超短超强激光脉冲辐照超薄碳膜电离状态研究

为了进一步理解极端条件下物质的电离特性, 特别是超短超强激光脉冲辐照超薄靶时等离子体的形成与分布, 本文以超薄碳膜为例, 细致研究了超短超强激光脉冲辐照下原子的离化过程. 分析和比较了强激光场直接作用电离和靶内静电场电离等两种场致电离形式, 在碰撞电离可以忽略的情况下, 发现更多的电离份额是来自靶内静电场的电离方式. 研究了激光脉冲强度对电离的影响, 发现激光脉冲强度越强, 电离速度越快, 产生的高价态离子所占比例也越高.当激光强度为1×10²⁰ W/cm²时, 尽管该强度高于电离生成C⁺⁶所需要的激光强度阈值, 但该激光脉冲并不能将整个靶电离成C⁺⁶离子, 对此本文进行了详细的分析. 在研究激光脉冲宽度的影响时, 发现激光脉宽越小, 电离速度越快, 但越小的激光脉冲电离获得的高价态离子越少.     

超短脉冲激光烧蚀石墨产生的喷射物的时间分辨发射光谱研究

本文使用不同激光能流(18 J/cm²–115 J/cm²)和脉冲宽度(50 fs–4 ps)的超短脉冲激光在真空中(4×10^-4 Pa)烧蚀高定向热解石墨. 通过测量烧蚀喷射物的时间分辨发射光谱研究喷射物的超快时间演化. 在喷射物发射光谱中, 观察到了C₂基团的天鹅带光谱系统, 416 nm附近C₁₅基团的由电子能级¹Σ_u⁺ 和¹Σ_g⁺之间的振动跃迁产生的光谱峰以及连续谱. 50 fs, 115 J/cm²的脉冲激光烧蚀产生的喷射物的连续谱的强度衰减分为快速下降和慢速下降两个阶段(以20 ns时间延迟为分界). 这表明连续谱是由两种不同的组分贡献的. 快速下降阶段, 连续谱主要由碳等离子体通过韧致辐射产生; 慢速下降阶段, 连续谱主要由烧蚀后期产生的大颗粒碳簇的热辐射贡献. 实验结果还揭示了激光能流的提高, 会明显增加喷射物中碳等离子体和激发态C₂的含量, 但对质量稍大的C₁₅的影响较小; 此外, 50 fs脉冲激光烧蚀产生的连续谱的存在时间会随着激光能流的减小而增大, 这说明低能流更有利于在烧蚀后期产生碳簇. 脉宽主要影响喷射物连续谱的时间演化. 4 ps脉冲激光烧蚀产生的连续谱的整个时间演化过程明显慢于50 fs脉冲产生的连续谱.     

超短超强激光与薄膜靶相互作用中不同价态碳离子的来源

研究了超短超强激光与不同厚度薄膜Al靶相互作用中靶背法线方向碳离子的最初来源. 通过对比分析碰撞电离率和场致电离率所起的作用, 发现C⁴⁺ 及更低价态的碳离子主要由场致电离产生, 而高价态的C⁵⁺和C⁶⁺ 离子主要来自于超热电子与靶表面的碰撞电离. 关键词： 超短超强激光与等离子体相互作用 离子加速 场致电离 碰撞电离     

Extending plasma accelerators: guiding with capillary tubes

In order to extend plasma accelerators, the laser beam has to be guided inside gas or plasma over a distance of the order of the dephasing length, which is typically much larger than the diffraction length z_R of the laser. A capillary tube can be used as a waveguide for high-intensity laser pulses over distances well in excess of z_R. Experimental demonstration of monomode guiding over 100 z_R of 10¹⁶ W/cm² pulses has been obtained in evacuated capillary tubes (45-70-μm inner diameter). A drop of transmission has been observed when the intensity of the amplified spontaneous emission (ASE) is high enough to ionize the capillary tube entrance. Propagation in helium gas-filled (10-40 mbar) capillary tubes has been studied at intensities up to 10¹⁶ W/cm²; a plasma column with on-axis density of the order of 10¹⁷ cm^-3 has been created on a length of the order of 4 cm. The use of a capillary tube for an extended accelerator is discussed for the ease of linear, resonant excitation of plasma waves by laser wakefield     

氢负离子在少周期激光场中解离时的干涉效应

本文利用强场近似理论研究了氢负离子在少周期激光场中的解离过程. 在计算中采用了数值积分和鞍点近似两种计算方法并得到了一致的结果. 更为重要的是, 利用鞍点法对激光脉冲中不同时刻解离产生的电子波包之间的干涉效应进行了研究, 发现光电子动量谱的主要结构是电子波包间的周期间干涉和周期内干涉共同作用的结果, 并分析了周期内和周期间干涉效应对光电子能量谱的影响. 最后, 讨论了激光脉宽对周期内和周期间干涉效应的影响. 本文的工作对进一步了解负离子光解离过程中的量子干涉效应和利用光场对其进行调控方面的研究具有意义.     

激光照射中Z薄靶等离子体状态的计算-激光等离子体相互作用的理论模拟(Ⅰ)

本文叙述用一维非平衡辐射流体力学激光打靶程序模拟计算高功率密度(~10¹³W/cm²)激光照射中Z介质薄靶形成的等离子体状态。考虑的物理过程有轫致、光电离、电子碰撞电离及它们的逆过程,Compton散射过程等。Compton散射采用Fokker-Planck近似;电子和离子热传导采用限流扩散近拟;光子方程采用多群限流扩散近似;用平均原子模型计算布居数。激光的吸收主要考虑逆轫致吸收。用功率密度分别为5×10¹³W/cm²和1×10¹⁴W/cm²,波长0.53μm,脉宽450ps的激光从两面和单面打se薄靶,模拟计算结果与国外的实验结果^[1]一致。     

Multiphoton double ionization of barium

The multiphoton double ionization of Ba from ~280 to 700 nm was investigated using laser pulses 5 ns long of peak intensity ~10¹⁰ W/cm². The spectrum consists of a number of strong resonances, which can be assigned to Ba⁺ transitions. Most of the assignments have been verified by pump-probe techniques. Thus, the Ba⁺⁺ observed is due to sequential ionization. The multiphoton ionization probability is highest for λ~500 nm, which matches a series of strong Ba and Ba⁺ transitions leading to double ionization     

Filippov type plasma focus as intense source of hard X-rays(Ex≃50 keV)

This paper evaluates the use of a plasma focus machine (Filippov type) as a pulsed intense source of hard X-rays. It is shown experimentally that discharging a capacitor bank of W=50 kJ in the new arrangement of the discharge parameters, one can deliver into the test cavity (volume of 6*10³ cm³) an average of Φ _x=8*10^-4 J/cm². The delivered energy fluence varies in the range of 2*10^-4 J/cm²⩽Φ_x⩽2.9*10^-3 J/cm², depending on the probe position. The X-ray energy spectra were established by the differential absorption method using thermo-luminescent detectors (time-integrated spectra) or plastic scintillators (time-resolved spectra). The average energy of X-ray photons is 40 keVx^av<50 keV (20 keV⩽E _x⩽170 keV) and remains quasi-constant during the main part of the pulse (~40 ns). The electron energy that can produce such bremsstrahlung radiation is in the range of 95 keV⩽E_e⩽170 keV. However, time-resolved experiments reveal that at each instant of time only one energy of electron beam occurs. The aforementioned radiation characteristics reveal new potentials for the plasma-focus machine for a variety of applications. Some insight into the physics behind production mechanism of quasi-monoenergetic relativistic-electron beams will be concurrently reviewed     

Plasma-based accelerator diagnostics based upon longitudinalinterferometry with ultrashort optical pulses

All-optical ultrafast time-resolved plasma diagnostics of plasma-based accelerators (PBA's) are described, with emphasis on the laser wakefield accelerator (LWFA). Specifically, the diagnostic techniques involve replacing the trailing particle bunch in the LWFA with a trailing photon bunch: a weak ultrashort laser pulse. Since this photon pulse is derived directly from the intense pump pulse, practical difficulties such as synchronization and dephasing are eliminated. The interaction of the photon bunch with the plasma wake is essentially a simple time-domain shift in optical phase, which can produce both “DC” phase shifts and frequency blue/red-shifting of the probe pulse spectrum. These phase/frequency shifts are recorded in frequency domain interferograms, which are formally equivalent to time-domain holograms. Experimental results of longitudinal plasma density profiling are presented in which plasma density oscillations (Langmuir waves) in the wake of an intense (I_peak~3×10 ¹⁷ W/cm²) laser pulse (~100 fs) were measured with ultrafast time resolution. Phase shifts consistent with large amplitude (~80%) density oscillations at the electron plasma frequency were observed in a fully tunnel-ionized He plasma, corresponding to longitudinal electric fields of ~10 GV/m. Strong radial ponderomotive forces enhance the density oscillations. Finally, proposed single-shot schemes for simultaneous transverse and longitudinal profiling are discussed     

超强圆偏振激光直接加速产生超高能量电子束

研究表明, 峰值强度为10²²–10²⁵ W/cm²量级的圆偏振激光脉冲的有质动力场可以直接加速并产生GeV–TeV的单能电子束, 其中被加速电子的能量与激光脉冲的峰值强度成线性定标关系. 为了获得更高能量的电子束, 通过对一维解析模型的分析得到: 如果电子束在激光传播的方向上具一个初始能量E₀, 那么这种线性的定标关系可以被打破, 被加速电子束最终的能量可以被放大E₀倍. 这是由于具有一定初始能量的电子束不容易被激光脉冲抛在后面, 进而获得更高的加速距离. 二维粒子模拟结果显示: 当电子束的初始能量E₀为MeV量级时这个方法是有效的, 而当E₀过大时这个方法失效. 这是因为当电子的加速距离远大于激光脉冲的瑞利长度时, 激光强度的衰减使得电子束的加速错过了最佳加速场.     

Coherent and incoherent XUV emission in helium and neon,laser-driven plasmas

The authors present results of measurements of high-order harmonic generation and XUV spontaneous emission in helium and neon plasmas excited by a short pulse laser at intensities between 10¹⁴ and 5×10¹⁷ W/cm². They compare the observed behavior of the harmonics with recent single atom calculations in helium. A wavelength dependence to the efficiency of harmonic generation that has not been previously reported is observed. Line emission from excited state transitions in Ne⁷⁺ in a short pulse laser-driven plasma is also observed. In particular, strong emission and a rapid recombination rate for the 9.8-nm (3d-2p) transition that is a possible candidate for a recombination-pumped X-ray laser is shown     

Absolute spectral distribution of soft X-ray emission from laserproduced gold plasma

Quantitative measurement of spectral distribution of soft X-ray emission from laser produced plasmas and estimation of X-ray conversion efficiency are reported. The X-ray emission from planar gold target irradiated by an Nd:glass laser was recorded using a high resolution transmission grating spectrograph. Spectral distribution of X-ray intensity was derived using calibrated film data and a deconvolution procedure to account for contribution of higher diffraction orders. Results of conversion efficiency per unit solid angle, at a laser intensity of ~4×10¹² W/cm² (λ_L = 1.054 μm), for 10< λ <80 Å and in the water window spectral region (23< λ< 44 Å) are presented. A three-fold increase in conversion efficiency was observed for second harmonic laser irradiation (λ_L = 0.527 μm) at an intensity of 8×10¹² W/cm²     

Multiple recollisions in nonsequential double ionization below the recollision-ionization threshold

By using the three-dimensional classical ensemble model, the recollision dynamics in nonsequential double ionization (NSDI) of Ar by 780-nm laser pulses at (6-1.2)×10¹⁴ W/cm² was extensively studied. We revealed the picture of multiple-recollision in the double ionization events at the laser intensity region below the recollision-ionization threshold. Via tracing the NSDI trajectories, it was found that the contribution of these multiple-recollision events increases as the laser intensity decreases. In this low intensity region, many multiple-recollision induced NSDI trajectories occur through the doubly excited states. The decay speed of the doubly excited state decreases with the decreasing laser intensity.     

Photo-ionized lithium source for plasma accelerator applications

A photo-ionized lithium source is developed for plasma acceleration applications. A homogeneous column of lithium neutral vapor with a density of 2×10^15-3 is confined by helium gas in a heat-pipe oven. A UV laser pulse ionizes the vapor. In this device, the length of the neutral vapor and plasma column is 25 cm. The plasma density was measured by laser interferometry in the visible on the lithium neutrals and by CO₂ laser interferometry on the plasma electrons. The maximum measured plasma density was 2.9×10 ¹⁴ cm^-3, limited by the available UV fluence (≈83 mJ/cm²), corresponding to a 15% ionization fraction. After ionization, the plasma density decreases by a factor of two in about 12 μs. These results show that such a plasma source is scaleable to lengths of the order of 1 m and should satisfy all the requirements for demonstrating the acceleration of electrons by 1 GeV in a 1-GeV/m amplitude plasma wake     

Ultrafast structural dynamics using time-resolved x-ray diffraction driven by relativistic laser pulses

Based on a femtosecond laser plasma-induced hard x-ray source with a high laser pulse energy( 100 mJ) at 10 Hz repetition rate,we present a time-resolved x-ray diffraction system on an ultrafast time scale.The laser intensity is at relativistic regime(2 × 10~(19) W/cm~2),which is essential for effectively generating K_α source in high-Z metal material.The produced copper K_α radiation yield reaches to 2.5 × 10~8 photons/sr/shot.The multilayer mirrors are optimized for monochromatizating and two-dimensional beam shaping of K_α emission.Our experiment exhibits its ability of monitoring the transient structural changes in a thin film SrCoO_(2.5) crystal.It is demonstrated that this facility is a powerful tool to perform dynamic studies on samples and adaptable to the specific needs for different particular applications with high flexibility.     

Measurements and interpretation of the absorption of 0.35 μm laser radiation on planar targets

We report on experimental plasma absorption of 0.35 μm radiation incident on plane targets. Absorption fractions between 50 and 98% were found for UV pulses of 90 and 450 ps duration on planar CH, nickel, and gold targets for intensities between 10¹³ and 3 × 10¹⁵ W/cm². The results are in agreement with computer calculations using inverse bremsstrahlung absorption and a thermal electron heat flux limiter between 0.03 and 0.06     

Spectral broadening induced by intense ultra-short pulse in 4H–SiC crystals

We report the observation of spectral broadening induced by 200 femtosecond laser pulses with the repetition rate of 1 kHz at the wavelength of 532 nm in semi-insulating 4H–SiC single crystals.It is demonstrated that the full width at half maximum of output spectrum increases linearly with the light propagation length and the peak power density,reaching a maximum 870 cm~(-1)on a crystal of 19 mm long under an incident laser with a peak power density of 60.1 GW/cm~2.Such spectral broadening can be well explained by the self-phase modulation model which correlates time-dependent phase change of pulses to intensity-dependent refractive index.The nonlinear refractive index n_2 is estimated to be1.88×10~(-15)cm~2/W.The intensity-dependent refractive index is probably due to both the nonlinear optical polarizability of the bound electrons and the increase of free electrons induced by the two-photon absorption process.Super continuum spectra could arise as crystals are long enough to induce the self-focusing effect.The results show that SiC crystals may find applications in spectral broadening of high power lasers.     

Further Acceleration of MeV Electrons by a Relativistic Laser Pulse

With the development of photocathode rf electron gun, electrons with high-brightness and mono-energy can be obtained easily. By numerically solving the relativistic equations of motion of an electron generated from this facility in laser fields modelled by a circular polarized Gaussian laser pulse, we find the electron can obtain high energy gain from the laser pulse. The corresponding acceleration distance for this electron driven by the ascending part of the laser pulse is much longer than the Rayleigh length, and the light amplitude experienced on the electron is very weak when the laser pulse overtakes the electron. The electron is accelerated effectively and the deceleration can be neglected. For intensities around 10¹⁹ W•μm²/cm², an electron's energy gain near 0.1 GeV can be realized when its initial energy is 4.5 MeV, and the final velocity of the energetic electron is parallel with the propagation axis. The energy gain can be up to 1 GeV if the intensity is about 10²¹ W•μm²/cm². The final energy gain of the electron as a function of its initial conditions and the parameters of the laser beam has also been discussed.     

激光诱导AlO自由基B2∑+–X2∑+跃迁光谱研究

基于激光诱导击穿光谱技术, 利用Nd:YAG脉冲激光激发Al₂O₃ (含量为99%)陶瓷片产生等离子体, 获得了AlO自由基B²∑⁺–X²∑⁺跃迁的33条发射谱线. 就AlO自由基光谱的时间演化规律和激光能量对谱线的影响规律进行了研究与分析. 结果表明, AlO自由基光谱出现在Al原子和Al离子光谱之后, 且持续时间较长. 当激光的脉冲能量由10 mJ起不断增加时, AlO自由基光谱强度逐渐减小, 且最大值出现时间随激光能量的增加而后移. 在此基础上, 进行了陶瓷等离子体在空气和氩气环境下的对比试验, 发现从Al₂O₃陶瓷片中激发所产生的AlO自由基必须有空气中O₂参与反应. 关键词： 激光诱导击穿光谱 AlO自由基 B²∑⁺–X²∑⁺跃迁光谱')" href="#">B²∑⁺–X²∑⁺跃迁光谱     

Spectral distribution of X-Ray yield of the M-shell emission fromlaser produced gold plasma

Experimental measurements of the spectral distribution of keV X-ray energy conversion of the M-shell emission from gold plasma produced by a 4 GW, 5 nS Nd:glass laser are presented. At a laser intensity of 2×10¹³ W/cm², the overall X-ray yield for 2.0 ⩽hv⩽3.6 keV is determined to be 0.1% of the laser energy. The effect of the keV X-ray spectral distribution on radiation preheat is discussed