Breakdown of the isobaric multiplet mass equation at A = 33, T = 3/2

Mass measurements on (33,34,42,43)Ar were performed using the Penning trap mass spectrometer ISOLTRAP and a newly constructed linear Paul trap. This arrangement allowed us, for the first time, to extend Penning trap mass measurements to nuclides with half-lives below one second ( 33Ar: T(1/2) = 174 ms). A mass accuracy of about 10(-7) (deltam approximately 4 keV) was achieved for all investigated nuclides. The isobaric multiplet mass equation was checked for the A = 33, T = 3/2 quartet and found to be inconsistent with the generally accepted quadratic form.     

Mass measurements of very neutron-deficient Mo and Tc isotopes and their impact on rp process nucleosynthesis

The masses of ten proton-rich nuclides, including the N=Z+1 nuclides ??Mo and ??Tc, were measured with the Penning trap mass spectrometer SHIPTRAP. Compared to the Atomic Mass Evaluation 2003 a systematic shift of the mass surface by up to 1.6 MeV is observed causing significant abundance changes of the ashes of astrophysical x-ray bursts. Surprisingly low α separation energies for neutron-deficient Mo and Tc are found, making the formation of a ZrNb cycle in the rp process possible. Such a cycle would impose an upper temperature limit for the synthesis of elements beyond Nb in the rp process.     

Experiments with thermalized rare isotope beams from projectile fragmentation: a precision mass measurement of the superallowed beta emitter 38Ca

The mass of the short-lived radio nuclide 38Ca (T(1/2) = 440 ms) has been measured with the 9.4-T Penning trap mass spectrometer of the Low-Energy Beam and Ion Trap Facility. A mass uncertainty of deltam = 280 eV has been achieved, corresponding to deltam/m = 8 x 10(-9). The result makes 38Ca, a superallowed beta emitter, a new candidate to test the conserved-vector-current hypothesis. The experiment is also the first demonstration that short-lived radioactive isotopes produced by projectile fragmentation of relativistic heavy-ion beams can be slowed down and prepared such that precision experiments of this kind are possible.     

Pseudo-dirac neutrinos: a challenge for neutrino telescopes

Neutrinos may be pseudo-Dirac states, such that each generation is actually composed of two maximally mixed Majorana neutrinos separated by a tiny mass difference. The usual active neutrino oscillation phenomenology would be unaltered if the pseudo-Dirac splittings are deltam(2) less, similar 10(-12) eV(2); in addition, neutrinoless double beta decay would be highly suppressed. However, it may be possible to distinguish pseudo-Dirac from Dirac neutrinos using high-energy astrophysical neutrinos. By measuring flavor ratios as a function of L/E, mass-squared differences down to deltam(2) approximately 10(-18) eV(2) can be reached. We comment on the possibility of probing cosmological parameters with neutrinos.     

New mass data for the rp-process above Z = 32

High-accuracy mass measurements have been performed with the Penning trap mass spectrometer ISOLTRAP at ISOLDE/CERN. The short-lived nuclides ^{70, 71, 72, 73}Se , ^{72, 73, 74, 75}Br , and ^{98, 99, 100, 101, 103}Ag have been measured with an average uncertainty of a few keV. The data are important input for nucleosynthesis calculations of the rp-process beyond Z = 32 .     

Creation of localized optical waves that Do not obey the radiation condition at infinity

X-ray bursts have been suggested as a possible site for the astrophysical rp-process. The time scale for the process is governed by beta-decay half-lives of several even-even N = Z waiting point nuclei, in particular, N = Z = 40 80Zr. A 4.1(+0.8/-0.6)-s beta(+)/EC half-life for 80Zr was determined by observing delayed 84-keV gamma rays depopulating a T(1/2) = 4-&mgr;s isomer at 312 keV in the daughter 80Y. As this half-life is lower than many previously predicted values, the calculated excessive production of A = 80 nuclides in astrophysical x-ray burst scenarios is reduced, and less extreme conditions are necessary for the production of heavier nuclides.     

Direct mass measurements of short-lived A=2Z-1 nuclides (63)Ge, (65)As, (67)Se, and (71)Kr and their impact on nucleosynthesis in the rp process

Mass excesses of short-lived A=2Z-1 nuclei (63)Ge, (65)As, (67)Se, and (71)Kr have been directly measured to be -46,921(37), -46,937(85), -46,580(67), and -46,320(141) keV, respectively. The deduced proton separation energy of -90(85) keV for (65)As shows that this nucleus is only slightly proton unbound. X-ray burst model calculations with the new mass excess of (65)As suggest that the majority of the reaction flow passes through (64)Ge via proton capture, indicating that (64)Ge is not a significant rp-process waiting point.     

Quadrupole deformation of the self-conjugate nucleus 72Kr

We report on the first determination of the absolute B(E2;0+(1)-->2+(1)) excitation strength in the N=Z nucleus 72Kr. 72Kr is the heaviest N=Z nucleus for which this quantity has been measured and provides a benchmark in a region of the nuclear chart dominated by rapidly changing deformations and shapes mediated by the interplay of strongly oblate and prolate-driving orbitals. The deduced quadrupole deformation strength is in agreement with a variety of self-consistent models that predict an oblate shape for the ground state of 72Kr. Large-scale shell-model Monte Carlo calculations reproduce the experimental B(E2) value and link the result to the occupation of the deformation-driving g9/2 orbit.     

New approach for measuring properties of rp-process nuclei

A new experimental approach was developed that can reduce the uncertainties in astrophysical rapid proton capture (rp) process calculations due to nuclear data. This approach utilizes neutron removal from a radioactive ion beam to populate the nuclear states of interest. Excited states were deduced by the gamma-decay spectra measured in a semiconductor Ge-detector array. In the first case studied, 33Ar, excited states were measured with uncertainties of several keV. The 2 orders of magnitude improvement in the uncertainty of the level energies resulted in a 3 orders of magnitude improvement in the uncertainty of the calculated 32Cl(p,gamma)33Ar rate that is critical to the modeling of the rp process. This approach has the potential to measure key properties of almost all interesting nuclei on the rp-process path.     

Beyond mean field approach to the beta decay of medium mass nuclei relevant for nuclear astrophysics

The Gamow-Teller strength distributions for the β decay of the ground state as well as the lowest excited states of the rp-process waiting point nuclei ⁶⁸Se and ⁷²Kr are obtained within the complex Excited Vampir variational approach using realistic effective interactions and a rather large model space. The shape mixing is consistently described for both the states in the even-even parent and the states in the odd-odd daugther nucleus. The influence of the shape mixing accounted by the different effective interactions used and comparison with the available data are presented. The possible influence of the decay of the lowest excited states of the parent nuclei in the astrophysical environment of X-ray bursts is discussed.Gamow-Teller strength distributions, β-decay half-lives, and β-delayed neutron emission probabilities for neutron-rich Zr nuclei are investigated for the first time within the complex Excited Vampir approach using a large model space. Comparison with available data and predictions relevant for the astrophysical r process are presented.     

Rayleigh instabilities in multiply charged sodium clusters

The stability of multiply charged sodium clusters Na(q+)(n) (q< or =10) produced in collisions between neutral clusters and multiply charged ions A(z+) ( z = 1 to 28) is experimentally investigated. Multiply charged clusters are formed within a large range of temperatures and fissilities. They are identified by means of a high-resolution reflectron-type time-of-flight mass spectrometer (m/deltam approximately 14 000). The maximum fissility of stable clusters is obtained for z = 28 and is X approximately 0.85+/-0.07, slightly below the Rayleigh limit (X = 1). It is mainly limited by the initial cluster temperature (T approximately 100 K).     

Carbon clusters for absolute mass measurements at ISOLTRAP

The cyclotron frequencies of singly charged carbon clusters C_n ⁺ (n ≥ 2) were measured with the Penning-trap mass spectrometer ISOLTRAP at ISOLDE/CERN. The present limit of mass accuracy δm/m = 1.2 ^. 10^-8 and the extent of the mass-dependent systematic shift (δm/m)_sys = 1.7(0.6) ^. 10^-10/u ^. (m - m _ref) of the setup were investigated for the first time. In addition, absolute mass measurements by use of pure clusters of the most abundant carbon isotope ¹²C are now possible at ISOLTRAP. Received: 21 March 2002 / Accepted: 16 May 2002 / Published online: 31 October 2002 RID="a" ID="a"Present address: CERN, CH-1211 Geneva 23, Switzerland; e-mail: klaus.blaum@cern.ch     

Direct mass measurement of the four-neutron halo nuclide 8He

A high-precision Penning trap mass measurement of the exotic 8He nuclide (T(1/2)=119 ms) has been carried out resulting in a reduction of the uncertainty of the halo binding energy by over an order of magnitude. The new mass, determined with a relative uncertainty of 9.2 x 10(-8) (deltam=690 eV) is 13 keV less bound than the previously accepted value. The mass measurement is of great relevance for the recent charge-radius measurement of 8He [P. Mueller, Phys. Rev. Lett. 99, 252501 (2007).10.1103/PhysRevLett.99.252501]. The 8He mass is the first result from the newly-commissioned Penning trap: TITAN (TRIUMF's Ion Trap for Atomic and Nuclear science) at the ISAC (Isotope Separator and Accelerator) radioactive beam facility at TRIUMF.     

Preparing a journey to the east of 208Pb with ISOLTRAP: Isobaric purification at A = 209 and new masses for 211-213Fr and 211Ra

With the Penning trap mass spectrometer ISOLTRAP, located at ISOLDE/CERN, preparatory work has been performed towards mass and decay studies on neutron-rich Hg and Tl isotopes beyond N = 126 . The properties of these isotopes are not well known because of large isobaric contamination coming mainly from surface-ionised Fr. Within the studies, production tests using several target-ion source combinations were performed. It was furthermore demonstrated around mass number A = 209 that the resolving power required to purify Fr is achievable with ISOLTRAP. In addition, masses of several isobaric contaminants, ^211-213Fr and ²¹¹Ra , were determined with a three-fold improved precision. The results influence masses of more than 20 other nuclides in the ²⁰⁸Pb region.     

ISOLTRAP: An on-line Penning trap for mass spectrometry on short-lived nuclides

ISOLTRAP is a Penning trap mass spectrometer for high-precision mass measurements on short-lived nuclides installed at the on-line isotope separator ISOLDE at CERN. The masses of close to 300 radionuclides have been determined up to now. The applicability of Penning trap mass spectrometry to mass measurements of exotic nuclei has been extended considerably at ISOLTRAP by improving and developing this double Penning trap mass spectrometer over the past two decades. The accurate determination of nuclear binding energies far from stability includes nuclei that are produced at rates less than 100 ions/s and with half-lives well below 100ms. The mass-resolving power reaches 10⁷ corresponding to 10keV for medium heavy nuclei and the uncertainty of the resulting mass values has been pushed down to below 10^-8. The article describes technical developments achieved since 1996 and the present performance of ISOLTRAP.     

Study of Muon-Catalyzed Fusion in Ortho–Para Controlled Solid Deuterium

Recently, the applicability of Penning trap mass spectrometry has been extended to nuclides with a half-life of less than one second. The mass of ³³Ar (T _1/2=174 ms) was measured using the ISOLTRAP spectrometer with an accuracy of 4.2 keV. This measurement provided a stringent test of the Isobaric Multiplet Mass Equation (IMME) at mass number A=33 and isospin T=3/2. The fast measurement cycle that shows the way to other measurements of very-short-lived nuclides is presented. Furthermore, the results of the IMME test are displayed. This revised version was published online in July 2006 with corrections to the Cover Date.     

Exploring new mass regions with the ISOLTRAP spectrometer

First direct mass measurements on rare earth isotopes around ¹⁴⁶Gd have been performed with the Penning trap mass spectrometer ISOLTRAP at ISOLDE/CERN. More than 40 isotopes of the elements Pr, Nd, Pm, Sm, Eu, Dy and Ho have been measured with an accuracy of typically 1 × 10^-7. In the case of ¹⁴¹Sm isomeric and ground state (ΔE = 175 keV) were resolved. Since isobaric contaminations are present in the ISOLDE beam, these measurements on rare earth isotopes became only possible after the installation of a new cooler trap which acts an isobar separator. This revised version was published online in August 2006 with corrections to the Cover Date.     

Binding energies of near proton-drip line Z = 22-28 isotopes determined from measured isotopic cross section distributions

A new method is proposed to determine the binding energy(B)of near proton-drip line isotopes from isotopic cross section distribution.To determine B of Z=22-28 isotopes(with T_z=-2 and-5/2),the lack of cross sections for proton-rich isotopes in the 345A MeV~(78)Kr+~9Be is overcome by predicting the proton-rich isotopes from a newly discovered scaling phenomenon found in the proton-rich isotopes measured in the 140A MeV~(40,48)Ca(~(58,64)Ni)+~9Be reactions.The cross sections for proton-rich isotopes are verified to exponentially depend on the average binding energy per nucleon,based on which B of the Z=22-28 isotopes with T_z=-2 and-5/2 are determined from cross sections.The determined B of the isotopes are justified from obeying the scaling phenomenon of the difference between the mass of mirror nuclei.The cross sections for the Z=22-28 isotopes with T_z=-1 and-3/2,which in potential can be experimentally studied in mass storage ring,are also predicted.     

Spectral property and its shape transition on 72—84Kr isotopes in microscopic core plus two—quasiparticle approach

By using a microscopic sdIBM-2+2q.p. approach, the levels of the ground-band, γ-band and partial two-quasi-particle bands for {}^{72-84}Kr isotopes are calculated. The data obtained are in good agreement with the recent experimental results, and successfully reproduce the nuclear shape phase transition of {}^{72-84}Kr isotopes at zero temperature. The ground-state band is described successfully up to J^π=18^+ and E_x=10.0MeV. Based on this model, the aligned requisite minimum energy has been deduced. The theoretical calculations indicate that no distinct change of nuclear states is caused by the abruptly broken pair of a boson, and predict that the first backbending of Kr isotopes may be the result of aligning of two quasi-neutrons in orbit g_{9/2}, which gains the new experimental support of the measurements of g factors in the {}^{78-86}Kr isotopes.     

Coherent development of neutrino flavor in the supernova environment

We calculate coherent neutrino and antineutrino flavor transformation in the supernova environment, for the first time including self-consistent coupling of intersecting neutrino and antineutrino trajectories. For neutrino mass-squared difference /deltam2/ = 3 x 10(-3) eV2 we find that in the normal (inverted) mass hierarchy the more tangentially-propagating (radially-propagating) neutrinos and antineutrinos can initiate collective, simultaneous medium-enhanced flavor conversion of these particles across broad ranges of energy and propagation direction. Accompanying alterations in neutrino and antineutrino energy spectra and fluxes could affect supernova nucleosynthesis and the expected neutrino signal.