Multiple small-angle scattering—A review

Small-angle scattering (SAS) is a powerful experimental technique in condensed matter physics for studying structural features of inhomogeneities of colloidal dimensions. So far the technique has been largely exploited to study thin samples for which the single scattering approximation, for the radiation-matrix interaction, holds good. The single scattering approximation is invalid when the thickness of the sample exceeds the scattering mean free path. This situation calls for a guideline to analyse the scattering data having significant contribution from multiple scattering. Since multiple scattering broadens the scattering profile, the beam broadening nature of multiple scattering can also be exploited, by making the sample suitably thick, to study large size inhomogeneities which are otherwise inaccessible to a small-angle scattering set up because of its resolution constraints. The present article presents a review and extension of the theoretical basis for analysing multiple scattering data from the point of view of a recent formalism on multiple small-angle scattering. The formalism is valid for both monodisperse and polydisperse scattering media characterized by the presence of large size inhomogeneities in the matrix. It is shown that multiple scattering from a polydisperse sample can be described by a system of coupled integrodifferential equation. However, multiple scattering from a monodisperse sample can be described by a Fokker-Planck type of equation. These equations have been analysed with an emphasis laid on the nature of the structural information pertaining to the inhomogeneities which is extractable from the multiple scattering profile. When the linear dimension of inhomogeneities becomes comparable to the scattering mean free path of the radiation in the sample, the statistical nature of the medium becomes pronounced. The statistical nature of the medium modulates the scattering profile. The modulation effect could be broadening or narrowing of the profile depending upon the nature of the inhomogeneities and their population distribution. The limiting regimes of validity and the implications of various approximations, frequently used to analyse the scattering data, have been indicated.     

Ballistic electron transport in wrinkled superlattices

Inspired by the problem of elastic wave scattering on wrinkled interfaces, we studied the scattering of ballistic electrons on a wrinkled potential energy region. The electron transmission coefficient depends on both wrinkle amplitude and periodicity, having different behaviors for positive and negative scattering potential energies. For scattering on potential barriers, minibands appear in the electron transmission, as in superlattices, whereas for scattering on periodic potential wells the transmission coefficient has a more complex form. Besides suggesting that tuning of electron transmission is possible by modifying the scattering potential via voltages on wrinkled gate electrodes, our results emphasize the analogies between ballistic electrons and elastic waves even in scattering problems on non-typical configurations.     

Method for solving the problems of multiple scattering by several bodies in a homogeneous unbounded medium

A method is developed for solving problems of multiple scattering by an aggregate of bodies in a homogeneous unbounded medium. For this purpose, the problem on the multiple scattering produced by two bodies in the field of a plane wave is first considered under the assumption that the initial unperturbed scattering amplitudes of both scatterers are known. The solution is constructed by considering plane waves multiply rescattered by the scatterers. Integral equations are obtained that allow one to calculate the resulting scattering amplitude of each scatterer and the combined scattering amplitude of the system of two scatterers. It is shown that knowledge of the solution to this problem is sufficient to solve the problem on the scattering field of a system consisting of an arbitrary number of scatterers. Expressions for the scattering amplitude in the case of an arbitrary primary field are presented. The relationship between the integral equations describing the multiple scattering in a homogeneous space and the multiple scattering by a single scatterer located near an interface is demonstrated. Approximate expressions are given for calculating the scattering amplitude in the case of multiple scattering.     

微纳粒子光学散射分析

为实现利用光学方式对微纳尺度粒子性质的研究,探讨了亚微米线及亚微米球对光电磁波的散射效应.微纳米尺度粒子的光学散射,散射粒子尺寸与入射光波长尺寸可满足米氏(Mie)散射条件.利用Matlab数值模拟的方式,将分析结果以模拟图的形式清晰地展现出来.满足尺寸条件的层状粒子以及任意多个散射粒子存在时对电磁波的散射都可采用Mie散射分析方法,并且针对多粒子散射,分析了散射体位于不同位置时对散射造成的影响.通过分析光学散射光场相关的微分散射截面及近场散射电磁场分布,可得出散射光场随散射角度的变化趋势,以及散射光场受各类因素的影响,包括入射光偏振态、散射粒子尺寸、散射粒子结构及粒子构成层数、散射粒子数量等的影响,也包括一些隐含因素对散射光场的影响,如散射粒子与周围介质的相对折射率.本文的科学意义体现在:与入射光波长尺寸可比的亚微米尺度的粒子,可用作传感器,对于其位移的探测可通过光学方式来实现,而由于粒子本身特性对散射光的影响具有一定的参考价值,从而使通过光学方式对机械位移的读出具有更高准确度.研究结果对于光学方式探测亚微米线机械振动具有指导意义.     

离轴球形粒子对高斯波束的散射光通量的计算

利用矢量球谐函数展开的方法,研究了离轴球形粒子对椭圆高斯波束的散射。根据其远区散射场的形式,得出了归一化散射场的斯托克斯参量(散射强度)与颗粒直径、折射率以及散射角的关系。建立了计算离轴球形粒子对高斯波束散射通量的解析模型,计算了散射光在任意散射方向上的光通量,得到了前向任意立体角内散射通量的计算公式,为激光散射探测提供了理论依据。     

Analysis of scattering medium structure from data on the multiple scattering of electromagnetic radiation

The radiation transfer equation for a semi -infinite scattering medium is solved. The solution provides information on the size distribution function of the scattering particles, starting from experimental data on the multiple scattering of electromagnetic radiation. A solution is obtained for the case where the probability of scattering is given by the solution of Mie's problem.     

Scattering by polar-optical phonons in a quasi-two-dimensional semiconductor

The scattering rate and momentum relaxation time for scattering of electrons in the quasi-two-dimensional quantized levels of an inversion or accumulation layer on a semiconductor surface is calculated for interactions via the polar-optical phonon. This interaction represents an important scattering mechanism in compound semiconcudctors. The quantization of the motion perpendicular to the surface enhances the scattering by this process over the bulk scattering.     

二维导体粗糙面电磁散射的分形特征研究

采用二维归一化带限Brown分形函数来模拟二维分形粗糙面,主要利用基尔霍夫近似给出了该导体粗糙面的电磁散射场.导出了平均散射场、平均散射系数和散射强度方差的计算公式.讨论了散射场分布与分维的关系,获得了散射场波峰拟合线的斜率与分维D满足线性关系这一重要结论. 关键词：     

Effects of Breaking Waves on Composite Backscattering from Ship-Ocean Scene

The existence of the sea surface is bound to affect the electromagnetic(EM) scattering from marine targets. When dealing with the composite scattering from targets over a sea surface by applying high-frequency EM theories,the total scattering field can be decomposed into three parts in low sea states, namely, the direct scattering from the sea surface, the direct scattering from targets and the coupling scattering between the sea surface and targets. With regard to high sea states, breaking waves make the direct scattering from the sea surface and the coupling scattering more complicated. To solve this issue, a scattering model is proposed to analyze the composite scattering from a ship over a rough sea surface under high sea states. To consider the effect of breaking waves,a three dimensional geometric model is adopted together with Ufimtsev's theory of edge waves for the scattering from a breaker. In addition, the coupling scattering between targets and breaking waves is taken into account by considering all possible scattering paths. The simulated results indicate that the influence of breaking waves on the scattering field from the sea surface and on the coupling field is non-negligible, and the numerical results also show the effectiveness of the proposed scattering model.     

Modeling of a microscopic optical pion-nucleon potential at energies in the (3, 3)-resonance region and nuclear-matter effect on the pion-nucleon amplitude

Differential cross sections for elastic pion scattering on a number of nuclei at energies between 130 and 290 MeV are calculated. For this purpose, use is made of a microscopic optical pion-nucleus potential that was obtained on the basis of the Glauber theory of high-energy scattering and which is determined by the density distribution of pointlike target nucleons and by the pion-nucleon scattering amplitude. The calculation of the cross sections in question is based on solving the respective relativistic wave equation. Three parameters of the pion-nucleon amplitude are fitted in performing a comparison with experimental data. These are the total cross section for pion-nucleon scattering, the ratio of the real to the imaginary part of the forward pion-nucleon scattering amplitude, and the slope parameter. The resulting values of these parameters are then compared with their counterparts for scattering on free nucleons. The character of nuclear-matter-induced changes in these parameters is studied.     

Acoustic scattering from a thermally driven buoyant plume revisited

Far-field weak scattering theory is applied to the case of high-frequency broad-bandwidth acoustic scattering from a thermally generated buoyant plume in a controlled laboratory environment. To first order, the dominant scattering mechanism is thermally driven sound-speed variations that are related to temperature deviations from ambient. As a result, the received complex acoustic scattering is a measure of the one-component three-dimensional Fourier transform of the temperature difference field measured at the Bragg wave number. The Bragg wave number vector is the difference between the scattered and incident wave vectors. Solving for its magnitude yields the Bragg scattering condition; this is the Fourier component of the plume variability that produces scattering. Results are presented for multistatic scattering from unstable and turbulent plumes using a parallel scattering geometry. The data justify application of the far-field weak scattering theory to the present case of a thermal plume. As a consequence, quantitative results on medium variability can be inferred using high-frequency broad-bandwidth acoustic scattering. Particular attention is given to the role of anisotropy of the variability of the scattering field in determining the validity of far-field Bragg scattering.     

中红外散射的基质折射率效应研究

本文利用Mie散射理论对中红外波段三种不同类型散射体的散射和消光进行了研究,发现基质在三种不同类型散射体的散射和消光中所起作用完全不同。对于无吸收的高折射率散射体,基质折射率越大面积散射比(或面积消光比)越低;对于反常色散散射体,基质折射率越大面积散射比和面积肖光比越高;而对于金属散射体,基质折射率的大小对于散射和消光影响极小。     

Enhanced scattering from a thin film with one-dimensional disorder

This paper deals with a TE plane wave scattering from a thin film with one-dimensional disorder by means of the stochastic functional approach. The thin film is one-dimensionally inhomogeneous in the horizontal direction with infinite extent, and is homogeneous in the vertical direction with finite thickness. Based on an approximate wavefield representation in terms of a Wiener–Hermite expansion in a preceding paper (Tamura et al., 2004, Waves in Random Media, 14, 435–465), the first- and second-order incoherent scattering cross-sections are presented in explicit forms and scattering properties are discussed. The scattering properties vary entirely with the film thickness. In a case where the thickness is smaller than a few wavelengths in the thin film, enhanced scattering and associated enhanced scattering may appear as sharp peaks or dips on the second-order incoherent scattering distribution if the thin film has guided wave modes. When the thickness becomes sufficiently larger than the wavelength inside the film, a new enhanced scattering phenomenon appears as gentle peaks on the second-order incoherent scattering distribution in four special directions. Such four directions are the directions of forward scattering, specular reflection, backscattering, and the symmetrical direction of forward scattering with respect to the normal of the film surface.The first-order incoherent scattering occurs distinctly in four such directions. Such enhanced scattering is independent of the existence of the guided wave modes inside the thin film, and deeply relates to the structure of the thin film with one-dimensional disorder that has infinite correlation in the vertical direction. For SiC and glass thin films having one-dimensional disorder with a Gaussian correlation and three types of exponential correlation, the first- and second-order incoherent scattering cross-sections are illustrated in figures. The narrow enhanced scattering peaks appear for the glass film in a thin case. The gentle enhanced peaks turn up for both the SiC and glass films in a thick case. Furthermore, the optical theorem is calculated for several cases. It is then found that the error of the optical theorem decreases and the performance of the wavefield is improved by taking into account the second-order incoherent scattering.     

光学厚度对颗粒媒质的多重散射的影响

基于辐射传播方程及多重散射基础理论,利用Fraunhofer近似,对颗粒媒质的多重散射光强进行了计算。研究了光学厚度对多重散射的影响,揭示了多重光散射的角分布特征,光强大小随光学厚度的变化,以及单散射引起的误差等方面的规律。为实际的颗粒媒质的光学测量等提供了理论根据。     

Enhanced scattering from a thin film with one-dimensional disorder

This paper deals with a TE plane wave scattering from a thin film with one-dimensional disorder by means of the stochastic functional approach. The thin film is one-dimensionally inhomogeneous in the horizontal direction with infinite extent, and is homogeneous in the vertical direction with finite thickness. Based on an approximate wavefield representation in terms of a Wiener-Hermite expansion in a preceding paper (Tamura et al., 2004, Waves in Random Media, 14, 435-465), the first- and second-order incoherent scattering cross-sections are presented in explicit forms and scattering properties are discussed. The scattering properties vary entirely with the film thickness. In a case where the thickness is smaller than a few wavelengths in the thin film, enhanced scattering and associated enhanced scattering may appear as sharp peaks or dips on the second-order incoherent scattering distribution if the thin film has guided wave modes. When the thickness becomes sufficiently larger than the wavelength inside the film, a new enhanced scattering phenomenon appears as gentle peaks on the second-order incoherent scattering distribution in four special directions. Such four directions are the directions of forward scattering, specular reflection, backscattering, and the symmetrical direction of forward scattering with respect to the normal of the film surface.The first-order incoherent scattering occurs distinctly in four such directions. Such enhanced scattering is independent of the existence of the guided wave modes inside the thin film, and deeply relates to the structure of the thin film with one-dimensional disorder that has infinite correlation in the vertical direction. For SiC and glass thin films having one-dimensional disorder with a Gaussian correlation and three types of exponential correlation, the first- and second-order incoherent scattering cross-sections are illustrated in figures. The narrow enhanced scattering peaks appear for the glass film in a thin case. The gentle enhanced peaks turn up for both the SiC and glass films in a thick case. Furthermore, the optical theorem is calculated for several cases. It is then found that the error of the optical theorem decreases and the performance of the wavefield is improved by taking into account the second-order incoherent scattering.     

基于Mie散射理论的铌酸锂晶粒散射特性

基于Mie散射理论,对铌酸锂晶粒光散射特性进行了理论分析与数值计算,得到了散射强度分布、偏振度与散射角、散射强度与粒子尺寸参数,以及光学截面与粒子半径的关系。研究表明:前向散射占优势,并随粒子半径的增大而增强;当粒子半径为0.1 μm 左右,散射截面和吸收截面达到最大值。     

有限波束作用下掩埋球体的散射声场计算

计算并分析了海底掩埋物体的三维散射声场。采用“等效垂直线列阵”方法来进行有限波束的建模,并将浅海波导中点声源散射声场的波数积分计算方法,推广到有限波束作用下海底掩埋物体的散射场计算,本文导出了物体位于沉积层中的散射声场计算公式。计算结果表明,在波导中垂直面内的散射声场,与沉积层中点源形成的声场非常相似;当距离较远时,散射声波呈柱面波衰减。文章还分析利用海面反射以提高散射能量的可能性,表明波束指向性及波束宽度对散射声场有较大影响。     

Fundamental Studies of Stimulated Raman Scattering and Adaptive Optics on the Basis of Stimulated Light Scattering

Some results associated with the fundamental investigations of stimulated scattering of light in various media are reported. A number of problems of adaptive optics based on stimulated scattering is studied. Concrete results of experimental investigations of physically important characteristics of conventional (spontaneous) and stimulated Raman scattering are presented and discussed. Among them are the scattering indicatrix and the relations between the phases of laser radiation incident on a substance and stimulated scattering. These results were first obtained in the G. S. Landsberg Optical Department of the P. N. Lebedev Physical Institute of the Russian Academy of Sciences. Data on excitation sources and the radiation detection technique are systematized. The main characteristics of spontaneous Raman scattering and forward and backward stimulated Raman scattering (energy parameters, pulse duration, pulse shape, divergence, brightness, spectral width, far- and near-field intensity distributions) are presented. The results on dynamic holography, phase conjugation of light in stimulated scattering, and reconstruction and recording of information (images) with the help of amplifying dynamic holograms are presented. The physical mechanisms responsible for the interference field recording and the phase conjugation of pump radiation in stimulated light scattering are discussed. The data on phase conjugation for stimulated scattering excited by picosecond optical pulses and the results associated with the effect of excitation geometry on the optical phase conjugation in the case of stimulated scattering excited by nanosecond pulses are presented.     

三维海洋波导中散射目标快速声学远场成像

研究用声传播远场分布信息成像海洋波导环境中三维散射目标的反问题,提出一种指示器样本成像方法,在不需要预先知道散射目标的任何声学和几何特性的情况下,可以快速得到其位置、形状等几何信息的一个理想的像.数值试验表明,该方法对成像海洋波导中三维散射目标是有效的,即使在有限孔径测量方式和具有噪声测量数据时,也能够得到散射目标的一个理想成像,表明海洋波导边界的多重反射效应对成像效果具有一定的正面影响.     

大尺度分层介质粗糙面电磁散射的特性研究

首先建立大尺度分层介质粗糙面散射的物理模型, 基于Stratton-Chu积分方程和Kirchhoff近似导出了粗糙面散射场的计算公式. 采用高斯随机粗糙面来模拟实际的分层介质粗糙面, 通过数值计算得到了正下视单站雷达接收到的后向散射回波. 理论推导了散射场强度与表面粗糙度之间的定量关系, 并从数值仿真的角度分析了表面和次表面的粗糙度对散射回波的影响, 给出了散射场随粗糙度变化的曲线. 最后考察了分层介质的电特性参数(介电常数和电导率)对分层粗糙面散射场的影响, 并对计算结果做出了分析.