Angular dependence of coercivity and remanence of Ni nanowire arrays and its relevance to magnetoviscosity

Ni nanowire arrays with varying wire dimensions (diameter d, length l) and center-to-center distances d_CC were synthesized by pulsed electrodeposition of Ni in porous Al templates. The magnetization-reversal behavior of the arrays was investigated by means of magnetometry for different angles θ between the wire axes and the applied magnetic field. The functional dependences of the characteristic parameters coercivity H_C(θ) and reduced remanence m_R/m_S(θ) exhibit a strong dependence on the wire dimensions and the center-to-center distance. For instance, for nanowire arrays with d=40 nm, d_CC=100 nm, and for θ=0°, the coercivity takes on a rather large value of μ₀H_C=85 mT and m_R/m_S≅94%; reducing d_CC to 30 nm and d to 17 nm results in μ₀H_C=49 mT and m_R/m_S≅57%, an observation which suggests an increasing magnetostatic interwire interaction at increased (d/d_CC)-ratio. The potential application of nanowires as the constituents of ferrofluids is discussed.     

Tunneling magnetoresistance in exchange-biased CoFeB/AlOx/Co/IrMn junctions

A series of exchange-biased magnetic tunneling junctions (MTJs) were made in an in-plane deposition field (h) = 500 Oe. The deposition sequence was Si(1 0 0)/Ta(30 Å)/CoFeB(75 Å)/AlO_x(d Å)/Co(75 Å)/IrMn(90 Å)/Ta(100 Å), where d was varied from 12 Å to 30 Å. The MTJ was formed by the cross-strip method with a junction area of 0.0225 mm². The tunneling magnetoresistance (ΔR/R) of each MTJ was measured. The high-resolution cross-sectional transmission electron microscopic (HR X-TEM) image shows the very smooth interface and clear microstructure. X-ray diffraction (XRD) demonstrates that the IrMn layer of the MTJ exhibits a (1 1 1) texture. From the results (ΔR/R) increases from 17% to 50%, as d increases from 12 Å to 30 Å. The tunneling resistance (R_o) of these junctions ranges from 150 Ω to 250 Ω. The exchange-biasing field (H_ex) of the MTJ is 50-95 Oe. Finally, the saturation resistance (R_s) was measured as a function of the angle (α) of rotation, where α is the angle between h and the in-plane saturation field (H_s) = 1.1 kOe. The following figure presents the dependence of R_s on α, instead of originally expected independence, the curve actually varies with a period of π.     

Semimetallic electrical transport in PbTe-SnTe superlattices on KCl substrate

The electrical resistivity and Hall coefficient (R_H) in PbTe-SnTe superlattices on KCl are measured between 4.2 and 300 K. Magnetic field dependence of R_H shows a sign inversion of R_H for a specimen of PbTe-SnTe with 100-50 A at 5 K. This is due to coexistence of electrons and holes. PbTe-SnTe superlattices are of type II, where the valence band edge of SnTe is higher than the conduction band edge of PbTe. From the magnetic field dependence of R_H, the electron and hole concentrations are calculated and the band-offset between PbTe and SnTe is estimated. The possibility of the structural phase transition of these superlattices is also discussed.     

First-order intertwining operators and position-dependent mass Schrödinger equations in d dimensions

The problem of d-dimensional Schrödinger equations with a position-dependent mass is analyzed in the framework of first-order intertwining operators. With the pair (H, H₁) of intertwined Hamiltonians one can associate another pair of second-order partial differential operators (R, R₁), related to the same intertwining operator and such that H (resp. H₁) commutes with R (resp. R₁). This property is interpreted in superalgebraic terms in the context of supersymmetric quantum mechanics (SUSYQM). In the two-dimensional case, a solution to the resulting system of partial differential equations is obtained and used to build a physically relevant model depicting a particle moving in a semi-infinite layer. Such a model is solved by employing either the commutativity of H with some second-order partial differential operator L and the resulting separability of the Schrödinger equation or that of H and R together with SUSYQM and shape-invariance techniques. The relation between both approaches is also studied.     

Canonical realizations of the lie algebras gl(n, R) and sl(n, R) I. Formulae and classification

The generators of the Lie algebra of the general linear group GL(n, R) and of the special linear group SL(n, R) are, recurrently, expressed through polynomials in the quantum canonical variables p_t and q_t. These realizations are skew-Hermitian, the Casimir operations are realized by constant multiples of identity element and, in dependence on the number of the canonical pairs used, they depend on d(d?1 for sl (n,R)), d = 2, …, n, free real parameters.     

Cu induced coercivity enhancement in the low viscosity GdCo5−xCux system

We investigate the influence of Cu substitution, on the coercivity and magnetic viscosity, in the ternary system GdCo_5−xCu_x (x=0, 0.5, 1, 1.5, 2 and 2.5) with different field sweep rates. All samples have been studied in the as cast state and crystallize in a single phase CaCu₅ structure. With Cu addition, the coercivity was 10 times enhanced for x =1.5. The behavior of the coercivity H_c against field sweep rate, dH/dt, shows that the GdCo_5−xCu_x system exhibits only a small magnetic viscosity effect, a desirable property for magnetic dynamic applications under high magnetic field.     

Electron transport,penetration depth,and the upper critical magnetic field in ZrB<Subscript>12</Subscript> and MgB<Subscript>2</Subscript>

We report on the synthesis and measurements of the temperature dependences of the resistivity ρ, the penetration depth λ, and the upper critical magnetic field H_c2, for polycrystalline samples of dodecaboride ZrB₁₂ and diboride MgB₂. We conclude that ZrB₁₂ behaves as a simple metal in the normal state with the usual Bloch-Grüneisen temperature dependence of ρ(T) and with a rather low resistive Debye temperature T_R = 280 K (to be compared to T_R = 900 K for MgB₂). The ρ(T) and λ(T) dependences for these samples reveal a superconducting transition in ZrB₁₂ at T_c = 6.0 K. Although a clear exponential λ(T) dependence in MgB₂ thin films and ceramic pellets was observed at low temperatures, this dependence was almost linear for ZrB₁₂ below T_c/2. These features indicate an s-wave pairing state in MgB₂, whereas a d-wave pairing state is possible in ZrB₁₂. In disagreement with conventional theories, we found a linear temperature dependence, of H_c2(T) for ZrB₁₂ (H_c2(0) = 0.15 T).     

Critical state of Josephson medium

A model of the critical state of a Josephson medium is developed on the basis of the Sonin theory of averaged Josephson medium. The model is used to explain the experimental data on the differential magnetic susceptibility _χd (H) and magnetoresistance R(H) of polycrystalline YBa₂Cu₃O_7?x samples in fields H<100 Oe.     

Evidence for a change of state in lithium tetra-ammine below 77 K

Using a novel modification of the standard crossed-coil helicon method, we have investigated the temperature dependence of the Hall coefficient, R_H, of the metal-ammonia compound lithium tetra-ammine, Li(NH₃)₄. When cooling from 77 K, there is a discontinuous change in R_H of 25 per cent near 64 K. This may be evidence of a new low temperature phase.     

Magnetizing process in R-Fe-B sintered permanent magnets studied on boron-rich R17Fe83−xBx magnets (R = Pr,Nd)

Minor loop coercivity (H_c) and remanent induction (B_r) of sintered R₁₇Fe_83−xB_x magnets are studied as a function of magnetizing field (H_M) and temperature for x = 8, 30 and 35. The boron-rich magnets (x = 30 and 35) are constituted of R₂Fe₁₄B hard-magnetic grains separated by paramagnetic R_1+ϵFe₄B₄ phases. A distribution of local demagnetization field is considered to be the principal origin of the observed dependence of H_c and B_r on H_M. Domain walls experience an energy barrier near grain boundary regions in the R-Fe-B magnets when they are driven to the regions by external magnetizing force. The barrier originates from large magnetostatic energy created by the local demagnetization fields created on sharp corners of R₂Fe₁₄B grains rather than the anisotropy energy.     

A diffusion model of chain-branching reaction of the explosive decomposition of heavy metal azides

A diffusion model of a solid-phase chain reaction of explosive decomposition of heavy metal azides was developed. The dimensional effects of initiation of the reaction were examined: the dependence of the critical fluence of initiation on the microcrystal size H(R) and on the irradiated zone diameter H(d). It was demonstrated that the diffusion model of the chain reaction closely describes the measured H(R) dependence at diffusion coefficients of D ∼ 0.2–0.3 cm²/s, values that correspond to experimentally measured mobility of electronic charge carriers of μ ∼ 10 cm²/(V s). To account for the measured H(d) dependence and the reaction front propagation velocity (V = 1.2 km/s), it is necessary that the diffusion coefficient be three orders of magnitude higher than the experimentally determined value. That the H(R) and H(d) dependences cannot be quantitatively described simultaneously is indicative of the underlying mechanisms of energy transfer being different.     

Epitaxial LSMO films grown on MgO single crystalline substrates

The manganite La_0.67Sr_0.33MnO₃ (LSMO) layers are deposited on single crystal MgO(0 0 1) substrates using a magnetron dc sputtering. The crystalline perfection of the layers, both the as-prepared and the annealed, are characterized by X-ray diffraction technique, rocking curve measurements, Rutherford backscattering spectroscopy (RBS) and transmission electron microscopy (TEM). TEM analyses give evidence of the epitaxial growth of the annealed LSMO with a nanocrystalline surface layer. The temperature dependence of resistance in the 77-340 K range is measured by a standard four-probe technique. While the as-prepared film does not show any transition from paramagnetic to ferromagnetic state, the film annealed in oxygen shows steep R(T) dependence with a peak at 330 K and maximal slope (dR/dT) at 290 K where the maximal sensitivity is 3% K⁻¹.     

Magnetic field penetration into the weak-link system of the YBa<Subscript>2</Subscript>Cu<Subscript>3</Subscript>O<Subscript>7−<Emphasis Type="Italic">x</Emphasis></Subscript> granular superconductor

The differential magnetic susceptibility χ_d(H) of YBa₂Cu₃O_7?x polycrystalline samples is studied experimentally in fields H<150 Oe. The empirical χ_d(H) dependence is determined. The results are explained on the basis of the critical-state model of a Josephson medium with hypervortices.     

Non-planar spin texture driven dissipation in a ferromagnet-superconductor bilayer

We report the observation of a pronounced dip in the in-plane magnetic field (H_∥) dependence of the critical current density J_c(H) and a peak in resistance R(H) of a NbN-HoNi₅ bilayer at temperatures below the magnetic ordering temperature (T_Curie ≈ 3.5 K) of HoNi₅, which is lower than the onset temperature (≈9 K) of superconductivity in the NbN layer. The extrema in J_c(H) and R(H) appear at fields much below the upper critical field of NbN. We attribute these features to a coupling between localized out-of-plane moments present in the magnetic film and Pearl vortices of the superconducting layer. A spin re-orientation transition of the localized moments by H_∥ breaks this coupling, leading to the observed excess dissipation.     

Magnetoresistance hysteresis in granular HTSCs as a manifestation of the magnetic flux trapped by superconducting grains in YBCO + CuO composites

Hysterestic behavior of the magnetoresistance of granular HTSCs and its interaction with the magnetic hysteresis are studied by measuring magnetoresistance R(H) and critical current I _c(H) of composites formed by HTSC Y_0.75Lu_0.25Ba₂Cu₃O₇ and CuO. A network of Josephson junctions is formed in such composites, in which the nonsuperconducting component plays the role of barriers between HTSC grains. Hysteretic dependences R(H) of magnetoresistance are studied in a wide range of transport current density j and are analyzed in the framework of the two-level model of a granular superconductor, in which dissipation takes place in the Josephson medium and the magnetic flux can be pinned both in grains and in the Josephson medium. The interrelation between the hysteresis of critical current I _c(H) and the evolution of the hysterestic dependence R(H) of the magnetoresistance upon transport current variation is demonstrated experimentally. The effect of the magnetic past history on the hysteretic behavior of R(H) and the emergence of a segment with a negative magnetoresistance are analyzed. It is shown for the first time that the R(H) dependences are characterized by a parameter that is independent of the transport current, viz., the width of the R(H) hysteresis loop.     

Bonding and composition diagrams for sputtered a-Si : H

The combined influence of H partial pressure (p_H) and deposition rate (R_D) on Si-H bonding and total H content in diode-sputtered a-Si : H is presented in two simple graphs for the case of substrate temperature (T_s) equal to 225°C. Similar to a phase diagram, the graphs predict the H content and Si-H bonding that will result if a deposition is carried out with any prescribed pair of values (p_H, R_D), where 0.04 < p_H < 10 Paand 0.01 < R_D < 1 nm/sec. Well defined regions of Si-H bonding represented by dominant infrared stretching absorptions at 2000, 2090 and 2150 cm^?1 are obvious in the bonding diagram. The absorption at 2090 cm^?1 is the most commonly observed and is obtainable over a wide range of intermediate values of p_H and R_D. The absorption at 2000 cm^?1 is dominant only for the lowest p_H and the highest R_D. The absorption at 2150 cm^?1 is dominant in films deposited at high p_H and low R_D. The composition diagram shows that highest total H content is obtained for low R_D and high p_H, and lowest total H content results for high R_D and low p_H     

不同分子取向下氢分子非次序双电离对核间距的依赖关系

利用三维经典系综模型研究了氢分子非次序双电离对核间距的依赖性.在不同分子取向下,氢分子双电离率随核间距的增大而先增大后减小,在核间距为4a.u.时取最大值.氢分子非次序双电离对核间距的依赖性随分子轴与激光偏振方向间夹角φ的增大而减弱.φ=0时,氢分子非次序双电离包含丰富的相关模式,对核间距有强烈的依赖性φ=π/2时,不同核间距下的相关模式相似,重碰撞在双电离过程中发挥更重要的作用.这些结果表明分子结构对双原子分子非次序双电离有重要影响. 关键词： 非次序双电离 核间距 关联动量分布     

A simple approach to the First Order Reversal Curves (FORC) of two-phase magnetic systems

The features that commonly appear in the First Order Reversal Curves (FORC) of magnetic composites, consisting of a hard and a soft phase, are reproduced by a simple mean-field approach in the limit of weak coupling. In this case the features corresponding to each phase are distinct and the effect of the interactions appears as biasing field on the soft phase and a coercivity reduction of the hard one. Interactions produce additional twin (positive/negative) interference features in the region of the (H, H_R) FORC diagram where there is a strong dependence on H through the soft phase and on H_R through the hard phase. The slope and the intensity of these twin features depend on interaction strength.     

Effect of carrier concentration on the reflectivity spectrum of Ge and InSb

We have measured at 5 K the derivative spectra (1/R) dR/dE around the E₁ and E₁ + Δ₁ structures, of Ge and InSb with different impurity concentrations. In the more highly doped samples, the peaks are broadened and shifted slightly to lower frequencies. The change in the value of (1/R) dR/dE is much larger than recently predicted by Seraphin and Aspnes, based on the surface field effect. Different possibilities for the effect are discussed. Wavelength modulation measurements on samples with an applied surface electric field have shown no difference.     

Dimensionality of a system of exchange-coupled grains and magnetic properties of nanocrystalline and amorphous ferromagnets

Characteristics of random magnetic anisotropy in ferromagnetic films of amorphous Co₉₀P₁₀ and nanocrystalline Ni₇₅C₂₅, Fe₈₀B₄C₁₆, and Co₈₀C²⁰ alloys and also in multilayer films [Co₉₃P₇(x)/Pd(14 Å)]₂₀ and [Co₉₀P₁₀(x)/Pd(14 Å)]₂₀ obtained by various technological procedures were studied experimentally. It was found that the spatial dimensionality (d) of the system of ferromagnetically coupled grains (2R _c ) in the materials under study determined the exponent in the power dependence of the approach of magnetization to saturation in the region of fields H<2A/MR _c ² . The dependence ΔM～H ^?1/2 was observed for nanocrystalline and amorphous films with a three-dimensional grain arrangement. The approach to saturation in multilayer films with a two-dimensional grain arrangement in an individual magnetic layer follows the law ΔM～H ^?1. The main micromagnetic characteristics of random anisotropy, such as the ferromagnetic correlation radius R _f and the average anisotropy 〈K〉 of a ferromagnetic domain with a size of 2R _f , were determined for multilayer Co/Pd films. Correlation was found between the coercive field and these characteristics of random anisotropy.