飞秒超强激光驱动太赫兹辐射特性的实验研究

强太赫兹源是太赫兹科学技术发展的关键,其中大能量强场太赫兹脉冲源在超快物态调控、新型电子加速器等领域具有重要的应用前景.超快超强激光与等离子体相互作用是近年来发展起来的一种新型的强场太赫兹辐射产生途径.本文报道了利用超强飞秒激光脉冲与金属薄膜靶作用产生太赫兹辐射的实验结果,研究了激光能量和离焦量对靶后太赫兹辐射能量的影响,并通过监测激光背向散射光谱,定性揭示了其变化规律与不同光强下的电子加热机制的相关性.实验表征了太赫兹辐射的频谱、偏振及聚焦光斑情况.测量结果表明,实验产生了脉冲能量达458μJ、聚焦场强高达GV/m量级的超宽带太赫兹辐射,为开展极端太赫兹脉冲与物质相互作用研究提供了一种新的强场太赫兹光源.     

Calcul de l'emission infrarouge de milieux laser CO2

Vibrationally-excited CO₂ present with inverted population emits infrared radiation at 4·26 μm. For an emitter consisting of optically-thick isolated lines, calculations allow determination of the emissivity and radiancy of a homogeneous layer of gas. Infrared emission is a useful tool for measurement of the energy contained in the upper laser level. A very thin layer of cold gas strongly alters the spectral distribution of the intensity and causes the total radiancy to decrease.     

激光脉冲宽度对有质动力加速电子的影响

基于真空中单电子运动模型,编程计算得到了高斯激光脉冲与初始位于激光传播轴上电子的相互作用结果。不同激光参鼍条件下,得到了电子的能量增益与激光强度、焦斑大小和脉冲宽度关系。结果表明,高斯激光脉冲焦斑较大时,电子没有明显的能量增益,高斯激光脉冲焦斑太小时,电子也没有明显的能量增益。电子的能量增益有一个最佳焦斑大小。在相同激光强度下,电子能量增益的最佳焦斑大小随脉冲宽度的增大而增大,但最佳焦斑大小与脉冲宽度的比值基本上是不变的。     

高能电子与超强激光束作用产生的阿秒脉冲列

利用非线性汤姆孙散射的理论，从理论和数值模拟上研究了单电子在横向穿越高斯激光束束 腰时所辐射的x射线阿秒脉冲列的性质. 主要分析了电子以初始能量γ₀=1M eV—100M eV横向穿越激光振幅参数为a₀=1—10的高斯光束束腰获得的阿秒辐射脉冲的 时间 和空间性质. 计算表明，辐射呈现脉冲列的形式. 脉冲列的包络宽度取决于激光强度、束腰 的宽度以及入射电子能量. 电子的初始能量比激光强度对电子辐射脉冲的影响更大. 辐射脉 宽、脉冲间隔和脉冲包络宽度都正比于1/γ²₀，辐射功率正比于 γ⁶₀，辐射能 量正比于γ⁴₀. 当改变激光振幅a₀时，辐射功率正比 于a²₀、辐射包络中单 个脉冲脉宽正比于1/a₀、脉冲之间的间隔正比于a₀. 当保持激光强 度不变，而改变光束 束腰半径w₀时，辐射的脉冲数量、包络和辐射能量正比于w₀. 当 激光功率保 持不变时而改变激光强度和束腰半径时，脉冲包络宽度和最大辐射能量都基本不变. 当激光 振幅参数a₀=1，电子初始能量为10MeV时，激光束腰为两个激光波长时，电子 辐 射脉冲包络宽度只有14×10^-3τ₀（τ₀为入 射激光周期），达到几个阿秒的量级. 关键词： 阿秒脉冲 非线性汤姆孙散射 高斯激光光束     

Formation of periodic surface nanostructures on Ti:Al2O3 crystals using femtosecond laser pulses

Periodic surface nanostructures are observed on Ti³⁺:Al₂O₃ single crystals that have been irradiated by a single focused beam from a femtosecond pulsed laser (wavelength: 800 nm; pulse duration: 130 and 152 fs). Atomic force microscopy images of single-ablated zones and modified structures created by fixing and translating samples through the focal region of a linearly polarized laser beam reveal self-organized periodic surface nanostructures (ripples) with a subwavelength spacing, which are oriented perpendicular to the electric-field vector of the laser beam. The period of the subwavelength ripples obtained by linearly polarized laser irradiation varies from ∼λ/5 to 2λ/5 (λ: incident laser wavelength) depending on the laser pulse energy. This phenomenon can be explained by assuming that the incident light field interferes with the electric field of electron plasma waves propagating inside the material; this interference periodically modulates the electron plasma density and modifies the surface ablation. In addition, for the first time, we observe screw-shaped nanostructures in the focal spot of circularly polarized beam irradiation. The morphology of these nanostructures appears to reflect the circular polarization of the laser light.     

On the focusing limit of high-power femtosecond laser pulse propagation in air

Focused propagation of high-power femtosecond laser radiation in air is considered. Based on numerical solution of the nonlinear Schr?dinger equation for complex envelope of light wave electric field, evolution of the beam effective radius is studied. The dependence of the effective (rms) size of a focal spot and the maximally achievable intensity of laser radiation at focal waist on the initial pulse power is established. It is shown that focal spot of tightly focused intensive ultrashort laser radiation can change its size during the pulse passage through the beam waist. This is the consequence of pulse intensity clamping in region of beam focusing caused by gas photoionization and plasma producing. This may prevent laser intensity from its further growth in the focal region and arrest the transversal compression of the beam in the linear focus as a whole.     

激光能量叠加过程中对准精度对焦斑的影响

利用多光束激光输出耦合叠加是一种提高激光器输出功率的有效方法。采用两束矩形激光对准系统,分析两光束不同对准情况下的焦斑特性。完全对准的情况下,两束光的远场焦斑重合在一起,焦斑能量是两光束能量之和。在实际光束对准系统中,讨论了三种常见的对准误差,并比较了这些误差对焦斑特性的影响。利用ZEMAX软件对设计系统进行了模拟分析,并进行了实验验证。结果表明,元件的位置误差会使远场焦斑能量集中度降低,焦斑半径增大。     

Laser plasmatron for diamond coating deposition

An experimental installation with a laser plasmatron based on a continuous wave CO₂ laser with a radiation power of up to 3.5 kW has been created. The plasmatron design makes it possible to bring out the plasma jet into atmospheric air both along and across the laser beam direction. The spatial temperature distributions on the metal substrate surface heated by the plasma jet are measured. The threshold power for optical discharge maintenance as a function of the gas flow rate and the focal length of the focusing lens are obtained for an Ar and Ar/CH₄/H₂ gas mixture under atmospheric pressure; the radiation spectrum of the discharge plasma is measured. A one-dimensional model of the discharge for estimation of its geometrical parameters in a convergent laser beam with consideration of radiation refraction on the discharge is given.     

Effect of phonon spectrum heating on the formation of laser-induced electron plasma in wide-gap insulators

The effect of lattice heating by laser pulses on the dynamics of electron plasma generation in transparent solids has been theoretically studied. Several ways of taking into account the contribution of the phonon spectrum heating to the electron avalanche dynamics, depending on the type of the effective (with respect to the field energy transfer to electrons) phonons and laser pulse duration, have been proposed. A comparative analysis of the results of Monte Carlo computation of electron gas heating in the laser pulse field, which were obtained for cold and heated lattices, has been performed. It is shown that the consideration of the effect of lattice heating on the probabilities of electron-phonon and electron-phonon-photon scattering leads to an increase in the avalanche rate, which is more pronounced at longer wavelengths of the incident radiation and under longer laser pulses. Some qualitative features of the redistribution of the energy, absorbed during a pulse, between the electron plasma and lattice are revealed, which suggest initiation of irreversible microscopic changes in the insulator. In particular, the ratio R of the energy accumulated in the electron subsystem to the excess (with respect to the initial equilibrium state) energy in the phonon subsystem has been calculated for different initial lattice temperatures. It is shown that this ratio increases with a decrease in the laser wavelength in the computation scheme with lattice heating disregarded and decreases at all pulse durations when the lattice heating is taken into account.     

超强激光与固体气体复合靶作用产生高能氦离子

激光氦离子源产生的MeV能量的氦离子因有望用于聚变反应堆材料辐照损伤的模拟研究而得到关注.目前激光驱动氦离子源的主要方案是采用相对论激光与氦气射流作用加速高能氦离子,但这种方案在实验上难以产生具有前向性和准单能性、数MeV能量、高产额的氦离子束,而这些氦离子束特性是材料辐照损伤研究中十分关注的.不同于上述激光氦离子产生方法,我们提出了一种利用超强激光与固体-气体复合靶作用产生氦离子的新方法.利用这种方法,在实验上,采用功率密度5×10~(18)W/cm~2的皮秒脉宽的激光脉冲与铜-氦气复合靶作用,产生了前向发射的2.7 MeV的准单能氦离子束,能量超过0.5 MeV的氦离子产额约为10~(13)/sr.二维粒子模拟显示,氦离子在靶背鞘场加速和类无碰撞冲击波加速两种加速机理共同作用下得到加速.同时粒子模拟还显示氦离子截止能量与超热电子温度成正比.     

Efficiency of an electron-beam-pumped chemical laser with an SF6-H2 working mixture

Results are presented from a study of HF lasers pumped by non-chain chemical reactions initiated by a radially convergent and by a planar electron beam. The main channels of formation of vibrationally excited HF molecules are analyzed. The distribution of the energy density of the radiation in the output beam of a wide-aperture laser is measured. In 30 liters of a mixture of SF₆:H₂=8:1 at a pressure of 1.1 atm an output energy of ∼200 J is obtained at an ∼11% efficiency with respect to the energy deposition. It is shown that the admixture of a buffer gas of neon or argon improves the uniformity of the radiation energy distribution in the output beam of an HF laser pumped by a non-chain chemical reaction and initiated by an electron beam, and it also increases the output energy. Zh. Tekh. Fiz. 69, 76–81 (January 1999)     

Radiation damping effects on the interaction of ultraintense laser pulses with an overdense plasma

A strong effect of radiation damping on the interaction of an ultraintense laser pulse with an overdense plasma slab is found and studied via a relativistic particle-in-cell simulation including ionization. Hot electrons generated by the irradiation of a laser pulse with a radiance of I lambda(2)>10(22) W microm(2)/cm(2) and duration of 20 fs can convert more than 35% of the laser energy to radiation. This incoherent x-ray emission lasts for only the pulse duration and can be intense. The radiation efficiency is shown to increase nonlinearly with laser intensity. Similar to cyclotron radiation, the radiation damping may restrain the maximal energy of relativistic electrons in ultraintense-laser-produced plasmas.     

Research of laser evaporation of fast-moving target

Evaporation of a stainless steel target moving with high speed (～50 m/s) under action of laser radiation was investigated theoretically and experimentally. In our experiments we used an electroionization CO₂—laser, which generated pulses with duration up to 1 ms and energy up to 100 J. We carried out the microscopic research of laser beam trace on the target surface and investigated the dynamics of the laser plume luminescence. For theoretical research we used 3D numerical model, which took into account: heating, melting and evaporation of target by laser beam, and, thermal effect of oxidation reaction. The results of calculations can explain the experimental data quite good. In particular, it is possible to explain occurrence of interrupted trace on the target at 12–24 kW laser power, that corresponds to intensity in the focal spot of ～10⁷ W/cm². This power is a threshold of unstable mode of laser evaporation. The unstable mode is caused by lack of oxygen, which was pushed away with metal vapor. The lack of oxygen leads to shutting down the oxidation reaction on target surface. The reaction resumes when the vapors fly away and oxygen riches the surface. As the result pulsed mode of evaporation takes place. This phenomenon was observed as pulse mode of laser plume luminescence and was obtained by calculations.     

High precision materials processing using a novel Q-switched CO2 laser

Holes with diameters of about 400 µm have been laser trepanned in Ti6Al4V and carbon fibre reinforced polymer (CFRP) thin sheets with a thickness of 0.5 mm. A commercial CO₂ laser (SM1500E, FEHA LaserTec, Germany) and a novel Q-switched CO₂ laser (µ-storm, IAI, Netherlands) were used as radiation sources. Optical microscopy, scanning electron microscopy and replicas of the processed holes were used to investigate the influence of the CO₂ laser pulse parameters (e.g. pulse energy, duration and peak power) on the processing quality. It was shown that melt formation and high temperature oxidation reactions of Ti6Al4V during thermal laser processing were reduced significantly by using short and high intense Q-switched CO₂ laser pulses. During trepanning of CFRP heat affected zones resulting from the extremely different thermal properties (melting and vaporisation temperature, heat conduction) of the reinforcing carbon fibres and the polymer matrix were reduced significantly by using the Q-switched CO₂ laser. The results demonstrate that Ti6Al4V and CFRP can be processed very precisely with CO₂ laser radiation and air as processing gas without melt formation and thermal damage.     

神光Ⅲ原型黑腔物理实验研究

总结了在神光Ⅲ原型激光装置上开展的一系列黑腔物理实验研究,从多个方面研究了黑腔内部等离子体状态和辐射场特性。用真空黑腔能量学研究获得了散射光、辐射温度和不同能段辐射流份额的定标规律,从能量学角度梳理和分析了整个激光黑腔相互作用过程。通过对黑腔中充入低密度低Z气体抑制了腔壁等离子体运动,明显减少了可能造成靶丸预热的金M带辐射流(1.6~4.4keV)份额。针对黑腔内部不同区域等离子体,研究了光斑区等离子体的运动,分析了其与电子热传导限流因子的关系;研究了冕区等离子体的运动,分析了不同充气等离子体条件对其的影响;在同一发次实验中同时测量了光斑区与再发射区的辐射流比值。     

Formation of nanobumps and nanoholes in thin metal films by strongly focused nanosecond laser pulses

Nanobumps and nanoholes have been formed in gold and silver films with various thicknesses on a dielectric substrate by strongly focused single nanosecond pulses of a Nd:YAG laser. An apertureless dielectric fiber probe and an aspherical lens with a numerical aperture of 0.5 were used to focus laser radiation into a diffraction-limited spot on the surface of gold and silver films, respectively. Atomic force and electron microscopy studies have demonstrated that the shape and dimension of nanostructures, as well as the threshold parameters of laser radiation for their formation, are determined by the thickness of a modified film (“size effect”) and by the duration of a laser pulse owing to the lateral heat conduction in films (nonlocal energy deposition effect). Mechanisms of the dynamic formation of such structures in metallic films by nanosecond laser pulses due to phase transformations of their material have been discussed.     

Attosecond X-ray pulse obtained from linear Thomson scattering

Linear Thomson scattering by a relativistic electron of a short pulse laser has been investigated by computer simulation. Under a laser field with a pulse of 33.3-fs full-width at half-maximum, and the initial energy of an electron of γ₀=10, the motion of the electron is relativistic and generates an ultrashort radiation of 76-as with a photon wave length of 2.5-nm in the backward scattering. The radiation under a high relativistic energy electron has better characteristic than under a low relativistic energy electron in terms of the pulse width and the angular distribution.     

超短超强激光导引及对电子加速的影响

使用粒子模拟程序对30 fs超短超强激光在均匀与抛物型两种密度分布等离子体中的传输, 以及在稳定传输状态下尾场的电子注入与加速形成的电子能谱进行了模拟与分析. 固定入射激光束斑尺寸, 在(0.4-2)×10¹⁹/cm³等离子体密度范围, 对比分析了归一化峰值强度从1-6范围的激光脉冲在上述两种密度分布等离子 体中传输时激光束斑尺寸的演化, 结果表明抛物型分布的等离子体密度通道能够对超短超强脉冲实现良好的导引, 有利于高能电子加速. 对于较高密度情况,即使在均匀等离子体中依靠相对论自聚 焦等机制也可以实现良好的自导引传输,有利于实验简化以及产生更大电量的加速电子.     

Numerical solution of Boltzmann tranport equation for TEA CO2 laser having nitrogen-lean gas mixtures to predict laser characteristics and gas lifetime

Selective laser isotope separation by TEA CO₂ laser often needs short tail-free pulses. Using laser mixtures having very little nitrogen almost tail free laser pulses can be generated. The laser pulse characteristics and its gas lifetime is an important issue for long-term laser operation. Boltzmann transport equation is therefore solved numerically for TEA CO₂ laser gas mixtures having very little nitrogen to predict electron energy distribution function (EEDF). The distribution function is used to calculate various excitation and dissociation rate of CO₂ to predict laser pulse characteristics and laser gas lifetime, respectively.Laser rate equations have been solved with the calculated excitation rates for numerically evaluated discharge current and voltage profiles to calculate laser pulse shape. The calculated laser pulse shape and duration are in good agreement with the measured laser characteristics. The gas lifetime is estimated by integrating the equation governing the dissociation of CO₂. An experimental study of gas lifetime was carried out using quadrapole mass analyzer for such mixtures to estimate the O₂ being produced due to dissociation of CO₂ in the pulse discharge. The theoretically calculated O₂ concentration in the laser gas mixture matches with experimentally observed value. In the present TEA CO₂ laser system, for stable discharge the O₂ concentration should be below 0.2%.     

Investigation of Shock Wave Loading and Crater Creation by Means of Single and Double Targets in the PALS-Laser Experiment

The efficiency of crater creation for different types of Al targets, namely, single massive targets and double targets consisting of a foil or a disk placed before the massive target at a chosen distance (300 and 500 µm), is studied. Targets were irradiated by the PALS facility laser beam with E _L = 100 – 400 J at the first harmonic λ = 1315 nm, a focal spot radius of 125 µm, and pulse duration of 400 ps. Velocities of the accelerated foil’s fragments or disks and electron density distributions of the plasma streams are determined by means of three-frame interferometry. Shapes and volumes of craters are obtained using the crater replica technology and microscopy measurements. It is shown that direct laser action is the most efficient way of energy transfer to the massive target and the most efficient method of crater creation. Somewhat lower efficiencies of shock wave loading and crater creation in comparison with direct laser action are found in the case of double targets where the energy is transferred to the massive target by colliding laser-driven foils or disks. The efficiencies of such a colliding energy transfer are close to 60% for foils and 40% for disks. The experimental results are in a good agreement with two-dimensional hydrodynamic models of shock wave generation under direct laser action and laser-driven macroparticle impact.