Coherent crystallization of bismuth under strong excitation by ultrashort laser pulses

By means of coherent control, fully symmetric bismuth phonons A _1og are investigated at helium temperature depending on the degree of crystal excitation. It is shown that coherent phonons with large amplitude show phase rigidity that is absent at small amplitude. Such a change in the phase properties of crystal lattice excitations can be understood using the concept of a coherent crystal, the achievement of which results from condensation of phonon modes arising with increasing degree of excitation.     

Controlling Rydberg excitation process with shaped intense ultrashort laser pulses

We perform a theoretical investigation on the control over the atomic excitation of Rydberg states with shaped intense ultrashort laser pulses. By numerically solving the time-dependent Schr?dinger equation(TDSE), we systematically study the dependence of the population of the Rydberg states on the π phase step position in the frequency spectra of the laser pulse for different intensities, central wavelengths and pulse durations. Our results show that the Rydberg excitation process can be effectively modulated using shaped intense laser pulses with the laser intensity as high as 1 × 10~(14) W/cm~2. Our work also have benefit to the future investigation to find out the dominant mechanism behind the excitation of Rydberg states in strong laser fields.     

Phase control of the excitation of a two-level system with short laser pulses

The possibility of the phase control for the excitation of a quantum system in the discrete spectrum under the action of a short high-intensity laser pulse with a controlled phase is theoretically analyzed. The analysis is performed using the example of the simplest two-level system (TLS) employing a numerical solution to equations for the optical Bloch vector. It is demonstrated that the excitation probability and the mean dipole moment of the quantum system, which determine the normal luminescence and the superradiance in the TLS ensemble, respectively, substantially depend on the phase of the laser pulse for relatively short and powerful laser pulses.     

Phase control of excitation of NV centers in diamond by ultra-short laser pulses

This Letter is a theoretical investigation of the excitation of NV centers in diamonds under ultra-short laser pulses with variable parameters. Calculations are based on the two-level approximation and Bloch formalism using dimensionless variables. The dependency of excitation probability on the carrier-envelope phase was examined for various values of electric field strength and pulse duration.     

Coherent excitation of molecular vibrational modes by high-power ultrashort infrared laser pulses

Coherent dynamics of multiphoton excitation of molecular vibrational modes by subpicosecond IR laser pulses differs greatly from that of picosecond pulse excitation. The resonance response of a molecule is primarily determined by the power broadening rather than the laser carrier frequency. Selective excitation of high vibrational levels is possible with the use of subpicosecond pulses.     

Measurement of ultrashort laser pulses

A proposal for measuring the pulse shape of ultrashort laser pulses is described. The proposed method consists of a Gamo triple intensity-interferometer to measure the triple-correlation function of the light pulses. A subsequent signal processing algorithm is used to reconstruct the true shape of the light pulses out of their triple-correlation function. The suggested method is quite insensitive to noise, as shown by means of computer simulations.     

Vortices in ultrashort laser pulses

The propagation of optical vortices nested in broadband femtosecond laser beams was studied both numerically and experimentally. Based on the nonlinear Schrödinger equation, the dynamics of different multiple-vortex configurations with varying topological charge were modelled in self-focussing and self-defocussing Kerr media. We find a similar behavior in both cases regarding the vortex–vortex interaction. However, the collapsing background beam alters the propagation for a positive nonlinearity. Regimes of regular and possibly stable multiple filamentation were identified this way. Experiments include measurements on pairs of filaments generated in a vortex beam on an astigmatic Gaussian background with argon gas as the nonlinear medium. Spectral broadening of these filaments leads to a supercontinuum which spans from the visible range into the infrared. Recompression yields <19 fs pulses. Further optimization may lead to much better recompression.     

Microablation with ultrashort laser pulses

This paper reports the micromachining results of different materials (Al, Si, InP and fused silica) using a Ti : sapphire laser at the wavelength of 800 and 267 nm with variable pulse lengths in the range from 100 fs to 10 ps. The hole arrays with a diameter up to a few μm through microdrilling are presented. We discussed how an effective suppression of the thermal diffusion inside the ablated materials and an effective microablation could be realized. If the laser fluence is taken only slightly above the threshold, a hole array can be drilled with diameters even smaller than the wavelength of the laser. Some examples are presented in the paper.     

Single-mode excitation of multimode fibers with ultrashort pulses

Single-mode excitation of step-index multimode fibers with light sources with short temporal coherence lengths is demonstrated. Multimode fiber designs with reduced microbending-induced mode coupling are described that allow the propagation of the fundamental mode over long lengths with negligible mode coupling even in the presence of tight fiber bends. At a wavelength of 1.56microm a fiber with a core diameter of 45microm can preserve the fundamental mode for a propagation length of ~20m . Such fibers allow coiling with a coil diameter as small as 7cm.     

Molecular wakes for ultrashort laser pulses

The molecular wake-assisted interaction between two collinear femotosecond laser pulses is investigated in air,which leads to the generation of a controllable 1.8 mJ super-continuum pulse with an elongated self-guided channel due to the cross-phase modulation of the impulsively aligned diatomic molecules in air. For two parallel launched femtosecond laser pulses with a certain spatial separation,controllable attraction and repulsion of the pulses are observed due to the counter-balance among molecular wakes,Kerr and plasma effects,where the molecular wakes show a longer interaction distance than the others to control the propagation of the intense ultrashort laser pulses.     

Phase modulation of intense ultrashort laser pulses reflected from steep, dense plasmas

The phase modulation of intense ( I = 10(18) W/cm(2)) ultrashort laser pulses ( tau(p) = 70 fs) after reflection from steep, dense plasmas has been temporally resolved for the first time in particle-in-cell simulations. The position of the turning point from where the pulse reflects has been compared to the phase modulation, over a range of angles of incidence. At normal incidence or s polarization the phase modulation almost exactly represents the movement of the turning point due to the light pressure. As the angle of incidence is increased for p polarization, the simple Fresnel relationship between phase modulation and displacement of the reflection position, Delta phi(t) = -2k(0)Delta x(t)cos theta(0), increasingly breaks down.     

Nonlinear transmission of ultrashort laser pulses by a thin semiconductor film under conditions of a two-photon two-pulse excitation of biexcitons

Specific features of the nonstationary transmission of two pulses exciting biexcitons from the ground state in a thin semiconductor film are studied. It is shown that one of the incident rectangular pulses is totally reflected from the film, whereas the second pulse passes through it as through an absolutely transparent medium. Criteria for appearance of a stationary bistable transmission are determined.     

Micromachining of quartz with ultrashort laser pulses

Received: 6 January 1997/Accepted: 1 April 1997     

Automated spatiotemporal diffraction of ultrashort laser pulses

We exploit the close similarities between time-frequency and position-wave-vector correspondences to control the spatiotemporal diffraction pattern of ultrashort laser pulses. This approach permits novel, automated generation of sophisticated two-dimensional femtosecond waveforms. A two-dimensional space-time version of a Gerchberg-Saxton algorithm is used to iteratively determine the phase pattern in position-frequency space that produces a user-defined intensity profile in wave-vector-time space.     

Real-time chirp diagnostic for ultrashort laser pulses

Using a real-time Fourier-transform algorithm, we present a simple technique for measuring the chirp of femtosecond laser pulses. We demonstrate significantly enhanced sensitivity compared with standard autocorrelation measurements.     

Hybrid optics for focusing ultrashort laser pulses

We present a specially designed hybrid optics comprising refraction and diffraction effects for tight spatial and temporal focusing of ultrashort laser pulses. Both aims can be put into practice by having a high numerical aperture (NA=0.45) and low internal dispersion at the same time. We are presenting what we believe is the first experimental realization of such a hybrid short plus focusing optics. The focusing properties are compared with a commonly used microscope objective (20 X, NA = 0.45) in theory and experimentally.     

New laser crystals for the generation of ultrashort pulses

Since the beginning of the 1990s, titanium sapphire has become the crystal of choice for the development of ultrashort laser systems producing very short and powerful pulses using the Chirped Pulse Amplification technique. In parallel to these developments leading to commercial products, new laser crystals have been studied in order to reach directly other wavelength ranges and to overcome the need to develop cw or pulsed green laser to pump the titanium sapphire crystal. In order to be able to directly pump the crystals with a very efficient and high-power semiconductor laser, new crystals doped with chromium or ytterbium ions have been developed. This article will review the latest development in this research field with the best performances obtained in terms of pulse duration. To cite this article: F. Druon et al., C. R. Physique 8 (2007).     

Remote sensing of the atmosphere using ultrashort laser pulses

Theoretical and experimental studies were performed on the propagation of ultrashort optical terawatt pulses through the atmosphere. Propagation simulations of intense sub-picosecond pulses show that non-linear processes, such as white light generation, can be initiated at a chosen distance by selecting an appropriate group velocity dispersion. With this technique, a white light continuum was generated in the atmosphere whose spectral distribution was characterised in the visible and near infra-red. Applications of this novel light source for atmospheric remote sensing were investigated, combining lidar and time-resolved broadband absorption spectroscopy techniques. Measurements were performed on the oxygen molecule and water vapour. A comparison between the experimental results and the tabulated spectroscopic data led to an excellent correlation with measurements made on water vapour whereas observations on the oxygen showed discrepancy. This study demonstrates that the remote generation of a white light source represents a new way to access the range-resolved multi-trace gas analysis in the atmosphere. Received: 8 December 1999 / Revised version: 18 May 2000 / Published online: 16 August 2000