Scaling behaviour of inner-shell ionization in superheavy quasi-molecules

We derive an approximate analytical formula for theK-shell ionization in collisions of very heavy atoms. The impact parameter and bombarding energy dependence are well described. The binding energy of the bound state at closest approach enters in a simple way, which could provide an experimental method for a spectroscopy of quasimolecular states.     

K X-ray satellite transitions in cobalt

Bombardment of cobalt with 42 MeV oxygen ions is seen to produce multiple inner shell electron excitation.Kα andKβ X-rays are measured and compared to Hartree-Fock-Slater calculated energies. This study of cobalt is the highestZ element where the satellite X-ray spectrum has been studied with good resolution.     

Dirac-Hartree-Fock studies of X-ray transitions in meitnerium

The K -shell and L -shell ionizations potentials for ²⁶⁸ ₁₀₉Mt were calculated at the Dirac-Hartree-Fock level taking into account quantum electrodynamic and finite nuclear-size effects. The K _α1 transition energies for different ionization states are accurately predicted and compared with recent experiments in the α -decay of ²⁷² ₁₁₁Rg .     

X-ray transitions from antiprotonic noble gases

The onset of antiprotonic X-ray transitions at high principal quantum numbers and the occurrence of electronic X-rays in antiprotonic argon, krypton, and xenon has been analyzed with the help of Multiconfiguration Dirac-Fock calculations. The shell-by-shell ionisation by Auger electron emission, characterised by appearance and disappearance of X-ray lines, is followed through the antiprotonic cascade by considering transition and binding energies of both the antiproton and the remaining electrons. Electronic lines could be attributed partly to specific states of the antiprotonic atom de-excitation.     

Pionic and muonic X-ray transitions in liquid helium

Energies and intensities of pionic and muonic X-rays in liquid ⁴He have been measured with a Si (Li) detector. The energy shift due to strong interaction effects of the pionic 1s level in ⁴He was determined to be ?75.7±2.0 eV. The natural line width of this level is 45±3 eV. These values are compared with different theoretical predictions. Cascade calculations, including external Auger effect and sliding transitions, have been performed to reproduce the yields of the muonic and pionic transitions. The pionic 2p level width is deduced: $\text{Γ}{}_{\mathrm{<mtext>2</mtext><mtext>p</mtext>}}\text{= (1.1 ± 0.5) × 10}{}^{12}\text{sec}{}^{\mathrm{?1}}\text{=}\text{(7.2±3.3) × 10}{}^{\mathrm{?4}}\text{eV}$.     

X-ray transitions in hydrogen-like,helium-like and lithium-like boron

The boron K X-ray spectra produced in heavy ion collisions using gas targets are reported. The observed X-ray transitions are used, to identify the one, two and three electron series of boron. The observed X-ray transition energies are found to agree well with theoretical calculations. A relatively large number of transitions involving double K-shell vacancies are observed. These transitions represent the first observation of double K-shell vacancies produced in collisions where the inner shell vacancies occur from electron promotion via molecular orbitals of the quasi-molecule formed during the collision.     

Magic numbers in superheavy elements

The energy density method is used to study the magic character of neutron and proton numbers corresponding to N > 126 and Z > 82. It is found that N = 184 and N = 228 are the next neutron magic numbers. For the protons, however, no sign of a shell closure appears for 82 < Z ? 130. Some simple criteria for the β^? - and α-stability of N = 184 and N = 228 isotones are also discussed.     

Interior electron shells in superheavy nuclei

The interior electron shells for superheavy nuclei (90≦Z≦250) have been investigated. Their binding energies are tabulated together with the vacuum polarization corrections for the various levels.     

Distinction between weak Auger transitions and internal X-ray photoemission

Estimates of the relative intensities of KLV Auger electrons and internally excited photoelectrons of similar energy show that the Auger process will dominate contrary to a recent suggestion by Powell.     

Doubly magic properties in superheavy nuclei

A systematic study of global properties of superheavy nuclei in the framework of the Liquid Drop Model and the Strutinsky shell correction method is performed. The evolution equilibrium deformations, TRS graphs and α-decay energies are calculated using the TRS model. The analysis covers a wide range of even-even superheavy nuclei from Z =102 to 122. Magic numbers and their observable influence occurring in this region have been investigated. Shell closures appear at proton number Z =114 and at neutron number N =184.     

Heavy and superheavy nuclei

The new elements 110, 111 and 112 were synthesized and unambiguously identified in experiments at SHIP. Due to strong shell effects the dominant decay mode is not fission, but emission of alpha particles. Theoretical investigations predict that maximum shell effects should exist in nuclei near proton number 114 and neutron number 184. Our measurements give hope that isotopes of element 114 close to the island of spherical Superheavy Elements could be produced by fusion reactions using ²⁰⁸Pb as target. Systematic studies of the reaction cross-sections indicate that transfer of nucleons is the important process to initiate the fusion.     

Doubly magic properties in superheavy nuclei

A systematic study of global properties of superheavy nuclei in the framework of the Liquid Drop Model and the Strutinsky shell correction method is performed. The evolution equilibrium deformations, TRS graphs and α-decay energies are calculated using the TRS model. The analysis covers a wide range of even-even superheavy nuclei from Z=102 to 122. Magic numbers and their observable influence occurring in this region have been investigated. Shell closures appear at proton number Z=114 and at neutron number N=184.     

Heavy-particle radioactivity of superheavy nuclei

The concept of heavy-particle radioactivity (HPR) is changed to allow emitted particles with Z(e) > 28 from parents with Z > 110 and daughter around (208)Pb. Calculations for superheavy (SH) nuclei with Z = 104-124 are showing a trend toward shorter half-lives and larger branching ratio relative to α decay for heavier SHs. It is possible to find regions in which HPR is stronger than alpha decay. The new mass table AME11 and the theoretical KTUY05 and FRDM95 masses are used to determine the released energy. For 124 we found isotopes with half-lives in the range of ns to ps.     

Research on some superheavy nuclei

Studies on some superheavy nuclei are performed. The α decay energies are calculated by an improved local binding energy formula, and the α decay half-lives are calculated by the Viola-Seaborg formula. Good agreements between theoretical and experimental results are reached.     

Transition rates of electrons in superheavy elements

Transition rates for electrons in the superheavy elementsZ=114, 126, 134, 145, 164 and 173 are calculated.K, L andM-shells are considered as final states. The 2s-1s transition of multipolarityM 1 is dominant for Z = 173 with a transition time of 10^?18 s. The radical expectation values 〈r〉 and 〈r²〉^1/2 are given.     

A pilgrimage through superheavy valley

We searched for the shell closure proton and neutron numbers in the superheavy region beyond Z = 82 and N = 126 within the framework of non-relativistic Skryme–Hartree–Fock (SHF) with FITZ, SIII, SkMP and SLy4 interactions. We have calculated the average proton pairing gap Δ_p, average neutron pairing gap Δ_n, two-nucleon separation energy S _2q and shell correction energy E _shell for the isotopic chain of Z = 112–126. Based on these observables, Z = 120 with N = 182 is suggested to be the magic numbers in the present approach.     

超重原子核与超重元素

研究超重原子核和超重元素,探索原子核的电荷和质量极限,是重要的科学前沿领域。超重原子核的存在源于量子效应。上个世纪60年代,理论预言存在一个以质子数114和中子数184为中心的超重稳定岛,这极大地促进了重离子加速器及相关探测设备的建造和重离子物理的发展。到目前为止, 实验室合成了118号及之前的超重元素。其中116号、114号和113号以下的新元素已被命名。利用重离子熔合反应合成更重的超重元素还面临着很多挑战,需要理论与实验密切结合,探索超重原子核性质与合成机制,以登上超重稳定岛。文章概要介绍了超重原子核和超重元素的研究背景、实验进展以及面临的挑战,并展望了未来的发展。     

Fusion-fission dynamics in the superheavy nucleus production

The fusion-fission reaction mechanism leading to the massive nucleus formation is studied. We investigate the superheavy nucleus formation in heavy-ion induced reactions by analysing the evaporation residue (ER) production in order to study the fusion dynamics and the decay properties of nuclei close to the stability island at Z=114. We consider the ⁶¹Ni+²⁰⁸Pb, ⁴⁸Ca+²³⁸U and ⁴⁸Ca+²⁴⁴Pu reactions that lead to the Z=110, 112 and 114 superheavy elements respectively. By using the dinuclear system (DNS) concept of the two interacting nuclei we calculate the quasifission-fusion competition in the entrance channel and the fission-evaporation competition along the de-excitation cascade of the compound nucleus. The dynamics of the entrance channel allows us to determine the beam energy window which is favorable to the fusion, while the dynamic evolution of the compound nucleus on the shell correction to the fission barrier and the dissipative effects influence the fission-evaporation competition in order to obtain the residue nuclei from the superheavy nucleus formation. We also calculate the τ _n /τ_tot ratio at each step of the de-excitation cascade of the compound nucleus and we present a systematics of τ _n /τ_tot (at first step of the cascade) for many reactions that lead to nuclei with Z=102–114.