility.     

Transverse compression of two-photon wave packets

A method for generating two-photon wave packets (biphotons) with a small width of the spatial intensity correlation function (correlation radius) has been considered. We propose to prepare a two-photon wave packet inhomogeneously broadened in the angle by means of spontaneous parametric down-conversion in an inhomogeneous crystal. Such biphotons are not diffraction limited; i.e., their correlation radius is much larger than the inverse width of the spatial spectrum. However, the correlation radius of such a biphoton decreases as the biphoton propagates in free space, and transverse compression occurs at a certain distance from the crystal; i.e., the biphoton becomes diffraction limited.     

周期极化铌酸锂中通信波段纠缠双光子的波长管理方法

理论研究了周期极化铌酸锂晶体中通过自发参量下转换产生的纠缠双光子的波长管理方法.简并自发参量下转换产生的单色偏振纠缠双光子的波长,可以通过调整晶体的极化周期或工作温度自由地调节,特别是在加工好的晶体中极化周期是确定的,因而调整晶体的工作温度更加便捷.对于双色偏振纠缠双光子来说,不需改变入射的泵浦光以及晶体的极化结构,仅通过调节晶体的工作温度就可以实现o光光子和e光光子波长的严格交换.     

Nonlocal pulse shaping with entangled photon pairs

Nonlocal shaping effects in the time or spectral profiles of an entangled photon pair emerging from a pulsed parametric down-converter are observed by spectrally or temporally filtering one of the twin beams. In particular, we demonstrate the appearance of fourth-order ("ghost") interference fringes in the spectrum of one beam conditioned by photodetection at the output of an unbalanced Michelson interferometer placed in the path of the other beam. The coherence time of the pump is the limiting factor for the sharpness of the details in the shaped biphoton spectrum.     

基于自发参量下转换源二阶激发过程产生四光子超纠缠态

目前,多光子纠缠态的制备大多通过线性光学器件演化自发参量下转换一阶激发过程产生的纠缠光子对得到.本文考虑由自发参量下转换源二阶激发产生四个不可区分的纠缠光子制备四光子超纠缠态的情况.通过几组分束器、半波片和偏振分束器等线性光学器件设计量子线路演化四光子系统,结合四模符合探测,可得到同时具有偏振纠缠和空间纠缠的四光子超纠缠态.     

Polarization States of Light and Their Quantum Tomography

The notion and main features of polarization states of light are discussed within the framework of classical and quantum optics. This notion is shown to be correctly defined for arbitrary light beams only within quantum optics by using the P-quasispin formalism developed earlier. Polarization states of quantum light are shown to be fully described by a polarization density operator (PDO) obtained via reducing the total field density operator. Theoretical foundations are given for quantum tomography of polarization states of light fields considered as a way of measuring PDO. Herewith, the main attention is paid to a method where proper polarization tomographic observables (PDO “measurers”) are used. The method is shown to be adequately formulated by means of quasi-spectral tomographic expansions of PDO in special operator bases (given by finite sums of partially orthogonal projectors), which determine probability distributions of tomographic observables as expansion coefficients. Matrix versions of such “tomographic” PDO representations are obtained. In particular, projections of these expansions on quasiclassical operator bases, determining polarization quasiprobability functions, are given. An example of experimental implementation of polarization tomography of unpolarized light (biphoton radiation with hidden polarization) is analyzed.     

Stationary generation of diode-pumped self-Raman Nd:YVO<Subscript>4</Subscript>/YVO<Subscript>4</Subscript> composite crystal laser

Output power dependences of composite Nd³⁺:YVO₄ Raman laser stationary generation on the longitudinal diode pump power are measured at different transmissions of the output mirror at the Stokes radiation frequency. The deviation of the measured dependences from linear is explained by the influence of thermal effects on both the overlap of the beams and diffraction losses. A method to estimate the laser and Stokes losses in the cavity and the parameters characterizing the overlap of the laser radiation with the pump and Stokes beams is proposed. A Stokes-component of power 2.1 W is obtained and corresponds to 12% diode-to-Stokes efficiency.     

Theory for quantum state of photon pairs generated from spontaneous parametric down-conversion nonlinear process

A theory is presented for the quantum state of photon pairs generated from spontaneous parametric down-conversion nonlinear process. In this theory, the influence of the final sizes of nonlinear optical crystals on optical eigenmodes is explicitly taken into consideration. It was found that these photon pairs are not in entangled quantum states. Polarization correlations between the signal beam and the idler beam are explained. It is also shown that the two photons generated from SPDC are not spatially separated, therefore the polarization correlation between the signal and idler beams is not an evidence for quantum non-locality. The text was submitted by the authors in English.     

Saturation of biphoton generation near atomic resonance

We have numerically investigated the biphoton generation rate as a function of several parameters in the spontaneous four-wave mixing in cold atoms.It has been found that the biphoton generation rate can easily reach saturation with the intensity of the coupling laser increasing.The saturation intensity is mainly dependent on the dephasing rate of the ground states,unrelated to the pumping laser.It implies that though the biphoton waveform can be manipulated by the coupling laser,the generation rate of the biphoton cannot increase markedly after the saturation.The saturation effect also suggests that there is an optimal coupling laser for obtaining the largest biphoton generation rate with a sufficiently long coherence time.     

Space-adjustable dark magneto-optical trap for efficient production of heteronuclear molecules

We present a simple, robust, space-adjustable dark magneto-optical trap(MOT) for the efficient production of heteronuclear molecules. Double-mixed beams made up of repumping beams and depumping beams propagate in nearly opposite directions in the dark MOT. This optical arrangement can easily adjust the spatial positions of two clouds by changing the power ratio of the two repumping beams, and ensure a good overlap, which is very necessary for the production of heteronuclear molecules. The imaging of cold atoms by camera and the collisioninduced loss rate obtained by recording the loading curve of the cold atoms show that we obtain a perfect overlap of atom clouds. The number of Rb Cs molecules with the double-mixed beams is improved by 70%, which is higher than the one with the single-mixed beam.     

Spontaneous parametric down-conversion

Spontaneous Parametric Down-Conversion (SPDC), also known as parametric fluorescence, parametric noise, parametric scattering and all various combinations of the abbreviation SPDC, is a non-linear optical process where a photon spontaneously splits into two other photons of lower energies. One would think that this article is about particle physics and yet it is not, as this process can occur fairly easily on a day to day basis in an optics laboratory. Nowadays, SPDC is at the heart of many quantum optics experiments for applications in quantum cryptography, quantum simulation, quantum metrology but also for testing fundamentals laws of physics in quantum mechanics. In this article, we will focus on the physics of this process and highlight a few important properties of SPDC. There will be two parts: a first theoretical one showing the particular quantum nature of SPDC, and the second part, more experimental and in particular focusing on applications of parametric down-conversion. This is clearly a non-exhaustive article about parametric down-conversion as there is a tremendous literature on the subject, but it gives the necessary first elements needed for a novice student or researcher to work on SPDC sources of light.     

Control of the spectrum of the biphoton field

The main methods for controlling the biphoton field, as well as the problems for which the width and the shape of the spectrum of the biphoton field are of decisive importance, are discussed. The method for controlling the spectrum of the spontaneous parametric downconversion of light based on the spatial modulation of the refractive indices of a nonlinear crystal in which the generation of biphotons has been analyzed. Modulation is due to the thermo-optic and electro-optic effects.     

Time-bin-modulated biphotons from cavity-enhanced down-conversion

We have generated a new type of biphoton state by cavity-enhanced down-conversion in a type-II phase-matched, periodically poled KTiOPO4 crystal. By introducing a weak intracavity birefringence, we obtained signal and idler photons whose quantum interference was modulated between singlet and triplet signatures according to their arrival-time difference. This cavity-enhanced biphoton source is spectrally bright, yielding a single-mode fiber-coupled coincidence rate of 0.7 pairs/s per mW of pump power per MHz of down-conversion bandwidth.     

Spontaneous parametric down-conversion

Spontaneous parametric down-conversion (SPDC) in media with no inversion center and the use of this phenomenon in the spectroscopy of natural oscillation states of a crystal lattice (i.e., optical phonons) are retrospectively described. We think that the SPDC spectroscopy method is estimated inappropriately and hope to again attract the attention of readers to one of the most interesting quantum phenomena of nonlinear optics that has no classical analog. The capabilities of SPDC spectroscopy will certainly be used in both fundamental science and technology of new materials.