Amplification without population inversion in molecules

We have studied the feasibility of amplification without population inversion (AWI) in LiH molecule for three-level ladder, V, and Λ schemes. We have shown the salient features of AWI in a molecular system in comparison to that in an atomic system, viz. the dependence of gain profile on the choice of different rotational and vibrational transitions. Under different three-level schemes, the effect of homogeneous and inhomogeneous broadening on the gain profile has been studied. We have also studied the dependence of gain on different external parameters. The temporal evolution of gain has been analyzed and it was found that AWI is achievable in both the transient and the steady state regime. For all the three-level schemes and in particular for the ladder scheme, amplification of the weak probe was obtained using a coupling laser of smaller frequency.     

Ultrafast control of coherent population transfer with a train of femtosecond pulse pairs

We investigate the ultrafast control of coherent population transfer in a Λ-type three-level system with a train of pump-Stokes femtosecond pulse pairs, where the pulse sequences can be produced either by optical delay line or by pulse shaping with sinusoidal phase modulation. It is shown that when the pump and Stokes pulses in each pair are applied in the counterintuitive order, similar to that in the stimulated Raman adiabatic passage technique, due to temporal quantum interference (besides optical interference in the case of overlapped subpulses), ultrafast control of coherent population transfer can be achieved by scanning the inter-pair time delay or by changing the sinusoidal phase modulation parameters. This method has potential applications in ultrafast control of chemical reactions and quantum information processing.     

Two-color pulse compression in aperiodically-poled lithium niobate

We experimentally demonstrate engineerable compression of two-colored pulses in a linearly-chirped quasi-phase-matching grating. Quadratic solitons generated from fundamental input are reshaped through cascaded parametric processes of second-harmonic generation (SHG) and the back-conversion. We use type-I (e: o + o) SHG geometry in a 50-mm-long aperiodically-poled MgO:LiNbO₃ device to satisfy the group-velocity matching condition. Simultaneously compressed fundamental and SH pulses of about 55-fs duration with small pedestal are generated from the fundamental input pulses of 95-fs duration.     

Localization of atoms in light fields: Optical molasses,adiabatic compression and squeezing

We present a theoretical study of the localization1 of atoms with an angular momentumJ _g=3 toJ _e=4 transition (e.g., chromium atoms) in quantized optical molasses created by two counterpropagating linearly polarized laser beams. We study the localization as a function of the potential depth, the angle between the polarizations and the interaction time with the molasses in the low-intensity limit, and discuss the possibility of adiabatic compression and squeezing of the atomic distribution.Dedicated to H. Walther on the occasion of his 60th birthday     

Intense femtosecond pulse shaping using a fused-silica spatial light modulator

We present the design concept of a setup of a pulse shaper to be used for high-power femtosecond lasers. The pulse shaper is constructed from a high-damage threshold fused-silica spatial light modulator and a 4-f optical system based on the design concept to avoid optical damage. We have successfully demonstrated a pulse compression of 20 fs, 5 mJ pulses obtained from a 1 kHz repetition rate Ti:sapphire chirped pulse amplification system at an average power of 5 W.     

Interaction of a two-level atom with squeezed light

We consider a degenerate parametric oscillator whose cavity contains a two-level atom. Applying the Heisenberg and quantum Langevin equations, we calculate in the bad-cavity limit the mean photon number, the quadrature variance, and the power spectrum for the cavity mode in general and for the signal light and fluorescent light in particular. We also obtain the normalized second-order correlation function for the fluorescent light. We find that the presence of the two-level atom leads to a decrease in the degree of squeezing of the signal light. It so turns out that the fluorescent light is in a squeezed state and the power spectrum consists of a single peak only.     

Eigenmode expansion of the polarization for a spherical sample of two-level atoms

We derive pseudo-orthogonality relations for both the magnetic and electric eigenmodes of a system of two-level atoms in a sphere configuration. We verify numerically that an arbitrary vector field can be reconstructed to a great accuracy from these eigenmode expansions. We apply this eigenmode analysis to explore superradiance from a sphere with initially uniform polarization.     

Anomalous Effects of Driving Field Linewidth on a One-Atom Dressed-State Laser

We examine the effects of driving field linewidth on a one-atom dressed state laser. Unexpectedly, the linewidth leads to anomalous effects on the cavity field. The mean photon number of the cavity field is raised or the normalized variance is reduced to a certain degree as the linewidth increases for an appropriate range of parameters. The responsible mechanism is attributed to the fluctuation-induced modification of the electromagnetic reservoir where the atom stays.     

Theory of nonlinear optical response of gauge invariant currents to linear and nonlinear couplings

When a gauge field interacts with a quantum condensed matter system, at first order of the gauge field it couples to the current operator of the electrons. Higher orders of the gauge field couple to electrons through other operators such as the stress tensor, etc. On the other hand, when one performs a measurement on a quantum system, not only the current operator, but also stress tensor operator of the electrons, etc. are hidden in the measurement, as they contribute to the gauge invariant current. We formulate a general problem of nonlinear optical response of the gauge invariant currents in presence of nonlinear couplings. We show that the new couplings along with new responses arising from field current have a very simple structure which can be formulated as time ordered multi-particle correlation functions. We also obtain their Lehman representation and thereby show that one need not use non-equilibrium formulations to deal with them. These new correlation functions suggest that in nonlinear optical response many new processes are possible. The experimental detection of the new terms in the current operator, and application corresponding multi-photon processes needs further theoretical and experimental investigations.     

Evolution of population in an equispaced three-level ladder-type atomic system

Transient response of nearly equispaced three-level ladder-type atomic system with a broad-band squeezed vacuum (SV) is investigated. We focus our attention in the interplay between the quantum interference and the squeezed field on the population distribution. It is shown that an atomic population inversion can be attained on one of the optical transitions due to the SV. Additionally, we show, with the proper value of the relative phase, the SV can also lead to unexpected population inversion on the transition between two different levels.     

Electromagnetic decay modes in a spherical sample of two-level atoms

We find the eigenmodes of the Lienard-Wiechert kernel for a spherical geometry. We show that these consist of two series corresponding to the classical electrodynamics multipole electric and magnetic series. The electric series possesses “anomalous modes”, absent in both the magnetic series and the “scalar photon” theory.     

Quantum interferences in coherent population trapping of a cold double Λ-type atom

We investigate quantum interferences in coherent population trapping of a cold double Λ-type four-level atomic system driven by two counterpropagating laser fields. We study both decoherence and enhanced-coherence actions resulting from the multi-transition pathways in building up the trapping state, and analyze the system operating with and without external coherences in various configurations of the atomic dipole moments.     

Reply to: “Comment on: ‘Effects of including the counterrotating term and virtual photons on the eigenfunctions and eigenvalues of a scalar photon collective emission theory’ [Phys. Lett. A 372 (2008) 2514]” [Phys. Lett. A 372 (2008) 5732]

We compute the emission amplitude for the collective emission from a sphere of identical atoms in the scalar photon theory for both the cases of the complex kernel (i.e. including virtual photons) and real kernel. We explicitly show that the single mode theory based on the real kernel neglects the effects of the different decay rates and frequency shifts associated with the eigenfunctions belonging to the same angular index but with different radial indices. We show that these effects modify, for k₀R?1, both the time dependence of the emission amplitude and its angular distribution, in clear contradiction to the assertions made by the Comment's authors.     

Trapping State in a System of Single Three-level Trapped Ion Driven by External Fields

We investigate the interaction of a single three-level trapped ion with two laser beams. By applying a unitary transformation and a small rotating transformation, an exact solution to this quantum system is obtained without performing the Lamb-Dicke approximation, and the trapping state is observed.     

Degenerate three-level cascade laser with the cavity mode driven by coherent light

We present the quantum statistical properties of the light produced by a degenerate three-level cascade laser with the cavity mode driven by coherent light. In this system three-level atoms in a cascade configuration, initially prepared in a coherent superposition of the top and bottom levels, are injected into a cavity coupled a vacuum reservoir. We find that although the driving coherent light has no effect on the degree of squeezing, it increases the mean photon number considerably. Therefore, this quantum optical system can be taken as a source of a bright squeezed light.     

Reconciling the eigenmode analysis with the Maxwell-Bloch equations approach to superradiance in the linear regime

The superradiance from a slab of inverted two-level atoms is theoretically analyzed in the linear regime from both the perspective of the expansion in eigenfunctions of the integral equation with the Lienard-Wiechert potential as kernel, and that of linearizing the Maxwell-Bloch equations. We show the equivalence of both approaches. We show that the so-called Reduced Maxwell-Bloch equations do not yield even approximately the correct solution when applied in the obvious way, but that they can be made to give the correct solution by adding a fictitious input field.     

Entangled Radiation through an Atomic Reservoir Controlled by Coherent Population Trapping

We show that it is possible to generate Einstein-Podolsky-Rosen （EPR） entangled radiation using an atomic reservoir controlled by coherent population trapping. A beam of three-level atoms is initially prepared in nearcoherent population trapping （CPT） state and acts as a long-lived coherence-controlled reservoir. Four-wave mixing leads to amplification of cavity modes resonant with RabJ sidebands of the atomic dipole transitions. The cavity modes evolve Jnto an EPR state, whose degree of entanglement is controlled by the intensities and the frequencies of the driving fields. This scheme uses the long-lived CPT coherence and is robust against spontaneous emission of the atomic beam. At the same time, this scheme is implemented in a one-step procedure, not in a two-step procedure as was required in Phys. Rev. Lett. 98 （2007） 240401.     

Superradiant Rayleigh scattering from a Bose-Einstein condensate with the incident laser along the long axis

We have realized the superradiant Rayleigh scattering in an elongated Bose-Einstein condensate, where the pump laser pulse travels along the long axis. In this incident configuration the spatial asymmetries and the backward scattering pattern are reported. The spatial and temporal evolution of the superradiant process is analyzed by our semiclassical model.     

Controlled generation of single photons from a strongly coupled atom-cavity system

We propose a new method for the generation of single photons. Our scheme will lead to the emission of one photon into a single mode of the radiation field in response to a trigger event. This photon is emitted from an atom strongly coupled to a high-finesse optical cavity, and the trigger is a classical light pulse. The device combines cavity-QED with an adiabatic transfer technique. We simulate this process numerically and show that it is possible to control the temporal behaviour of the photon emission probability by the shape and the detuning of the trigger pulse. An extension of the scheme with a reloading mechanism will allow one to emit a bit-stream of photons at a given rate. Received: 7 July 1999 / Revised version: 3 September 1999 / Published online: 20 October 1999