A study of some resonances in the 54Fe(p, γ)55Co reaction

Excitation functions for the ⁵⁴Fe(p, γ)⁵⁵Co reaction have been recorded in the energy region E_p = 1100–1760 keV. The decay schemes and branching ratios of ten resonances have been investigated. Angular distributions of primary γ-rays have been measured for three resonances to establish resonance spins. Resonance strengths for six resonances and gamma widths for three resonances have been determined. The isobaric analogues of the ground ($\text{J}{}^{\mathrm{\pi }}\text{=}\text{7}\text{2}{}^{\mathrm{?}}\text{)}\text{and}\text{1919}\text{keV}$$\text{J}{}^{\mathrm{\pi }}\text{=}\text{3}\text{2}$^?) states of the parent nucleus ⁵⁵Fe have been identified at 4722 and 6712 keV respectively in ⁵⁵Co. The Coulomb displacement energies of the observed analogue pairs (0–4722 keV) and (1919–6712 keV) have been obtained. The strengths of the possible analogue-antianalogue transitions for the proton capture state at E_p = 1679 keV have also been determined.     

Microscopic calculation of cross sections for the reactions 12C(p, 2p) and 16O(p, 2p): U. Wille and R. Lipperheide Nucl. Phys. A189 (1972) 113

Isomeric states of ⁶⁹Se were produced via the heavy-ion compound-nucleus process and from the positon decay of ⁶⁹Br, the former producing a high-spin state and the latter preferentially populating a low-spin state. Ge(Li) detectors as well as scintillation counting showed that the high-spin state decays with T_{$\text{1}\text{2}$} = 14.0 ± 1.0 min to levels in ⁶⁹As, giving rise to γ-rays of 116, 166 and 282 keV. The low-spin state decays predominantly to a state giving rise to a 145 keV γ-ray with T_{$\text{1}\text{2}$} = 1.8 ± 0.2 min. The beta end-point energy of both isomers is 5.2 ± 0.2 MeV. It is deduced that the high-spin state, assigned J^π = $\text{9}\text{2}$⁺, is the ground state; the isomeric state had J^π = $\text{3}\text{2}$^?. The angular momentum inversion as compared to neutron-excess Se isotopes is attributed to Coriolis coupling to a deformed core as described by Malik and Scholz.     

Spectroscopic investigations of the decay 223Ra → 219Rn

Internal conversion electron spectra of the transitions 4.4 keV, 10.0 keV, 14.4 keV, and 324.1 keV in the decay ²²³Ra → ²¹⁹Rn were measured. E2/M1 mixing ratios of these γ-transitions were deduced from conversion electron intensity ratios: δ² = 3.8(4) · 10^?3, 2.35(18) · 10^?3, 12.85(36) · 10^?3, 0.23(3). The half-lives of the 4.4 keV and 14.4 keV levels were determined as $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 15.4(1.3)}$ nsec and 0.875(30) nsec. Reduced transition probabilities were calculated and compared to the Weisskopf estimates. αγ angular correlation measurements of the transitions 269.6 keV, 324.1 keV, and 338.6 keV and an αγ linear polarization measurement of the 269.6 keV transition were performed for spin determination. We assign $\text{I =}\text{7}\text{2}$ to the ²¹⁹Rn ground state and $\text{I =}\text{5}\text{2}$ or $\text{9}\text{2}$ to the 269.6 keV state. All other low excitations including the 338.6 keV level have spins $\text{I =}\text{5}\text{2}$, $\text{7}\text{2}$, or $\text{9}\text{2}$. The spins of the states 158.7 keV and 14.4 keV are equal. The ²²³Ra ground state spin is $\text{I =}\text{7}\text{2}$ or $\text{9}\text{2}$. The possibility of an interpretation of the transitional nucleus ²¹⁹Rn in the frame of the collective model is discussed.     

Electromagnetic properties of levels in 55Mn

Excited levels of ⁵⁵Mn were produced by the reaction ⁵²Cr(α, p) at 10.5 and 11.1 MeV beam energy. A series of γ-ray measurements was made, all in coincidence with protons detected near 180°. A Ge(Li) γ-ray detector was used at 4 angles, and extensive angular-correlation measurements were made with an array of NaI(Tl) detectors. Excitation energies of 25 levels up to 3161 keV were determined, including a new level at 2215 keV. Only the level at 2285 keV and the $\text{1}\text{2}{}^{\mathrm{?}}$ state near 1290 keV were not observed in this range. From Doppler-shift attenuations, the mean lifetimes of 14 levels up to 2565 keV were deduced. Branching ratios and multipole mixing ratios were obtained for most of these levels. The following spin assignments were determined: 1530 keV, $\text{J =}\text{3}\text{2}$; 1885 keV, $\text{J =}\text{7}\text{2}$ or $\text{5}\text{2}$; 2565 keV, $\text{J =}\text{3}\text{2}$. Reduced transition probabilities, B (M1) and B (E2), of many transitions were calculated from these experimental results and are compared with the available theoretical values.     

The half-lives of the first and second excited states in 66Ga

The half-lives of the first and second excited states at 43.9 and 66.3 keV in ⁶⁶Ga were determined by measuring the time dependence of the 43.9 and 22.4 keV γ-transition intensities. The levels in ⁶⁶Ga were populated by the ⁶⁶Za(p, n)⁶⁶Ga and ⁶³Cu(α, n)⁶⁶Ga reactions. The results are T_{$\text{1}\text{2}$}(43.9 keV) = 16(4) ns and T_{$\text{1}\text{2}$}(66.3 keV) = 23(2) ns. A g-factor measurement reported in the literature is reanalysed.     

Nuclear spectroscopic studies of the 23.7 h 248Bk

Main features of the decay of the 23.7 h ²⁴⁸Bk have been determined by spectroscopy with scintillation and semiconductor detectors. The results are as follows: half-life 23.7 ± 0.2 h; branching is (30 ± 5)% to ²⁴⁸Cm (≈ 23% EC decay to 0⁺ ground state and ≈ 7% to first 2⁺ state) and (70 ± 5)%β^? decay to ²⁴⁸Cf(5 % to 592 keV K^π = 2^? state and (65 ± 5)% to the ground-state band). The β^? decay energy, Q_β^?, has been measured to be 860 ± 20 keV, and the electron capture decay energy, Q_EC, has been derived from closed cycle to be 705 ± 25 keV. The deduced logft values of β^? and EC transitions restrict the spin of the ²⁴⁸Bk ground state to 1, with configuration assignment $\text{{}\text{n}\text{[734]}\text{9}\text{2}{}^{\mathrm{?}}$; $\text{p}\text{[633]}\text{7}\text{2}{}^{\mathrm{+}}$. It has also been deduced that the long lived isomer lies 65 ± 40 keV abovethe 23.7h ²⁴⁸Bk ground state.     

Spins and lifetimes of levels in 55Mn

The study of excited ⁵⁵Mn levels with the ⁵²Cr(α, pγ) reaction was extended to levels up to 3161 keV. With a Ge(Li) detector, DSA measurements in gold-backed targets were made, as well as angular correlations; both of these experiments were done in coincidence with protons detected near 180°. A multiple-detector NaI(Tl) array was also used in the same reaction geometry for better γ-ray detection efficiency. Mean lifetimes of 12 levels from 2727 to 3161 keV are reported. Spins and sometimes parities of the following levels were deduced from the angular-correlation analyses and lifetime results: 1885 keV, $\text{7}\text{2}$^?; 2199 keV, $\text{7}\text{2}$(^?); 2311 keV, ($\text{13}\text{2}$); 2366keV, $\text{5}\text{2}$^?; 2727 keV, $\text{7}\text{2}$; 2823 keV, $\text{9}\text{2}$. Multipole mixing ratios and M1 and E2 transition rates of the radiations from these and from the 1292 keV level are presented. The similarity of the low-lying level structure and of interlevel transitions in ⁵⁵Mn to those in certain other f_{$\text{7}\text{2}$}³ nuclei is examined.     

Analysis of the properties of excited states in 165Er

An analysis of ¹⁶⁵Tm decay has shown that precision measurements of the γ-ray and internal conversion electron intensities, in combination with angular correlation measurements, provide additional data useful for the determination of the mixing and intensity ratios of γ-transitions with a small energy difference. The spin of the 589.868 keV state is found to be $\text{I}{}^{\mathrm{\pi }}\text{=}\text{1}\text{2}{}^{\mathrm{?}}$. Doublet opposite-parity transitions from states at 1103.495, 920.632 and 745.968 keV to levels near 590 keV with an energy difference ΔE = 108 ± 22 eV are identified.     

Electromagnetic transitions in 51Mn

The nuclear structure of ⁵¹₂₅Mn was studied by γ-ray spectroscopy in the ⁵⁴Fe(p, α)⁵¹ Mn reaction (E_p = 9.0–13.2 MeV) and the ¹⁴N+³⁹K, ¹⁶O+⁴⁰Ca and ¹⁴N+⁴⁰Ca fusion-evaporation reactions (E_beam = 36 MeV). In the ⁵⁴Fe(p, αγ)⁵¹Mn reaction γ-rays were detected in coincidence with α-particles emitted near 180°; mean lifetimes and γ-ray mixing and branching ratios were deduced from Doppler shift attenuation and α-γ angular correlation measurements, respectively. Definite spin assignments are: 237 and 2416 keV, $\text{J}{}^{\mathrm{\pi }}\text{=}\text{7}\text{2}{}^{\mathrm{?}}$; 1140 keV, $\text{9}\text{2}$^?; 1488 keV, $\text{11}\text{2}$^?; 1825 and 2140 keV, $\text{3}\text{2}$^?. The results for other states below 3 MeV are consistent with the existence of rotational bands (/kh²/2/OI/t~ 95 keV) built on the ($\text{3}\text{2}$⁺) 1817 keV and $\text{1}\text{2}$⁺ 2276 keV hole states. The various measurements together with an earlier value for the lifetime of the first-excited state determine unambiguously the B(M1) and B(E2) values for all of the decay branches of the $\text{7}\text{2}$^?, $\text{9}\text{2}$^? and $\text{11}\text{2}$^? lowest three excited states. From the γ-singles and γ-γ coincidence observations with fusion-evaporation reactions, the yrast cascade proceeds through these three states and higher states at 2957, 3250,3680 and 4139 keV which are suggested to have $\text{J}{}^{\mathrm{\pi }}\text{=}\text{13}\text{2}{}^{\mathrm{?}}$, $\text{15}\text{2}$^?,$\text{15}\text{2}$^? and $\text{19}\text{2}$^?, respectively. The various experimental results for the $\text{5}\text{2}$^? → ($\text{19}\text{2}$^?) yrast states are in good overall agreement with shell-model calculations in the (f_{$\text{7}\text{2}$}¹ space.     

Coulomb excitation of 85Rb and 87Rb

Energy levels of ⁸⁵Rb and ⁸⁷Rb have been studied via de-excitation γ-rays following Coulomb excitation with ³⁵Cl ions. In addition to the known negative-parity states at 151.2 keV and 868.2 keV in ⁸⁵Rb, two states at 281.0 keV and 731.8 keV have been found with fourγ-ray transitions of 129.8, 281.0, 450.8 and 731.8 keV. Only one Coulomb excited state at 402.6 keV in ⁸⁷Rb has been observed. The B(E2↑) values (in units e² · b²) have been determined as 0.0035±0.0004 (151.2 keV), 0.0016±0.0002 (281.0 keV), 0.0101 ±0.0010 (731.8 keV), and 0.036±0.004 (868.2 keV) for the states in ⁸⁵Rb, and as 0.0054±0.0006 (402.6 keV) for the state in ⁸⁷Rb. The mean lifetimes of the 731.8 keV and 868.2 keV states have been measured by the Doppler shift attenuation method as 6.4±0.7 psec and 4.2±0.5 psec respectively. Angular distribution measurements allow unique spin and parity assignments of $\text{1}\text{2}{}^{\mathrm{?}}$ and $\text{3}\text{2}{}^{\mathrm{?}}$ to the 281.0 keV and 731.8 keV levels respectively. The spin and parity of the 868.2 keV level has been restricted to $\text{5}\text{2}{}^{\mathrm{?}}$ or $\text{7}\text{2}{}^{\mathrm{?}}$.     

Spins of the levels and multipole mixing ratios of transitions in 125Sb determined from γ-γ directional correlation and polarization-directional correlation measurements

In order to resolve several discrepancies in spin assignments to levels in ¹²⁵Sb, directional correlations and polarization-directional correlations have been measured for several γ-γ cascades in ¹²⁵Sb populated from the decay of ¹²⁵Sn. Earlier results obtained from using NaI and Ge(Li) and NaI detectors were difficult to interpret due to the complex structure of the decay scheme. To improve the experimental situation, we have used two coaxial Ge(Li) detectors for the angular correlation measurements and a coaxial Ge(Li)-planar Ge(Li) combination for the polarization-directional correlations. Combination of the results of these measurements give unique spin assignments of $\text{11}\text{2}$^?, $\text{11}\text{2}$^?, $\text{9}\text{2}$⁺, $\text{11}\text{2}$⁺ and $\text{9}\text{2}$⁺ to the 1982 keV, 1890 keV, 1420 keV, 1089 keV and 1067 keV levels, respectively. The determined E2/M1 mixing ratios are : δ(470) = 0.010±0.027, δ(1067) = ?0.86±0.18, and δ(916) = ?0.02±0.01.     

Isomers in the N = 83 nucleus 149Dy

Energy levels in the N = 83 nucleus ¹⁴⁹Dy were studied by the reaction ¹⁵²Gd(α, 7n) at 106 MeV bombarding energy using in-beam γ-ray spectroscopy methods. The measurements identified three isomers in this nucleus, at 1073 keV (13 ± 3 ns), at 2700±150keV (5 μs < T_{$\text{1}\text{2}$} < 0.5 s), and above 3.5 MeV (50 ± 15 ns). The low-lying isomer is interpreted as i_{$\text{13}\text{2}$}. The configuration $\text{27}\text{2}$^?(πh_{$\text{11}\text{2}$}²)₁₀₊ ×vf_{$\text{7}\text{2}$} is suggested for the state at 2.7 MeV.     

Level structure of the 89-neutron nucleus 153Gd: (I). Levels and gamma-transitions in 153Gd excited in the decay of 153Tb

Investigations of the properties of ¹⁵³Gd excited states populated in ¹⁵³Tb decay were continued. The following measurements were performed: coincidence spectra e^?γ with L41, K93 + L52, K110, K129 + L87 + L88 and K195 + L152 keV conversion electron lines, angular correlations of high energy γ-cascades going through the 109.7 keV level, delayed e^?γ and e^?e^? coincidence spectra to determine the half-lives of 41.5, 93.3, 109.7, 129.1,183.5, 212.0 and 216.1 keV states, R(135°, ± B) parameters of IPAC for the 102–110 and 83–129 keV cascades using ¹⁵³Tb sources implanted into Fe foil.A decay scheme of ¹⁵³Tb containing 50 excited levels is proposed. Their spins, parities, $\text{log}\text{?t}$ and, for low-lying levels, also the mean half-lives have been determined. An estimation of the g-factors of the 109.7 and 129.1 keV levels has been given. On the basis of half-lives of investigated states absolute values of reduced γ-transition probabilities for these states have been calculated. The structure of the ground state of ¹⁵³Gd is discussed.     

High spin states in 57Co

High spin states of ⁵⁷Co have been studied via prompt γ-ray spectroscopy in the reactions ⁴⁸Ti(¹²C, p2n) and ⁵⁴Fe(α, p) at 26–48 MeV and 12–24 MeV, respectively. The energies and decay modes of these levels were determined from the analysis of γ-ray singles and γ-γ coincidence spectra, excitation functions, angular distributions and correlations. The relevant lifetimes were measured by the Doppler-shift attenuation method. The new levels established in this work are at 4037, 4814 and 5918 keV with the most probable J^π assignment of $\text{15}\text{2}{}^{\mathrm{?}}$, if $\text{17}\text{2}{}^{\mathrm{?}}$ and $\text{19}\text{2}{}^{\mathrm{?}}$, respectively. The previously known level at 2524 keV was assigned to have $\text{J}{}^{\mathrm{\pi }}\text{=}\text{13}\text{2}{}^{\mathrm{?}}$. These together with the known $\text{9}\text{2}{}^{\mathrm{?}}$(1224 keV) and $\text{11}\text{2}{}^{\mathrm{?}}$(1690 keV) levels constitute the yrast states of ⁵⁷Co. The measured lifetimes of the above six levels are (in order of increasing energies) 0.085±0.030, 0.32±0.10, 0.16±0.06, 0.10_?0.07^+0.06, 1.5_?0.5⁴ and 0.17_?0.07^+0.08 ps, respectively. Comparisons with some theoretical calculations are presented.     

The γ-decay of the g92 analogue state in 59Cu

An investigation of the γ-decay of the $\text{1}\text{g}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}$ analogue state in ⁵⁹Cu has been performed using the ⁵⁸Ni(p, γ)⁵⁹Cu reaction. The (p, γ) excitation function has been taken in the range E_p = 3450–3650 keV. The decay schemes of the (p, γ) resonances at E_p = 3483, 3532 and 3547 keV, measured with Ge(Li) detectors, lead to eight new levels in ⁵⁹Cu with excitation energies between 1.8 and 4.7 MeV and to spin assignments of several states. The spins of the first two resonances are found to be ($\text{1}\text{2}$, $\text{3}\text{2}$) and ($\text{5}\text{2}$). The spin of the E_p = 3547 keV resonan is, from angular distributions, uniquely determined to be $\text{J}{}^{\mathrm{\pi }}\text{=}\text{9}\text{2}{}^{\mathrm{+}}$ and this state is found to be the unfragmented analogue state of the $\text{E}{}^1\text{= 3.062}\text{MeV}$, $\text{J}{}^{\mathrm{\pi }}\text{=}\text{9}\text{2}{}^{\mathrm{+}}$ parent state in ⁵⁹Ni. The measured complete decay scheme of this resonance shows that its isovector M1 decay is in disagreement with all existing theoretical predictions.     

Analyzing powers for the (p, α) reactions on 58, 60, 62Ni at Ep = 22 MeV

Measurements of both the analyzing power and cross section were made for the (p, α) reactions on ^58,60,62Ni at an incident energy of 22 MeV. Data were taken for the strongly populated proton-hole states (0f_{$\text{7}\text{2}$}, 1s_{$\text{1}\text{2}$} and 0d_{$\text{3}\text{2}$}) in the residual cobalt isotopes and for 8 weakly populated low-lying states in ⁵⁵Co and ⁵⁹Co. Angular distributions were taken between θ_lab = 10° and 140° for the ground state and θ_lab = 10° and 80° for the excited states. Both the cross sections and analyzing powers exhibit a similar angular distribution for states having the same J^π values except in the transition to the $\text{3}\text{2}$^? state in ⁵⁹Co at 1.099 MeV. Using the observed J-dependence of the analyzing power, the unknown J^π values for the states at 2.982 MeV in ⁵⁵Co and 3.090 MeV in ⁵⁹Co are assigned to be $\text{9}\text{2}$^?. The shapes of the differential cross sections were well reproduced by the zero-range DWBA calculations using a triton-cluster form factor. However, all the measured analyzing powers could not be reproduced within the framework of such a simple DWBA calculation.     

Low lying states of 96Tc

The ⁹⁶Mo(p, n) and ⁹⁶Mo(p, nγ) reactions have been studied for proton energies between 3.8 and 5.5 MeV. Energy levels in ⁹⁶Tc up to 632 keV excitation energy have been determined. Possible spin and parity assignments are given for several levels based on the neutron enhancement and angular distributions observed on and off resonance of the $\text{5}\text{2}{}^{\mathrm{>+}}$ isobaric analog state in ⁹⁷Tc, as well as the observed γ-yields. The first excited state reported at 34 keV was found to be a close doublet only 0.8 keV apart. The observation of this doublet in the (p, n) reaction was used to determine the ground state Q-value Q = ? 3.760±0.010 MeV.     

Das Niveauschema von 47V aus dem γ-zerfall von Analogresonanzen

A high-accuracy investigation of the level scheme of ⁴⁷V has been performed using the ⁴⁶Ti(p, γ)⁴⁷V reaction. The γ-decay schemes of the strong (p, γ) resonances at E_p = 1546, 1549, 1565 and 1572 keV lead to 17 new energy levels in ⁴⁷V with excitation energies between 2.7 and 5.1 MeV. From the (p,γ) angular distributions mixing ratios of the primary γ-transitions and J^π values of the resonances and of many states populated in the γ-decay have been determined. The total width of the E_p = 1549, 1565 and 1572 keV resonances for γ-decay are found to be Γ_γ = 0.12, 0.15 and 0.03 eV, respectively. The Q-value of the ⁴⁶Ti(p,γ)⁴⁷V reaction is found to be 5168.6 keV. The two resonances at E_p = 1549 and 1565 keV, which have $\text{J}{}^{\mathrm{\pi }}\text{=}\text{3}\text{2}{}^{\mathrm{?}}$, are interpreted as fine structure components of the analogue state of the $\text{E}{}^1\text{= 2.545}\text{MeV}\text{J}{}^{\mathrm{\pi }}\text{=}\text{3}\text{2}{}^{\mathrm{?}}$ level in ⁴⁷Ti while the ($\text{7}\text{2}$) resonance at E_p = 1546 keV might correspond to the $\text{E}{}^1\text{= 2.615}\text{MeV}\text{7}\text{2}{}^{\mathrm{?}}$ parent state in ⁴⁷Ti. The analogue-antianalogue M1 transition strength of the split $\text{3}\text{2}{}^{\mathrm{?}}$ analogue state is 0.01 single-particle units and fits well into our systematics of IAS → AIAS transitions in fp-shell nuclei.     

Optical pumping measurement of the hyperfine structure of cadmium ion ground state

The 5²S_{$\text{1}\text{2}$} ground state of Cd⁺ ions has been oriented by Schearer's technique. The hyperfine structure constant for this level has been determined as ¦A¦ = 14700 ± 700 MHz for the odd isotopes 111 and 113.     

Spectroscopy of 41K by thermal neutron capture in 40K

The γ-ray spectrum emitted after thermal neutron capture in ⁴⁰K has been studied at the ILL high flux reactor with curved crystal Bragg, pair and Ge(Li) spectometers. 585 transitions were assigned to the reaction ⁴⁰K(n, γ)⁴¹K and 490 of them were placed into a ⁴¹K level scheme; 68 new states are proposed. On the basis of γ-ray branches to states with established spin and parity, many new spin-parity assignments were made. The level energies up to 4 MeV were measured with a precision of 8–50 eV relative to the 411.8 keV ¹⁹⁸Au standard, those above 4 MeV with a precision of 50–100 eV. The spin of the capture state was found to be $\text{I =}\text{7}\text{2}$; the neutron binding energy was determined to E_B = 10095.25(10) keV. The level density of $\text{I}{}^{\mathrm{\pi }}\text{=}\text{5}\text{2}{}^{\mathrm{\pm }}\text{,}\text{7}\text{2}{}^{\mathrm{\pm }}\text{,}\text{9}\text{2}{}^{\mathrm{\pm }}$ states was analyzed in terms of the constant-temperature Fermi gas model. It was shown that in this spin window the level scheme is almost complete up to an excitation energy of 5 MeV.