Quantized orbital angular momentum transfer and magnetic dichroism in the interaction of electron vortices with matter

Following the very recent experimental realization of electron vortices, we consider their interaction with matter, in particular, the transfer of orbital angular momentum in the context of electron energy-loss spectroscopy, and the recently observed dichroism in thin film magnetized iron samples. We show here that orbital angular momentum exchange does indeed occur between electron vortices and the internal electronic-type motion, as well as center-of-mass motion of atoms in the electric dipole approximation. This contrasts with the case of optical vortices where such transfer only occurs in transitions involving multipoles higher than the dipole. The physical basis of the observed dichroism is explained.     

Mechanism of angular momentum exchange between molecules and Laguerre-Gaussian beams

We derive the interaction Hamiltonian between a diatomic molecule and a Laguerre-Gaussian beam under the assumption of a small spread of the center of mass wave function of the molecule in comparison with the beam waist. Considering the dynamical variables of the center of mass, vibrational, rotational, and electronic motion, we show that, within the electronic dipole approximation, the orbital angular momentum of the field couples with the rotational and electronic motion. The changes in the transition probabilities and selection rules induced by the field orbital angular momentum and the applicability of the derived interaction mechanisms for polyatomic molecules are discussed.     

Generation of light carrying orbital angular momentum via induced coherence grating in cold atoms

We report on the generation of light carrying orbital angular momentum through Bragg diffraction into an electromagnetically induced coherence grating in a degenerate two-level system of cold cesium atoms. The induced Zeeman coherence grating is shown to contain the spatial phase structure of the incident beams. The exchange of phase information between a light beam with orbital angular momentum and a long-lived atomic coherence opens up the way to process quantum information encoded in a multidimensional state space.     

Electric-dipole increase in NMR intensity in mixed-valence complexes

The possibility of a considerable increase in NMR intensity has been shown for absorption on mixed-valence 3d ions in magnetically ordered crystals. This effect is determined by the high intensity of electric dipole transitions between the ground and low excited levels of a mixed-valence complex, as well as by the existence of the unfrozen orbital angular momentum in such complexes, which mixes nuclear and electron states.     

Binary-black-hole encounters, gravitational bursts, and maximum final spin

The spin of the final black hole in the coalescence of nonspinning black holes is determined by the "residual" orbital angular momentum of the binary. This residual momentum consists of the orbital angular momentum that the binary is not able to shed in the process of merging. We study the angular momentum radiated, the spin of the final black hole, and the gravitational bursts in a sequence of equal mass encounters. The initial orbital configurations range from those producing an almost direct infall to others leading to numerous orbits before infall, with multiple bursts of radiation. Our sequence consists of orbits with fixed impact parameter. What varies is the initial linear momentum of the black holes. For this sequence, the final black hole of mass M_{h} gets a maximum spin parameter a/M_{h} approximately 0.823, with this maximum occurring for initial orbital angular momentum L/M_{h};{2} approximately 1.176.     

Wave-particle duality of solitons and solitonic analog of the Ramsauer-Townsend effect

We study the interaction of light beams carrying angular momentum with a single, trapped and well localized ion. We provide a detailed calculation of selection rules and excitation probabilities for quadrupole transitions. The results show the dependencies on the angular momentum and polarization of the laser beam as well as the direction of the quantization magnetic field. In order to optimally observe the specific effects, focusing the angular momentum beam close to the diffraction limit is required. We discuss a protocol for examining experimentally the effects on the S_1/2 to D_5/2 transition using a ⁴⁰Ca⁺ ion. Various applications and advantages are expected when using light carrying angular momentum: in quantum information processing, where qubit states of ion crystals are controlled, parasitic light shifts could be avoided as the ion is excited in the dark zone of the beam at zero electric field amplitude. Such interactions also open the door to high dimensional entanglement between light and matter. In spectroscopy one might access transitions which have escaped excitation so far due to vanishing transition dipole moments.     

The angular momentum of light: optical spanners and the rotational frequency shift

An introduction is given to the concepts of the spin and orbital angular momentum of light beams. Both spin and orbital angular momentum can be transferred from a light beam to particles held within optical tweezers, so forming an optical spanner. Each also give rise to a frequency shift when the light beam is rotated. This arises because quarter or half-wave plates and /2 or mode converters play equivalent roles for spin and orbital angular momentum respectively.     

Orbital and spin photon angular momentum transfer in liquid crystals

All-optical angular control of the molecular alignment in liquid-crystal films is demonstrated using a laser beam having an elliptically shaped intensity profile. The material birefringence is unimportant, as proven by the fact that good alignment is obtained with unpolarized light. This raises the possibility of achieving optical angular control of transparent isotropic bodies. A general theoretical approach, based on light and matter angular momentum conservation, shows that the optical alignment is due to the internal compensation between the transfer of the orbital and the spin part of angular momentum of the incident photons to the material.     

Orbital-angular-momentum based origin of Rashba-type surface band splitting

We propose that the existence of local orbital angular momentum (OAM) on the surfaces of high-Z materials plays a crucial role in the formation of Rashba-type surface band splitting. Local OAM state in a Bloch wave function produces an asymmetric charge distribution (electric dipole). The surface-normal electric field then aligns the electric dipole and results in chiral OAM states and the relevant Rashba-type splitting. Therefore, the band splitting originates from electric dipole interaction, not from the relativistic Zeeman splitting as proposed in the original Rashba picture. The characteristic spin chiral structure of Rashba states is formed through the spin-orbit coupling and thus is a secondary effect to the chiral OAM. Results from first-principles calculations on a single Bi layer under an external electric field verify the key predictions of the new model.     

Slow light in ultra-cold atomic gases

We investigate the influence of slow light with an orbital angular momentum on the mechanical motion of ultra-cold atomic gases including both the atomic Bose–Einstein condensates and degenerate Fermi gases. We present a microscopic analysis of the interplay between light and matter and show how slow light can provide an effective magnetic field acting on the electrically neutral atoms.     

The propagation of a polarized gaussian beam in a smoothly inhomogeneous isotropic medium

In the frame of the eikonal-based complex geometrical optics, which describes the phase front and cross section of a light beam using the quadratic expansion of a complex-valued eikonal, we investigate the transverse deflections of a polarized Gaussian beam (GB) in a smoothly inhomogeneous isotropic medium, which is called the spin Hall effect of the beam. The linear complex-valued eikonal terms are introduced firstly to describe the polarization-dependent transverse shifts of the beam in the inhomogeneous medium. We find that the polarization-dependent transverse shifts of the beams include two parts: one originates from the coupling between the spin angular momentum and the extrinsic orbital angular momentum due to the curve trajectory of the center of gravity of the polarized GB, and the other from the coupling between the spin angular momentum and the intrinsic orbital angular momentum due to the rotation of the beam with respect to the central ray.     

Delocalized correlations in twin light beams with orbital angular momentum

We generate intensity-difference-squeezed Laguerre-Gauss twin beams of light carrying orbital angular momentum by using four-wave mixing in a hot atomic vapor. The conservation of orbital angular momentum in the four-wave mixing process is studied as well as the spatial distribution of the quantum correlations obtained with different configurations of orbital angular momentum. Intensity-difference squeezing of up to -6.7 dB is demonstrated with beams carrying orbital angular momentum. Delocalized spatial correlations between the twin beams are observed.     

Hall effect of light

We derive the semiclassical equation of motion for the wave packet of light taking into account the Berry curvature in momentum-space. This equation naturally describes the interplay between orbital and spin angular momenta, i.e., the conservation of the total angular momentum of light. This leads to the shift of wave-packet motion perpendicular to the gradient of the dielectric constant, i.e., the polarization-dependent Hall effect of light. An enhancement of this effect in photonic crystals is also proposed.     

Black hole solutions in heterotic string theory on a torus

We construct the general electrically charged, rotating black hole solution in the heterotic string theory compactified on a six-dimensional torus and study its classical properties. This black hole is characterized by its mass, angular momentum, and a 28-dimensional electric charge vector. We recover the axion-dilaton black holes and Kaluza-Klein black holes for special values of the charge vector. For a generic black hole of this kind, the 28-dimensional magnetic dipole moment vector is not proportional to the electric charge vector, and we need two different gyromagnetic ratios for specifying the relation between these two vectors. We also give an algorithm for constructing a 58 parameter rotating dyonic black hole solution in this theory, characterized by its mass, angular momentum, a 28-dimensional electric charge vector and a 28-dimensional magnetic charge vector. This is the most general asymptotically flat black hole solution in this theory consistent with the no-hair theorem.     

Analytical description of shape transition in nuclear alternating parity bands

The angular momentum dependencies of parity splitting and electric dipole transitions in the alternating parity bands of heavy nuclei have been analyzed. It is shown that these dependencies can be treated in a universal manner with a single critical angular momentum parameter, which characterizes phase transition from octupole vibrations to the stable octupole deformation. Using the simple but useful model of axially-symmetric reflectionasymmetric mode, the analytical expressions for parity splitting and electric dipole transitional moment have been obtained. The findings are in good agreement with the experimental data for various isotopes of Ra, Th, U, and Pu.     

Mechanical equivalence of spin and orbital angular momentum of light: an optical spanner

We use a Laguerre-Gaussian laser mode within an optical tweezers arrangement to demonstrate the transfer of the orbital angular momentum of a laser mode to a trapped particle. The particle is optically confined in three dimensions and can be made to rotate; thus the apparatus is an optical spanner. We show that the spin angular momentum of +/-?per photon associated with circularly polarized light can add to, or subtract from, the orbital angular momentum to give a total angular momentum. The observed cancellation of the spin and orbital angular momentum shows that, as predicted, a Laguerre-Gaussian mode with an azimuthal mode index l=1 has a well-defined orbital angular momentum corresponding to ? per photon.     

Second Order Lagrangian and Angular Momentum of Scalar Field

The class of second order Lagrangian for the scalar field is including free divergence terms giving rise to new canonical conservation laws by means of Noethers theorem. The appearance of a spin like tensor S within angular momentum is nothing but a redefinition of orbital angular momentum. S is mainly giving a new definition of center of mass for the field, indicating that the variation for the motion of singularities is nothing but a redefinition for the motion, since the sum for the additional forces, coming from divergence part of Lagrangian, is zero. Thus, the physical content of the theory will not be affected by the divergence part of Lagrangian, is zero. Thus, the physical content of the theory will not be affected by the divergence termes; it is only an other formulation.     

Angular momentum of gaussian light beams

Analysis of the orbital angular momentum of paraxial light beams shows that a key role in the formation of this quantity is played by phase relations between longitudinal and transverse radiation fields. When a light beam is circularly polarized or has a helical wave front, the azimuthal component of the Poynting vector and the density of orbital angular momentum prove to be non-zero. In the case of circularly polarized radiation, the azimuthal component of the Poynting vector and the density of the orbital angular momentum can change the sign at different points in the cross section of the light beam, while the total orbital momentum of the beam remains quantized.     

Photoexcitation of graphene with twisted light

We study theoretically the interaction of twisted light with graphene. The light-matter interaction matrix elements between the tight-binding states of electrons in graphene are determined near the Dirac points. We examine the dynamics of the photoexcitation process by posing the equations of motion of the density matrix and working up to second order in the field. The time evolution of the angular momentum of the photoexcited electrons and their associated photocurrents are examined in order to elucidate the mechanisms of angular momentum transfer. We find that the transfer of spin and orbital angular momentum from light to the electrons is more akin here to the case of intraband than of interband transitions in semiconductors, due to the fact that the two relevant energy bands of graphene originate from the same atomic orbitals.     

Observation of the transfer of the local angular momentum density of a multiringed light beam to an optically trapped particle

We observe the spinning and orbital motion of a microscopic particle trapped within a multiringed light beam that arises from the transfer of the spin and orbital components of the light's angular momentum. The two rotation rates are measured as a function of the distance between the particle and the axis of the trapping beam. The radial dependence of these observations is found to be in close agreement with the accepted theory.