Annealing studies on the absorption spectrum of 41K-atoms trapped in an argon matrix

Argon crystals were doped with 0.2 ppm of ⁴¹K through the nuclear reaction ⁴⁰Ar (n, β^-) ⁴¹K. The absorption spectrum from 300 nm to 800 nm was measured as a function of the annealing temperature. Absorption ← 4²s_{$\text{1}\text{2}$} transition of the free atom could be bands corresponding to the 4²p_{$\text{1}\text{2}$}, _{$\text{3}\text{2}$} ← 4²s_{$\text{1}\text{2}$} and 5²p_{$\text{1}\text{2}$}, _{$\text{3}\text{2}$} ← 4²s_{$\text{1}\text{2}$} transition of the free atom could be observed. The absorption bands depend strongly on the annealing temperature. An increase in the annealing temperature results in a blue shift of the absorption bands.     

Particle-hole states in 42K studied by the 44Ca(d, α)42K reaction

The ⁴⁴Ca(d, α)⁴²K reaction was studied at a bombarding energy of 11 MeV using a broadrange magnetic spectrograph and solid-state detectors. About thirty energy levels were identified in ⁴²K, up to an excitation energy of 3.5 MeV. Excitation functions corresponding to some of the low-lying energy states of ⁴²K were measured in the incident energy range from 10.4 to 11.6 MeV. Angular distributions of the α-particle groups corresponding to the excitation of about twenty energy levels in ⁴²K have been measured. DWBA calculations were performed and L-values for most of the above transitions were deduced. The results were compared with previous information and possible spin and configuration assignments are proposed for some of the states. Centroids of states interpreted as belonging to the (1d_{$\text{3}\text{2}$}^?1)_p (1f_{$\text{7}\text{2}$}³)_n, (2s_{$\text{1}\text{2}$}^?1)_p (1f_{$\text{7}\text{2}$}³)_n and the (1d_{$\text{3}\text{2}$}^?1)_P (1d_{$\text{3}\text{2}$}^?1 1f_{$\text{7}\text{2}$}⁴)_n configurations were found to be in good agreement with calculations based on the weak-coupling model.     

KMS condition in a Schrödinger picture of the dynamics

Given the C¹-algebra $\text{A}$ of observables, the KMS condition is formulated in terms of the time evolution α¹_t of a set $\text{S}$₀ ? $\text{S}$($\text{A}$) of “physical” states subject to certain natural conditions. α¹_t need not be defined by an automorphism group of $\text{A}$. It is shown that, for a KMS state ω, α¹_t induces a 1-automorphism α^ω_t of the von Neumann algebra π_ω($\text{A}$)″ generated by the representation π_ω belonging to ω.     

Preferential excitation transfer in Cs1(6D32)- Cs(6S12) collisions

A cw dye laser beam, tuned near the Cs 8761 Å resonance (Cs¹(6P_{$\text{1}\text{2}$}) → Cs¹(6D_{$\text{3}\text{2}$}) transition) is focused into a Cs vapor. At a Cs density higher than 5 × 10¹⁵ cm^-3, we observe a greater 6P_{$\text{1}\text{2}$} population when the laser is on resonance than when it is off resonance. However, at a lower Cs density, the reverse is observed. This phenomenon is explained as due to the preferential excitation transfer process: Cs¹(6D_{$\text{3}\text{2}$}) + Cs(6S_{$\text{1}\text{2}$}) → Cs¹(6P) + Cs¹(6P), and the corresponding cross secti on is estimated to be (1.5^+1.5_-0.7) × 10^-14 cm² by fitting the experimental results to an approximate rate-equation analysis.     

Collisional quenching of HgBr(B2∑+12)

Rate coefficients for the quenching of HgBr(B²∑⁺_{$\text{1}\text{2}$}) by HgBr₂, H₂, CO₂, CO, O₂, N₂, Xe, and Br₂ are reported. HgBr(B²∑⁺_{$\text{1}\text{2}$}) is formed by the photolysis of HgBr₂ with the output from an ArF laser. The rate coefficients are determined by monitoring the time resolved B²∑⁺_{$\text{1}\text{2}$} → X²∑⁺_{$\text{1}\text{2}$} emission as quenching species are added. Radiative lifetimes at particular emission frequencies are also reported, and quenching mechanisms are discussed.     

Intrinsic states,high-spin rotational bands and rotation alignment in 177Os and 179Os

Low-lying intrinsic states and their associated rotational bands have been identified in ¹⁷⁷Os and ¹⁷⁹Os. They are the mixed i_{$\text{13}\text{2}$} neutron states and the $\text{1}\text{2}$^?[521] states in ¹⁷⁷Os and ¹⁷⁹Os, as well as the $\text{5}\text{2}$^?[512] state in ¹⁷⁷Os and the $\text{7}\text{2}$^?[514] state in ¹⁷⁹Os. The $\text{1}\text{2}$^? sta is assumed to be the ground state, the other intrinsic states giving rise to isomers. The in-band decay properties of the $\text{7}\text{2}$^?[514] band, and the i_{$\text{13}\text{2}$} bands show the effect of mixing. In the rotational bands in ¹⁷⁷Os a low frequency backbending anomaly is observed but no anomaly is observed in the i_{$\text{13}\text{2}$}. band. In ¹⁷⁹Os the i_{$\text{13}\text{2}$} band does backbend but at a higher frequency than in the yrast bands of the even neighbours. The systematics of the backbending frequencies, and the effects of blocking, are discussed. The rotation aligned angular momentum is deduced, and a comparison made between the i_{$\text{13}\text{2}$} bands and the s-bands in the even neighbours. The results broadly support the identification of the s-bands with the aligned (i_{$\text{13}\text{2}$})² configuration.     

Neutron-hole strengths and isobaric analog states in 95Zr

The ⁹⁶Zr(τ, α)⁹⁵Zr reaction at 39 MeV incident energy was used to populate both the low-lying and highly excited (up to an excitation energy of 18 MeV) analog states in ⁹⁵Zr and some low-lying levels in other Zr isotopes. The main components of the 2d_{$\text{5}\text{2}$}. and 1g_{$\text{9}\text{2}$}. hole strengths and the analogs of the 2p_{$\text{1}\text{2}$}., 2p_{$\text{3}\text{2}$}. and 1f_{$\text{3}\text{2}$}. proton hole states in ⁹⁵Y have been observed in this work. Angular distributions of transitions to 27 levels in ⁹⁵Zr have been extracted and analysed with DWBA calculations to yield spectroscopic factors. Between the excitation energies of 1 and 3 MeV in ⁹⁵Zr a number of levels with l = 2, 4 and 5 angular distributions have been identified. These are associated with the 2d_{$\text{3}\text{2}$}, 1g_{$\text{7}\text{2}$} and 1h_{$\text{11}\text{2}$} components already observed in the previous study of the ⁹⁴Zr(d, p) and (α, τ) reactions. The total strength and center of gravity for levels assigned to the (1g_{$\text{9}\text{2}$})^?1 configurations in ⁹⁵Zr are presented and compared to the results obtained from the studies of neutron pick-up reaction on ⁹¹Zr and ⁹⁸Mo. For the isobaric analog states observed between the excitation energies of 15 and 17 MeV, total widths, Coulomb displacement energies and spectroscopic factors are also determined from this experiment and the results compared with the properties of the low-lying proton hole states in the ⁹⁵Y parent nucleus.     

Resonant absorption in LiNdP4O12 lasers

The resonant loss in LiNdP₄O₁₂ (LNP) lasers has been investigated. The effective resonant loss coefficient for the 1.047(7) μm laser emission was measured to be 0.042 cm^-1. This value can be explained by resonant absorption due to the ⁴I_{1$\text{1}\text{2}$}→⁴F_{$\text{3}\text{2}$} transition including the reabsorption effect of the fluorescence resulting from the ⁴I_{$\text{9}\text{2}$}→⁴F_{$\text{3}\text{2}$} transition.     

Collisional enhancement of the I(52P12) emission at 1.3μm by parent molecules CF3I,C2F5I,i-C3F7I and n-C3F7I

The magnetic dipole transition I(5²P_{$\text{1}\text{2}$}-5²P_{$\text{3}\text{2}$}) at 1.3152 μm is shown to be enhanced by collisions of the metastable iodine atoms with the parent RI molecules CF₃I, C₂F₅I, i-C₃F₇I and n-C₃F₇I. The enhancing mechanism is exciplex emission of the RI·I(5²P_{$\text{1}\text{2}$}) molecule at 1.3 μm, with different rates for each iodide. The influence of this effect on the measurement of the quantum yields to I(5²P_{$\text{1}\text{2}$}) and of the respective reaction rates by infrared fluorescence is discussed.     

A hyperfine filter for the 3776 Å thallium resonance line

A magnetic hyperfine filter for the resonance line ²P_{$\text{1}\text{2}$} → ²S_{$\text{1}\text{2}$} of thallium is described. This line is a hyperfine triplet and this filter transmits only the 0→1 component connecting the lower sublevel of the ²P_{$\text{1}\text{2}$} ground state. This filter may thus be used for obtaining a population inversion in the ground state of Tl.     

On the cyclotron resonance width of an electron impurity system in two dimensions

Using the proper connected diagram expansion which incorporates the quasi-particle effect naturally we calculated the cyclotron resonance width γ in the extreme quantum limit.(a) γ ∝n

$\text{1}\text{2}$

_s B

$\text{1}\text{2}$

for a short range interaction, and (b) γ = π

$\text{1}\text{2}$

ze² κ^-1 <?crossed h.c.h;^-1 n

$\text{1}\text{2}$

_s for Coulomb interaction, are obtained. The field (B) and concentration (n_s)-dependence is in satisfactory agreement with experimental data. The variation γ = (γ²₁ + γ²₂ + …)

$\text{1}\text{2}$

of Matthiessen's rule γ = γ₁ + γ₂ + …, holds when there exist scattering centers of different kinds in the system.     

Pionic and radiative decay widths of charmed hadrons in a badly broken SU(4) symmetry

The width of ψ(4.414) is surprisingly small for a c$\text{c}$ state far above the charm threshold, Γ_exp ≈ 33 MeV. This fact can be qualitatively understood if one makes the conservative assignment 4 ³S₁. The nodes of the wave function reflect as zero's of the decay amplitude in the momentum of the decay products, and are responsible for the suppression of the couplings to the ground state charmed mesons, Γ(ψ(4.414)→D$\text{D}$+ D$\text{D}$¹ + $\text{D}$D¹ + D¹$\text{D}$¹ + F$\text{F}$ + F$\text{F}$¹ + $\text{F}$F¹ + F¹$\text{F}$¹) ≈ 15 MeV. All the modes are suppressed by factors of the order of 10³ with respect to the k³ spin counting prediction. The dominant modes are predicted to be D¹$\text{D}$¹, F$\text{F}$¹ + $\text{F}$F¹ and D$\text{D}$. Moreover, we show that the contributions from P-wave charmed mesons are reasonably expected to be suppressed either by phase space or by the nodes if their masses lie within certain range. We emphasize however that the smallness of the photon coupling remains to be understood.     

Excitation processes leading to ruby emission

We excited the ²T₁-levels in ruby by tunable laser light, pumped bya pulsed YAG:Nd³⁺ laser, and observed the low temperature emissions from the 2$\text{A}$ and $\text{E}$ sublevels of ²E in the mild bottlenecking regime. The R₂-line decay time was about five-fold longer and the ratio of intensities R₂/R₁ higher (by up to a factor 10) than after pumping into ⁴T₂. It is suggested that when ⁴T₂ is pumped the relaxation is nonadiabatic, so that transitions between the sublevels occur while the ²E state relaxes to its normal (trigonal) configuration. The time-development of the relaxing state is studied. It is shown that its coherence between the 2$\text{A}$ and $\text{E}$ sublevels leads to a narrowing of the spectral width in transition between the sublevels.     

Relaxation of the 4G92 state of Nd3+ in LaCl3 and Nd3+ in La(Cl99.6Br0.4)3

The decay of the ⁴G_{$\text{9}\text{2}$} state of Nd³⁺ in LaCl₃ and La(Cl_99.6 Br_0.4)₃ was measured after pulsed laser excitation as a function of temperature. The decay rate is shown to depend besides the radiative transition on single-phonon relaxation between the states ⁴G_{$\text{9}\text{2}$} ($\text{μ =}\text{1}\text{2}$) and ⁴G_{$\text{9}\text{2}$} ($\text{μ =}\text{3}\text{2}$) and on multiphonon orbit-lattice relaxation from ⁴G_{$\text{9}\text{2}$} to ²G_{$\text{9}\text{2}$}. Partial substitution of Cl by Br only alters the radiative lifetime.     

Determination of some atomic-state densities in an Xe-Br2 mixture

The atomic-state densities of the 6s[1 $\text{1}\text{2}$]⁰ metastable Xe energy level and of the 5s⁴P_{$\text{1}\text{2}$}, 5s⁴P_{$\text{3}\text{2}$} and 5s⁴P_{$\text{5}\text{2}$}Br energy levels in an Xe-Br₂ mixture have been determined as a function of current strength.     

The radial distribution of the 1f72 neutron in 41Ca from the 40Ca(13C, 12C)41Ca reaction

The reaction ⁴⁰Ca(¹³C, ¹²C)⁴¹Ca leading to the ground and low-lying $\text{3}\text{2}$^? levels has been studied at bombarding energies of 18.5 and 19.0 MeV, close to the Coulomb barrier. The cross sections have been analysed using the DWBA with previously measured calibrations to obtain the rms radii of 1f_{$\text{7}\text{2}$} and 2p_{$\text{3}\text{2}$} orbits in the ⁴¹Ca levels. The rms radius of the 1f_{$\text{7}\text{2}$} point neutron orbit in the ground state relative to the ⁴⁰Ca core was determined to be 3.89 ± 0.12 fm. This is compared with various theoretical predictions based on Hartree-Fock theory. The 1f_{$\text{7}\text{2}$} orbit radius gives the point neutron excess size to a good approximation for comparison with the value of 3.45 fm deduced from Coulomb energy differences. The consistency of the results with ⁴⁰Ca(t, d)⁴¹Ca experiments using a (t/d), zero-range normalization of 3.26 × 10⁴ MeV² · fm³ is demonstrated, and trends in neutron size parameters through the Ca isotopes are discussed.     

Laser probing of ions confined in a cylindrical radiofrequency trap

We measure the lifetime of the 5 ²D_{$\text{5}\text{2}$} metastable level of Ba⁺ ions confined in a cylindrical radiofrequency trap as well as some parameters which characterize the confining properties of the trap. This is accomplished by studying the ion response to a short pulsed optical excitation saturating the 6 ²S_{$\text{1}\text{2}$}–6 ²P_{$\text{3}\text{2}$} transition.The measured lifetime of the 5 ²D_{$\text{5}\text{2}$} metastable level is 47 ± 16 s. The storage voltages for which the ion number shows a maximum are experimentally investigated. Their change when a light buffer gas is added is observed. The effect of this gas on the storage time is also specified.     

Isomers in the N = 83 nucleus 149Dy

Energy levels in the N = 83 nucleus ¹⁴⁹Dy were studied by the reaction ¹⁵²Gd(α, 7n) at 106 MeV bombarding energy using in-beam γ-ray spectroscopy methods. The measurements identified three isomers in this nucleus, at 1073 keV (13 ± 3 ns), at 2700±150keV (5 μs < T_{$\text{1}\text{2}$} < 0.5 s), and above 3.5 MeV (50 ± 15 ns). The low-lying isomer is interpreted as i_{$\text{13}\text{2}$}. The configuration $\text{27}\text{2}$^?(πh_{$\text{11}\text{2}$}²)₁₀₊ ×vf_{$\text{7}\text{2}$} is suggested for the state at 2.7 MeV.     

Energies of the n2S12 and n2D32,52 states of Cs

Using the technique of Doppler-free two-photon spectroscopy the energies of the n²S_{$\text{1}\text{2}$} (12 ? n ? 35) and n²D_{$\text{3}\text{2}$,$\text{5}\text{2}$} (11 ? n ? 48) states of CsI have been measured with a thermionic detector. The absorption spectrum of molecular iodine was used as a reference giving us a total estimated accuracy of about 2 × 10^-7. Taking also into account the energies of the 7–11 ²S_{$\text{1}\text{2}$} and 5 and 6 ²D_{$\text{3}\text{2}$,$\text{5}\text{2}$} states measured by other authors and using an extended Ritz-formula we found the ionization limit to be E_i = 31406.468 ± 0.006 cm^-1.     

The photoelectron angular distributions of HBr and HI AT hν = 21.2 eV

Photoelectron angular distributions for the ²Π_{$\text{3}\text{2}$, $\text{1}\text{2}$}(pπ)^?1 and ²Σ_{$\text{1}\text{2}$}⁺(pσ)^?1 ionic states of HBr and HI have been measured at a photon energy of 21.2 eV. The asymmetry parameters for the highly localized pπ orbitals closely follow those of the “lone-pair” orbitals of the related CH₃X molecules and the outer np atomic orbitals of the corresponding united atoms. Furthermore, the asymmetry parameters for the ²Π_{$\text{3}\text{2}$} and ²Π_{$\text{1}\text{2}$} states were found to be equal within experimental uncertainty, despite the large spin—orbit splittings of these heavy molecules. The asymmetry parameters for the ²Σ⁺(pσ)^?1 ionic states are significantly smaller than for the ²Π(pπ)^?1 states, in contrast to recent predictions based on angular momentum transfer theory.