In-beam study of 102Sn

Excited states in ¹⁰²Sn have been identified for the first time, in an in-beam γ-ray spectroscopic experiment. Two γ-ray transitions with energies 1472 and 497 keV following the decay of the seniority 6⁺ isomer with t_1/2 = 1.0(5) μs were unambiguously assigned to ¹⁰²Sn. Due to the very low cross section of about 2 μb for producing ¹⁰²Sn in the reaction ⁵⁰Cr(⁵⁸Ni,1α2n), a highly selective detector setup utilizing NORDBALL ancillary detectors and a recoil catcher device was used. High γ-ray detection efficiency was achieved with two EUROBALL Ge cluster detectors.     

In-beam study of102Sn

Excited states in¹⁰²Sn have been identified for the first time, in an in-beamγ-ray spectroscopic experiment. Twoγ-ray transitions with energies 1472 and 497 keV following the decay of the seniority 6⁺ isomer with t_1/2=1.0(5)μs were unambiguously assigned to¹⁰²Sn. Due to the very low cross section of about 2µb for producing¹⁰²Sn in the reaction⁵⁰Cr(⁵⁸Ni,1α2n), a highly selective detector setup utilizing NORDBALL ancillary detectors and a recoil catcher device was used. Highγ-ray detection efficiency was achieved with two EUROBALL Ge cluster detectors.     

Low-lying states of 109Sn from the 106Cd(α, nγ) reaction

Measurements of γ-ray, γγ-coincidence and internal conversion electron spectra from the ¹⁰⁶Cd(α, nγ)¹⁰⁹Sn reaction were carried out at 15–20 MeV α-particle bombarding energies with Ge(HP) γ-ray and superconducting magnetic lens plus Si(Li) electron spectrometers. The energies, relative intensities, internal conversion coefficients and coincidence relations of the ¹⁰⁹Sn transitions were determined, and a more complete, consistent level scheme has been deduced. Spin and parity values have been determined from the internal conversion coefficients, the bombarding-energy dependence of the side-feeding intensities of the states and the available γ-ray angular distribution data. The level scheme was interpreted in the framework of the quasi-particle shell model.     

The decay of115 mIn

The decay of^115m In has been investigated using accurate counting methods. The emission rate of conversion electrons plusβ ^?-particles was determined with a 4π proportional flow counter. The total andK-shell internal conversion coefficients of the 336 keVγ-ray in¹¹⁵In were measured by the electron X-ray coincidence method using combinations of a Si surface barrier with a NaI(Tl) detector and of a magneticβ-spectrometer with a high energy resolution Si(Li) detector, respectively. The conversion ratioR=K/(L+M+...) was deduced from electron spectra recorded with the magneticβ-spectrometer. The 336 keVγ-ray emission rate of all used sources was determined with a calibrated NaI(Tl)γ-ray spectrometer. A Ge(Li) detector has been used to determine the relative intensity of the 497 keVγ-ray in¹¹⁵Sn. As results have been deduced the 336 keVγ-ray emission per decay (N _γ1/N ₀=(45.9 ± 0.1)%), the total internal conversion coefficient (α=1.073 ± 0.014), theK-shell internal conversion coefficient (α _K=0.843±0.012), the conversion ratioR=3.63±0.07, theβ ^?-transition per decay going to the ground state (N _β1/N ₀=(5.0 ± 0.7)%) and to the first excited level in¹¹⁵Sn¹¹⁵Sn(N _β2/N ₀=(0.047 ± 0.002)%), and the 497 keVγ-ray emission (N _γ2/N _γ1=(0.103 ± 0.004)%). From the obtained internal conversion data it follows that the 336 keVγ-ray transition is ofM4 character with anE5 admixture of less than (3.5±1.5)%. The half-life of the isomeric state¹¹⁵ mIn has been determined with four different methods. The result isT _1/2=(4.486±0.004) h.     

Particle × phonon multiplets in 65 147 Tb82

High-spin states of¹¹⁵Sb were studied by inbeamγ-ray spectroscopy using the⁸⁹Y (²⁹Si, 2pn) fusionevaporation reaction at a beam energy of 108 MeV. The experiments includedγ-γ coincidence and directional correlation of oriented nuclei (DCO) ratio measurements using six BGO Compton suppressed Ge detectors. An intruderΔJ=2 rotational band has been identified for the first time and it is interpreted as the h_11/2 proton coupled to a two particle-two hole (2p ? 2h) deformed state of the¹¹⁴Sn core. A ΔJ=1 rotational band based on the 2p ? 1h, π{g ₇ ^2/2 ?g ₉ ^2/?1 }, configuration has been extended to the 29/2⁺ state at an excitation energy of 5241 keV.     

Collective bands in even mass Sn isotopes

Positive parity bands in ^{112, 114, 116, 118}Sn have been excited up to levels with spin and parity J^π = 12⁺ using Cd(α, 2nγ)Sn reactions. The experiments consisted of γ-ray excitation function, γ-γ coincidence, lifetime, γ-ray angular distribution, γ-ray linear polarization and conversion electron measurements. The observed bands show strong resemblances with ground-state bands of transitional nuclei in this mass region. It is pointed out that the J^π = 0⁺ band-heads originate from 2p-2h excitations in the Z = 50 proton shell. The excitation energies of the band-heads are calculated by means of the macroscopic-microscopic renormalization method. Pair correlations between the 2h and 2p configurations are included separately in a phenomenological way by taking into account the pairing energies of the Cd and Te ground states with respect to the Sn ground state.     

High-energy γ-rays in α-accompanied spontaneous fission of 252 C f

An experiment was performed on prompt γ-ray emission in binary and α-particle accompanied spontaneous fission of ²⁵² C f using the Darmstadt-Heidelberg 4π NaI Crystal Ball spectrometer. The enhancement in γ-ray yield, denoted as the “high-energy component”, which appears between 3.5 and 8 MeV and in the region of near-symmetric fragment mass splits, was observed to be equally pronounced in both fission modes. Analyzing the fragment mass dependence of the mean γ-ray multiplicity in both fission modes clearly identifies the disintegration of equilibrated fission fragments in a narrow mass range around the double-magic ¹³²Sn as the source of these γ-rays.     

High-energy gamma rays emission in coincidence with light charged particles from the32S +74Ge reaction at 210 MeV

High-energyγ-rays from the³²S+⁷⁴Ge reaction at 210 MeV bombarding energy were measured in coincidence with light charged particles detected in a large area hodoscope. Experimental results show that energeticγ-rays in coincidence with light charged particles are essentially emitted in the compound nucleus decay. The parameters of the giant dipole resonance (GDR) have been extracted from alineshape analysis of the experimentalγ-ray spectrum. The derived values of mean energyE _D, widthΓ and strengthS are in good agreement with results from previous experiments on Sn isotopes obtained by using different experimental techniques.     

Search for an isomer in94Rb

Measurements of theβ-ray half-life,γ-ray and X-ray spectra andγ-ray half-lives have been done with a plastic scintillation detector, a high resolution Ge(HP) detector and a 142 cm³ Ge(Li) detector to search for an isomeric state in⁹⁴Rb. Mass-separated activities of⁹⁴Rb were obtained from the He-jet type on-line mass-separator at the Kyoto University reactor. No isomeric transition was found in theγ-ray and X-ray measurements with the upper limits of 3×10^?4 and 8×10^?5, respectively, as compared with the 836.9 keV transition. Half-lives obtained from theγ-ray decay measurements are discussed in the light of classification given byQ _β -value measurements.     

High spin level structure in127Ba produced by the118Sn(12C, 3n) reaction

High-spin states in¹²⁷Ba have been produced by the reaction¹²⁸Sn(¹²C,3n)¹²⁷Ba and studied by in-beamγ-ray spectroscopic techniques. The odd-parity states form a level system based upon a 9/2^? state and generated by an odd neutron in theh _11/2 shell coupled to a triaxial core. Theg _7/2 shell is responsible for theΔ I=1, even-parity band.     

Gamma decay of the giant dipole resonance and feeding of superdeformed states in 143Eu

The γ decay of the giant dipole resonance (GDR) built on excited nuclear states has been measured in coincidence with the low-energy γ discrete transitions for the nucleus ¹⁴³Eu. The reaction used was ¹¹⁰Pd(³⁷Cl, 4n)¹⁴³Eu at a beam energy of 165 MeV. The EUROBALL spectrometer (for the measurement of discrete γ transitions) coupled with the HECTOR array (for high-energy γ-ray detection) has been used. The high-energy γ-ray spectrum in coincidence with superdeformed (SD) discrete transitions of ¹⁴³Eu shows an “excess” between 9–12 MeV if compared with the one associated to cascades which do not pass through the SD configurations. Such an “excess” is in the energy region where one expects the low-energy component of the GDR strength function built on a SD state. The measured intensity can be reproduced by the statistical model assuming that the superdeformation survives only few MeV above the yrast line. A similar and consistent scenario has also been obtained by comparing the high-energy γ-ray spectra of ¹⁴³Eu in coincidence with its spherical (which is fed by the SD configuration) and its triaxial configuration (which is bypassed by the decay of the SD states).     

Low-lying excited states of106Ag studied with the103Rh (α,nγ)106Ag and104Pd (α,pnγ)106Ag Reactions

The level scheme of¹⁰⁶Ag has been studied using the¹⁰³Rh(α,nγ)¹⁰⁶Ag and¹⁰⁴Pd(α,pnγ)¹⁰⁶Ag Reactions. The experimental information is taken fromγ-ray coincidence data using Ge(Li)-Ge(Li) and HPGe-planar Ge(Li) configurations andγ-ray angular distributions. With these measurements 126 γ rays have been assigned to¹⁰⁶Ag with 116 deexciting 78 states below 2.26 MeV in excitation. The location of the 8.4-day 6⁺ isomer is established at 89.63±0.09 keV. Many of the low-lying states are interpreted in terms of a slightly deformed rotor model.     

Competition between few nucleon emission andγ-ray deexcitation for the reaction systems65Cu+87Rb and40Ar+110Pd

Bothγ-ray and neutron emission have been studied for the reaction systems⁶⁵Cu(237MeV) +⁸⁷Rb→¹⁵²Dy^* and⁴⁰Ar(158MeV)+¹¹⁰Pd→¹⁵⁰Gd^*. By using a sum spectrometer in coincidence with neutron counters, Ge(Li) or Nal detectors, we have measured the totalγ-ray energy and the average totalγ-multiplicity distributions as well as the neutron spectra for various exit channels. These measurements provide strong evidence for thermal equilibrium in reactions involving a small number of emitted neutrons (i.e.⁸⁷Rb(⁶⁵Cu,n or 2n)) at rather high excitation energy (～54MeV). This statistical emission of only a few neutrons is controlled by very strong y-ray competition: theγ-entry line is found not to be parallel to the yrast line. Instead the energy gap is about 8MeV for J～27? and rises to at least 13MeV for J～36?. There are some indications that the main part of the energy from this gap is removed by statisticalγ-ray cascades. The main features of the experimental data for both entrance channels are well reproduced by statistical model calculations with proper attention to the yrast line position and an adjustement of the dipoleγ-ray normalization coefficient. It is conceivable that the y-ray enhancement that we introduce may be related to a lack of knowledge of the absolute level densities at high energy and spin, or possibly to the presence of new or additional degrees of freedom that may enter into the competition between neutron andγ-ray emission.     

In-beam study of the doubly-odd nucleus 61 140 Pm79

A detailed -γ-ray study of¹⁵²Dy has been performed using the¹²⁴Sn(³²S,4n) reaction at low bombarding energy. Several γ rays deexciting non-Yrast states have been identified, among them transitions previously observed in coincidence with the superdeformed band. However we have no evidence for the lowest members of this band.     

Cross section of metastable state population in the photoneutron decay of the E1 giant resonance for 110Pd, 112Cd, and 113In nuclei

The cross sections of isomeric state excitation in the ¹¹⁰Pd(γ, n)^109m Pd, ¹¹²Cd(γ, n)^111m Cd, and ¹¹³In(γ, n)^112m In reactions have been investigated. The measurements were performed in the γ-ray energy range 9–18 MeV with a step ΔE = 0.5 MeV. The dependences of the isomeric ratios on the γ-ray energy are obtained. The experimental data are compared with the results of calculations within the cascade-evaporation model.     

On-line γ-ray investigation of the14N+27Al reaction at 30 MeV/u

The cross-sections of target-like residues following the¹⁴N+²⁷Al reaction at 30 MeV/u have been measured from in-beam and radioactiveγ-ray spectra. The recoil velocities of some fragments have been estimated from theγ-ray Doppler broadening.     

High-spin states in107Sn

High-spin states in¹⁰⁷Sn were studied using the reaction⁵⁴Fe(⁵⁶Fe, 2pn)¹⁰⁷Sn. An odd-parity band was identified as based on thevh _11/2 orbit by measuring theγ-ray linear polarization. Also were confirmed the excited states based on thevd _5/2 andvg _7/2 orbits. The halflives of the 17/2⁺ and 11/2^? states were measured to be 0.25(4) ns and 28(11) ps, respectively. The experimental level structure and its interpretation were in good agreement with a shell model calculation.     

Spectroscopy of highly excited states in29Si

Particleγ-ray coincidences have been measured in the²⁸Si (d,pγ) reaction at 6.5 and 7 MeV bombarding energy, in the²⁶Mg (α,nγ) reaction at 12, 14 and 15 MeV, and in the²⁷A1 (τ,pγ) reaction at 9 MeV. Theγ-decay has been observed for all bound states of²⁹Si and for 56 unbound states up to 12,960 KeV excitation energy. Particleγ-ray angular correlations were measured in the²⁸Si (d,pγ) reaction at 6.5 MeV and in the²⁶Mg (α,nγ) reaction at 12 MeV. Spin (-parity) assignments or restrictions were obtained for nearly all bound states and some high-spin states above the binding energy. The assignment of mirror levels in²⁹Si and²⁹P has been extended to 8.2 MeV excitation energy. The excitation energies of 41 positive-parity states are reproduced by shell model calculations. The possible existence of aK ^π=5/2⁺ band with prolate deformation is discussed.     

High-spin states in106Cd

Levels of¹⁰⁶Cd, populated by¹⁰⁴Pd(α, 2nγ)¹⁰⁶Cd have been studied measuring direct and delayedγ-ray spectra,γ-γ coincidences andγ-ray angular distributions. A decay level scheme is proposed including states up to 4659.8 keV. IntenseE2 transition cascades have been observed. The half-life of an isomeric level located at 4659.8 keV has been measured:T _1/2= 62±6ns. Nuclear Reactions ¹⁰⁴Pd(α, 2nγ),E _α=31MeV; measuredE _γ,I _γ,γ-γ coinc, σ(θ)T _1/2.¹⁰⁶Cd deduced levels,J, π, Enriched targets. Ge(Li) detectors.