Shape coexistence near the double-midshell nucleus 111Rh

The decay of ¹¹¹Ru obtained from fast on-line chemical and mass separation has been investigated by β-γ-t and γ-γ coincidence techniques. Earlier spin and parity assignments of ¹¹¹Rh levels based on extrapolations of level systematics are confirmed. In particular, the K=1/2 intruder band is supported by the hindrance of E2 transitions between deformed and spherical states and enhancement of intraband E2 transitions. The excitation energies of intruder band members in Rh isotopes show a minimum at ¹⁰⁹Rh₆₄, with two neutrons less than ¹¹¹Rh at the N=66 midshell. This trend, which differs from the one in the higher-Z neighbouring elements Ag and Cd with minima at N=66, follows the evolution of deformation observed in the lower-Z elements Ru and Mo. Received: 25 June 1997 / Revised version: 10 September 1997     

New results on elements 111 and 112

Experiments on the synthesis and identification of the nuclei ²⁷²111 and ²⁷⁷112 were performed in order to confirm previous results. Three additional decay chains were measured in the reaction ⁶⁴Ni + ²⁰⁹Bi →²⁷³111^*. The study revealed considerably improved data on the decay chain originating from ²⁷²111. One additional chain was measured in the reaction ⁷⁰Zn + ²⁰⁸Pb →²⁷⁸112^*. The decay properties of the chain starting at ²⁷⁷112 are in excellent agreement with the second chain of the first experiment down to ²⁶⁵Sg, where the new chain ends by a previously unknown spontaneous-fission branch. A re-analysis of all the data on elements 110, 111, and 112 measured at GSI since 1994 (a total of 34 decay chains was investigated) revealed that for 2 chains (the second chain of ²⁶⁹110 measured in 1994 and the first chain of ²⁷⁷112 measured in 1996) the results of the new analysis differed from the previous one. In all other cases the earlier data are exactly reproduced. Received: 21 December 2001 / Accepted: 15 January 2002     

Dipole and quadrupole cascades in the yrast region of 143Gd

The high spin states of ¹⁴³Gd have been studied via the ¹¹¹Cd(³⁵Cl,1p2n) reaction at 170 MeV. One dipole cascade has been newly found and two dipole cascades have been extended to higher spin states. A relatively long E2 cascade consisting of irregular transition energies has been found, which has only weak connections to the other dipole and quadrupole cascades. This resembles the ones recently found in ^142,143,144Eu and ¹⁴⁴Gd. The dipole and quadrupole cascades have been found to appear by turns in an energy increment of about 0.2 MeV above the yrast line. Received: 1 November 1997     

Half-lives of platinum isotopes from photoactivation

The half-lives of the platinum isotopes ^189,191,197Pt and of the 4-day isomer in ^195mPt have been measured with high precision using the photoactivation technique. The γ-ray activity was counted over several half-lives with a high-purity germanium detector. The measured half-lives are: T_1/2(¹⁸⁹Pt) = 12.1 ± 1.5 h; T_1/2(¹⁹¹Pt) = 2.862 ± 0.007 d; T_1/2(¹⁹⁷Pt) = 19.96 ± 0.05 h; T_1/2(^195mPt) = 4.0104 ± 0.0047 d. Received: 13 September 1999     

Decay modes of 24Mg excited at 46.4 MeV

⁸Be_gs coincidences with ¹²C, ⁸Be_gs and α-particles produced in the ¹²C +¹²C interaction at 65 MeV have been measured in a wide in-plane angular range. The 3 −⁸Be_gs final state is found to be produced, even if poor statistics prevent any identification of the ¹⁶O states involved in the first stage of the process. The ⁸Be_gs−α and ⁸Be_gs−¹²C coincidence yields are found to be due to ¹²C and ¹⁶O excited states, decaying into the ⁸Be_gs+α and ¹²C +α systems, respectively. Received: 15 June 1998 / Revised version: 4 December 1998     

The A = 51 mirror nuclei 51Fe and 51Mn

Eighteen previously unknown γ-ray transitions were identified in the T _z = - 1/2 nucleus ⁵¹Fe following the fusion-evaporation reaction ³²S(²⁸Si,2α1n)⁵¹Fe. The level scheme reaches the fully aligned I ^π = 27/2^- terminating state of the five holes in the f _7/2 shell. The 17/2^- state was found to be isomeric, and the lifetime was measured to be 2.87 ns. The mirror symmetry of ⁵¹Fe and ⁵¹Mn is discussed, and the level scheme of ⁵¹Fe is compared to shell-model calculations. Received: 20 July 2000 / Accepted: 1 August 2000     

A new high-spin isomer in 145Sm

A new high-spin isomer in ¹⁴⁵Sm was observed by in-beam γ-ray spectroscopy with the reaction ¹²²Sn(²⁷Al,3np) at 127 MeV performed at the Nordball multi-detector array in Roskilde. The excitation energy of the isomer was determined to be E _x= 11147 keV, and using the generalized centroid-shift method its half-life was found to be T _1/2= (7.4 ± 1.0) ns. Received: 23 October 1998     

Selective laser ionization of N≥82 indium isotopes: The new r-process nuclide 135In

Production yields and β-decay half-lives (T _1/2) of very neutron-rich indium isotopes were determined at CERN/ISOLDE using isobaric selectivity of a resonance-ionization laser ion-source. Beta-delayed neutron (βdn) multiscaling measurements have yielded improved T _1/2 for 206(6) ms ¹³²In, 165(3) ms ¹³³In and 141(5) ms ¹³⁴In. With 92(10) ms ¹³⁵In, a new r-process nuclide has been identified which acts as an important “waiting point” in the In isotopic chain for neutron densities in the range n _n≃ 10²⁴-10²⁶ n/cm³, where the r-matter flow has already passed the A≃ 130 abundance peak region. Received: 17 January 2002 / Accepted: 30 January 2002     

Measurement of the lifetime of the first 2+ state in 124Ba

The lifetime of the first 2⁺ state in the nucleus ¹²⁴Ba has been measured by γ-γ coincidence recoil-distance Doppler shift method. The ¹⁰⁹Ag(¹⁹F, 4n)¹²⁴Ba reaction at a beam energy of 75 MeV was employed to populate excited states in ¹²⁴Ba. The mean lifetime was determined to be 275(12) ps using the differential decay curve method. The value of B(E2;0₁ ⁺→ 2₁ ⁺) for ¹²⁴Ba deduced from the lifetime is in reasonable agreement with the prediction of the proton-neutron interacting boson model(IBM-2) without Pauli blocking effect. Received: 23 February 1998     

Lattice Location of 181Ta and 111Cd Probes in Hafnium and Zirconium Aluminides Studied by Perturbed Angular Correlation

The perturbed angular correlation technique was applied to study the lattice location of the ¹¹¹In/¹¹¹Cd and ¹⁸¹Hf/¹⁸¹Ta probe atoms in hafnium and zirconium aluminides. Compounds of different stoichiometries and crystallographic structures were the subject of investigation. According to the expectation, in all investigated compounds ¹⁸¹Hf/¹⁸¹Ta probes occupy the Hf(Zr) crystallographic sites. The ¹¹¹In/¹¹¹Cd probes are placed at the sites of all constituent metals—aluminum, hafnium and zirconium, depending on the crystallographic structure of compound, concentration of the constituent metals and temperature of the sample.     

Dynamic polarization potential of 12C+12C system at molecular-resonance energies

The nuclear reaction dynamics leading to the formation of recently discovered resonance in the mutual-0₂ ⁺ channel of the ¹²C+¹²C inelastic scattering around E _c.m.≃ 32 MeV is studied in terms of the dynamic polarization potential (DPP) induced by the channel coupling among various excited states in ¹²C. The microscopic 3α cluster-model wave functions are used to generate the ¹²C−¹²C diagonal and coupling potentials in the double-folding model. It is found that DPP for the 0₂ ⁺+ 0₂ ⁺ channel is an unusually strong attractive potential which even exceeds the zeroth-order folding-model potential of this channel around the nuclear surface region and that the strong coupling between the 0₂ ⁺ and 2₂ ⁺ states is predominantly responsible for the unusual DPP in this channel. The effective potential, the sum of the original folding-model potential and the attractive DPP, is found to generates resonance states in the same energy region as that of the resonance states generated by the original folding-model potential but the former states are found to be higher-nodal states having four additional radial nodes. Similar but more moderate property of DPP is also found in the entrance (elastic) channel. These results suggest that the reaction dynamics of generating the resonance in the ¹²C(0₂ ⁺) +¹²C(0₂ ⁺) channel may rather differ from that of the simple crossing of the zeroth-order molecular band generated by the potentials in the entrance and exit channels suggested by the standard band-crossing model. Received: 17 December 1998 / Revised version: 1 March 1999     

On the nature of the 17 μs isomer of the <Superscript>133</Superscript>Sb valence nucleus

The decay of the 17 μs isomer of ¹³³Sb was re-investigated experimentally. It was produced by thermal neutron induced fission of ²⁴¹Pu. Its detection is based on time correlation between fission fragments selected by the LOHENGRIN spectrometer at ILL (Grenoble), and the γ-rays, and conversion electrons from the isomer. The interpretation of the level scheme is based on shell model calculations, where empirical two-body matrix elements were employed. The good agreement between theory and experiment suggests that the isomer is the 21/2⁺ member of the 2p-1h πg _7/2ν(f _7/2 h _11/2 ⁻¹) configuration. Received: 20 January 2000 / Revised version: 28 February 2000     

Systematics of related high-spin isomers in 144Sm and other N = 82 nuclei

An in-beam experiment with the reaction ¹²²Sn(²⁷Al,4np) at 127 MeV was performed at the Nordball multi-detector array in Roskilde. It provided evidence for a new high-spin isomer in ¹⁴⁴Sm. This isomer with T _1/2= (2.6 ± 0.5) ns at an excitation energy E _x= 9232 keV seems to belong to a family of isomers of similar configuration in neighbouring N= 82 nuclei. Received: 16 November 1997     

Alpha decay of the new isotopes 188,189Po

New neutron-deficient isotopes ^188,189Po have been produced in the complete fusion reaction of ⁵²Cr ions with a ¹⁴²Nd target at the velocity filter SHIP. The evaporation residues were separated in-flight and subsequently identified on the basis of α-γ and α-conversion electron coincidence measurements and of α-α position and time correlations. In ¹⁸⁹Po a ground state to ground state α decay with E_α1= 7540(20) keV, T_1/2= 5(1) ms and two fine structure α-decays at E_α2= 7264(15) keV and E_α3= 7316(15) keV have been observed. In ¹⁸⁸Po (T_1/2= 400⁺²⁰⁰ ₋₁₅₀μs) a ground state to ground state α decay at E_α= 7915(25) keV and a fine structure α decay at E_α= 7350(40) keV have been found. Improved data on the α-decay of ¹⁸⁹Bi were obtained. Received: 15 October 1999     

High-spin states in 160Lu

High-spin states of ¹⁶⁰Lu have been studied through the ¹⁴⁴Sm( ¹⁹F, 3n) reaction. The previously known πh _11/2⊗υi _13/2 yrast band is extended from I ^π = 21^- to 25^- and a four quasiparticle band with configuration πh _11/2[523]7/2 ^-⊗υh _9/2[521]3/2 ^-⊗ (υi _13/2)² is reported. Received: 21 May 2001 / Accepted: 19 July 2001     

Rotational bands in 181Ta

High-spin states in ¹⁸¹Ta have been studied via the ¹⁷⁶Yb(¹¹B,α2n) reaction at 52 MeV using the PEX array and at 57 MeV using the NORDBALL array, with α-particle detection. The previously known, K^π=(7/2)⁺ ground state band and K^π=(9/2)⁻ band have been extended to spins (29/2)⁺ and (31/2)⁻, respectively. Two new one-quasiparticle bands, the K^π=(5/2)⁺ band built on the known (5/2)⁺ isomer and a K^π=((1/2)⁻) band have been observed. Two other rotational bands with three-quasiparticle structure, K^π=(15/2)⁻ and ((19/2)⁺ with π(7/2)[404]ν²(1/2)[510](9/2)[624] and π(9/2)[514]ν²(1/2)[510](9/2)[624] configurations, respectively, have been newly observed. The half-life of the K^π=((19/2)⁺) bandhead which decays to the head of the (15/2)⁻ band has been measured to be 140(36) ns. However, transitions from the ((19/2)⁺) state to the (15/2)⁻ band have not been observed. Received: 26 August 1998     

Terminating high-spin bands in 101Rh

High spin states of ¹⁰¹Rh have been populated using the reaction ⁷⁰Zn+³⁶S at 130 MeV. γ-rays were detected with the EUROGAM2 array. New high-spin bands have been observed in this nucleus up to 45/2⁻, 57/2⁻ and 65/2⁺ states. They have been interpreted using the Nilsson-Strutinsky cranking formalism as terminating configurations. Two of the bands were observed up to the predicted terminating states which are built up from g_9/2 protons as well as d_5/2, g_7/2 and h_11/2 neutrons relative to a ⁹⁰Zr core. Received: 30 October 1998     

New high-spin microsecond isomers in 131Sb

In this work we have identified and studied the decay of two new microsecond isomers 19/2^- and 23/2⁺ in ¹³¹Sb. This neutron-rich nucleus was produced by thermal neutron-induced fission of ²⁴¹Pu. The detection is based on time correlation between fission fragments selected by the LOHENGRIN spectrometer at ILL (Grenoble) and the γ-rays or conversion electrons from isomers. These new data on high-spin states complete the level scheme previously obtained from β-decay. A large fraction of the members of the πg _7/2ν(h _11/2 ^-1 d _3/2 ^-1) and πg _7/2νh _11/2 ^-2 multiplets are now known and were compared with a multi-particle shell model calculation. Received: 7 June 2000 / Accepted: 19 September 2000     

First evidence for a new spontaneous fission decay produced in the reaction 30Si +238U

Mean lifetimes of the high spin states in the yrast band of ¹²⁶Ba were measured by using the Doppler shift attenuation method in connection with the reaction ¹¹⁶Sn (¹⁶O, 2p4n)¹²⁶Ba at a beam energy of 73 MeV. The corresponding normalized B(E2) values are obviously reduced in the vicinity of the backbending. The results are compared with the theoretical predictions based on a realistic nucleon-nucleon interaction. Received: 9 June 1997 / Revised version: 16 October 1997