The stimulated Raman scattering competition between solute and solvent in Rhodamine B solution

The competition between the stimulated resonance Raman scattering (SRRS) of Rhodamine B (RhB) and the stimulated Raman scattering (SRS) of ethanol (C₂H₅OH) is observed at the RhB in C₂H₅OH solution. For different concentrations of the solution, the peak wavelengths of the SRRS, the amplified spontaneous emission (ASE), the fluorescence and the absorption of RhB are different. The SRRS of RhB and the SRS of C₂H₅OH are simultaneously generated when the concentration of the solution is 10^-5 mol/L and the energy of the excitation laser is 20.4 mJ. Otherwise, only either the SRRS of RhB or the SRS of C₂H₅OH is generated. The SRRS can be amplified by the ASE gain when the SRRS is near the peak of the ASE, and the peak wavelength of the SRRS coincides with the wavelength of the maximal intensity ASE.     

罗丹明B荧光增强苯受激拉曼散射研究

将液芯光纤技术与荧光增强受激拉曼散射技术相结合,能够大大增强受激拉曼散射光谱强度,降低受激拉曼散射阈值。通过对罗丹明B苯溶液在液芯光纤中的受激拉曼散射进行研究,结果表明:荧光染料Rhodamine B可以降低苯溶液的各阶受激拉曼散射阈值近一个数量级;在一定浓度范围内(10-6mol/L~10-8mol/L)各阶Stokes阈值随浓度降低而降低,并在理论上给出了解释。并且理论推导了在荧光种子作用下的四阶耦合波方程。液芯光纤中的受激拉曼光谱技术在对实现宽带受激辐射激光器、种子激光,以及生物大分子结构研究、生物分子的非生物过程研究等领域等有光明应用前景。     

Soliton experiments in stimulated Raman scattering

Experimental observations of solitons in stimulated Raman scattering are reported. Soliton formation resulted from the introduction of a phase shift in the incident Stokes beam as predicted by theory. Pulse sharpening and retardation on propagation in the Raman medium have been observed along with amplitude diminution. The first two features were predicted and the third was not. Spontaneous soliton formation has been observed in the absense of any amplitude modulation or apparent phase shift in the optical fields, indicating that additional sets of initial conditions may result in soliton formation.Work performed under the auspices of the U.S. Department of Energy.     

水中受激拉曼散射的能量增强及受激布里渊散射的光学抑制

为提高液体介质中受激拉曼散射的输出能量,提出了通过温度调控来抑制受激布里渊散射的方法,设计了532 nm多纵模宽带脉冲激光泵浦的受激拉曼散射发生系统,测量了不同温度下水中前向受激拉曼散射及后向受激布里渊散射的输出能量,分析了水温、泵浦激光线宽及热散焦效应对受激拉曼散射输出能量影响的物理机制.实验结果表明:通过降低水温可实现对受激布里渊散射过程的有效抑制,同时减小热散焦效应带来的光束畸变,从而有效提高受激拉曼散射的输出能量.研究结果对液体介质中的受激拉曼散射多波长转换具有重要意义.     

分子间费米共振增强二元溶液体系的受激拉曼散射研究

研究了液芯光纤内不同体积比的甲苯和间二甲苯二元混合溶液的受激拉曼散射.实验结果表明:在不同的体积比之下二元溶液的环呼吸振动模式1002 cm^-1,甲基的CH伸缩振动模式2920 cm^-1 以及芳香环CH对称伸缩振动模式3058 cm^-1的拉曼带同时产生受激拉曼辐射,并且2920 cm^-1 和 3058 cm^-1 拉曼带的一阶受激拉曼散射阈值要低于1002 cm^-1拉曼带的二阶 关键词： 分子间费米共振 二元溶液 受激拉曼散射 拉曼散射截面     

碰撞对受激Raman散射的影响

从动力学方程出发，引入有效碰撞，讨论了碰撞对受激Raman散射线性增长率的影响.结果表 明，碰撞阻尼和Landau阻尼使得受激Raman散射线性增长率有了实质性的下降，受激Raman散 射只能发生在电子温度和电子密度平面的一个有限区域.现在的理论模型能够解释受激Raman 散射光谱上存在的“缝”(gap)现象. 关键词： 受激Raman散射 碰撞阻尼 线性增长率     

光纤中强受激喇曼散射时的自相位调制

在光纤-光栅对激光脉冲压缩中,由于受激喇曼散射和自相位调制的竞争,使得泵浦激光脉冲波形重整,且自相位调制谱极不对称。本文用2m的单模保偏光纤,在产生较强的受激喇曼散射的情况下,得到较为对称的泵浦激光的自相位调制功率谱,并讨论了自相位调制功率谱的一些特点。     

KDP晶体受激拉曼散射特性

详细比较了磷酸二氢钾(KDP)晶体的自发拉曼散射和受激拉曼散射光谱,在受激拉曼散射(SRS)中观察到了自发拉曼散射中最强的振动模的三阶Stokes光(559.43,589.74,623.50nm),由于其他振动模的受激拉曼散射增益系数较小,其SRS光谱未观察到。另外,比较了传统生长的未退火和退火后的KDP晶体及快速生长的锥区和柱区KDP晶体的受激拉曼散射增益系数,结果表明生长方法和热退火对KDP晶体的受激拉曼散射增益系数无明显影响。     

KDP晶体受激拉曼散射特性

详细比较了磷酸二氢钾(KDP)晶体的自发拉曼散射和受激拉曼散射光谱,在受激拉曼散射(SRS)中观察到了自发拉曼散射中最强的振动模的三阶Stokes 光(559.43, 589.74, 623.50 nm),由于其他振动模的受激拉曼散射增益系数较小,其SRS光谱未观察到。另外,比较了传统生长的未退火和退火后的KDP晶体及快速生长的锥区和柱区KDP晶体的受激拉曼散射增益系数,结果表明生长方法和热退火对KDP晶体的受激拉曼散射增益系数无明显影响。     

Optimization of a Raman/EDFA hybrid amplifier based on dual-order stimulated Raman scattering using a single-pump

Based on dual-order stimulated Raman scattering (SRS) of a single 1395 nm Raman fiber laser in 75 km single mode fiber and its corresponding dispersion compensation module, a hybrid Raman/Erbium doped fiber amplifier (EDFA) for long wavelength band (L-band) amplification is realized by inserting a segment of EDF within the span. By comparing the performance of gain and noise in four hybrid amplifiers with different span configurations, we find that the distribution of the secondary L-band amplification obtained from the EDF along the link has a great influence on the performance of the hybrid amplifier. Both gain and noise performance of hybrid amplifier can be improved significantly by optimizing the location of the EDF. Moreover, we can extend the flat gain bandwidth from L-band to central wavelength band (C-band) plus L-band by recycling the residual first-order SRS to pump a segment of EDF with proper length.     

高保偏光纤前方受激拉曼散射光谱特性的研究

系统的研究了石英系高保偏双折射光纤的受激拉曼光谱的特性,给出了七级斯托克斯谱和一级反斯托克斯谱.测试了各级拉曼谱的阈值、谱宽和拉曼增益，分析了形成各级拉曼谱的能量转移机理.     

用激光增益获取弱增益拉曼模式的受激拉曼散射光谱

当酒精的弱增益拉曼模式处于罗丹明640染料分子的激光增益范围时，在由悬垂液滴构成的圆形谐振腔中，观察到乙醇分子C—H伸缩系列模中多个弱增益拉曼模式的受激拉曼散射（SRS）光谱.随着抽运光的增强，迅速增长的强增益拉曼模式的受激辐射抑制了其他弱增益模式的SRS，并导致染料激光的完全淬灭.通过分析圆形腔腔模的光子速率方程和激光染料分子的三能级粒子数速率方程，解释了观察到的实验现象. 关键词： 受激拉曼散射 悬垂液滴 弱拉曼增益模式 激光增益     

激光等离子体相互作用的受激拉曼散射饱和效应

在激光等离子体相互作用过程中,受激拉曼散射（SRS）会通过Langmuir波衰减不稳定性（LDI）和电子俘获两种机理饱和.文章给出均匀一维等离子体和低强度非相对论激光作用中,LDI和电子俘获两种机理下的SRS饱和时间的解析表达式.SRS饱和时间与入射激光强度,电子密度,电子温度,初始电子密度微扰等参数有关.解析理论计算得到了与模拟和实验相符的结果. 关键词： 受激拉曼散射 饱和 Langmuir波衰变不稳定性（LDI） 电子俘获     

光纤通信中有色散影响的受激喇曼散射信道特性研究

提出了在波分复用光纤通信系统中，考虑光纤色散“走离”时受激喇曼散射(SRS)信道的新模型,给出了计算中距离步长的选取公式。根据该模型，数值计算了各信道在随机数字序列调制下和在受激喇曼散射(SRS)非线性效应作用下经过有色散“走离”的波分复用光纤系统的传输功率。得出光纤色散会降低SRS效应引起的输出功率波动的结论,画出了在SRS效应作用下输出功率标准差随色散系数变化的曲线，并对产生该现象的机理进行了定性分析。该模型适合于任意光纤色散、任意输入功率和任意信道数目。     

激光等离子体受激Raman散射光谱的时间分辨测量

采用光学多道谱仪和光学条纹相机耦合,组成时间分辨的Raman散射光谱测量系统,可实现0.5nm的光谱分辨和好于10ps的时间分辨。采用该测量系统,在神光Ⅱ装置上开展了脉宽1ns、波长351nm的激光与两种不同尺寸柱腔靶相互作用的物理实验,获得了时间分辨的SRS光谱实验结果。研究表明,SRS光谱在时间上相对于入射激光有一定的延迟,腔靶尺寸减小时,延迟时间随之减小。通过长、短波截止波长分析电子密度方法,计算得出了Ⅰ型和Ⅱ型腔靶SRS散射光最短波长光谱发生的密度区分别为0.069nc和0.027nc。     

Femtosecond soliton generation induced by intrapulse stimulated Raman scattering in optical fibers

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苯C—H伸缩振动弱增益模式的受激拉曼散射

对苯的长拉曼振动模式C—H(3060 cm^-1线)伸缩振动的一阶受激拉曼散射进行了实验研究.利用在苯溶液中加入甲苯溶液,在液芯光纤内实现了苯的全对称C—H伸缩振动3060 cm^-1线的受激拉曼散射.利用等离子体解释了这一增强机理. 关键词： 液芯光纤 受激拉曼散射 等离子体     

基于光纤中SRS效应的全光波长转换

提出利用光纤中非线性效应受激喇曼散射（stimulated Raman scattering, SRS）实现波长转换的原理方案和相应的理论分析模型,并进行实验验证,将经过放大后的信号光和连续探测光同时注入光纤,在光纤中进行SRS放大,实现信号之间的转换。结果表明:利用SRS可实现波长转换,可实现跨几个THz的波长之间的转换。得到最大转换效率和消光比分别为-17.3 dB和15.7 dB。通过改变探测光的波长,可实现相隔几个THz光信号的全光波长转换和可调谐波长转换。     

Effects of Landau damping and collision on stimulated Raman scattering with various phase-space distributions

Stimulated Raman scattering (SRS) is one of the main instabilities affecting success of fusion ignition. Here, we study the relationship between Raman growth and Landau damping with various distribution functions combining the analytic formulas and Vlasov simulations. The Landau damping obtained by Vlasov-Poisson simulation and Raman growth rate obtained by Vlasov-Maxwell simulation are anti-correlated, which is consistent with our theoretical analysis quantitatively. Maxwellian distribution, flattened distribution, and bi-Maxwellian distribution are studied in detail, which represent three typical stages of SRS. We also demonstrate the effects of plateau width, hot-electron fraction, hot-to-cold electron temperature ratio, and collisional damping on the Landau damping and growth rate. They gives us a deep understanding of SRS and possible ways to mitigate SRS through manipulating distribution functions to a high Landau damping regime.     

Temperature measurements in condensed phases using non‐resonant femtosecond stimulated Raman scattering

We have previously demonstrated the capability of femtosecond stimulated Raman scattering (FSRS) data to measure the temperature (T) of condensed matter at the molecular vibrational level. [Phys. Rev. Lett. 2011, 107, 43001] In this paper, we expand the theory for the FSRS temperature dependence by considering the effects of an isolated change of T as well as a coupled change of T and chemical concentration. We point out that the origin of the temperature sensitivity of the Stokes to anti‐Stokes ratio of FSRS lies in the exponential nonlinearity of the gain and loss. We establish that FSRS of two Raman modes can be used to simultaneously determine the vibrational temperature and the change in concentration of the species contributing to those two modes. Single‐shot experimental results using FSRS are presented to demonstrate over four orders of magnitude higher efficiency than spontaneous Raman in small volume samples with picosecond resolution. Copyright © 2012 John Wiley & Sons, Ltd.