Lifetimes of a dipole cascade in 192Hg

The β-spectrum of the 3^?-2⁺ transition in the decay of¹⁴⁶Pm has been investigated with a 4π-Si(Li)-semiconductor spectrometer in a β-γ-coincidence experiment for the first time. The shape factor has been determined: C(W)=1?0.394W}-0.275/W+0.044 W². The spin and parity of the ground state of¹⁴⁶Pm can be determined to be 3^?. The shape of this non-allowed spectrum indicates the existence of the “cancellation” or “selection rule” effect.     

The 1-(1.9 MeV β-)2+ transition in the decay of148Pm

The non-unique first-forbidden 1^?(1.9 MeVβ ^?)2⁺ transition in the decay of¹⁴⁸Pm is studied. The nuclear matrix elements are evaluated using for the ground state of the odd-odd¹⁴⁸Pm a phenomenological wave function derived in a previous work in the framework of the two-quasiparticle model and assuming that the first excited 2⁺ state in¹⁴⁸Sm can be described as the first quadrupole phonon state. This model provides nuclear matrix elements which are capable of describing experimental data like the spectrum shape factor, the longitudinal polarization of the electrons and a particular set ofβ-γ directional correlation coefficients, but it fails to interpret the large logft value of this transition. In addition, the validity of theξ-approximation is discussed.     

Decay of the 4.2-min152Pm into levels of152Sm

After bombardments of enriched¹⁵²Sm with 14-MeV neutrons, three isomers of¹²⁵Pm reaction, have been observed with half-lives of 4.2±0.2 min, 7.5±0.2 min and 15.0±1.0 min. Sources of pure 4.2-min¹⁵²Pm were obtained by separating the promethium from its parent 11-min¹⁵²Nd produced by thermal-neutron induced fission of²³⁵U. The beta and gamma radiations of the 4.2-min¹⁵²Pm have been investigated using semiconductor and scintillation spectrometers. Most of theγ-ray transitions could be placed in a level scheme for 152Sm. Especially interesting is a level at 1083 keV for which the assignmentI ^π=0⁺ is proposed. In a 4πβγ experiment, the ground state feeding of¹⁵²Sm in theβ ^?-decay of the 4.2-min¹⁵²Pm has been measured to be 61% of allβ-ray transitions. AQ _β-value of 3.4±0.2 MeV has been obtained.     

The decay scheme of the 3-s Isomer of100Nb and the properties of levels in100Mo

Theβ ^? decay of the longer-lived isomer in¹⁰⁰Nb has been studied at the fission-product separator JOSEF. Measurements ofγ-ray singles spectra, ofγ-γ coincidences and ofγ-γ angular correlations have been performed. A value oft _1/2=2.99(11)s has been determined for the isomer which probably hasI ^π=4⁺ or 5⁺. A scheme of the levels of¹⁰⁰Mo which are populated in the decay of this isomer has been established. Information on the spins of several states of¹⁰⁰Mo has been obtained. Thus,I=0 levels have been identified at 1,505, 2,038 and 2,087 keV. The mixing ratios have been determined for the 2₂ ⁺→2₁ ⁺ and 2₃ ⁺→2₁ ⁺ transitions. The results provide evidence for a vibrational structure of¹⁰⁰Mo with separate bands based on the ground state and on the first excited 0⁺ level.     

β + ratio andβ-delayedγ-decay of146Eu

The positron decay of¹⁴⁶Eu was investigated, firstly to derive for the allowed transition to the 2046 keV state in¹⁴⁶Sm the electron capture to positron decay ratio. The experimental valueEC/β ⁺=43.7(42) is found to be in agreement within the respective error intervals with the ones calculated from the formalism of allowed decay using the recentQ-values of¹⁴⁶Eu. Further on, theγ-decay properties of¹⁴⁶Eu have been reinvestigated with emphasis on implied modifications of the hitherto accepted decay scheme: 42 new levels and 33 newγ-transitions were placed in the revised level scheme, 12 of the previously reported levels were deleted. The level distribution of¹⁴⁶Sm is discussed within a statistical model. The indication for a non-statisticalβ-strength function is observed.     

States inN=80140Nd populated in the decay of140Pm

The level structure of theN=80,¹⁴⁰Nd has been investigated through the beta decay of^140m Pm and^140g Pm, whose decay half-lives were measured to be 5.95±0.05 min and 9.1±0.5 sec, respectively. Decay schemes for the two isomers have been constructed fromγ-ray measurements. With the help of the beta decayft values and internal conversion electron measurements, spins and parities were deduced for levels in¹⁴⁰Nd. Among the levels a 7^? state at 2222.0 keV and a 5^? state at 2273.3 keV are identified as two-neutron quasiparticle states. The (ie233-01) for^140m Pm and^140g Pm have been deduced as 7^? and 1⁺, respectively. From beta end-point measurements, the decay energies of the two isomers have been determined asQ _EC=6.48±0.07 MeV^140m (Pm) andQ _EC=6.08±0.10 MeV (^140gPm). The results are discussed in the light of nuclear systematics of theN=79 and 80 isotones.     

Shape coexistence and other aspects of nuclear structure in40Ar

Theγ-decay of⁴⁰Ar has been studied by particle-γ-ray coincidence measurements in the³⁷Cl(α, pγ) reaction at 12 and 13 MeV bombarding energy. Particle-γ-ray angular correlations and linear polarizations ofγ-rays were measured at 12 MeV. A lifetime measurement using the Doppler-shift attenuation method was performed at 11 MeV. The coexistence of spherical and deformed states in⁴⁰Ar could be concluded from the observation of aK ^π=0⁺ rotational band which has itsI ^π=0⁺ through 6⁺ members at 2,121, 2,524, 3,515 and 4,959 KeV excitation energy. The intrinsic quadrupole moment derived fromB(E2) values is ∥Q ₀∥=1,320 _?120 ⁺⁶⁰ mb. Negative-parity states with high spin were observed at 4,858(5^?), 4,494(5^?), 4,226(4^?) and 4,991 KeV(4^?) excitation energy. A complete account of all levels below 5 MeV excitation energy is obtained by a model in which twod _3/2 proton holes couple weakly to the⁴²Ca levels below 4.75 MeV excitation energy.     

Tentative level diagram of146Pm below 1.1 MeV

The level scheme of the doubly odd nucleus¹⁴⁶Pm was investigated by means of in-beam spectroscopy. The¹⁴⁶Nd(p, n) reaction in the 3.5–8 MeV proton energy interval on enriched targets has been used to populate the exited states of¹⁴⁶Pm. High resolutionγ-ray spectra using Ge(Li) and hyperpure Ge detectors and conversion electrons with a mini-orange spectrometer were measured. Withγ-exitation functions andnγ-coincidences usingnγ-discriminated NE231 neutron detectors transitions in¹⁴⁶Pm were identified,γγ-coincidences gave information aboutγ-cascades. With these data a level scheme of 38 levels below 1.1 MeV exitation energy has been deduced including 73 transitions. For 12 transitions experimental conversion coefficients have been evaluated, which agree with the expected values forM1/E2-transitions.     

Non-yrast level structure of135Pr

Levels of¹³⁵Pr populated in the (p,2n) reaction were studied using methods of in-beamγ-ray and conversion electron spectroscopy. Many low-lying positive-parity states give evidence of a deformation ofβ=0.15–0.20. The same conclusion is evident from band structures built on these positive-parity states and on theh _11/2 negative-parity state. The triaxial rotor-plus-particle model reproduces quite well band structures withβ=0.20 andγ= 21°.     

Messung von fünf β-γ-Zirkularpolarisationskorrelationen beim Zerfall Eu152→Gd152

In the decay Eu¹⁵²→Gd¹⁵² fiveβ(circularly polarizedγ) correlations have been measured (Table). The Fermi matrix element of the 3^?–3^? β transition is small or vanishing. The levels of 344 and 755 keV (I=2⁺ and 4⁺, respectively) seem to be collective states.     

Coulomb excitation of230Th with32S,84Kr and142Nd projectiles

The Coulomb excitation measurements for the²³⁰Th nucleus with³²S,⁸⁴Kr and¹⁴²Nd projectiles are presented. The use of different projectiles allowed us to get information in the ground-state band and side bands. The energy spectrum of the ground-state band and of the lowest negative-parity band have been investigated up to the spin valueI=24⁺ andI=19^?(21), respectively. Five side bands (K ^π=0⁺, 2 ₁ ⁺ , 2 ₂ ⁺ , 1^?, 2^?) were observed also. The branching ratios for a large number of transitions in the spin regionI≦10 for π=+1 andI≦9 for π=? 1 are analysed. The full set of experimental data contains information on the mixing of the adiabatic states and on the nuclear response to the electromagnetic field ofγ-radiation. It is shown that the experimental data may be explained taking into account the coupling of the ground-β- and twoγ-bands and also of theK ^π=0^?, 1^? and 2^? negative-parity bands. An enhancement of the transitions from theγ-to theβ-band in respect to the transitions from theγ to the ground band and from theβ- to the ground band is reported. The mixing of the negative-parity bands is found to be typical for the alignment of the octupole-vibrational angular momentum. The strong spin dependence of the intrinsic matrix elements of the electric-dipole operator follows from the branching ratios of inter- and intra-band transitions from theK ^π=0^? states.     

Levels in182W populated in the decay of182Ta

Theγ-rays emitted in theβ-decay of¹⁸²Ta have been reinvestigated with improved statistics in attempting to clarify the reported new levels at 1460.41, 1592.98, 1620.36, 1712.29 and 1762.91 keV in¹⁸²W observed in theβ-decay of¹⁸²Ta. The present study demonstrated that the fifteen newγ-rays, which were used to support the existence of the five new levels, are not relevant to theγ-decay of¹⁸²Ta. Therefore the five new levels are not populated in this decay. Additionally, theγ-ray with an energy of 1035.6 keV (0 ₂ ⁺ →2 ₁ ⁺ ) deexciting theβ-band head in¹⁸²W is observed for the first time in the present decay study and the previous tentative placement of the 351.0 keVγ-ray in the level scheme is confirmed by the present coincidence measurements.     

Gamma-ray-L-x-ray directional correlations in182W

Directional correlations between gamma radiation andL x-rays in¹⁸²W have been measured. The x-rays are emitted following the internal conversion process of the 100.1 keV 2⁺ → 0⁺ transition. The experimental results for anisotropies involving gamma radiation emitted in the 1189.0 keV transition andL x-rays are A(γ?L _l )=?0.073(27),A(γ?L _α)=?0.0102(45),A(γ?L _β)=?0.0031(35), andA(γ?L _γ)=?0.007(13). The value deduced for the coefficientU ₂(e) pertaining to the converted transition isU ₂(e)=0.52(8) in reasonable agreement with the theoretically expected value 0.410. A note is given on the use of internal conversion radial matrix elements.     

Structure of even-even138Nd from the decay of138Pm

The structure of¹³⁸Nd is investigated through theβ ⁺-decay of¹³⁸Pm, whose decay half-life is measured to be 3.24±0.05 min. A level structure comprising 27 excited states and 52 transitions is constructed. With the help of deducedft values and internal conversion coefficients, spin-parity assignments are made to many states in¹³⁸Nd and to the ground states of¹³⁸Pm. From the positron end-point energy measurement, the total decay energy is determined to be 5.4±0.2 MeV, which is compared with the predictions of several mass formulae and with the decay energy systematics of theN=77 isotones. The structure of¹³⁸Nd is discussed in the light of nuclear systematics of theN=78 isotones.     

Nuclear levels in228Th populated in the decay of228Pa

The electron-capture decay of²²⁸Pa to levels in²²⁸Th has been studied using mass-separated sources and high-resolutionγ-ray and conversion-electron spectroscopy. A level at 979.5 keV is assigned as 2⁺ member of a second excited K_π=0⁺ band, with the 0⁺ band head at 938.6 keV. The 2⁺ and 3⁺ members of a second excited K_π=2⁺ band at 1153.5 and 1200.5 keV, which decay by strongE0 transitions to the 969 keVγ-vibrational band, are confirmed. In addition we tentatively propose a K_π=1⁺ band at 944 keV. The K_π=0^?, 1^? and 2^? members of the octupole quadruplet are confirmed, and theγ decay of these levels is analysed in an approach, in which the mixing of the octupole bands by the Coriolis interaction is taken into account. It is suggested that octupole correlations might be important for theE1 transition moments. A total of 29 levels is observed between ～1.4 and ～2.0 MeV, for which the nuclear structure, and the possible assignment to rotational bands, is unclear.     

Measurement of radiative Σ±→nπ±γ decay

The radiativeΣ ⁺ → nπ⁺ γ decay mode was analysed in the 81 cm SACLAY hydrogen bubble chamber exposed to a stoppingK ^? beam at the CERN PS. The pion spectrum was measured up to momenta of 150 MeV/c in theΣ rest frame. We obtain the following branching ratios based on 180 Σ⁺→nπ⁺γ and 292Σ ^?→ nπ^?γ events:Γ(Σ⁺ → nπ⁺ γ)/Γ(Σ⁺→nπ⁺)=(0.93±0.10)×10^?3 Γ(Σ^?→nπ^? γ)/Γ(Σ^?→nπ^?)=(0.46±0.06)×10^?3. An unambiguous assignment ofS-wave to the Σ^?→nπ^? andP-wave toΣ ⁺→nπ⁺ was obtained. The absolute and differential decay rates as well as the parity assignments are in good agreement with theoretical predictions.     

Spins und γ-Multipolordnungen beim Zerfall Fe59→Co59

In the decay of Fe⁵⁹ the following quantities have been measured:γ-ray intensities, conversion coefficients andβ-(circularly polarizedγ) correlations. The conversion coefficients were found to be: for the 1.10 MeVγ-transition, α_tot.=(1.36±0.10)·10^?4 and for the 1.29 MeVγ-transition, α_tot.=(1.07±0.08)·10^?4. The asymmetry parameterA of the correlationβ(0.27 MeV)?γ(1.29 MeV) were measured to beA= ?0.17±0.10, and forβ(0.46 MeV)?γ(1.10 MeV),A=?0.13±0.04. From these data and publishedγ?γ angular correlation measurements the following spins of Co⁵⁹ levels could be deduced: 1.10 MeV,I=5/2^?; 1.29 MeV,I=5/2^?; and 1.43 MeV,I=3/2^?. The two strongβ-ray groups are pure Gamow-Teller transitions (ΔI=1). The multipolarities of all fiveγ-rays are given.     

Decay of the134Cs isomers and the levels of134Xe,134Cs,and134Ba

A precision study of the decay of¹³⁴Cs ^g and¹³⁴Cs ^m has been made, using ordinary Ge(Li) spectrometers and ā Compton-suppression spectrometer. The logft value of the second forbidden nonuniqueβ-decay to¹³⁴Xe has been measured to be 13.0±0.2. TheM4γ-ray transition in¹³⁴Cs^m(8^?) decay has been measured to haveα _K= 73±7 and a hindrance of 7.0 over the Moskowski estimate. This is discussed in terms of the level configurations and the analogous transition in¹³³Xe. A new intensity limit of 2×10^?6 has been set for the zero-phonon transition between the 4⁺ and 2⁺ members of the two-phonon triplet. This leads to an upper limit forB(E2)_4→2′, greater than 905. This and the more preciseγ-ray intensity values are discussed in relation to presently available nuclear models.     

Nuclear orientation study of97, 103, 105Ru in Fe

Angular distributions have been measured forγ-rays emitted following the decays of^{97, 103, 105}Ru oriented in an iron matrix at temperatures down to 2.8mK. From the temperature dependence of theγ-anisotropies the magnetic hyperfine splitting frequenciesν _M =|gμ _N B _HF/h| of^{97, 103, 105}RuFe were found to be 110(7), 57(15) and 80 _?50 ⁺¹⁷ MHz, respectively. With the known hyperfine fieldB _HF=?489.6(4.0) kG the nuclearg-factors are derived as ∣g(⁹⁷Ru;j ^π=5/2⁺)∣=0.29(2), ∣g(¹⁰³Ru;j ^π=3/2⁺)∣=0.15(4) and ∣g(¹⁰⁵Ru;j ^π=3/2⁺)∣=0.21 _-0.13 ^+0.05 . The analysis for¹⁰³RuFe has been performed with the assumption ofj ^π=3/2⁺ and 5/2⁺ for the ground state of¹⁰³Ru. Taking into account experimentally knowng-factors of 3/2⁺ and 5/2⁺ states in this mass region, our data strongly favour the assignmentj ^π=3/2⁺ for the¹⁰³Ru ground state.