温度调谐MgO：LiNbO3晶体光参量振荡器

采用调Q Nd:YAG激光倍频光(0.532μm)泵浦温度调谐MgO:LiNbO_3晶体单、双谐振光参量振荡器(OPO包括DRO、SRO)的实验结果.双谐振(DRO)调谐范围达844.1～1411.3nm,最低泵浦阈值0.22mJ/pulse;单谐振(SRO)调谐范围达738.9～1032.2nm,最低泵浦阈值0.66mJ/pulse.最大能量转换效率为10.4%.     

Continuous spectral measurements of the optical absorption of glasses over the visible and near-infrared wavelength ranges

A calorimetric method for continuous measurements of the optical absorption of bulk glasses over the spectrum extending from the visible to the near-infrared wavelength ranges is presented. A relation between the absorption and the induced temperature rise of the sample, at thermal equilibrium, is derived. Details for the most convenient arrangement of source, lens and monochromator are given. As an example, experimental results are plotted for a F2 glass.     

Efficient intracavity generation of visible pulses in a femtosecond near-infrared optical parametric oscillator

We have achieved efficient simultaneous intracavity doubling of the signal frequency and sum-frequency generation between the signal and the pump in a periodically poled LiNbO(3) femtosecond optical parametric oscillator pumped by a Ti:sapphire laser. The responsible mechanisms are second-, third-, and fourth-order quasi-phase matching (QPM). An ~56% poling duty cycle permits efficient even-order QPM. Femtosecond pulses tunable in the visible were generated with a total efficiency of more than 8% for only 480-mW pump power at 80 MHz. Optimization of the poling duty cycle can improve the efficiency further.     

Efficient periodically poled stoichiometric lithium tantalate optical parametric oscillator for the visible to near-infrared region

A compact, efficient optical parametric oscillator (OPO) for the visible to near-infrared region based on periodically poled stoichiometric lithium tantalate pumped by a frequency-doubled multikilohertz Q-switched Nd:YAG laser is demonstrated. Up to 61% photon conversion with a 71% slope efficiency for photon conversion from 532 nm to the signal radiation was measured. We observed that the efficient conversion diminished the potential for photorefractive damage induced by the 532 nm radiation in the crystal and made sustained operation of the OPO device possible.     

High-energy quasi-phase-matched optical parametric oscillation in a 3-mm-thick periodically poled MgO:LiNbO3 device

We have demonstrated high-energy quasi-phase-matched optical parametric oscillation in a 3-mm-thick periodically poled 5-mol. % MgO-doped LiNbO3 device with a 32.1-microm grating period and a 30-mm length. With a large-spot-size pump laser of 2.2-mm diameter, we obtained a total output pulse energy of 22 mJ for both the signal (wavelength 1.82 microm) and the idler (2.56 microm) waves at an input pump energy of 46 mJ.     

High-efficiency mid-infrared laser from synchronous optical parametric oscillation and amplification based on a single MgO:PPLN crystal

This paper presents a specially designed optical parametric oscillator (OPO) which achieved high-efficiency mid-infrared laser of 2.83 μm. The cascaded nonlinear interactions of OPO and optical parametric amplifier (OPA) were simultaneously realized in a single MgO:PPLN crystal. The signal oscillation of 1.70 μm was used to pump a secondary parametric process that resulted in amplification of the idler laser of 2.83 μm. When the MgO:PPLN crystal with a grating period of 31.2 μm was pumped by a 1.064 μm laser and operated at 148°C, the quasi-phase-matching of both OPO and OPA could be simultaneously achieved. Average output power of 7.68 W at 2.83 μm was obtained for 25 W of pump at 7 kHz. The power conversion efficiency of 2.83 μm laser was 30.7%, which was evidently higher than common OPOs.     

High-energy quasi-phase-matched optical parametric oscillation in a periodically poled MgO:LiNbO3 device with a 5 mm x 5 mm aperture

Fabrication of a 5 mm thick periodically poled MgO-doped LiNbO3 device with a 32.1 microm period for mid-infrared generation was demonstrated. The periodic structure was evaluated by measurement of second-harmonic generation with the d31 coefficient. Optical parametric oscillation using this device with an uncoated 5 mm x 5 mm aperture and a 36 mm effective length realized a high-energy output of 77 mJ for both signal (wavelength 1.83 microm) and idler (2.54 microm) waves with a 72% slope efficiency at 110 mJ pumping of a Q-switched Nd:YAG laser with a 12 ns pulse duration.     

Low-threshold mid-IR MgO:PPLN optical parametric generation with high reflectivity mirror for signal wavelength

A low-threshold middle-infrared(mid-IR) MgO:PPLN optical parametric generation(OPG)pumped by a laser diode(LDl end-pumped Z-type Nd:YLF laser at 1047 nm is realized with high reflectivity(HR) mirror for signal.At repetition rate of 10 kHz,the OPG threshold of 50μJ has been achieved with HR mirror for signal.Compared with the threshold without mirror,the threshold decreases by 17%.Using HR mirror for pump at output side of crystal,the threshold of 40μJ is achieved.The 2.7-4.1μm continuous tunable output is produced with seven grating periods from 28.5 to 31.5μm and temperatures from 30 to 200℃.When the incident average pump power is 3 W.the OPG idler output power is 0.46 W at 3.26 μm,which corresponds to optical-to-optical conversion efficiency up to 15.3%.     

Single optical cycle laser pulse in the visible and near-infrared spectral range

Since the inception of the laser, pulse duration has been continuously decreased by the use of a variety of techniques: Q-switching, mode-locking, and pulse compression. We would like to present a new technique based on the addition of laser sub-harmonic, ALS, that allows the production of a single-cycle pulse with single-femtosecond pulse duration. This simple technique takes advantage of the recent progress made in the generation of a few optical cycles and in optical parametric amplification. Received: 10 March 1999 / Revised version: 17 May 1999 / Published online: 30 July 1999     

Efficient noncollinear parametric amplification of weak femtosecond pulses in the visible and near-infrared spectral range

We report measurement of efficient amplification of weak femtosecond supercontinuum seed pulses by use of a noncollinear optical parametric process in BBO crystal pumped with 150-fs pulses from a frequency-doubled regenerative-amplified Ti:sapphire laser at 390nm . The highest amplification factor, 10(8) , was achieved for 3x10(-16)J energy seed pulses at wavelength of 560nm.     

Refractive,dispersive and thermo-optic properties of twelve organic solvents in the visible and near-infrared

We report on experimental measurements of the refractive index of twelve organic solvents at five different wavelengths (450, 532, 632.8, 964 and 1,551 nm) and a temperature of 300 K. Based on these new data visible to near-infrared dispersion relations are constructed. Group-velocity dispersion (GVD) is theoretically calculated. Zero- and negative-GVD situations are identified for two common solvents in near-infrared wavelengths. Via comparison with refractive index data available in bibliography, estimated values of thermo-optic coefficients are also presented.     

Tunable femtosecond laser in the visible range with an intracavity frequency-doubled optical parametric oscillator

We demonstrated experimentally a synchronously pumped intracavity frequency-doubled femtosecond optical parametric oscillator (OPO) using a periodically-poled lithium niobate (PPLN) as the nonlinear material in combination with a lithium triborate (LBO) as the doubling crystal. A Kerr-lens-mode-locked (KLM) Ti:sapphire oscillator at the wavelength of 790 nm was used as the pump source, which was capable of generating pulses with a duration as short as 117 fs. A tunable femtosecond laser covering the 624-672 nm range was realized by conveniently adjusting the OPO cavity length. A maximum average output power of 260 mW in the visible range was obtained at the pump power of 2.2 W, with a typical pulse duration of 205 fs assuming a sech2 pulse profile.     

Internal Q-switching and self-optical parametric oscillation in a two-dimensional periodically poled Nd:MgO:LiNbO3 laser

We report on an internally Q-switched self-optical parametric oscillator (SOPO) based on a monolithic two-dimensional (2D) periodically poled Nd:MgO:LiNbO(3) (Nd:MgO:PPLN) integrating three device functionalities of a laser gain medium, an electro-optic Bragg Q-switch, and an optical parametric gain medium (OPGM). The quasi-phase-matching conditions required by the Bragg Q-switch and OPGM are both satisfied in the 2D nonlinear photonic crystal (NPC) structure formed in the Nd:MgO:PPLN. A 1525 nm signal with a pulse energy of ～3.3 μJ (>350 W peak power) was obtained from the SOPO at 8.5 W diode pump power. An off-angle signal at 1612 nm, amplified by a unique gain-enhancement effect in this 2D NPC, was also observed. Tuning of the SOPO in the eye-safe region was demonstrated.     

Photorefractive properties of highly-doped lithium niobate crystals in the visible and near-infrared

Light-induced refractive-index changes, bulk-photovoltaic current densities, and photoconductivities of photorefractive iron-doped lithium niobate crystals (iron concentrations between 0.02 and 0.17 wt. %) are investigated in detail using visible and near-infrared light. It turns out that the one-center model predicts the material performance correctly for small iron concentrations (c_Fe<0.06 wt. % Fe₂O₃), only. A strong increase of the photoconductivity for higher doping levels limits the space-charge fields. Refractive-index changes up to 7×10^-4 for green and 2.8×10^-4 for near-infrared ordinarily polarized light are obtained. The corresponding hologram multiplexing numbers are 11 for green and 5 for near-infrared light. Received: 18 November 1998 / Revised version: 8 January 1999 / Published online: 7 April 1999     

飞秒光参量振荡器中非线性晶体的空间啁啾与角色散

对飞秒光参量振荡器的空间啁啾和角色散进行了理论计算和分析.给出了在非线性晶体中的空间啁啾表达式，以及在BBO晶体Ⅰ类非共线相位匹配情况下，在角度调谐过程中非线性晶体包括角色散在内的二阶、三阶色散的解析表达式，并精确计算了角色散对其二阶、三阶色散的影响. 关键词： 飞秒光参量振荡器 空间啁啾 角色散 二阶、三阶色散     

Visible,near-infrared and infrared optical properties of silica aerogels

Silica aerogel is an excellent thermal insulation material with a low thermal conductivity and a high porosity and has attracted great concern in applications. This paper was to experimentally investigate the optical properties of optically thick silica aerogel in the visible, near-infrared and infrared spectrum region. The fiber-loaded silica aerogel sample was prepared through sol–gel technique and supercritical drying process. Silica fibers were added into the aerogel during the preparation procedure to strength the skeleton of aerogel. As a comparison with the fiber-load silica aerogel, a silica fiber composite sample with the same chemical component and different physical structure was also prepared. A simplified two-flux model neglecting the boundary effect was used to describe the radiation propagation characteristics inside the samples. The spectral normal-hemispherical reflectances, transmittances, and normal emittances of silica aerogel and silica fiber samples were measured and compared in the wavelengths of 0.38–15 μm. Then the spectral optical constants of samples were determined using the experimental data. The spectral absorption and scattering coefficients of silica aerogel were within (0.01 cm⁻¹, 31.0 cm⁻¹) and (1.4 cm⁻¹, 25.8 cm⁻¹). The results showed that the spectrum region where the scattering coefficient is low usually corresponds to a high absorption coefficient. In addition, the total radiation properties of samples were predicted at high temperatures. The analysis of optical properties of silica aerogel is necessary to provide valuable data in applications.     

Tunable synchronously-pumped fiber Raman laser in the visible and near-infrared exploiting MOPA-generated rectangular pump pulses

We report a tunable synchronously pumped fiber Raman laser (SPFRL) in the near-infrared (NIR) and visible wavebands pumped by a pulsed, all-fiber PM 1060 nm master oscillator power amplifier (MOPA) and its frequency-doubled output, respectively. The seed was adaptively shaped to deliver rectangular output pulses, thereby enabling selective excitation of individual Raman Stokes lines. Using filtered synchronous feedback of the desired Raman Stokes line, the linewidth of the SPFRL was reduced by a factor of 4 and the extinction ratio of the desired Raman Stokes was improved by more than 3 dB relative to a simple single-pass conversion scheme. A continuous tuning range of 2.2 THz was obtained for each of the Raman Stokes orders in the visible (spanning from green to orange-first to fifth Stokes lines). A larger 5.0 THz tunable range was achieved in the NIR spectral region.     

Linear and nonlinear optical properties of MgO:LiTaO3

We derive new temperature dependent Sellmeier equations for the extra-ordinary and ordinary refractive indices of 0.5% MgO-doped stoichiometric LiTaO₃ crystal. The equations are based on quasi phase-matched frequency conversion measurements, as well as on interferometric measurements of the thermal expansion and thermal dispersion. These equations fit experimental data over wide spectral ranges: 0.35–6 μm for the extra-ordinary wave and 0.375–3.75 μm for the ordinary wave, from room temperature up to 200°C. The nonlinear optical measurements set lower-limit values for the d ₃₃, d ₂₂, and d ₂₄ elements of the second-order susceptibility tensor χ ⁽²⁾ of 12.9, 1.54, and 0.46 pm/V, respectively. The interferometric measurements enable one to determine the linear and quadratic expansion coefficients of 1.45762e?5 1/°C, and 2.68608e?8 (1/°C)², respectively. The Sellmeier equations are in good agreement with previously published data.     

Pulse-front-matched optical parametric amplification for sub-10-fs pulse generation tunable in the visible and near infrared

A noncollinear optical parametric amplifier is presented that generates transform-limited sub-10-fs pulses that are tunable in both the visible and the near infrared (NIR). The pulse-front-matched pump geometry realizes tilt-free signal amplification, and pulses as short as 6.1 fs can be obtained from 550 to 700 nm. The large angular dispersion of the idler specific to the group-velocity-matching interaction is effectively eliminated by a grating-telescope compensator, and 9-fs NIR pulses are also successfully obtained from 900 to 1300 nm. This is believed to be the first tunable sub-10-fs light source.     

Diode-pumped singly resonant continuous-wave optical parametric oscillator with wide continuous tuning of the near-infrared idler wave

We demonstrate wide, continuous tuning of the single-frequency idler wave of a cw singly resonant optical parametric oscillator (SRO). The SRO consists of a periodically poled LiNbO(3) crystal for quasi-phase matching in a four-mirror signal-resonant ring cavity. The SRO, excited by 2.25 W of 924-nm radiation from an InGaAs diode laser, generates as much as 200 mW of single-frequency 2.1-mum idler radiation. We tune the idler frequency continuously within a range as large as 56 GHz by changing the wavelength of the diode pump laser. The versatility of this continuously tunable single-frequency infrared source is demonstrated by recording of N(2)O rovibrational absorption lines near 2.1 mum.