15N excitation contribution to 48Ca(16O, 15N)49Sc reaction

The effect of ¹⁵N excitation process is studied in the reaction ⁴⁸Ca(¹⁶O, ¹⁵N)⁴⁹Sc. The excitation process is included into a generalized non-local optical potential for a scattersing ¹⁵N-⁴⁹Sc and is found to be responsible for a shift of a grazing peak in the exact finite-range DWBA calculation.     

Traces of Landau-Zener transitions in the fusion cross section of heavy nuclei?

Nucleus-nucleus collisions with center-of-mass energies E_c.m. close to the Coulomb barrier are investigated within the framework of time-dependent two-center shell-model states. The influence of Landau-Zener transitions on the nucleus-nucleus potential is studied in detail as a function of E_c.m. Dynamical barrier shifts and barrier fluctuations are evaluated for central collisions of ⁹⁰Zr + ⁹⁰Zr, ⁹²Zr + ⁹²Zr, ⁹⁶Zr + ⁹⁶Zr and their effect on the fusion probability is discussed explicitly. While for ⁹⁰Zr + ⁹⁰Zr no modification of the barrier penetration is found a relative enhancement (reduction) of the fusion probability up to a factor of 4 is obtained for ⁹²Zr + ⁹²Zr and⁹⁶Zr + ⁹⁶Zr.     

Possibility of radionuclide production for PET diagnostics and brachyteraphy on the INR RAS linac

The technology of radionuclide production for positron-emission tomography on the proton linac of the Institute for Nuclear Research, Russian Academy of Sciences, is considered. A prototype of a combined target unit for production of positron-emitting radionuclides ¹¹C, ¹³N, and ¹⁸F in the proton linac beam is presented. The production of medical isotopes ¹⁰³Pd, ^{124, 125}I, and ¹³¹Cs is briefly discussed.     

A microscopical DWBA description of the charge-exchange reactions (7Li, 7Be)

The charge-exchange reaction (⁷Li, ⁷Be is described in the frame of a microscopical DWBA with central effective forces. The transition density for ⁷Li-⁷Be is calculated in two ways: with a one-particle model and with a cluster model, taking full account of recoil effects. The formalism is used for the cases of (⁷Li, ⁷Be reactions with ⁶Li and ⁴⁰Ca. Further cross sections for reactions on ¹²C and ¹⁶O with $\text{E(}{}^7\text{Li) = 78 MeV}$ and excitation energies around 4.5 and 6.2 MeV, respectively, are compared to new data obtained at the Kurchatov Institute. Here particle-hole states in an oscillator model were used to characterize the heavy system. Angular distributions are well reproduced, but absolute cross sections are 6–7 times too small. This indicates that the assumption of a direct one-step process is correct, but that tensor forces should be included as a component of the effective nucleon-nucleon force.     

Light ion fusion in deformation model

Experiments with heavy ions at moderate energies show the importance of deformation in heavy ion collisions. A deformation model which takes deformation dynamically into account is developed. Having described fusion and deep inelastic collision for a very heavy system (Xe + Bi) and a medium heavy system (Ar + Th) at various energies successfully, we turn to some comparatively lighter heavy ions where fusion is the most dominant feature. Fusion cross-sections for six pairs of lighter systems (³⁵Cl +¹¹⁶Sn,⁵⁸Ni+⁶²Ni,³⁵Cl+⁶²Ni,³²S+²⁴Mg,²⁴Mg+²⁴Mg and¹²C+²⁷Al) have been obtained using our deformation model which agree well with experiment. The two-slope-behaviour of fusion excitation function which is an important feature of light ion fusion systematics is also obtained, in our model calculations for all the systems studied.     

Partial fusion of a weakly bound projectile with heavy target at energies above the Coulomb barrier

Partial-fusion cross-sections for the systems ⁶Li + ²⁰⁸Pb, ⁹Be + ²⁰⁹Bi have been determined. The effect of breakup on fusion for weakly bound projectiles ⁶Li and ⁹Be incident on ²⁰⁸Pb or ²⁰⁹Bi targets has been discussed comparing experimental fusion cross-section excitation functions to those evaluated with a semi-classical approach. It is shown that complete fusion of a weakly bound projectile with heavy target is reduced, whereas the breakup process has very little influence on the total-fusion cross-section for some of the studied systems at energies above the Coulomb barrier.     

A theoretical study of the spectroscopic states of the CF molecule

LCAO-MO SCF calculations on the ground and excited states of CF are described. Close agreement with observed term values is obtained. The calculation of some molecular properties is discussed, and a very good result is obtained for the spin-orbit coupling in the ground state. The positive spin-orbit coupling in the ²Δ state is not explained. It is shown that the observed predissociation in the A state must be attributed to a curve crossing at a smaller internuclear distance than equilibrium, and that the ⁴Σ^- state from 5σ 2π² is responsible. Calculations show that a second-order treatment of the A ²Σ⁺-⁴∑^- interaction is necessary and sufficient to account for the predissociation.     

Microscopic description of low-energy neutron scattering by nuclei

The Bloch and Gillet shell-model formalism extended to continuum states is applied to lowenergy neutron scattering by nuclei. It is shown that complete antisymmetrization leads in the r-representation to corrective terms which yield important corrections to the scattering lengths. Calculations are performed within a model restricted configuration space for the target nuclei ¹²C, ¹³C, ¹⁶O, ¹⁷O and ⁴⁰Ca. We predict values for the spin-dependent scattering amplitude for ¹³C and ¹⁷O. The antisymmetrization problem in the case of a large configuration mixing is studied for the ¹⁹F target nucleus. The resonant effects of the compound nucleus are then very important and the results become very sensitive to the configuration space and the interaction parameters.     

Charged pion production and projectile breakup cIN 85A MeV 12C-induced heavy-ion reactions

Charged pions have been measured at 70° in coincidence with projectile-like fragments in ¹²C + ¹²C, ¹²C + ¹¹⁶Sn and ¹²C + ¹²⁴Sn reactions at 85A MeV. Neither the π⁺ emission nor the π⁻/π⁺ ratio exhibit differences for ¹²⁴Sn and ¹¹⁶Sn targets outside those expected from the isospin difference. Inconsistencies in the target mass dependence of the pion yield disappear if a correction for reabsorption is included. After this correction, we observe a strong, ~ A^1.1, mass dependence. The projectile breakup is significantly stronger for pion-producing collisions than for the average collision indicating a much stronger abundance of central collisions.     

Infrared spectra for co isotopes chemisorbed on Pt “111”: Evidence for strong absorbate coupling interactions

Previous results for ¹²C¹⁶O chemisorbed on a Pt“111” recrystallised ribbon revealed that the infrared absorption band due to the CO stretch appears at low coverages at 2063 cm^?1 and shifts to ~2100 cm^?1 at saturation coverage at 300 K. The cause of this shift is studied in the present work, by investigating the vibrational spectra from a variety of mixtures of ¹²C¹⁶O and ¹²C¹⁶O. The results show that there is a strong dipole-dipole coupling interaction between adsorbate molecules in the overlayer, and provide conclusive evidence that the 35 cm^?1 frequency shift observed with increasing coverage for ¹²C¹⁶O is attributable to coupling.     

194Pt(12C, 12C′) reaction and the triaxial-rotor model

Elastic and inelastic scattering differential cross sections for the ¹⁹⁴Pt(¹²C, ¹²C′) reaction at a bombarding energy of 78 MeV have been measured. Data have been obtained for 0⁺, 2⁺, 4⁺, and 2^+′, states in ¹⁹⁴Pt. The data have been analyzed using a rigid asymmetric-rotor model in coupled-channels reaction calculations. It is found that satisfactory fits to all data can be obtained but only if the hexadecapole deformation is included in the asymmetric-rotor model.     

Relaxation of the conductivity of CsI-Tl after excitation by subnanosecond electron pulses

The pulsed conductivity is investigated for a CsI-Tl crystal having a Tl⁺ concentration N=8×10¹⁷cm⁻³ and excited by an electron beam (0.2 MeV, 50 ps, 10²–10⁴ A/cm ²). It is shown that the amplitude of the conduction current pulse is almost an order of magnitude lower than for “pure” CsI crystals irradiated under like conditions. The conduction current relaxation time is preserved up to τ=100 ps in this case. Under the experimental conditions, therefore, the lifetime of electrons in the conduction band is controlled by trapping at Tl⁺ centers. The electron capture cross section at a Tl⁺ center is determined: σ=7×10⁻¹⁶ cm², which agrees in order of magnitude with estimates of the capture cross section for a neutral trapping center. Fiz. Tverd. Tela (St. Petersburg) 40, 66–67 (January 1998)     

Non-empirical CI potential curves for the ground and excited states of PH and its positive ion

A series of calculated potential curves is reported for the low lying valence and (selected) Rydberg states of the PH molecule by employing the multi-reference (single- and) double-excitation CI method. A large AO basis including f functions on phosphorous is chosen for this study and up to twenty main configurations are used to generate a given MRD-CI space in the accompanying theoretical treatment. Very good agreement is obtained between calculation and experiment for a variety of spectroscopic constants and a number of predictions for electronically excited states of PH are made for cases in which no comparable empirical data are yet available. The repulsive ⁵∑^- state is shown to be responsible for the predissociation of several states of the neutral system and is also thought to explain the failure to detect a number of low lying Rydberg states experimentally. Analogous calculations for the PH⁺ molecular ion have also been carried out and spectroscopic constants for this system are reported. In this case the ⁴Π state plays much the same role as the neutral ⁵∑^- species in bringing about predissociation in its electronic spectrum. Finally a comparison is made throughout between the results for PH and PH⁺ and a number of isovalent systems, especially NH and NH⁺ and also SiH.     

Alpha transfer at sub-coulomb energies in the 9Be + 16O reaction

From a detailed comparison of the sub-Coulomb-barrier cross sections for the ⁹Be + ¹⁶O and ¹²C + ¹³C reactions, it is demonstrated that there is a strong α-transfer in the channel ⁹Be + ¹⁶O→²⁰Ne¹ + ⁵He, in accord with the near optimum Q-value for the α-transfer.     

Fission fragment energy correlation measurements for the sub-barrier (nth, f) of 241Am and 243Am

Fission-fragment mass and kinetic-energy distributions and their correlations have been studied for the sub-barrier fission of the odd-odd ²⁴²Am and ²⁴⁴Am nuclei resulting from thermal neutron capture in ²⁴¹Am and ²⁴³Am. Unwanted events were eliminated by a coherence test based on the time of flight. The ²⁴³Am mass distribution is more asymmetric and shows structures at μ_H ≈ 139 and 144, compared with that for ²⁴¹Am which is smooth and structureless. The structure at μ_H ≈ 144 is caused by deformed neutron shells at N ≈ 88 in the heavy fragment and $\text{N ≧ 60}$ in the light fragment. While the 〈E_K〉 at symmetry for ²⁴¹Am is ≈ 19 MeV higher than that for ²³⁵U, it is shifted upwards only ≈ 6.5–10 MeV in the other mass regions. However, 〈E_K〉 at symmetry for ²⁴³Am is ≈ 6 MeV lower than for ²⁴¹Am and this decrease tapers down to ≈ 1 MeV for μ_H > 135. These data show a decrease in the total fragment deformation for ²⁴¹Am at symmetry as predicted by calculations. However, the ²⁴³Am data show a sudden change back to higher deformation.     

First evidence for the 2+ level in the very neutron-rich nucleus102Sr

Evidence for the 2⁺ level in¹⁰²Sr is obtained from theβ-decay of¹⁰²Rb, mass separated at the ISOLDE facility. The energy of 126 keV and the collectivity of the 2⁺→0⁺ transition indicate that¹⁰²Sr is a strongly deformed rigid rotor. In addition, a sizeable lifetime is measured for the 94 keV transition in¹⁰²Y.