Total internal reflection diffraction grating in conical mounting

The main conditions and parameters for obtaining surface relief total internal reflection diffraction gratings in conical mounting are presented. Calculated and experimental investigations reveal that there are ranges of grating periods, incidence angles, diffraction angles and gratings depths for which such gratings could be obtained, both for TE and TM polarizations. With optimized grating parameters the diffraction efficiency of the total internal reflection diffraction gratings can be greater than 90%.     

Observation of superluminal and slowdown light propagation in doped lithium niobate crystals

We investigate the group velocity of light in a one-dimensional volume grating inside lithium niobate crystals doped with different impurities. The superluminal and slowdown light propagations are both observed in the crystals. The relationships between the group refractive index and the grating amplitude and phase shift are presented and discussed.     

Resolution improvement of surface plasmon-enhanced, liquid crystal spatial light modulator: Simulation studies

Spatial resolution is an important performance characteristic of spatial light modulators (SLM). One of the key factors affecting the spatial resolution of liquid crystal (LC)-based SLM is the fringing field effect. This effect can be reduced in thin LC cells with corresponding reduction in the electro-optical response. A strong electro-optic response in thin LC layer can be attained using the surface plasmon resonance (SPR) phenomenon. While SPR-based LC SLMs were already demonstrated about 15 years ago, their development has been hampered in part by low resolution, due to the finite propagation length of the surface plasmons (SPs). A fine patterning of the metal layer supporting the propagation of SPs is studied as a possible solution for reducing the spatial blurring associated with the long propagation length of SPs. The results of detailed computer simulations showing improved resolution SPR-LC-SLM are presented.     

Display method with compensation of the spatial frequency response of a liquid crystal spatial light modulator for holographic femtosecond laser processing

Liquid crystal spatial light modulators, which are widely used as display devices for computer-generated holograms, have modulation characteristics that depend on spatial frequency. We describe a method for displaying a computer-generated hologram on a liquid crystal spatial light modulator with compensation of its spatial frequency response. Using this method, we demonstrate a binary phase grating with smaller dependence on the spatial frequency. We also demonstrate application of the display method to holographic femtosecond laser processing.     

Inscription of holographic gratings using circularly polarized light: influence of the optical set-up on the birefringence and surface relief grating properties

The polarization properties of the optical set-up used for holographic recording of diffraction gratings on azopolymer thin films are analyzed. The state of polarization of circularly polarized light is fully analyzed after reflection on a mirror at various incidences (Lloyd-mirror set-up). The Stokes analysis is performed using a photopolarimeter and the phase shift, the ellipticity and the azimuth orientation are compared with those calculated from Fresnel formulae. At large angles of incidence, an initially right circularly polarized (RCP) beam becomes elliptically polarized with an azimuth of nearly +45°. From these results, holographic diffraction gratings are recorded on an azobenzene-containing polymer thin film using (i) co- and contra-circularly polarized beams and (ii) a right circularly polarized beam interfering with a +45° linearly polarized light beam. Using Jones-matrix formalism, the polarization states of the diffracted orders from the birefringence (Δn) and the surface-relief (2Δd) gratings are derived and compared with experimental measurements. Finally, the induced local birefringences and surface-relief amplitudes are discussed in connection with atomic force microscopy measurements. The diffraction efficiencies obtained under the (+45°+RCP) and (LCP + RCP) (where LCP = left circularly polarized) configurations are thus compared and discussed. Received: 5 October 2001 / Revised version: 26 November 2001 / Published online: 17 January 2002     

Orthogonal geometry of wave interaction in a photorefractive crystal for linear phase demodulation

We present a novel configuration of an interferometer which is implemented by using vectorial wave mixing in the orthogonal geometry of wave interaction in a cubic photorefractive crystal, for the detection of small phase transients. The orthogonal geometry of wave interaction allows the linear regime of the phase-to-intensity transformation even when phase transients are encrypted in a depolarized wave without using any polarizing element. The use of a depolarized beam without a polarizing element strongly diminishes the noise level, thus increasing the sensitivity to phase transients.     

The effect of impedance boundary conditions on the potential function of the boundary diffraction wave theory

A novel potential function of the boundary diffraction wave theory is obtained for the impedance surfaces by the asymptotic reduction of the modified theory of physical integrals. The function is expressed in terms of the direction vectors of the incident and scattered rays. The application of the method is performed on the problem of diffraction of plane waves by an impedance half plane for oblique incidence.     

Intense femtosecond pulse shaping using a fused-silica spatial light modulator

We present the design concept of a setup of a pulse shaper to be used for high-power femtosecond lasers. The pulse shaper is constructed from a high-damage threshold fused-silica spatial light modulator and a 4-f optical system based on the design concept to avoid optical damage. We have successfully demonstrated a pulse compression of 20 fs, 5 mJ pulses obtained from a 1 kHz repetition rate Ti:sapphire chirped pulse amplification system at an average power of 5 W.     

Tunable grating-assisted surface plasmon resonance by use of nano-polymer dispersed liquid crystal electro-optical material

This paper reports on the experimental observation of the displacement of a surface plasmon resonance (SPR) excited by a metallic diffraction grating. This effect is achieved by the use of an electro-optical material composed of nano-sized droplets of liquid crystals dispersed in a host polymer. The average refractive index of this material in the form of a thin film on the undulated metal surface can be modified with the application of an external electric field and to tune the wavelength at which the SPR excitation leads to a reflection minimum. The theoretical design and experimental demonstration of the principle of this component are described.     

Effects of recording wavelength on three-dimensional vector holograms in photoreactive liquid crystal composites

Effects of recording wavelength on the recently proposed (Sasaki, 2008) three-dimensional vector holograms, in which the optical anisotropy is three-dimensionally modulated, are presented experimentally and theoretically. The polarization states of the interference light are three-dimensionally modulated due to both the polarization interference and optical anisotropy in the recording medium. These spatial distributions of the polarization states and the resulting diffraction properties in the three-dimensional vector holograms are strongly dependent on the recording wavelength. Theoretical consideration based on the finite-difference time-domain (FDTD) method reveals the mechanism of the optical characteristics of the three-dimensional vector holograms recorded by various kinds of light sources with different wavelengths.     

Effect of optical activity and crystal symmetry on maximal diffraction efficiency of reflection holograms in cubic photorefractive piezocrystals

The dependence of the maximal diffraction efficiency of a volume reflection hologram recorded in a cubic optically active photorefractive piezocrystal on the crystal thickness is investigated. The theoretical analysis is fulfilled on the basis of the coupled wave equations in a static grating approximation taking into account the linear electro-optic, inverse piezoelectric, and photoelastic effects. The optimal cuts of the crystals with various thickness for which the maximal diffraction efficiency of the reflection hologram can be attained are determined. It is shown that the optical activity of the crystal is responsible for a variety of the optimal cuts corresponding to different crystal thicknesses. Effect of the crystal on the dependence of the maximal diffraction efficiency of the reflection hologram on a crystal cut is discussed.     

The photo-neutronrefractive effect

Since its discovery in 1966, the photorefractive effect, i.e. the change of the refractive index upon illumination with light, has been studied extensively in various materials and has turned out to play a key role in modern optical technologies like photonics. This article focuses on substances that change their refractive index for neutrons when irradiated with light. In analogy to light optics, we call them photo-neutronrefractive. After a short introduction to the relevant concepts of neutron optics, two materials exhibiting this effect, a photopolymer and an electrooptic crystal, are presented. Further, we discuss the progress made concerning the development of creating light-induced gratings for neutron diffraction, which culminated in the setup of an interferometer for cold neutrons. Experiments performed on photo-neutronrefractive materials are surveyed and the variety of corresponding results obtained is presented, including a discussion of their impact on material science, neutron optics, and the foundations of physics. Received: 23 July 2002 / Published online: 25 October 2002 RID="*" ID="*"Corresponding author. Fax: +43-1/4277-9511, E-mail: martin.fally@exp.univie.ac.at     

Arrangement of a 4Pi microscope for reducing the confocal detection volume with two-photon excitation

The main advantage of two-photon fluorescence confocal microscopy is the low absorption obtained with live tissues at the wavelengths of operation. However, the resolution of two-photon fluorescence confocal microscopes is lower than in the case of one-photon excitation. The 4Pi microscope type C working in two-photon regime, in which the excitation beams are coherently superimposed and, simultaneously, the emitted beams are also coherently added, has shown to be a good solution for increasing the resolution along the optical axis and for reducing the amplitude of the side lobes of the point spread function. However, the resolution in the transverse plane is poorer than in the case of one-photon excitation due to the larger wavelength involved in the two-photon fluorescence process. In this paper we show that a particular arrangement of the 4Pi microscope, referenced as 4Pi′ microscope, is a solution for obtaining a lateral resolution in the two-photon regime similar or even better to that obtained with 4Pi microscopes working in the one-photon excitation regime.     

Prevailing effects of interference or diffraction by multiple apertures

The effects of interference and diffraction produced by a bidimensional structure composed of multiple and identical apertures are studied. Such effects are competitive during the propagation, that is, in some planes the interference effects are more visible, while in others prevail the diffraction ones. Using the number of Fresnel zones, the spatial domains where the interference or diffraction effects prevail are defined and parameterized. Simulation and experimental results are further introduced to verify the proposed method.     

Off-Bragg-angle light diffraction and structure of dynamic interband photorefractive gratings

Steady-state and time-resolved off-Bragg-angle diffraction experiments are used to determine the structure and the dynamics of photorefractive gratings induced by interband photoexcitation. In potassium niobate, we identify in such gratings basically a two-layer structure. Close to the surface, we find a space-charge electric field generated by a charge modulation stored directly in the bands. This grating component is typically 50 μm thick, the amplitude of the refractive index modulation is larger than 10^-4, and the response time is a few μs for resonant intensities of 100 mW cm^-2. This component is also robust under non-resonant illumination. Deeper in the crystal, a second holographic layer extends over a few hundreds of μm, its amplitude is smaller, and its slower response time is in the ms range. The mutual phase shift between the grating components is also determined. Received: 23 November 1998 / Revised version: 14 January 1999 / Published online: 12 April 1999     

Influence of auxiliary violet light on holographic kinetics at low and high recording intensities in bacteriorhodopsin film

The photochromic bacteriorhodopsin (BR) film can be used as a rewritable holographic recording medium. Due to the saturation absorption and the scattering and reflecting lights from the BR film, the grating contrast-ratio of the hologram is diminished during the hologram recording. When the intensity of the recording light is low, the influence of the saturation absorption and the scatter and reflection of BR film on the grating contrast-ratio is weak. But for the case of intense recording light, this influence is more serious. It is found that the influence of the auxiliary violet light on the holographic kinetics of diffraction efficiency is distinct under different recording intensities. At the low recording light intensity, the steady diffraction efficiency is increased and the peak diffraction efficiency is suppressed by the auxiliary violet light. But for intense recording light, the steady diffraction efficiency and the peak diffraction efficiency are both increased by the auxiliary violet light. Based on the two-state model of BR photochromism, we give a good theoretical explanation to the above phenomena.     

Single laser exposure fabrication of diamond-like 3-dimensional photonic crystal microstructures using circularly polarized light

Phase tunable multi-level diffractive optical elements define an attractive approach for single laser exposure fabrication of 3-dimensional photonic crystal microstructures. The significant advantage of these multi-level diffractive optical elements over two-level diffractive optical elements is the flexibility of fabricating a wide range of 3-dimensional periodic structures by manipulating the relative phase of different diffracted beams. Here, phase tuning was applied to demonstrate fabrication of a hybrid 3-dimensional structure intermediate between previously reported diamond-like Woodpile-type structure of tetragonal symmetry and structure having body-centered-tetragonal lattice symmetry. Circularly polarized light was applied for the first time to balance the diffraction order efficiencies and improve the structural uniformity. Design guidelines are presented for generating diamond-like photonic crystal template that possesses complete photonic bandgap when inverted with high refractive index materials.     

Reconstruction of parasitic holograms to characterize photorefractive materials

Photoinduced light scattering is a serious drawback that limits the applicability of thick holographic recording media but provides valuable information on the recording medium. As long as there is no correlation between the scattering centers in the crystal, photoinduced light scattering may be explained to result from the interference pattern of the incident beam and the field scattered from a single point-like scattering center. The hologram of this ellipsoidally scattered wave field will have practically the same structure in the reciprocal space modified by a response function which reflects the anisotropic properties of the recording medium. We studied photoinduced light scattering in LiNbO₃:Fe, a model system for photorefractive materials. The transmitted intensity in the stationary state of the scattering process is investigated as a function of the reconstruction angle at different wavelengths and polarizations of the reconstructing beam. The experimental results are analyzed by a simple phenomenological model based on the Ewald construction and can be used to choose suitable conditions at which holographic scattering can be minimized as well as to extract some physical parameters of the crystal. Received: 27 September 2000 / Revised version: 1 December 2000 / Published online: 21 February 2001     

Color dispersion in two-dimensional phase array based on polymer-dispersed liquid crystal film

This work proposes a feasible method for fabricating a two-dimensional periodic structure with a sub-micrometer periodicity using a single laser beam, based on polymer-dispersed liquid crystal (PDLC) films. The resulting nano-PDLC morphology is highly symmetrical, and similar to that written using multi-beam interference. The increase in the electric-tunability of the optical behavior, including spatial diffraction and color dispersion, is examined. The color dispersion provides optical evidence of the periodic structure of the PDLC film.     

Experimental observations of the spectrum of light diffracted at a slit as a secondary source

In this paper, we investigated both theoretically and experimentally the normalized spectrum of partially coherent light radiated from a secondary source which is produced by an imaging system. The experimental results show that, if the imaging lens is achromatic, the normalized spectrum of the light radiated from a secondary source shifts either towards the red side or towards the blue side, compared to the spectrum of the source, and the spectral shifts change for different position of the observation points. It is found that the experimental results are consistent with the theoretical ones. A chromatic lens, acting as the imaging lens, is used to investigate the effect of the chromatic aberration on the normalized spectrum of the light field. The results show that the influence of the chromatic aberration on the normalized spectrum is considerable and cannot be neglected in high-precision spectral measurement experiments.