Single-particle and core-excited states in 49Sc: (I). The 48Ca(3He,d)49Sc reaction

The ⁴⁸Ca(³He, d)⁴⁹Sc reaction has been studied at 25 MeV incident energy. Angular distributions have been measured from 5° to 40° using a split-pole spectrometer, for about 160 levels located up to 18 MeV excitation energy. A local zero-range DWBA analysis has been carried out, using Gamow functions as form factors in the case of unbound states; l-assignments and spectroscopic factors are obtained for a large number of levels, most of them previously unknown. The summed experimental spectroscopic strengths for the T_<, l = 1 and l = 3 levels are in good agreement with the shell-model sum-rule limits for 1f-2p proton states, and their energy centroids have been determined. The $\text{lg}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}$ strength in ⁴⁹Sc is strongly fragmented: about 27% of the T_< strength is carried by twenty-three levels located between 6.5 and 13.5 MeV. Spectroscopic factors for analog states are compared with those from previous (p, p), (³He, dp) and (d, p) experiments.     

The 16O(d, 3He)15N reaction at 29 MeV: Reaction mechanism and nuclear structure

The reaction ¹⁶O(d, ³He)¹⁵N has been investigated using 29 MeV deuterons, and angular distributions were obtained for levels in ¹⁵N up to 10 MeV excitation energy. The measured distributions were subjected to distorted-wave (DWBA), compound nucleus (Hauser-Feshbach) and coupled-channel (CCBA) analyses. Only the strong transitions to the $\text{1}\text{2}$^? ground state and the $\text{3}\text{2}$^? state at 6324 keV exhibit distributions which are well described by DWBA. The spectroscopic factors are in agreement with shell-model estimates. The weak transitions generally show little structure and the spectroscopic factors extracted for these transitions tend to be unreasonably large. Contributions from compound nucleus formation were estimated and found to vary between about 10 % and 100 % of the observed cross sections with an average of the order of 30 %. The CCBA analysis for the transitions to the $\text{5}\text{21}{}^{\mathrm{+}}$, $\text{5}\text{22}$⁺ and $\text{7}\text{2}$⁺ states at 5271, 7155 and 7566 keV, respectively, was performed using the spectroscopic amplitudes from weak coupling shell-model wave functions. Inelastic excitations to one-phonon states in the target and residual nuclei were included. The agreement between calculated and experimental distributions is good for both shape and magnitude, a conclusion which is not disturbed by the addition of small compound nucleus contributions. It is evident that spectroscopic factors extracted for the weak transitions on the basis of a direct one-step reaction mechanism alone are unreliable.     

Single-particle and core-excited states in 49Sc: (II). The 48Ca(α, t)49Sc reaction

The ⁴⁸Ca(α, t)⁴⁹Sc reaction has been studied at 36 MeV incident energy. About eighty levels have been observed up to 7.5 MeV excitation energy and angular distributions were measured from 6° to 58°, using a split-pole spectrometer. A local zero-range DWBA analysis has been carried out, and the deduced l-assignments and spectroscopic factors are compared with those obtained from the (³He, d) reaction. In the other hand, a large number of angular distributions cannot be reproduced by the DWBA calculations; they have been compared with the results of coupled-reaction-channel calculations, assuming two-step excitation of weak coupling states with a [${}^{48}\text{Ca}{}^1\text{?}\text{f}{}_{\mathrm{<mtext>7</mtext><mtext>2</mtext>}}$] structure. Good agreement between experimental angular distributions and two-step predictions is obtained for several ⁴⁹Sc levels, suggesting spin and parity assignments. Moreover, as rather large cross sections are predicted for two-step excitations, it is concluded that, generally, these processes cannot be neglected in the analysis of (α, t) reactions.     

A survey of the (3He, 7Be) reaction at 70 MeV

A study of the (³He, ⁷Be) reaction has been undertaken using a 70 MeV ³He beam. By surveying a wide range of target nuclides, namely ^{12, 13}C, ¹⁶O, ^{24, 26}Mg, ^{40, 42, 44}Ca, ^{58, 60, 62, 64}Ni, ⁹⁰Zr, ^{120, 124}Sn, ¹⁴⁴Sm and ²⁰⁶Pb, systematics of the α-clustering phenomenon were investigated. In addition, masses and energy levels of ⁶⁰Fe and ¹²⁰Cd were measured. The ⁷Be particles were detected in a single wire proportional counter backed by a plastic scintillator in the focal plane of an Enge spectrometer to ensure adequate particle identification. Total energy resolution as small as 140 keV full width at half maximum was obtained, although in most cases the target thickness limited the energy resolution to larger values. Differential cross sections as low as 20 nb/sr were measured. The finite range programs LOLA and LOLITA were used to calculate differential cross sections for comparison to data, assuming the reaction to proceed by a direct α-transfer. The spectroscopic factors which were extracted show a marked decrease with increasing atomic mass number, implying a decrease in surface α-clustering for heavier nuclei.     

Cross section measurements and thermonuclear reaction rates for 48Ca(p, γ)49Sc and 48Ca(p,n)48Sc

Absolute cross sections have been measured for the reaction ⁴⁸Ca(p, γ)⁴⁹Sc for 0.579 MeV ≦ E_{p, lab} ≦ 2.670 MeV and for the reaction ⁴⁸Ca(p, n)⁴⁸Sc for 0.956 MeV ≦ E_{p, lab} ≦ 2.670 MeV. Substantial competition effects in the cross section for ⁴⁸Ca(p, γ)⁴⁹Sc were observed at the thresholds for neutron emission to the 623 keV (3⁺), 1143 keV (2⁺) and 1402 keV (2^?) excited states of ⁴⁸Sc. Thermonuclear reaction rates were calculated from the measured cross sections for 0.1 ≦ T₉ ≦ 10.0. The new rates differ considerably from those used in earlier calculations of the production of the rare, neutron-rich intermediate mass nuclides during explosive carbon burning. In particular, the new rates may change the predicted abundances for ⁴⁸Ca, ^{49, 50}Ti and ⁵⁰V substantially. The good agreement between current global Hauser-Feshbach models and the experimental data indicates that Hauser-Feshbach calculations can provide sufficiently reliable rates for astrophysical calculations in cases where experimental data are non-existent.     

The 208Pb(α, 3He)209Pb reaction at 58 MeV

The ²⁰⁸Pb(α, ³He)²⁰⁹Pb reaction at 58 MeV has been used to search for high-spin states in ²⁰⁹Pb. Only three levels are excited with appreciable intensity: the ground state $\text{(2}\text{g}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}\text{)}$ and levels at $\text{0.781 (}\text{li}{}_{\mathrm{<mtext>11</mtext><mtext>2</mtext>}}\text{)}\text{and}\text{1.426}\text{MeV}\text{(}\text{lj}{}_{\mathrm{<mtext>15</mtext><mtext>2</mtext>}}\text{)}$. The angular distributions for these levels have been measured and analyzed using standard DWBA calculations to obtain spectroscopic strengths. The ²⁰⁸Pb(α, α) elastic scattering was measured and optical parameters deduced from the data. A normalization value N = 50 yields spectroscopic values which are close to the values measured in the (d, p) reaction. The (α, ³He) reaction should easily pick out any appreciable components of the $\text{j}{}_{\mathrm{<mtext>15</mtext><mtext>2</mtext>}}$ shell model state, which weak-coupling calculations predict should be fragmented. However only three weak transitions previously seen in a (d, p) experiment are observed.     

The (He, t) reaction at intermediate energies : Spin-isospin multipole transitions

Data for the (³He, t) reaction at 900 MeV and 2 GeV on the targets ²⁶Mg, ⁴⁰Ca, ⁴⁸Ca, ⁵⁴Fe, ⁹⁰Zr and ²⁰⁸Pb are presented. A multipole decomposition for the data at 900 MeV has been made and the different distributions have been analysed. From the L = 0 cross section the Gamow-Teller strength distributions are extracted and compared with (p, n) data. The L = 1 and 2 distributions are analysed in a schematic model which describes the general systematics fairly well. The spectra at 2 GeV and Θ = 4° show for all targets a well-developed quasi-elastic peak. The A-dependence of the cross section is analysed in a simple model.     

The (3He,t) reaction on 24Mg and 28Si

The (³He, t) charge exchange reaction on ²⁴Mg and ²⁸Si has been studied at 38.5 MeV. The angular distributions provide a number of new spin assignments in ²⁴Al and ²⁸P. A two-step excitation through intermediate α-particle channels was used to predict the ²⁴Al cross sections. The fits are fair in shape, but about a factor of three too large when a perfect overlap of initial and final shapes is assumed. The data to three 1⁺ states of ²⁸P are compared to the known electromagnetic reduced transition rate B(M1) to the analog states in ²⁸Si.     

Polarization and polarization transfer in the 2H(d,n)3He reaction at 10 MeV

Angular distributions of six polarization transfer coefficients $\text{K}{}_{\mathrm{x}}{}^{\mathrm{x\prime }}\text{(θ), k}{}_{\mathrm{x}}{}^{\mathrm{z\prime }}\text{(θ), K}{}_{\mathrm{z}}{}^{\mathrm{<mtext>x</mtext><mtext>?</mtext>}}\text{(θ), K}{}_{\mathrm{z}}{}^{\mathrm{<mtext>z</mtext><mtext>?</mtext>}}\text{(θ),}\text{and}\text{K}{}_{\mathrm{yy}}{}^{\mathrm{<mtext>y</mtext><mtext>?</mtext>}}\text{(θ)}$; of the four analyzing powers A_y(θ), A_xx(θ), A_yy(θ), and A_zz(θ); and of the polarization function P^ý(θ), have been measured atE_d = 10.00 MeV for the reaction ²H(d, n)³He. Measurements were made for neutron lab angles between 0° and 80° in 10° steps. Additionally the y-axis associated quantities were measured at θ_1ab = 99°. Most of the measured coefficients are large at some angles and all show considerable variation with angle.     

Study of the W(t, p)W reaction at 20 MeV

The ¹⁸²W(t, p)¹⁸⁴W reaction has been studied at 20 MeV. The outgoing protons were detected in an Elbek broad range magnetic spectrograph. Absolute cross sections and angular distributions were measured. Evidence for inelastic effects in the reaction mechanism was observed for the first excited 2⁺ state, the 3⁻ level at 1221 keV and the 5⁺ state at 1295 keV. The 0⁺ level at 1002 keV was populated with ≈ 2% the ground state cross section. A 4⁺ level at 1536 keV was observed with ≈ 50% the ground state cross section. Calculations of the absolute (t, p) cross sections to this and other states with known structure resulted in excellent agreement with the measured values.     

Cross sections and thermonuclear reaction rates for 42Ca(p, γ)43Sc, 44Ca(p, γ) 45Sc, 44Ca(p,n) 44Sc and 45Sc(p,n)45Ti

The yield of γ-rays from the reaction ⁴²Ca(p, γ)⁴³Sc has been measured as a function of bombarding energy over the range 0.63–3.01 MeV, from ⁴⁴Ca(p, γ)⁴⁵Sc over the range 0.775–4.00 MeV, from ⁴²Ca(p, p'γ)⁴²Ca over the range 2.24–3.01 MeV, and from ⁴⁴Ca(p, p'γ)⁴⁴Ca over the range 1.90–5.03 MeV. The cross section of the reaction ⁴⁴Ca(p, n)⁴⁴Sc has been measured from threshold to a bombarding energy of 5.05 MeV by observation of the 1157 keV γ-ray associated with the residual ⁴⁴Sc activity, and the cross section of the reaction ⁴⁵Sc(p, n)⁴⁵Ti has been measured from threshold to a bombarding energy of 4.00 MeV both by observation of the annihilation radiation associated with the residual ⁴⁵Ti activity and by measurement of the total neutron yield with a wide-angle BF₃ tube and paraffin detector. All these data are compared with statisticalmodel calculations and satisfactory agreement is achieved. Thermonuclear reaction rates for the (p, γ) and (p, n) reactions are calculated for the temperature range 5 × 10⁸-10¹⁰K and the significance of these results for explosive nucleosynthesis in stars is discussed.     

Study of the 182W(t,p)184W reaction at 20 MeV

The ¹⁸²W(t, p)¹⁸⁴W reaction has been studied at 20 MeV. The outgoing protons were detected in an Elbek broad range magnetic spectrograph. Absolute cross sections and angular distributions were measured. Evidence for inelastic effects in the reaction mechanism was observed for the first excited 2⁺ state, the 3^? level at 1221 keV and the 5⁺ state at 1295 keV. The 0⁺ level at 1002 keV was populated with ≈ 2% the ground state cross section. A 4⁺ level at 1536 keV was observed with ≈ 50% the ground state cross section. Calculations of the absolute (t, p) cross sections to this and other states with known structure resulted in excellent agreement with the measured values.     

Large-angle enhancements in the 16O(6Li, α)18F reaction at 48 MeV

The elastic scattering of ⁶Li + ¹⁶O at 48 MeV has been measured and fitted with an optical model calculation. Measurements have been made of the ¹⁶O(⁶Li, α)F reaction at 48 MeV populating the 1⁺ g.s., 3⁺ 0.927 MeV and 5⁺ 1.122 MeV states in ¹⁸F. The data exhibit cross sections at large angles comparable to those at forward angles, and have been compared with exact finite-range DWBA calculations. Exchange contributions were included for the 1⁺ g.s. and were unable to account for the large-angle data. Calculated statistical compound nucleus cross sections were approximately a factor of 100 below the data. The same conclusions are reached for previously published data at 34 MeV.     

Proton polarization and differential cross section for the (3He,p) reaction on 6Li and 9Be at 14 MeV

Angular distributions of the proton polarization and the differential cross section have been measured for the reaction (³He, p) initiated by 14 MeV incident ³He particles and proceeding to the ground and the first excited states of the final nuclei ⁸Be and ¹¹B. Large polarization values were observed, especially for the ⁹Be(³He, p)¹¹B reaction leading to both the ground and the first excited states in ¹¹B. The experimental results have been analysed in terms of a two-nucleon transfer spindependent distorted-waves theory using finite-range formalism and including corrections due to the non-locality of the optical potentials. A proper coherent summation over L and S, whenever necessary was included in the DWBA calculations of the polarization and the differential cross section as implied by the presence of the spin-orbit terms in the optical-model potentials used to generate the distorted waves.     

Spectroscopy of low-lying positive parity states in 30P from the study of the reaction (3He,d) at 14.0 MeV

The reaction ²⁹Si(³He, d)³⁰P was studied at an incident energy of 14.0 MeV. Spectroscopic strengths for 14 positive parity states up to an excitation of 4.50 MeV have been obtained using DWBA analysis. The incident channel optical-model parameters for the DWBA calculations were extracted from elastic scattering cross sections measured also at 14.0 MeV.     

The reaction 67Zn(t, α)66Cu

Levels of ⁶⁶Cu have been studied using the (t, α) reaction on ⁶⁷Zn at 18 MeV. Orbital and, in some cases, total angular momentum transfer were inferred from a comparison of differential cross sections with those measured for the same reaction on the even zinc isotopes. The quartet of levels corresponding to the p_{$\text{3}\text{2}$} proton pick-up from the $\text{5}\text{2}$^? target was identified. In addition, a strong set of l = 3 transitions was found corresponding to pickup from the f_{$\text{7}\text{2}$} proton shell.     

Direct and compound nuclear contributions to the 13C(6Li,t) reaction at Elab = 25 MeV

The reaction ¹³C(⁶Li, t)¹⁶O has been studied in the incident energy range 24–26 MeV. Complete angular distributions have been measured at E_⁶Li, = 25 MeV in the angular range θ_lab = 8°–172°, with the reaction ⁶Li(¹³C, t)⁶O being used for the backward angle measurements. Cross sections for evaporation residues from the fusion of the ⁶Li + ¹³C system have been measured in the incident ⁶Li energy range 9.2–35.1 MeV. Compound nuclear contributions to the transfer cross sections have been calculated using the Hauser-Feshbach statistical theory with the assumption that the compound-nucleus formation cross section is equal to the measured fusion cross section. By comparison of the compound nuclear calculations with backward angle data it is found that the sharp cutoff approximation commonly used to represent the initial angular momentum distribution of the compound nucleus is not adequate for the ¹³C(⁶Li, t)¹⁶O reaction. Good fits to the backward angle data can be obtained by using a smooth cutoff approximation. The forward angle cross sections have been compared with exact finite-range distorted-wave Born approximation calculations to extract transferred angular momenta and spectroscopic strengths. The present results differ from those of an earlier study. These differences are due to the inclusion of forward angle data in the present study.     

A study of the Ti(He, t) and Ni(He, t) reactions to isobaric analogue states

The (³He, t) reaction populating 0⁺ and 2⁺ states in ^{58, 60}Cu and ^{46, 48}V which are isobaric analogue states (IAS) of the 0⁺ ground states and 2⁺ first excited states in ^{58, 60}Ni and ^{46, 48}Ti have been studied at an incident ³He energy of 24.6 MeV. Triton spectra were measured for the targets ^46,48Ti, ^natNi and ⁵⁸Ni and angular distributions for the 0⁺ and 2⁺ IAS of ^{46, 48}Ti and ^{58, 60}Ni determined. The data were obtained using a magnetic spectrometer and position-sensitive detectors. The results have been analysed using DWBA theory. The 0⁺ → 0⁺ transitions to analogue states are described quite well using a microscopic form factor derived from a nucleon-nucleon interaction. However, with a Gaussian form, the m.s. radius of this interaction is only limited to the region 0–9 fm². Comparisons with data at other incident energies indicate that the strength of the effective interaction is strongly energy dependent. The Coulomb energies and (³He, t) angular distributions of the states assigned as the 2⁺ analogues in ⁴⁸V and ^58,60Cu are not described well by the models investigated. The ⁴⁶V 2⁺ IAS angular distribution is reproduced by a microscopic calculation, however. The ratios of the 0⁺ → 2⁺ IAS to the 0⁺ → 0⁺ IAS transitions are used to deduce a quadrupole deformation for the valence neutrons. The difference in the quadrupole deformations of the matter and proton distributions, as determined by other means, is found to be correlated with those of the valence neutrons. Several transitions to non-analogue states are also investigated.     

Semi-microscopic analysis of multi-nucleon transfer and the 40Ca(α, p)43Sc reaction

A semi-microscopic model for analyzing multi-nucleon transfer reactions in the distorted-wave Born approximation is presented. This model, which is shown to be compatible with other semi-microscopic models, employs cluster form factors. The cluster spectroscopic factors are calculated using shell-model wave functions. Data from the ⁴⁰Ca(α, p)⁴³Sc reaction are presented and used to test the model. The relative cluster spectroscopic factors for a number of levels are found to be in agreement with those calculated using wave functions in an $\text{(}\text{f}{}_{\mathrm{<mtext>7</mtext><mtext>2</mtext>}}\text{)}{}^3$ basis.     

Inelastic processes and form factor effects in the 162, 164Dy(3He,d) reactions at 46.5 MeV

The 162, 164Dy(³He, d) reactions at E_3He = 46.5 MeV are analyzed using the coupled channels Born approximation (CCBA) and improved form factors derived from a deformed Woods-Saxon potential. The latter are generated using the coupled channels procedure of Rost. The transitions considered populate the $\text{7}\text{2}$^?[523], $\text{1}\text{2}$⁺[411], $\text{3}\text{2}$⁺[411], $\text{1}\text{2}$^?[541] and $\text{5}\text{2}$⁺ orbitals in ^{163, 165}Ho. Indirect processes induced by inelastic scattering are found to have an influence on the cross sections comparable to that deduced for neutron transfer reactions on rare earth nuclei at lower energies. Considered alone, these can alter the cross sections even of strong transitions by a factor of two and of weaker ones by an order of magnitude. For the weaker transitions equally large changes can result when the improved form factors, rather than conventional spherical Woods-Saxon functions, are used in the calculations. In the examples considered these two effects tend to cancel, often, but not always, resulting in predicted cross sections similar in magnitude to the results of conventional DWBA calculations made with spherical Woods-Saxon form factors. The CCBA angular distributions are generally similar in shape to DWBA predictions, which usually give good fits to the experimental angular distributions over the 0–35° range of the data. Compared with DWBA predictions which use (he same optical parameters, but spherical Woods-Saxon form factors, the CCBA with deformed Woods-Saxon form factors is in better overall agreement with the experimental cross-section magnitudes. However there are a number of cases in which the CCBA, although usually predicting larger cross sections than the DWBA, still underestimates the experimental cross sections by nearly factor of two. These cases all occur in the $\text{71}\text{2}$^?[541] band or in the strongly Coriolis mixed $\text{1}\text{2}$⁺[411] and $\text{3}\text{2}$⁺[411] bands, and include the majority of transitions populating these orbitals. Since both nuclear structure and reaction mechanism effects are interwoven m the calculations, further data would be most useful in probing the origin of the discrepancy.