双原子分子多光子电离强场效应的含时波包动力学研究

强激光非线性条件下分子的多光子电离过程呈现出较为明显的强场效应．由于这种效应不能用传统的量子微扰论来处理。“缀饰态”模型方法提供了物理图象清晰的处理光与物质相互作用的方案．本文基于含时波包动力学的基本理论，将激光场看作经典场，利用“缀饰态”模型研究了强场下双原子分子（NO、RbI等）的多光子电离过程．研究表明，激光场的强度、泵浦-探测脉冲延迟时间等对多光子电离光电子能谱的形状有着重要的影响。而这种影响是由光诱导势引起的．另外，在研究具有两个连续态的Rbl体系时，自电离现象的发生也与势能面的交叉密切相关，并受外场强度的影响．本文计算模拟外场中分子的光电子能谱时所得到的强场效应对理解和实现原子分子过程的激光搛控具有重要的意义．     

碘原子共振多光子电离光谱研究

用可调谐的染料激光(4600～5000(?)),共振(3+2)和(4+1)多光子电离探测了I(5p~2P_(3/2)~0)和1~#(5p~2P_(1/2)~0).碘原子是由碘分子(I_2)经激光解离而产生的.在上述激光波段中共观察到12个原子跃迁,其中,(4+1)多光子电离跃迁是首次观察到的.     

双原子分子多光子电离强场效应的含时波包动力学研究

强激光非线性条件下分子的多光子电离过程呈现出较为明显的强场效应.由于这种效应不能用传统的量子微扰论来处理,"缀饰态"模型方法提供了物理图象清晰的处理光与物质相互作用的方案.本文基于含时波包动力学的基本理论,将激光场看作经典场,利用"缀饰态"模型研究了强场下双原子分子(NO、RbI等)的多光子电离过程.研究表明,激光场的强度、泵浦-探测脉冲延迟时间等对多光子电离光电子能谱的形状有着重要的影响,而这种影响是由光诱导势引起的.另外,在研究具有两个连续态的RbI体系时,自电离现象的发生也与势能面的交叉密切相关,并受外场强度的影响.本文计算模拟外场中分子的光电子能谱时所得到的强场效应对理解和实现原子分子过程的激光操控具有重要的意义.     

双原子分子多光子电离强场效应的含时波包动力学研究

强激光非线性条件下分子的多光子电离过程呈现出较为明显的强场效应.由于这种效应不能用传统的量子微扰论来处理,“缀饰态”模型方法提供了物理图象清晰的处理光与物质相互作用的方案.本文基于含时波包动力学的基本理论,将激光场看作经典场,利用“缀饰态”模型研究了强场下双原子分子(NO、RbI等)的多光子电离过程.研究表明,激光场的强度、泵浦-探测脉冲延迟时间等对多光子电离光电子能谱的形状有着重要的影响,而这种影响是由光诱导势引起的.另外,在研究具有两个连续态的RbI体系时,自电离现象的发生也与势能面的交叉密切相关,并受外场强度的影响.本文计算模拟外场中分子的光电子能谱时所得到的强场效应对理解和实现原子分子过程的激光操控具有重要的意义.     

连续变量量子态的光学操控

量子态的光学操控是指在光场的传输、存储和频率变换等过程中用光学方法对光场的量子态进行操作与控制.量子态操控是量子通讯及量子态制备和应用的基础.在简要介绍连续变量多组份纠缠态光场制备的基础上,概述基于多组份纠缠态光场的连续变量量子通讯网络及在执行压缩态和纠缠态光场操控方面的实验研究进展.     

Gd原子的共振多光子电离研究

本文首次报道了用共振多光子电离(RMPI)技术探测到四条在可见光范围内的Gd原子强双光子跃迁线.观察到双色三光子Gd原子激光同位素分离.研究了高分辨率Gd原子电离谱,并解释了电离谱的线型.     

激光场中H原子的多光子电离速度

 建立了激光与原子相互作用的伪分立态模型,并用此模型计算了激光场中H原子的多光子电离速率。对于光子能量较小的激光,计算结果与其它理论计算结果相符合。     

激光场中H原子的多光子电离速度

建立了激光与原子相互作用的伪分立态模型,并用此模型计算了激光场中H原子的多光子电离速率。对于光子能量较小的激光,计算结果与其它理论计算结果相符合。     

铅原子非共振多光子电离过程的研究

在激光波长为1064nm、532nm和355nm下,研究了铅原子的非共振多光子过程.通过改变激光脉冲的线宽研究了铅原子非共振7-光子电离速率和激光统计性的依赖关系.     

Polarization control of multi-photon absorption under intermediate femtosecond laser field

It has been shown that the femtosecond laser polarization modulation is a very simple and well-established method to control the multi-photon absorption process by the light–matter interaction. Previous studies mainly focused on the multiphoton absorption control in the weak field. In this paper, we further explore the polarization control behavior of multiphoton absorption process in the intermediate femtosecond laser field. In the weak femtosecond laser field, the secondorder perturbation theory can well describe the non-resonant two-photon absorption process. However, the higher order nonlinear effect(e.g., four-photon absorption) can occur in the intermediate femtosecond laser field, and thus it is necessary to establish new theoretical model to describe the multi-photon absorption process, which includes the two-photon and four-photon transitions. Here, we construct a fourth-order perturbation theory to study the polarization control behavior of this multi-photon absorption under the intermediate femtosecond laser field excitation, and our theoretical results show that the two-photon and four-photon excitation pathways can induce a coherent interference, while the coherent interference is constructive or destructive that depends on the femtosecond laser center frequency. Moreover, the two-photon and fourphoton transitions have the different polarization control efficiency, and the four-photon absorption can obtain the higher polarization control efficiency. Thus, the polarization control efficiency of the whole excitation process can be increased or decreased by properly designing the femtosecond laser field intensity and laser center frequency. These studies can provide a clear physical picture for understanding and controlling the multi-photon absorption process in the intermediate femtosecond laser field, and also can provide a theoretical guidance for the future experimental realization.     

Time-dependent theoretical approach to the influence of laser fields on the resonance enhanced multi-photon ionization of SH radical

This paper reports that the (2+1) resonance enhanced multi-photon ionization spectra of SH radical in external fields are simulated using the split-operator scheme of time-dependent wave-packet method. Two ionic states, i.e.~a¹Δ and b¹∑⁺, are involved in the simulation. It gives the simulated photoelectron spectra, the population in each electronic state, as well as the projection of the wave-packet in each electronic state on different vibrational states. These results show that the so-called four-state model can represent the experimental results well.     

初始振动态对氢分子离子电离通道的影响

通过数值求解非Born-Oppenheimer近似条件下的一维含时薛定谔方程,理论模拟了H2+在不同核初始振动态条件下(=0到=7)的库仑爆炸核初始动能释放谱。模拟结果表明：强激光场中氢分子离子的电离通道主要包括直接多光子电离、电荷共振增强电离及有中间过程的电荷共振增强电离,并且可以通过选取不同的初始振动态实现对氢分子离子电离通道的控制。     

初始振动态对氢分子离子电离通道的影响

通过数值求解非Born-Oppenheimer近似条件下的一维含时薛定谔方程,理论模拟了H2+在不同核初始振动态条件下(=0到=7)的库仑爆炸核初始动能释放谱。模拟结果表明：强激光场中氢分子离子的电离通道主要包括直接多光子电离、电荷共振增强电离及有中间过程的电荷共振增强电离,并且可以通过选取不同的初始振动态实现对氢分子离子电离通道的控制。     

理论研究强激光场中2pz态氢原子的电离

运用强场近似速度规范理论研究了激发态氢原子的电离情况,当 a.u. 时（ω是激光场的频率,γ是Keldysh绝热参数）,在线性极化激光场中推导了2pz态氢原子电离率的简单表达式,从公式中可以看出在低频极限的情况下,电离率和激光场频率ω成正比,这一公式对激发态氢原子电离机制的研究提供了重要的理论参考。     

Vibrational excitation of diatomic molecular ions in strong field ionization of diatomic molecules

A model based on the strong-field and Born-Oppenheimer approximations qualitatively describes the distribution over vibrational states formed in a diatomic molecular ion following ionization of the neutral molecule by intense laser pulses. Good agreement is found with a recent experiment [X. Urbain et al., Phys. Rev. Lett. 92, 163004 (2004)]. In particular, the observed deviation from a Franck-Condon-like distribution is reproduced. Additionally, we demonstrate control of the vibrational distribution by a variation of the peak intensity or a change of frequency of the laser pulse.     

Nonsequential double ionization of the aligned hydrogen molecule in strong field

This paper studies the nonsequential double ionization(NSDI) process of diatomic molecules aligned parallel and perpendicular to an intense linearly polarized laser field by using a three-dimensional semiclassical model.With this model,it achieves insight into the ion momentum distribution under the combined influence of a two-centre Coulomb potential and an intense laser field,and this result shows the significant influence of molecular alignment on the ratio between double and single ionization rate.Careful investigations show that the NSDI process for different alignment molecules has a close relation to the laser intensity and the different bounding electron distribution has a significant influence on the final ion momentum distribution.     

非序列双电离向饱和区过渡的电子最大关联度

本文采用三维半经典再散射模型系统地研究了 He 原子在 光强从域下到近序列双电离区强场作用下的非序列双电离问题, 统计了各种场强下最终电离的两个电子正负关联的几率之比, 发现发生最大正关联的场强处于向非序列 双电离饱和区过渡的区域, 并在关联纵向动量谱中展示了形成最大关联度的过程. 最后通过轨道"回溯"分析, 进一步研究了其背后的物理机理, 发现在碰撞后其中一个电子再散射和隧穿电子高速弱碰撞分别 是低场强和高场强下负关联比例增加的原因.     

原子非序列双电离的多次返回碰撞电离机理分析

本文采用三维半经典再散射模型研究了He原子在高光强(1.5×10¹⁵ W/cm²)、少周波激光脉冲作用下的非序列双电离问题,重点分析了沿激光电场极化方向的动量关联谱.发现两个电子沿相反方向发射的比例明显比中等光强区(7×10¹⁴ W/cm²)和低光强区(2.5×10¹⁴ W/cm²),以及同等光强的长脉冲情形都偏高, 同时V形结构也更加明显.通过轨道"回溯"分析, 进一步深入 关键词： 强场 非序列双电离 再散射     

Multiphoton and tunneling ionization of atoms in an intense laser field

We study the ionization probabilities of atoms by a short laser pulse with three different theoretical methods,i.e.,the numerical solution of the time-dependent Schro¨dinger equation(TDSE),the Perelomov-Popov-Terent’ev(PPT) theory,and the Ammosov-Delone-Krainov(ADK) theory.Our results show that laser intensity dependent ionization probabilities of several atoms(i.e.,H,He,and Ne) obtained from the PPT theory accord quite well with the TDSE results both in the multiphoton and tunneling ionization regimes,while the ADK results fit well to the TDSE data only in the tunneling ionization regime.Our calculations also show that laser intensity dependent ionization probabilities of a H atom at three different laser wavelengths of 600 nm,800 nm,and 1200 nm obtained from the PPT theory are also in good agreement with those from the TDSE,while the ADK theory fails to give the wavelength dependence of ionization probability.Only when the laser wavelength is long enough,will the results of ADK be close to those of TDSE.