Gamma-gamma directional correlation study in92Zr

The gamma-gamma directional correlation of the 2⁺′-2⁺-0⁺, 913(Iγ=1.69)-934(Iγ =100)keV cascade in⁹²Nb decay has been investigated with a NaI-Ge(Li) system. Our results yieldδ=?0.013 _?0.024 ^+0.041 . This is one of a very few cases where the second 2⁺ to first 2⁺ transition is not predominatelyE2. This may be related to the closed neutron shell, as earlier suggested. [Radioactivity⁹²Zr; measuredγ-γ(θ), deducedδ]     

Structure of the Triplet of low-lying states in101Mo

The properties of the triplet of low-lying states in¹⁰¹Mo have been studied through spectroscopy of theγ radiation following thermal neutron capture in¹⁰⁰Mo and β^? decay of¹⁰¹Nb and through a measurement of the proton angular distributions in the¹⁰⁰Mo(d,p) reaction with 14 MeV deuteron energy. The half-lives of the 13.5 keV state and the 57.0 keV 5/2⁺ state have been measured as 226(7) and 133(7)ns, respectively. These values and the quadrupole/dipole mixing ratios of the 13.5 keV and 43.5 keV transitions yield spin and parity 3/2⁺ for the 13.5 keV level. The E2 components in the 13.5 (3/2⁺ →1/2⁺) and 43.5 keV (5/2⁺→3/2⁺) transitions are ≦ 8·10^?4 and 54(9)%, respectively. The possibility of an additional state near to the 57.0 keV level is discussed. IBFM/PTQM calculations, taking into consideration the transitional character of the¹⁰⁰Mo boson core, account for the electromagnetic-transition and transfer-reaction pattern of the triplet of states.     

Investigation of neutron deficient Zr and Nb nuclei with heavy ion induced compound reactions

³²S and¹²C induced compound reactions on Fe, Ni and Se targets have been used to produce neutron deficient nuclei in the mass region 84≦A ≦87. In-beamγ-ray spectroscopy consisting of the measurement of excitation functions,γγ coincidences andγ-ray angular distributions has been performed. The following level energies and spin-parity values have been deduced:⁸⁴Zr: 540 keV, 2⁺; 1262.8, (4⁺); 2137.2, (6⁺); 3089.2⁸⁶Zr: 751.9, 2⁺; 1666.6, (4⁺); 2670.0, (6⁺); 2705.5, (5); 3271.3; 3298.5, (8⁺); 3423.5, (7); 3531.5, (10⁺); 3645.9; 4326.1; 4417.3 Half-lives and energies ofγ-rays from the residual activities have been measured. The existence of three new isotopes could be established by their radioactive decay:⁸⁴Nb(12±3 s)→⁸⁴Zr⁸⁶Nb(80±12 s)→⁸⁶Zr⁸⁷Mo(14.6±1.5 s)→⁸⁷Nb→⁸⁷Zr     

The decay of the 11.80 MeV isobaric analog resonance in93Tc to negative parity states in92Mo

The 2,524 keV 5^? state and 2,848 keV3^? state in⁹²Mo were excited by inelastic proton scattering going through the 11.80 MeV isobaric analog resonance in⁹³Tc. Angular distributions of the 3^?→ 2⁺ and 5^?→ 4⁺ γ-rays were measured and analyzed in order to obtain the partial waves of the outgoing protons.     

Very proton rich nuclei withN≈82

Postaccelerated⁵⁸Ni and⁶⁰Ni beams from the Munich MP tandem have been used to study the compound reactions⁵⁸Ni→⁹³Nb,⁹²Mo,⁹⁴Mo and⁶⁰Ni→⁹²Mo. The final nuclei¹⁴⁸Er,¹⁵⁰Er and¹⁴⁷Ho have been investigated with in-beamγ-spectroscopic methods, such as excitation functions,γγ coincidences, bunched-beam and pulsed-beam techniques. Level schemes of¹⁴⁸Er,¹⁵⁰Er and¹⁴⁷Ho have been established with the following level energies, spins, parities and half-lives:¹⁴⁸Er: 646.6 keV 2⁺; 1,524.0(4⁺); 2,254.3(5^?); 2,526.9(6⁺); 2,537.3(7^?), 2,706.0(7^?, 8^?); 2,784.4(8⁺); 2,915.5(10⁺) 13±3 μs¹⁵⁰Er: 1,578.9 keV 2⁺; 1,786.4 3^?; 2,261.2(5^?); 2,634.1(7^?); 2,734.3(8⁺); 2,798.3(10⁺) 2.7±0.2 us; 4,001.9; 4,491.8; 4,886.0; 5,222.7¹⁴⁷Ho: 765.4; 1,737.2; 2,355; 2,656.6 The level scheme of¹⁵⁰Er has been discussed in the framework of the seniority scheme. Perfect agreement with the experiment has been found for the predictions of this scheme for the half-lives of 10⁺ states inN=82 isotones. This is the first nuclear region where the predictions of the seniority scheme have been observed without strong perturbation.     

Level structure of106Mo

The level scheme of the very neutron rich nucleus ₁₀₆ ⁴² Mo₆₄ has been studied for the first time through theβ decay of¹⁰⁶Nb. Six new excited states were observed inγ singles andγ-γ coincidence experiments in addition to the 2⁺, 4⁺ and 6⁺ members of the ground state band. The excitation energies and the deexcitation pattern suggest the interpretation of the levels at 710, 885 and 956 keV as the 2 ₂ ⁺ , 3 ₁ ⁺ and 0 ₂ ⁺ states, respectively. The data support the assumption of a non-axial deformation of¹⁰⁶Mo. A half-life of (1.02±0.05) s has been determined for theβ decay of¹⁰⁶Nb.     

Level structure of 184W from the 183W(n, γ) reaction

The level structure of ¹⁸⁴W has been studied from the prompt γ-rays emitted following the capture of both thermal and 2 keV neutrons by ¹⁸³W. Energies and intensities were measured for both the primary and the secondary (low-energy) prompt γ-rays. From these data, a level scheme is proposed for ¹⁸⁴W in which all the I^π = 0⁺, 1⁺ and 2⁺ states below ≈ 2.0 MeV are observed. Where possible, rotational-band assignments have been made to these and other levels. Additional evidence is presented which confirms the 1130 keV state as being the band head of a K^π = 2^? octupole vibrational band. Admixed K^π = 0⁺ and 2⁺ bands are established at 1322 and 1386 keV, respectively, with the I^π = 2⁺ states (at 1431 and 1386 keV) having a mutual admixture of ≈ 12%. In the energy region above 1.5 MeV, the following bands and band-head energies are identified: K^π = 1⁺, 1613 keV; K^π = 0⁺, 1614 keV; K^π = 1⁺, 1713 keV; K^π = 2⁺, 1877 keV. The neutron binding energy in ¹⁸⁴W has been determined to be 7411.1±0.6 keV. The band structure of the 1613 keV (1⁺) and 1614 keV (0⁺) bands is observed to be strongly distorted, the observed $\text{A (}\text{h}\text{?}{}^2\text{/2}\text{I}\text{)}$ values being ≈ 3.6 keV and ≈ 32 keV, respectively. This strong distortion is shown to be explainable in terms of Coriolis coupling of reasonable strength between the two bands. A similar explanation is shown to account for the somewhat less anomalous A-values (22.8 keV and 14.0 keV, respectively) of the 2⁺ band at 1386 keV and the 3⁺ band at 1425 keV. The results of a phenomenological fiveband-mixing analysis involving the K^π = 0⁺ and 2⁺ bands below ≈ 1.5 MeV are presented and discussed. These calculations indicate, among other things, that the direct E2 matrix element connecting the 1322 keV, K^π = 0⁺ band and the ground-state band is quite small, possibly zero. They also indicate that a nonzero E2 matrix element exists between this excited K^π = 0⁺ band and the γ-vibrational band and that the magnitude of this element is comparable with that between the γ-vibrational and ground-state bands. Arguments favoring and apparently refuting the interpretation of the 1322 keV, 0⁺ band as a “two-phonon γ-vibration” are presented.     

Study of low-lying states in151Eu via (n,n′γ) reaction

The levels of¹⁵¹Eu have been investigated in the (n,n′γ) reaction using nuclear reactor fast neutrons. The energies, intensities and angular distributions of theγ-rays have been measured with the Ge(Li) spectrometer. Four rotational bands with the following band heads and Nilsson configurations have been identified: ground state band, 5/2⁺ [402]; 21.5 keV, 7/2⁺[404]; 196.5 keV, 3/2⁺[411]; 260.5 keV, 5/2⁺[413]. The low spin states at 332.2 and 336.2 keV have been tentatively assigned to the l/2⁺[411] Nilsson orbital, but 522.8, 580.0 and 587.0 keV states to the 1/2⁺[420] Nilsson orbital. The negative parity levels at 353.7, 522.1 and probably 546.2 keV have been proposed basing on theh _11/2 proton state.     

Gamow-teller strength distribution in the vicinity of A = 90: (I). Schematic calculation of GT strength in 90, 92, 94Nb

The distributions of Gamow-Teller strength in ^{90, 92, 94}Nb have been calculated utilizing the so-called GT force in the random phase approximation. For ⁹⁰Nb the calculated distribution is in striking agreement with that part of the ⁹⁰Zr(p, n) excitation function leading to 1⁺ excitations in ⁹⁰Nb and qualitative agreement is demonstrated for data from the reactions ^{92, 94}Zr(p, n). Some 25 % of the GT strength is found to lie well below the structureless giant resonance proposed by Ikeda et al. The implications of this result to the β-decay properties of neutron rich nuclei near A = 90 are discussed.     

Study of energy levels of 92Nb observed in the 92Zr(p,n) reaction

The energy levels of ⁹²Nb were observed in the ⁹²Zr(p, n) reaction by use of the neutron time-of-flight technique. Limits on the spins and parities of the ⁹²Nb levels were placed by observing the enhancement in the relative yield of the final states at an isobaric analog resonance and by the measurement of the relative yield off resonance. The measured enhancements and off-resonance yields are compared with values calculated using the statistical compoundnucleus model. Comparison of results from the two methods is used to obtain spin-parity assignments for nine energy levels lying between 976 and 1739 keV in ⁹²Nb.     

Energy levels of92Nb from 92Zr(p,nγ)92Nb

The energy levels of⁹²Nb were studied by means of the⁹²Zr(p, nγ) reaction. The deexcitation γ-rays were observed with a high-resolution Ge(Li) detector in the proton energy range 3.00–4.80 MeV in steps of about 25 keV. Many new excited states of ⁹²Nb were populated by this reaction. Excitation energies up to 1.77 MeV were determined with high precision, and a level scheme of ⁹²Nb is proposed. From a Hauser-Feshbach analysis, the γ-decay scheme and other information, the spin-parities of many levels were assigned.     

The 2+-2+ transition of 879 keV in160Dy investigated by electron-gamma directional correlation

e-γ directional correlation measurements of 2⁺(879 keV)2⁺(87 keV)0⁺ cascade in¹⁶⁰Dy have been made and the magnitude of electric monopole to quadrapole mixing ratio for 879 keV transition was found to beq _k =?0.03(10) for λ=0 (λ-according to Hager-Saltzer definition).     

Nuclear structure of low-lying 0+ states in Ge and Se isotopes

The following meanlives of levels in⁷²Se have been measured using the recoildistance Doppler-shift method:Τ(2⁺, 862 keV)=3.1±0.6 ps,Τ(2⁺′, 1317 keV)=12.5±2.6 ps,Τ(4⁺, 1638 keV)=1.2±0.3 ps andΤ(6⁺, 2469 keV)≦0.7 ps. These meanlives yield sixB(E2) values which are discussed together with the known data of the depopulation of the excited 0⁺′ state at 937 keV. Systematics of 0⁺′ states in the mass region 70?A?100 show that the low excitation energy of the 0⁺′ states is correlated with subshell closures. This suggests that the previous interpretation of the 0⁺′ state in⁷²Se as a rotational band head is questionable.     

Study of the excited states of119Sn by the decay of119g+m In

The decay of^119g+m In to the excited states of¹¹⁹Sn was investigated.¹¹⁹In was produced by the¹²⁰Sn(γ,p)¹¹⁹In reaction on an enriched SnO₂ target. The isomeric transition of 311.25 keV to the¹¹⁹In ground state was observed. In the beta decay of^119m In excited states at 23.9, 920.5, 921.4, 1089.0, 1187.9 and 1249.6keV in¹¹⁹Sn withJ ^π values of 3/2⁺, 3/2⁺, 5/2⁺, 5/2⁺, 3/2⁺ and 1/2⁺ respectively, are fed. In the decay of the¹¹⁹In ground state only the 7/2⁺ level in¹¹⁹Sn at 787.0 keV is fed.     

Untersuchung des Zerfalls von134Cs durch γ-γ-Winkelkorrelationsmessungen

γ-γ-angular correlation measurements with Ge(Li) detectors and NaJ(Tl) detectors provided theE2/M1 mixing ratios of the following gamma transitions: 3 ₁ ⁺ →2 ₂ ⁺ (475.3 keV), 2 ₂ ⁺ →2 ₁ ⁺ (563.3 keV), 4 ₂ ⁺ →4 ₁ ⁺ (569.4 keV), 3 ₁ ⁺ →2 ₁ ⁺ (1,039 keV). The angular correlation measurements were only consistent with spin 3 of the 1,643 keV level. The half life of the 1,401 keV level was determined by delayed coincidence techniques to beT _1/2 (1,401 keV)≦30 ps.     

Investigation of vibrational levels in226Ra by coulomb excitation and by the226Ra(d,pnγ) reaction

Vibrational bands in²²⁶Ra were studied by Coulomb excitation and by the²²⁶Ra(d,pnγ) reaction. The first-excitedK ^π = 0⁺ and 1^? bands with known band heads at 825 and 1049 keV, respectively, were extended up to the 8⁺ and 7^? levels. A new 2⁺ level at 1110 keV and the known 2⁺ level at 1156 keV were observed following Coulomb excitation and interpreted asγ vibration and possible member of a second-exitedK ^π = 0⁺ band, respectively. TheE1 andE2 branching ratios from these vibrational bands to the ground and first-excited 0^? band are explained within the rotational model including band mixings. No evidence was found for a 0⁺ level at 650 keV proposed earlier.     

Theβ + decay of the new isotope86Mo and the first observation of86m Nb

Theβ ⁺ decay of⁸⁶Mo has been firstly investigated by means ofβγ spectroscopy. The⁸⁶Mo nuclei were produced by fusion-evaporation reactions of⁵⁴ Fe (³⁵Cl, 1 p2n) and⁵⁸Ni (³²S,2p 2n) at beam energies of 103 and 120 MeV, respectively. Threeγ rays of 47.3, 49.8 and 187.0 keV were unambiguously identified to follow theβ ⁺ decay of⁸⁶Mo by results ofXγ andβγ coincidence and cross-bombardment. A half life and a maximumβ ⁺-ray energy of⁸⁶Mo were determined to be 19.6±1.1 s and 3.9±0.4 MeV, respectively. A decay scheme of⁸⁶Mo is proposed in this article. Furthermore, a decay of⁸⁶Nb has been studied using the same combinations of projectiles and targets, and a newβ-decaying isomer^86m Nb was observed with a half life of 56.3±8.3 s.     

Spin des 921 keV-Zustandes in99Tc

The angular correlation of the⁹⁹Tc 739-181 keV gamma-gamma cascade has been measured in a liquid molybdenium source. The result was:A ₂=0.0930 ± 0.0028,A ₄=?0.0095 ± 0.0042. The spin of the 921 keV level was determined to 3/2⁺. The mixing ratio of the 739 keV gamma-transition was measured to δ (E2/M1)=5.9 _?0.3 ^+0.4 .     

Richtungskorrelationsuntersuchungen an den γ-Kaskaden des131Cs

The¹³¹Cs decay has been studied by angular correlation measurements of the (404-216), (832-216), and (247-373) keV γ-cascades using NaJ(Tl)-detectors in connection with a two parameter multi-channel analyzer. Unique spin assignments are obtained for the 216 (Jπ=3/2⁺) and 373 (Jπ=3/2⁺) keV levels. A previously discussed value ofJπ=5/2⁺ for the 1048 keV level is ruled out. The multipole character of the 404 keV transition is found to beE2 with less than 2%M1.