Propagation of Gaussian beams in negative-index metamaterials with cubic nonlinearity

Propagation of Gaussian beams in the negative-index metamaterials (NIMs) with cubic nonlinearities is investigated, both theoretically and numerically. The role of the status of the incident Gaussian beam, which is scaled by a converging parameter in this paper, in beam self-focusing and self-defocusing in NIMs is specially identified. The expressions for beam self-focusing and self-defocusing for different converging parameter cases, and the dependence of the critical power and the focus location of self-focusing in NIMs on the converging parameter are obtained. It is found that it is the divergent rather than convergent incident beams which are self-focused more quickly in NIMs with defocusing nonlinearities, in sharp contrast with the propagation property of Gaussian beams in conventional Kerr media, in which beam self-focusing only occurs in the media with focusing nonlinearities and a convergent incident beam self-focuses more quickly than a divergent one. By adjusting the converging parameter of incident Gaussian beam or the controllable magnetic permeability of NIM, or both, one can manipulate the beam self-focusing in NIMs at will.     

Propagation of four-petal Gaussian beams in strongly nonlocal nonlinear media

The propagation of four-petal Gaussian beams in strongly nonlocal nonlinear media has been studied. The analytical solution and the analytical second-order moment beam width are obtained. For the off-waist incident and the waist incident cases, the intensity pattern evolves periodically during propagation in strongly nonlocal nonlinear media. Under the off-waist incident condition, the second-order moment beam width varies periodically during propagation, whatever the input power is. But under the waist incident condition, there exists a critical power. When the input power equals the critical power, the second-order moment beam width remains invariant, otherwise the second-order moment beam width varies periodically. Numerical simulations based on the nonlocal nonlinear Schrödinger equation are carried out for comparison with the theoretical predictions. The results show that the numerical simulations are in good agreement with the analytical results in the case of strong nonlocality.     

Phase matched vectorial three-wave mixing in isotropic Kerr media

A theoretical analysis of vectorial three-wave mixing in isotropic Kerr media is presented. The analysis based on the coupled-wave equations describes the amplification of a weak wave by coupling with a strong pump wave phase matched by optically induced change of average refractive index. The phase matching condition for interacting waves with different polarizations is calculated, allowing a large amplification of a weak wave by three-wave mixing in thick Kerr media. The main conclusions of our theoretical analysis are supported by the results of experiments in CS₂ liquid medium.     

Formation of Hot Images in Laser Beams through a Self-defocusing Kerr Medium Slab

A nonlinear hot image is usually thought as of a special case of self-focusing, and thus occurs when a laser beam propagates through a slab of self-focusing medium. Here we show theoretically that a hot image may also be formed by a thin slab of self-defocusing medium. The physical origin for this hot image formation is akin to the in-line volume-phase holographic imaging due to the intensity-dependent refractive-index modulation of the self- defocusing medium. NumericM simulations confirm the theoretical prediction and further identify the dependence of the hot image on the beam power, the modulation depth of obscuration and the thickness of self-defocusing medium. The analysis presented here brings new insight into the physics of hot image formation in the high power laser system.     

Theoretical study of saturable Kerr nonlinearity using top-hat beam Z-scan technique

Saturable Kerr nonlinearity is theoretically investigated by use of the top-hat beam Z-scan technique. The saturation intensity changes the nonlinear refractive profile and decreases the sensitivity of the Z-scan measurements, which were quantitatively analyzed. An empirical formula for the saturable Kerr nonlinearity, which gave the relationship between the light intensity and the peak-valley transmittance difference, was accomplished. A high-accuracy method to determine the nonlinear refractive index and the characteristic saturation intensity was proposed.     

Wavefront study in a Gaussian beam passed through a nonlinear optical medium

We present a numerical model to study the wavefront of a Gaussian laser beam propagated through a nonlinear Kerr media. The model is based on the Gaussian decomposition method. The interaction between a laser beam and a self-focusing or self-defocusing media is discussed from the viewpoint of wavefront distortion. The method is useful for simulation of the wavefront of the beam next to the sample. We also compare our results with those obtained from z-scan method. There is a quite good agreement between data from z-scan method and our results.     

Optical vortices in self-focusing Kerr nonlinear media

In this work we numerically compare the interaction of optical vortices (OVs) in self-defocusing and self-focusing Kerr nonlinear media. We find that the basic scenarios (attraction/repulsion, translation/rotation vs. background) in the interaction of two and three vortices with equal and alternative topological charges (TCs) are the same in both media. However, the vortex dynamics under self-focusing conditions is influenced by the reshaping of the surrounding part of the background. Square structure of OVs with alternating TCs is found to be stable with respect to the vortex positions in self-focusing media. This elementary cell is successfully generalized in a large square array of OVs with alternative TCs which brings ordering in the multiple filamentation of the background beam in self-focusing conditions.     

Ultra fast third-order non-linear response of amino-triazole donor-acceptor derivatives by optical Kerr effect

We report the study of the temporal dependence of the non-linear optical response of novel organic materials in solution. The experimental results of the optical Kerr gate using 70 fs pulses show a quasi-instantaneous response for three derivatives of an amino-triazole donor-acceptor system. The non-linearity of the compounds is identified as arising from the electronic contribution to the third-order non-linear susceptibility. The non-linear parameters of each sample were obtained using the optical Kerr response of CS₂ as reference.     

Transformation of a hollow Gaussian beam into a ring-shaped beam using a phase aperture

Propagation of a hollow Gaussian beam diffracted by a circular phase aperture is studied without making the paraxial approximation. The analytical expression of the intensity of the apertured hollow Gaussian beam is presented in the far field. The influences of the truncation parameter and the order of hollow Gaussian beam on the intensity distributions are discussed. It is shown that a circular ?-phase aperture can be used to transform a hollow Gaussian beam into a ring-shaped beam in the far field with the appropriate parameters.     

Polarization properties of SC generated in CaF2

Polarization of SC generated by 80 fs pulses of Ti:Sapphire laser strongly depends on the orientation of CaF₂ plate with respect to the plane of polarization of the pump light. Intensity modulation of the broad blue-shifted wing of SC against crystal rotation for the polarization parallel and orthogonal to the polarization of the pump beam is observed with CaF₂ and Sapphire. Observed modulation is due to evolution of the polarization state along the propagation distance in crystal.     

High sensitive measurements of absorption coefficient and optical nonlinearities

Accurate knowledge of absorption coefficient of a sample is a prerequisite for measuring the third-order optical nonlinearity of materials, which can be a serious limitation for unknown samples. We introduce a method, which measures both the absorption coefficient and the third-order optical nonlinearity of materials with high sensitivity in a single experimental arrangement. We use a dual-beam pump-probe experiment and conventional single-beam z-scan under different conditions to achieve this goal with communication relevant wavelength. We also demonstrate a counterintuitive coupling of the non-interacting probe-beam with the pump-beam in pump-probe z-scan experiment.     

The origin of the super-resolution via a nonlinear thin film

In laser applications, resolutions beyond the diffraction limit can be obtained with a thin film of strong optical nonlinear effect. The optical index of the silicon thin film is modified with the incident laser beam as a function of the local field intensity n(r)∼E²(r). For ultrathin films of thickness d?λ, the transmitted light through the film forms a profile of annular rings. Therefore, the device can be related to the realization of super-resolution with annular pupils. Theoretical analysis shows that the focused light spot appears significantly reduced in comparison with the diffraction limit that is determined by the laser wavelength and the numerical aperture of the converging lens. Analysis on the additional optical transfer function due to the thin film confirms that the resolving power is improved in the high spatial frequency region.     

Theoretical study on stability of Z-scan technique by use of quasi-one-dimensional slit beam

The modified Z-scan technique using the quasi-one-dimensional slit (QODS) beam for characterizing the third-order optical nonlinearity has been reported recently. In the present work, we investigate the effect of the finite length of the slit in the QODS beam Z-scan for the practical experimental conditions, and then give an empirical expression that allows the direct estimation of nonlinear refraction coefficient from the measured normalized peak-valley transmittance difference. In particular, we explore relatively in detail the influences of the sample imperfection on the Z-scan traces, such as the hollow hole of the sample and the nonuniform nonlinearity. Compared with the other Z-scan techniques, such as the top-hat and Gaussian-beam Z-scans, we find that the QODS beam Z-scan has the great improvement for the sample imperfections. The results suggest that the QODS beam Z-scan is a more promising and useful technique for characterizing the optical nonlinearity of an imperfect sample.     

Simultaneous estimation of optical nonlinear refractive and absorptive parameters by solvent induced changes in optical density

With picosecond pulses at the wavelength of 532 nm, we have determined the optical nonlinear refractive and absorptive parameters of the dye N,N′-bis(2,5-di-tert-butylphenyl)-3,4,9,10-perylenedicarboximide (DBPI) by a single closed-aperture (CA) Z-scan technique. This technique uses a theoretical model that elucidates the refractive and absorptive optical nonlinearity present simultaneously in the CA Z-scan profile. The observed remarkable red shift in the absorption spectrum of the dye in the acidic medium as compared to that in the polar medium has been used to vary the optical density at a single frequency. We find that the effect of saturable absorption (SA) is complete at higher concentrations. The effect of reverse saturable absorption (RSA) is dominating in dilute concentrations. The observed variations in the excited state refractive cross-section (σ_r) with the concentration and the energy have been attributed to the contributions of higher order nonlinearity along with the existing third-order nonlinearity.     

Weak localization effects in the second-harmonic light scattered by random systems of particles

We report rigorous numerical simulations that show the presence of coherent backscattering effects in the second-harmonic generation and scattering of light by random systems of two-dimensional particles. Since the medium composing the particles is assumed to be homogeneous and isotropic, the second-harmonic field is generated mainly by surface effects. For the fundamental frequency, the results present a clear enhanced backscattering peak. In contrast, the second-harmonic scattering patterns present an intensity dip in the backscattering direction.     

Talbot effect in metallic gratings under Gaussian illumination

Metallic gratings can be found in applications such as optical metrology. Due to their fabrication process, the surface presents a certain roughness. In this work, the effect of roughness on Talbot effect has been analyzed when the grating is illuminated with a Gaussian beam. A model based on Fresnel regime is used in order to determine the intensity distribution in the near field. Contrast of the self-images is obtained and it is found that it decreases in terms of the distance between the grating and the observation plane. When the autocorrelation function of roughness presents a Gaussian behaviour, the diffracted beams are still Gaussian although some of their properties change. For example, the width of the diffracted beams increases with respect to the case of the standard chrome on glass gratings. On the other hand, the power of each diffracted beam is independent on the roughness properties of the surface.     

Modulation instability with incoherent white light in self-defocusing photorefractive crystal

We report on the first experimental observation of modulation instability and spontaneous pattern formation with incoherent white light emitted from an incandescent lamp in self-defocusing photorefractive LiNbO₃:Fe crystal. Experimental results show that the modulation instability of white light in self-defocusing medium is related to the input intensity, illumination time and the direction of the crystalline c-axis with respect to that of the lamp filament. At the illumination time t = 0 and the steady-state of MI, we give the spatial distribution of the optical Fourier power spectrum experimentally and the corresponding Fourier transformation of the output intensity numerically, and observe the emergence of the high frequency component along the c-axis.     

Abnormal properties of spontaneous emission in a Kerr nonlinear blackbody

We reexamine the atomic spontaneous decay in a Kerr nonlinear blackbody by contrast with our previous paper [M. Yin, Z. Cheng, Phys. Rev. A 78 (2008) 063829]. In the process of deriving the atomic decay rate, we use the temperature-dependent velocity of photons to take the full nonlinearity of a KNB into account. It is found that below a transition temperature T_c, the atomic spontaneous emission in a KNB might be enhanced or inhibited compared with that in a normal blackbody whose interior is filled with a nonabsorbing linear medium. The physical origin of the enhancement and inhibition of spontaneous emission is also discussed.     

Debye series expansion of shaped beam scattering by GI-POF

We derive Debye series expansion (DSE) for infinitely long multilayered cylinders normally incident by shaped beam. Typically the interaction between multilayered cylinders and Gaussian beam is derived in detail, and localized approximation is introduced to calculate the beam shaped coefficients. Finally DSE is employed to the study of rainbow scattering by graded-index polymer optical fiber (GI-POF).