Lifetimes of excited electrons in Fe and Ni: first-principles GW and the T-matrix theory

We present the results of an ab initio calculation of excited electron lifetimes in ferromagnetic materials which incorporates non-spin-flip and spin-flip processes within GW and T-matrix approaches. The method we develop is applied to low-energy electron excitations in Fe and Ni. It is found that the spin-wave generation in Fe essentially reduces the lifetimes of the spin-minority d states whereas the free-electron-like spin-minority states and all the spin-majority states are affected much less. The influence of spin-flip scattering on the lifetimes in Ni appears to be weak. The T-matrix non-spin-flip processes are important for the lifetimes of excited spin-minority states.     

Inelastic quasiparticle lifetimes of the Shockley surface state band on Ni(111)

We present a study of the low-energy quasiparticle lifetimes of the Shockley surface state on the Ni(111) surface with scanning tunnelling spectroscopy. By measuring the coherence length of the decaying standing wave pattern at straight step edges electron and hole lifetimes have been determined. The values of the lifetime measured on this ferromagnetic surface show to be considerable smaller than the values obtained from noble metal surfaces. This is explained by differences in the electron density of states at the Fermi energy but has to include substantial spin-flip scattering. Furthermore hole lifetimes appear to be larger than electron lifetimes with the same excitation energy. Although only results for the majority spin component are presented, a spin-dependent selfenergy is expected.     

Search for isovector giant monopole resonances via the Pb(3He,tp) reaction

The (nat)Pb(3He,tp) reaction at E(3He) = 177 MeV was studied to identify 2Planck's over 2piomega isovector monopole strength in Bi isotopes. Monopole strength was found in the region -45相似文献   

Observation of the 7 MeV excited spin-flip and non-spin-flip partners in 16 ΛO by γ -ray spectroscopy

We have observed three γ -ray transitions in _Λ ¹⁶ O from both 7MeV excited spin-flip and non-spin-flip partners ( 2^-, 1^- ₂ to the ground-state doublet ( 1^- ₁, 0^- via the ¹⁶O(K ^-,π^-) reaction. The 7MeV excitation energies of the spin-doublet members ( 2^-, 1^- ₂ were determined to be 6784±4±4 keV and 6562±1±2 keV, respectively, and thus the spacing was obtained to be 222±4±5 keV. This is the first observation of the spin-flip state directly populated by the ( K ^-,π^- reaction. Moreover, such directly populated spin-flip and non-spin-flip partners were resolved for the first time.     

Kinetics of formation of the excited states of krypton atoms and ions upon electron-induced desorption from a solid surface

The kinetics of formation of the excited states of the atomic krypton ion is studied in pure krypton at a low pressure. The excited states are formed due to the dissociation of excited molecular ions desorbed from a solid surface by an electron beam. The lifetimes of these ions and their dissociation channels are determined.     

Tunneling conductance of a two-dimensional electron gas with Dresselhaus spin-orbit coupling

We theoretically studied the spin-dependent charge transport in a two-dimensional electron gas with Dresselhaus spin-orbit coupling (DSOC) and metal junctions. It is shown that the DSOC energy can be directly measured from the tunneling conductance spectrum. We found that spin polarization of the conductance in the propagation direction can be obtained by injecting from the DSOC system. We also considered the effect of the interfacial scattering barrier (both spin-flip and non-spin-flip scattering) on the overall conductance and the spin polarization of the conductance. It is found that the increase of spin-flip scattering can enhance the conductance under certain conditions. Moreover, both types of scattering can increase the spin polarization below the branches crossing of the energy band.     

Strain-modulated ultrafast magneto-optic dynamics of graphene nanoflakes decorated with transition-metal atoms

We perform first-principles calculations and coherent laser-matter interaction analyses to investigate the laser-induced ultrafast spin flip on graphene nanoflakes(GNFs) with transition metal elements attached on the boundary [TMGNFs(TM = Fe, Co, Ni)]. It is shown that the spin-flip process on TMGNFs is highly influenced by the involved element species and the position attached to the nanoflakes. Furthermore, taking NiGNF as an example, the first-principles tensile test predicts that the variation of the C–Ni bond length plays an important role in the spin density distribution, especially for the low-lying magnetic states, and can therefore dominate the spin-flip processes. The fastest spin-flip scenario is achieved within 80 fs in a NiGNF structure under 10% tensile strain along the C–Ni bond. The local deformation modulation of spin flip provides the precursory guidance for further study of ultrafast magnetization control in GNFs, which could lead to potential applications in future integrated straintronic devices.     

The nuclear deformation versus the spin-flip like excitations and the suppression of the 2νββ decay amplitude

The suppression mechanism of the Gamow-Teller double beta decay amplitude M_GT is studied using a many body Hamiltonian which describes a composite system of protons and neutrons moving in a projected spherical single particle basis. Alike nucleons interact through pairing while protons and neutrons by a separable dipole-dipole force both in the particle-hole (ph) and particle-particle (pp) channels. The spin-flip and non-spin-flip components of the QRPA phonons have a differents contribution to the M_GT values. The relative magnitudes and phases depend both on the strength of the particle-particle interaction (g_pp) and on the nuclear deformation. The deformation yields a fragmentation of the M_GT value on one hand and washes out the separation of states of pure spin-flip and non-spin-flip structures. Due to this effect M_GT has only one fragmented resonance structure in the low part of the spectrum.     

基于双激发态对稠密等离子体中双电子复合速率系数的研究

讨论了稠密等离子体中双电子复合速率系数的计算方法,推导出了在双激发态间跃迁过程和关于双激发态的碰撞电离和自电离过程的影响下双电子复合速率系数作为关于电子密度函数的计算公式,并以类氖镍离子为例进行了计算.计算结果展示了双电子复合速率系数随电子密度增大的具体变化趋势.此外,还给出了在不同原子过程影响下双电子复合速率系数的数据,并进行了分析.     

Laser-induced down-conversion parameters of singly and doubly doped ZnS phosphors

Singly and doubly doped ZnS phosphors have been synthesized using flux method. Laser-induced photoluminescence has been observed in ZnS-doped phosphors when these were excited by the pulsed UV N₂ laser radiation. Due to down-conversion phenomenon, fast phosphorescence emission in the visible region is recorded in milliseconds time domain for ZnS:Mn while in the case of ZnS:Mn:killer (Fe, Co and Ni) the lifetime reduces to microseconds time domain. Experimentally observed luminescent emission parameters of excited states such as, lifetimes, trap-depth values and decay constants have been reported here at room temperature. The high efficiency and fast recombination times observed in doped ZnS phosphors make these materials very attractive for optoelectronic applications.     

Photon structure functions in quantum chromodynamics: (I). Operator product expansion method

A study of the polarized photon structure functions is made using the operator product expansion in the framework of perturbative chromodynamics. The non-spin-flip function is corrected as in the unpolarized case but the spin-flip function is unchanged.     

Magnetic neutron-wave resonator

Expressions for the neutron density and reflection amplitude have been obtained in the case of a magnetic neutron-wave resonator placed in a static magnetic field or in static and rotating magnetic fields. It is shown that the enhancement of the spin-flip neutron reflection coefficient and that of spin-flip neutron density are proportional to the squared and cubic enhancements of nuclear neutron absorption or the non-spin-flip neutron density, respectively. The conditions for neutron measurements with a high sensitivity of the parameters of magnetic structures have been determined.     

Dirac R-matrix calculations of photoionization cross sections of Ni XII and atomic structure data of Ni XIII

We performed R-matrix calculations for photoionization cross sections of the two ground state configuration 3s²3p⁵ (²P^o_3/2,1/2) levels and 12 excited states of Ni XII using relativistic Dirac Atomic R-matrix Codes (DARC) across the photon energy range between the ionizations thresholds of the corresponding states and well above the thresholds of the last level of the Ni XIII target ion. Generally, a good agreement is obtained between our results and the earlier theoretical photoionization cross sections. Moreover, we have used two independent fully relativistic GRASP and FAC codes to calculate fine-structure energy levels, wavelengths, oscillator strengths, transitions rates among the lowest 48 levels belonging to the configuration (3s²3p⁴, 3s3p⁵, 3p⁶, 3s²3p³3d) in Ni XIII. Additionally, radiative lifetimes of all the excited states of Ni XIII are presented. Our results of the atomic structure of Ni XIII show good agreement with other theoretical and experimental results available in the literature. A good agreement is found between our calculated lifetimes and the experimental ones. Our present results are useful for plasma diagnostic of fusion and astrophysical plasmas.     

GRID lifetime measurements in59, 61, 63Ni following thermal neutron capture

The GRID-method has been used to measure the lifetimes of ten excited states in^{59, 61, 63}Ni following thermal neutron capture in Ni targets of natural isotopic composition. Four of the lifetimes have been determined for the first time, the other six lifetimes can be compared with the results of conventional DSA-measurements following charged particle induced reactions. Cascade feeding effects have been included in the analysis. Level energies and electromagnetic properties of negative parity states in⁵⁹Ni have been compared with the results of shell model calculations in 3p0h and 4p 1h model spaces. Statistical model estimates of the lifetimes as function of excitation energy and spin are also given.Work partially supported by Deutsches BMFT under contract 06GOE141     

Spin-flip processes and ultrafast magnetization dynamics in Co: Unifying the microscopic and macroscopic view of femtosecond magnetism

The femtosecond magnetization dynamics of a thin cobalt film excited with ultrashort laser pulses has been studied using two complementary pump-probe techniques, namely, spin-, energy-, and time-resolved photoemission and the time-resolved magneto-optical Kerr effect. Combining the two methods, it is possible to identify the microscopic electron spin-flip mechanisms responsible for the ultrafast macroscopic magnetization dynamics of the cobalt film. In particular, we show that electron-magnon excitation does not affect the overall magnetization even though it is an efficient spin-flip channel on the sub-200 fs time scale. Instead, we find experimental evidence for the relevance of Elliott-Yafet-type spin-flip processes for the ultrafast demagnetization taking place on a time scale of 300 fs.     

Nonequilibrium transport through a vertical quantum dot in the absence of spin-flip energy relaxation

We investigate nonequilibrium transport in the absence of spin-flip energy relaxation in a few-electron quantum dot artificial atom. Novel nonequilibrium tunneling processes involving high-spin states, which cannot be excited from the ground state because of spin blockade, and other processes involving more than two charge states are observed. These processes cannot be explained by orthodox Coulomb blockade theory. The absence of effective spin relaxation induces considerable fluctuation of the spin, charge, and total energy of the quantum dot. Although these features are revealed clearly by pulse excitation measurements, they are also observed in conventional dc current characteristics of quantum dots.     

Spin-flip transitions of two-dimensional electrons in nonsymmetric heterostructures

The absorption of far-infrared radiation due to electron transitions between spin-split states in nonsymmetric quantum wells excited by a plane-polarized electric field is considered. It is shown that a relative contribution of the exchange renormalization of spin-flip transitions decreases as the concentration of two-dimensional electrons increases. The shape of the absorption peak under resonance transitions is calculated for the case when the line broadening is determined using scattering by static defects. The effect of the Coulomb interaction on the shape of the peak is taken into account, and the suppression of spin-flip absorption due to temperature growth is described.     

Effects of adsorbates on the formation of doubly excited He atoms during impact of He2+ ions on Fe(110) and Ni(110) surfaces

The formation of doubly excited states of He atoms during collisions of He²⁺ ions with projectile energies between 74 eV and 124 eV with an Fe(110) and a Ni(110) surface is studied via Auger electron spectroscopy. We observe that the electron spectra from autoionization of doubly excited states of 2s², 2s2p, 2p² configurations show a pronounced dependence on the coverage with oxygen for both surfaces. For a controlled O₂ adsorption on the Fe(110) and Ni(110) surfaces we can explain the resulting changes in the electron spectra by the modification of the measured work functions of the target surfaces. In terms of thermal desorption and dissolution into the bulk of surface contaminations at elevated temperatures, we present an alternative interpretation of similar previous studies by another group, where the local electron spin polarization of Fe(110) and Ni(110) surfaces was deduced from changes in the electron spectra as function of target temperature.     

Magnetic metastability in tetrahedrally bonded magnetic III-nitride semiconductors

Results of density-functional calculations for isolated transition metal (TM = V, Cr, Mn, Fe, Co, Ni on cation sites) doped GaN demonstrate a novel magnetic metastability in dilute magnetic semiconductors. In addition to the expected high spin ground states (4muB/Mn and 5muB/Fe), there are also metastable low spin states (0muB/Mn and 1muB/Fe)--a phenomenon that can be explained in simple terms on the basis of the ligand field theory. The transition between the high spin and low spin states corresponds to an intraionic transfer of two electrons between the t2 and e orbitals, accompanied by a spin-flip process. The results suggest that TM-doped wideband semiconductors (such as GaN and AlN) may present a new type of light-induced spin-crossover material.     

Reappearance of fine structure as a probe of lifetime broadening mechanisms in the 4f(N) --> 4f(N-1)5d excitation spectra of Tb3+, Er3+, and Tm3+ in CaF2 and LiYF4

High-energy transitions in the 4f(N) -->4f(N-1)5d excitation spectra of lanthanide ions in host crystals are usually broadened due to the short excited-state lifetimes, whereas low-energy transitions, with longer excited-state lifetimes, may show fine structure. We report the surprising observation that for some materials fine structure is observed not only for the low-energy excitation bands but also for some high-energy transitions. The excited states that display fine structure are those for which the 5d electron is in the lowest crystal-field level but the 4f(N-1) core is in a highly excited state, indicating that the broadening depends only on the energy of the 5d electron and not on the total energy of the 4f(N-1)5d excited state.