高电荷态离子Arq+与不同金属靶作用产生的X射线

研究了高电荷态离子Arq+(q=16,17,18)入射金属Be,Al,Ni,Mo,Au靶表面产生的X射线谱.实验结果表明,Ar的Kα-X射线是离子在与固体表面相互作用过程中固体表面之下形成空心原子发射的.电子组态1s2的高电荷态Ar16+离子在金属表面中性化过程中,存在的多电子激发过程使Ar16+的K壳层电子激发产生空穴,级联退激发射Ar的Kα特征X射线.Ar17+离子在金属表面作用过程中产生的X射线谱形与靶材料没有明显的关联,入射离子的Kα-X射线产额与其最初的电子组态有关,靶原子的X射线产额与入射离子的动能有关.     

近玻尔速度氙离子激发钒的K壳层X射线

测量了2.4—6.0 MeV Xe~(20+)离子轰击V靶表面过程中辐射的X射线.计算了V的K壳层X射线发射截面,并将实验结果与平面波恩近似、ECPSSR、两体碰撞近似的理论计算进行了对比.讨论了近玻尔速度非对称碰撞过程中,BEA模型估算高电荷态重离子激发内壳层电离的修正因素.结果表明,综合考虑库仑偏转和有效电荷态修正后,BEA理论与实验结果符合较好.     

高电荷态离子Arq+与不同金属靶作用产生的X射线

研究了高电荷态离子Ar^q+(q=16，17，18)入射金属Be，Al，Ni，Mo，Au靶表面产生的X射线谱.实验结果表明，Ar的Kα-X射线是离子在与固体表面相互作用过程中固体表面之下形成空心原子发射的.电子组态1s²的高电荷态Ar¹⁶⁺离子在金属表面中性化过程中，存在的多电子激发过程使Ar¹⁶⁺的K壳层电子激发产生空穴，级联退激发射Ar的Kα 特征X射线.Ar¹⁷⁺离子在金属表面作用过程中产生的X射线谱形与靶材料没有明显的关联,入射离子的Kα-X射线产额与其最初的电子组态有关，靶原子的X射线产额与入射离子的动能有关. 关键词： 高电荷态离子 空心原子 多电子激发 X射线     

近Bohr速度的152Eu20+入射Au表面产生的X射线谱

测量了动能为2.0–6.0 MeV的高电荷态离子¹⁵²Eu²⁰⁺ 入射Au表面产生的特征X射线谱, 结果表明, 相互作用不仅激发出了Au的 M_ζ, M_α和M_δ特征X射线, 还激发出了Eu的M_α X射线, 且X射线总产额随入射离子动能的增加而增加. 计算了Au的M壳层总的X射线产生截面, 并与理论模型的计算结果做了比较分析. 关键词： 高电荷态离子 X射线 产额 截面     

近Bohr速度129Xeq+离子入射Ta靶发射近红外光谱线

用动能一定的高电荷态¹²⁹Xe^q+(17≤q≤27)离子,分别入射洁净的Ta靶表面,测量中性化的激发态Xe原子从组态5p⁵(²P°_3/2) nl退激到组态5p⁵(²P°_3/2) ml’过程中辐射的近红外光谱线.实验结果表明:多激发态的空心原子退激发射其特征光谱线,部分典型的跃迁按照阶梯方式退激.Xe原子发射的谱线的单粒子荧光产额和激发的Ta原子发射谱线的单粒子荧光产额随入射离子电荷态的增加而增加,其增加的趋势与入射离子携带的势能随电荷态增加的趋势一致.证明在近Bohr速度的能区,经典过垒模型是成立的.     

近玻尔速度不同离子碰撞产生Al的KX射线

在玻尔速度附近能区,测量了H⁺,He²⁺和I²²⁺,Xe²⁰⁺离子作用于Al靶时碰撞激发靶的K壳层X射线.得到了相应X射线的发射截面,并与不同理论模型进行对比.研究表明,单核子能量相同时,轻离子入射激发的X射线产生截面比高电荷态重离子轰击时小了大约4个数量级.质子、He²⁺离子激发的实验截面可以由ECPSSR理论来很好的估算,而I²²⁺,Xe²⁰⁺的实验结果与考虑有效电荷、低速库仑偏转修正的BEA理论计算符合较好.     

H+和Ar11+激发Si的K壳层X射线发射研究

测量了50–250 keV H⁺和1.0–3.0 MeV Ar¹¹⁺ 轰击Si表面过程中辐射的X射线. 结果表明, 在Ar¹¹⁺入射的情况下, 引起了Si的L壳层上3, 4个电子的多电离.计算了Si的K壳层X射线产生截面, 并将两体碰撞近似(BEA), 平面波恩近似, ECPSSR理论计算与实验值进行了对比. ECPSSR理论与质子产生的截面数据能够很好地符合; 而考虑多电离后, BEA理论与Ar¹¹⁺的实验结果符合较好. 关键词： X射线 高电荷态重离子 多电离     

采用薄靶方法测量低能电子致Al,Ti,Cu,Ag,Au元素K壳层电离截面与L壳层特征X射线产生截面

使用5—27 keV能量范围内的单能电子束轰击薄碳衬底上的薄Al (Z=13),Ti (Z=22),Cu (Z=29),Ag (Z=47),Au(Z=79)靶,使用硅漂移型探测器(SDD)收集产生的特征X射线,测量了Al,Ti,Cu的K壳层电离截面以及Cu,Ag和Au的L壳层特征X射线的产生截面,并且使用蒙特卡罗PENELOPE程序对实验结果进行了修正.本文给出了Cu的L壳层特征X射线产生截面.与半相对论扭曲波玻恩近似(semi-relativistic distorted-wave Born approximation,DWBA)理论值相比,本文的大多数实验值在7%的范围内与理论值符合.研究表明,中重元素的L壳电离截面的理论计算以及相应的原子参数有待更精确的确定.     

高电荷态离子Arq+入射在金属表面形成靶原子X射线谱

本文报道低能高电荷Ar12+、Ar13+ 、Ar14+离子与金属Mo表面作用过程中Mo原子受激发射X射线和X射线强度随入射能量变化的实验结果.结果表明,低速高电荷离子与金属表面原子相互作用可有效地激发靶原子或靶离子内壳层电子而发射X射线.     

Xe~(26+)入射Au靶离子L壳层空穴的产生与退激辐射

基于两体碰撞过程的能量与角动量守恒,推导出Xe26+离子与Au原子碰撞过程,单离子的L壳层空穴产额与离子动能的理论关系.实验测定了动能2.4-3.6Me V的Xe26+离子入射Au靶,产生的Xe的L-X射线谱,获得了射线产额与离子入射动能的实验关系.结果表明,碰撞过程产生Xe L壳层空穴的同时,产生了一定数目的 M壳层空穴,导致L壳层空穴平均荧光产额显著变大,在实验能量范围,空穴产额的理论值与射线产额的实验值存在较好的一致性.     

X-ray emission for Ar11+ ions impacting on various targets in the collisions near the Bohr velocity

X-ray emission from the collisions of 3 MeV Ar¹¹⁺ ions with V, Fe, Co, Ni, Cu, and Zn is investigated. Both the x-rays of the target atom and projectile are observed simultaneously. The x-ray yield is extracted from the original count. The inner-shell ionization cross section is estimated by the binary encounter approximation model and compared with the experimental result. The remarkable result is that the Ar K-shell x-ray yield is diminished with the target atomic number increasing, which is completely opposite to the theoretical calculation. That is interpreted by the competitive consumption of the energy loss for the ionization of inner-shell electrons between the projectile and target atom.     

Nd L-shell x-ray emission induced by light ions

The L-shell x-ray of Nd has been obtained for 300-600 keV He²⁺ ions impacting, and compared with that produced by H⁺ and H₂⁺ ions. The threshold of projectile kinetic energy for L-shell ionization of Nd is crudely verified in the energy region of about 300-400 keV. It is found that the energy of the distinct L-subshell x-rays has a blue shift. The relative intensity ratios of Lβ_{1, 3, 4} and Lβ_{2, 15} to Lα_{1, 2} x-ray are enlarged compared to the atomic data, and they decrease with the increase of the incident energy, and increase with increasing the effective nuclear charge of the incident ions. That is interpreted by the multiple ionization of outer-shells induced by light ions.     

中低能非全裸C离子与He原子的碰撞研究

采用反冲离子飞行时间-散射离子位置灵敏符合测量技术，测量了能量范围在0.7v₀—4.4v₀(v₀为玻尔速度)的碳离子C^q+(q=1—4)与He原子碰撞过程不同出射道靶原子的双电离与单电离截面比R，包括入射离子不损失电子(直接电离)的出射道(R_q,q),入射离子俘获一个电子的出射道(R_q,q-1)和入射离子损失一个电子的出射道(R_q,q+1)，并研究了R随入射C离子的能量及电荷态的变化关系.实验表明，对给定电荷态的入射离子，靶原子的双电离与单电离截面比R与出射道有很强的依赖关系，即R_q,q<R_q,q+1<R_q,q-1.直接电离出射道截面比R_q,q与入射离子电荷态几乎无关，而入射离子俘获一个电子的出射道和损失一个电子的出射道靶原子双电离与单电离截面比R_q,q-1和R_q,q+1却与入射离子电荷态有很强的关系.采用原子极化理论和电子屏蔽与反屏蔽作用对实验结果进行了解释. 关键词： 离子-原子碰撞 电离 截面比     

C3+与Ne碰撞过程纯电离绝对截面的测量和研究

介绍了离子-原子碰撞过程中双微分绝对截面的计算方法.利用符合技术测量了中能区C³⁺+Ne碰撞系统的纯电离微分绝对截面. 将实验结果与多体经典蒙特卡罗方法计算结果进行对比后发现，纯电离截面随入射能量变化的趋势基本一致，对理论与实验产生差异的原因作了分析. 对多重电离的电离机制分析表明：高价态的反冲离子主要来自于俄歇贡献；随着入射能量的升高，电子-电子间的库仑作用也逐渐显现. 此实验方法可以用于相同实验装置上的各种反应出射道的绝对截面测量，入射离子种类及入射离子能量范围将得到拓展. 关键词： 离子-原子碰撞 绝对截面 纯电离     

Multiple ionization of argon accompanied by electron loss and capture of 0.22-6.35 MeV C^q＋ ions

In this paper a projectile ions recoil ions coincidence technique is employed to investigate the target ionization and projectile charge state changing processes in the collision of 0.22-6.35 MeV Cq^＋ （q = 1 - 4） ions with argon atoms. The partial cross section ratios of the double, triple, quadruplicate ionization to the single ionization （or the single capture） of argon associated with single electron loss （or single electron capture） by the projectile are measured and compared with the previous experimental results. In the present experiment, it is observed that the ratios of ionization cross sections R associated with single loss and single capture depend strongly on the projectile charge state and vary significantly with different reaction channels as impact energy increases. In addition, this paper gets empirical scaling laws for the ionization cross section ratios R corresponding to the projectile single loss and finds that the ratios of the double ionization to the single ionization associated with single electron capture remain constant in the present energy range.     

Use of a diabatic molecular expansion in studies on electron capture by He2+ ions in helium at keV energies

In this preliminary work, using a 3-state diabatic molecular expansion without any excited channels, we have studied within the semiclassical impact parameter approximation the single charge transfer process He²⁺+He(1s ²)→He⁺(1s)+He⁺(1s). Our results agree very well with experiment, which demonstrates the usefulness of this type of diabatic molecular basis in doubly charged ion-atom collision systems.     

X-ray emission from 424-MeV/u C ions impacting on selected target

The K-shell x-rays of Ti, V, Fe, Co, Ni, Cu, and Zn induced by 424-MeV/u C~(6+) ion impact are measured. It is found that the K x-ray shifts to the high energy side and the intensity ratio of Kβ/Kα is larger than the atomic data, owing to the L-shell multiple-ionization. The x-ray production cross sections are deduced from the experimental counts and compared with the binary encounter approximation(BEA), plane wave approximation(PWBA) and energy-loss Coulomb-repulsion perturbed-stationary-state relativistic(ECPSSR) theoretical predictions. The BEA model with considering the multipleionization fluorescence yield is in better consistence with the experimental results. In addition, the cross section as a function of target atomic K-shell binding energy is presented.     

Production of recoil ions He^i＋ accompanied by single electron loss of 0.2-7 MeV C^q＋ and 0.25-5 MeV O^q＋ （q = 1- 4） ions

Target ionization accompanied with projectile electron loss is investigated for 0.2-7 MeV C^q＋ （q = 1 - 4） with He and 0.25-5 MeV O^q＋ （q = 1 - 4） with He collisions. For projectile single-electron loss channel, the He double-to-single ionization ratio R is nearly independent of projectile charge state but dependent on the nuclear charge of projectile Zp. The results are analysed with atomic structure qualitatively. So far there have not existed the experimental data comparable with our results, to our knowledge. The ratio R is interpreted in terms of the two-step mechanism. This analysis agrees well with similar experiments in the literature.     

Transfer ionization cross-sections measured in collisions of highly charged argon ions with neon target

: Multiple electron transfer processes are studied for Arq+n- Ne (q= 8, 9, 11, 12) collisions by using multi-parameter coincidence techniques. Various electron transfer processes are identified experimentally and the related cross-sections are measured. The dependence of transfer ionization cross-sections on the recoil charge states is compared with the results from the modified molecular classical overbarrier model. It is found that the modified model described the experimental results reasonably.     

应用ECPSSR理论研究重离子引起原子的内壳层电离

ECPSSR理论是解释离子-原子碰撞内壳层电离最成功的理论之一.我们用VISUAL FORTRAN编写了ECPSSR理论计算程序,修正了ISICS程序中的错误,本程序可以对各种入射离子与靶原子的组合进行计算,给出K,L,M的壳层及次壳层电离截面以及相应的X射线产生截面,并根据需要选择是否对入射离子运动进行相对论修正.采用所编写的程序计算了一些碰撞体系的电离截面和X射线产生截面,并与其他程序的计算结果和实验数据分别进行了比较.