抽运光强度对光学抽运重水气体产生THz激光的影响分析

利用半经典理论，对脉冲光学抽运重水气体产生THz激光信号过程进行分析，对其中抽运光强度与输出THz信号光之间的关系进行了数值计算和求解，结果表明，THz信号出射光强度跟抽运源入射光强度之间不满足简单的线性关系，而是呈现高阶的非线性关系.在工作介质腔长、气压和工作温度一定的条件下，存在最佳抽运光强度，在一定的抽运光强范围内，THz信号出射光强度与抽运源入射光强度的关系呈现近似线性的增长关系，抽运光能量和信号光能量之间的转换效率相对较高，当抽运光强超过一定值时，由于瓶颈效应的发生会导致THz输出信号的逐步减弱，并产生一定的频率调谐范围.     

Raman自由电子激光的半经典理论

采用Ｔｈｏｍａｓ-Ｆｅｒｍｉ近似势，将多电子系统简化为单电子问题，并用微扰论求解了Ｋｌｅｉｎ-Ｇｏｒｄｏｎ方程．由电子的零级波函数求得了电荷密度和电流密度的零级表达式．通过适当简化Ｋｌｅｉｎ-Ｇｏｒｄｏｎ方程，用分离变量和ＷＫＢ近似，求得了电子波函数及相应的电荷密度与电流密度的表达式 关键词：     

THz自由电子激光椭圆型耦合输出光腔

在对中国工程物理研究院高功率太赫兹（THz）自由电子激光（FEL）装置理论分析和设计的基础上,针对目前THz FEL光腔设计面临的主要难点,提出了椭圆型耦合输出光腔的设计方案,并对椭圆型耦合输出光腔代替传统FEL光腔的优势、光腔品质、耦合效率等进行了分析研究。研究表明,椭圆型耦合光腔的设计更适合目前THz FEL波导光腔的光斑特点,可使光腔输出功率提高33%以上,输出耦合效率即光腔品质可提高30%~70%;随着辐射频率的提高,椭圆孔耦合输出光腔的优势提高更为明显。     

THz自由电子激光椭圆型耦合输出光腔

在对中国工程物理研究院高功率太赫兹（THz）自由电子激光（FEL）装置理论分析和设计的基础上,针对目前THz FEL光腔设计面临的主要难点,提出了椭圆型耦合输出光腔的设计方案,并对椭圆型耦合输出光腔代替传统FEL光腔的优势、光腔品质、耦合效率等进行了分析研究。研究表明,椭圆型耦合光腔的设计更适合目前THz FEL波导光腔的光斑特点,可使光腔输出功率提高33%以上,输出耦合效率即光腔品质可提高30%~70%;随着辐射频率的提高,椭圆孔耦合输出光腔的优势提高更为明显。     

激光能量对气体等离子体产生太赫兹波的影响

双色激光脉冲激励气体等离子体产生太赫兹波是得到高强度宽频带太赫兹波的重要方法,本文利用光电流模型研究了该方法中激光能量对产生太赫兹波的影响。理论计算表明,太赫兹波随激光能量的增大而增强,而太赫兹波的频谱结构不受激光能量的影响。分析了双色激光能量影响太赫兹波强度的原因,并利用自由电子浓度和电子电流密度诠释了该影响的内在物理机制。该研究为提高太赫兹辐射强度提供了一种有效的途径。     

自由电子激光辐射场的经典理论分析

以经典电动力学分析自由电子激光辐射场,讨论辐射场的一般特性,并利用麦克斯韦方程组、波动方程、电子连续性方程以及相对论电子运动的洛伦兹力方程和能量方程一起系统地建立了自由电子激光辐射场的自洽解方法. 关键词：     

光泵亚毫米波激光的理论模型及计算方法(Ⅰ)——半经典密度矩阵理论

该作者曾对光泵亚毫米波激光作过系统深入地的研究。重点论述在小型光泵亚毫米波激光的理论研究中所应用的量子系统的半经典密度矩阵理论。     

中物院高功率THz FEL装置的理论分析和优化设计

在1~3 THz频段内设计了11个分点频率,对每一频率的对应的场强和电子束能量进行了选取和计算。模拟结果表明:采用目前参数基本能够达到设计要求;辐射频段在2.6 THz附近时装置输出功率和增益都比较高,可以先锁定这个频段附近进行实验的调试;在长波段即1 THz左右时,滑移效应显著,腔增益和输出功率较低,实验实现比较困难,因此在1 THz频段附近必须积极想办法来提高输出功率。     

中物院高功率THz FEL装置的理论分析和优化设计

在1~3 THz频段内设计了11个分点频率,对每一频率的对应的场强和电子束能量进行了选取和计算。模拟结果表明:采用目前参数基本能够达到设计要求;辐射频段在2.6 THz附近时装置输出功率和增益都比较高,可以先锁定这个频段附近进行实验的调试;在长波段即1 THz左右时,滑移效应显著,腔增益和输出功率较低,实验实现比较困难,因此在1 THz频段附近必须积极想办法来提高输出功率。     

非三维空间的经典气体模型

类似于三维空间中的方法，推导了一、二、四维空间中经典气体的气体动理论的相应的公式和常数，与三维空间的情况做了比较。     

Injection seeding for single-mode operation in an optically pumped high-power D2O laser

Spectrally narrow, pulsed outputs consisting of almost a single mode have been obtained from an optically-pumped high-power (200kW) D₂O laser by adopting the injection seeding method, where single-mode radiation (seed pulse) from a low-power, compact D₂O laser has been injected into the main D₂O laser. Spectrally narrow outputs with high power having spectral widths as narrow as 5 MHz have been obtained, when the seed pulses with frequency tuned to one longitudinal mode of the main D₂O laser have been injected at a time sufficiently before the lasing of the main laser took place. The experimental results have been compared with those of numerical simulation modified to include the injection field with varying injection times.     

Far-infrared hydrazine laser pumped by an N2O laser

We have used an N₂O laser to optically pump N₂H₄ molecules in a far-infrared cavity and observed 17 new laser lines in the wavelength range 93.0 to 374.2 μm, the 136.8 μm line pumped by 10P(16) being a doublet. We measured the frequencies of the laser lines by heterodyne mixing of the far-infrared radiation with radiation from two frequency-stabilized CO₂ lasers.     

The rotational Raman spectra and cross sections of H2O, D2O, and HDO

We report the experimental rotational Raman spectra of H₂O, and of a mixture of D₂O and HDO in the vapor phase at room temperature, and their interpretation in terms of rotational–vibrational energies, wavefunctions, and transition moments of the molecular polarizability. These transition moments are based on high-level ab initio calculations of the wavelength dependent polarizability surface, and on wavefunctions where the rotational–vibrational coupling is considered in detail. As a byproduct of this analysis several tables have been compiled including scattering strengths and assignments for individual rotational transitions of the three species. From these tables the rotational Raman spectra can be simulated over the range of temperatures up to 2000 K for H₂O, and up to 300 K for D₂O and HDO.     

The Raman spectra and cross-sections of the ν2 band of H2O, D2O, and HDO

We report the experimental Raman spectra of the ν₂ band of H₂O, D₂O, and HDO in the vapor phase at room temperature. A complete interpretation of the Raman intensities is carried out employing the variational rovibrational wavefunctions obtained from a Hamiltonian in Radau coordinates and an ab initio polarizability surface at 514.5 nm. We show the importance of the rotation-vibration coupling to obtain the correct line intensities. Several tables with the assignments of the individual rotational-vibrational transitions and their Raman scattering strengths are reported. From these tables, the ν₂ Raman spectra can be simulated up to 2000 K for H₂O, and up to 300 K for D₂O and HDO.     

Submillimeter emission lines from CD2Cl2 optically pumped lasers

Fifty-five new submillimeter laser lines from optically pumped CD₂Cl₂, have been obtained in a FIR metallic waveguide resonator. Twenty-seven lines, ranging from 184 m to 1387 m, and twenty-eight lines, from 219 m to 888 m, have been observed when using CW CO₂ laser and CW N₂O laser optical pumping, respectively. The accuracy of wavelength measurements are of the order of 3.10^–3.     

不同初始振动态下D2O在B带的态-态光解动力学

利用高精度的非绝热从头算势能面,采用量子实波包方法研究了D₂O在3个不同初始振动态(0,1,0)、(1,0,0)和(0,0,1)下光激发到~B态解离过程的态-态量子动力学．结果表明,由于初始振动波函数的形状不同,从不同振动态产生的吸收光谱、产物分布和产物分支比具有不同的动力学特性．弯曲振动态(010)的吸收谱呈现出两波瓣的形状且中间具有较浅的极小值,其基态产物OD( ~X)在高能量区域会出现轻微的振动态反转现象．所有初始振动态得到的激发态产物OD(_?)的振-转态分布都随能量的变化出现强烈的震荡,这是由于受到了激发态势能面上长寿命共振态的影响．反对称伸缩振动态(0,0,1)在高能量区域具有较大的产物分支比OD(_?)/OD( ~X),表明绝热通道在某些情形下是主要的解离通道．     

Frequencies of cw FIR laser lines from optically pumped CH2F2

The frequencies of 48 optically pumped cw FIR CH₂F₂ laser lines have been measured relative to stabilized CO₂ lasers. Uncertainties are estimated to be about 5 parts in 10⁷.     

Far-infrared laser action in vinyl chloride, vinyl bromide, and vinyl fluoride optically pumped by a CW N2O laser

This paper reports the first use of a N₂O laser for optically pumping vinyl halides, to obtain new cw submillimeter laser lines. Eighteen far-infrared (FIR) emissions have been observed in vinyl chloride, twenty five in vinyl bromide and thirty eight in vinyl flouride.     

The Raman spectra and cross-sections of H2O, D2O, and HDO in the OH/OD stretching regions

We report the OH and OD stretching regions of the vapor phase Raman spectra of H₂O, and of a D₂O/HDO mixture, at room temperature. Also, the corresponding spectrum of H₂O at ∼2000 K in a methane/air flame is reported. These spectra are interpreted in terms of transition moments of the molecular polarizability, based on high-level ab initio calculations of the polarizability surface, and on variational wavefunctions considering the rotational-vibrational coupling in full. As a byproduct of this analysis several tables have been compiled including scattering strengths and assignments for individual rotational transitions of the three species. From these tables the Raman spectra in the OH/OD stretching regions can be simulated over the range of temperatures up to 2000 K for H₂O, and up to 300 K for D₂O and HDO.