Determination of the spectroscopic quadrupole moments of 131Cs, 132Cs and 136Cs

Nuclear spectroscopic quadrupole moments of the radioactive isotopes ¹³¹Cs, ¹³²Cs, and ¹³⁶Cs have been determined from the hyperfine structure of the $\text{6}{}^2\text{P}{}_{\mathrm{<mtext>3</mtext><mtext>2</mtext>}}$ state by the level crossing method. The results including a Sternheimer correction are: $\text{Q}{}_{\mathrm{<mtext>s</mtext>}}\text{(}{}^{131}\text{Cs}\text{) = ?0.625(6)}\text{b}$, $\text{Q}{}_{\mathrm{<mtext>s</mtext>}}\text{(}{}^{132}\text{Cs}\text{) = +0.508(7)}\text{b}$, $\text{Q}{}_{\mathrm{<mtext>s</mtext>}}\text{(}{}^{136}\text{Cs}\text{) = +0.225(10)}\text{b}$. The quadrupole moments of all the Cs isotopes from A = 131 to A = 137 are recalculated. It is shown, that nuclear quadrupole moments of a specific isotope obtained from different atomic P-states only agree within the limits of error after application of the Sternheimer correction. The increase of Q_s with decreasing neutron number conforms with other observations and theoretical calculations stating that for elements around Z = 55 nuclear deformation develops below N = 82. The staggering of the sign of Q_s may be interpreted as consequence of an oblate-prolate degeneracy of the nuclear energy surface. Some magnetic moments have been slightly improved: $\text{μ}{}_{\mathrm{<mtext>I</mtext>}}\text{(}{}^{132}\text{Cs}\text{) = 2.219(7) μ}{}_{\mathrm{<mtext>N</mtext>}}$, $\text{μ}{}_{\mathrm{<mtext>I</mtext>}}\text{(}{}^{136}\text{Cs}\text{) = 3.705(15)μ}{}_{\mathrm{<mtext>N</mtext>}}$ (corrected for diamagnetism).     

Absolute E1, ΔK = 1 transition probabilities between multi-quasiparticle high-spin states in 176Hf and 178Hf

Applying the generalized centroid shift method in (α, 2n) reactions, the half-lives of the 3080 keV 15⁺ state in ¹⁷⁶Hf and of the 1637 keV 5^? state in ¹⁷⁸Hf have been measured as $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 0.20}{}^{\mathrm{+0.12}}{}_{\mathrm{?0.08}}\text{ns}$ and $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 0.40 ± 0.10}\text{ns}$, respectively. B(El) values of K-allowed E1 transitions $\text{n}\text{9}\text{2}{}^{\mathrm{+}}\text{[624]→}\text{7}\text{2}{}^{\mathrm{?}}\text{[514]}$ are derived, and together with other data on similar transitions in odd-A nuclei, compared with predictions of the Nilsson plus pairing model. In ¹⁷⁶Hf, the 15⁺ and 14^? states at 3080 and 2866 keV, respectively, appear as quite pure deformed 4QP configurations. In the 2QP state at 1637 keV in ¹⁷⁸Hf, possible strong mixing of vibrational components is discussed coupled via 2QP K-admixtures arising from the partial alignment of the $\text{i}{}_{\mathrm{<mtext>13</mtext><mtext>2</mtext>}}$ neutron.     

Measurement of the magnetic moment of the 7+ isomer in 198Tl

Using the atomic beam magnetic resonance method the hyperfine structure separation of $\text{1.9}\text{h}{}^{\mathrm{198m}}\text{Tl}\text{(I}{}^{\mathrm{\pi }}\text{= 7}{}^{\mathrm{+}}\text{)}$ has been measured in the ${}^2\text{P}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}$ atomic ground state. From the hyperfine structure splitting the nuclear magnetic dipole moment has been deduced. The results are: Δν = 4500 (68) MHz, μ_I = 0.641(10)μ_N. This is an improvement of approximately one order of magnitude compared to a previous measurement. The quoted value of the magnetic dipole moment includes corrections for the hyperfine structure anomaly and for diamagnetic shielding.     

Nuclear magnetic moment of the 9.7 h 12− isomer 196mAu

The magnetic hyperfine splitting v_M=|gμ_NB_HF/h| of ^196mAu (j^π=12^?; configuration ¦(π$\text{11}\text{2}$($\text{v}\text{13}\text{2}{}^{\mathrm{+}}\text{)〉}{}_{12}{}^{\mathrm{?}}$; $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 9.7}\text{h}\text{)}$ as dilute impurity in Ni has been determined with nuclear magnetic resonance on oriented nuclei as 96.0(2) MHz. With the known hyperfine field B_HF = ?264.4(3.9) kG corrected for hyperfine anomalies the g-factor and magnetic moment of ^196mAu are deduced to be |g| = 0.476(7) and |μ| = 5.72(8) μ_N. Taking into account the known magnetic properties of $\text{π}\text{1}\text{2}{}^{\mathrm{?}}$ and $\text{v}\text{13}\text{2}{}^{\mathrm{+}}$ isomeric states in the neighbouring odd Pt, Au and Hg nuclei the structure of the 12^? state is discussed.     

High-spin positive-parity states in 179Hf studied by the 180Hf(τ, α)179Hf reaction AT 32 MeV

Full angular distributions are presented for states populated in the reaction ¹⁸⁰Hf(τ, α)¹⁷⁹Hf at 32 MeV beam energy. Positive-parity states associated with the i_{$\text{13}\text{2}$} unique parity intruder orbital are given special attention. Thus, angular distributions for the five first members of the [624$\text{9}\text{2}$] groundstate sequence are given, as well as for a number of more highly excited states, some being new assignments. The distribution of l = 6 transfer strength is quite characteristic, two $\text{13}\text{2}$⁺ states being substantially more populated than the rest. The characteristic features of the data are explained by a quasiparticle-rotor calculation employing deformed Woods-Saxon orbitals, but only if the hexadecapole shape parameter of the nuclear potential is β₄ ～ ?0.08. The often anomalous differential cross sections for $\text{I}{}^{\mathrm{\pi }}\text{≠}\text{13}\text{2}{}^{\mathrm{+}}$ band members are well accounted for by a rotor model CCBA calculation employing transfer form factors extracted from the orbitals of the deformed Woods-Saxon field, and including non-adiabatic Coriolis mixing effects.     

Backbending in 167Hf and 168Hf and the band-crossing picture

Using two Compton-suppression spectrometers in an E_γ?E_γ coincidence experiment, the yrast bands in ^167,168Hf were extended up to $\text{49}\text{2}$ and 28 ?, respectively. The i ${}_{\mathrm{<mtext>13</mtext><mtext>2</mtext>}}$ positive parity band in ¹⁶⁷Hf experiences backbending at a higher frequency than the first backbending in ¹⁶⁸Hf, and no second backbending is obseerved in ¹⁶⁸Hf. New information is threby obtained on the nature and interaction strength of the crossing bands in the vicinity of N = 96.     

Nuclear moments of the low abundant natural isotope 176Lu and hyperfine anomalies in the lutetium isotopes

The atomic beam magnetic resonance method combined with laser-induced state- and isotopeselective detection of metastable atoms has been used to investigate the hyperfine structure of the ²D ground multiplet in ¹⁷⁵Lu and ¹⁷⁶Lu. The analysis of the data yields not only accurate values for the hyperfine interaction constants, the nuclear magnetic dipole moment of ¹⁷⁵Lu, and the electronic g_J, factors, but also the first directly measured value of the nuclear magnetic dipole moment of the low abundant isotope ${}^{176}\text{Lu}\text{: μ}{}_{\mathrm{I}}\text{(}{}^{176}\text{Lu) = 3.1692 (45)μ}{}_{\mathrm{<mtext>N</mtext>}}$ (corrected for diamagnetic shielding). The spectroscopic quadrupole moment of ¹⁷⁶Lu was calculated from the ratio of the B-factors and the quadrupole moment of ${}^{175}\text{Lu}\text{: Q}{}_{\mathrm{<mtext>s</mtext>}}\text{(}{}^{176}\text{Lu}\text{) = 4.92 (3)}\text{b}$. Moreover, the magnetic hyperfine anomalies for the isotopic chain ^{175,176,176m,177}Lu were determined. A quadrupole hyperfine anomaly between ¹⁷⁵Lu and ¹⁷⁶Lu was not found when comparing the ratio of the B-factors in the states ${}^2\text{D}{}_{\mathrm{<mtext>3</mtext><mtext>2</mtext>}}\text{and}{}^2\text{D}{}_{\mathrm{<mtext>5</mtext><mtext>2</mtext>}}$. From a comparison of the quadrupole moment of ¹⁷⁵Lu obtained from the hyperfine structure data and the quadrupole moment measured in muonic lutetium atoms semi-empirical Sternheimer shielding factors could be estimated.     

Recoil-distance lifetime measurements in 51Cr, 53Cr, 53Mn and 53Fe

Levels in ⁵¹Cr, ⁵³Cr, ⁵³Mn and ⁵³Fe were excited via (α, n) or (α, p) reactions. Using the recoil-distance method, mean-lives (in ps) have been obtained for excited states (keV) in the residual nuclei: ${}^{51}\text{Cr}\text{(2256) = 66±2,}{}^{53}\text{Cr}\text{(1536) = 21.5±3.5,}{}^{53}\text{Cr}\text{(2173) = 6.7±3.1,}{}^{53}\text{Mn}\text{(2564) = 20}{}^{\mathrm{+8}}{}_{\mathrm{?6}}\text{and}{}^{53}\text{Fe}\text{(1424) = 4.0±1.0}$. Reduced transition probabilities calculated from these values are compared with the available theoretical values.     

Magnetic moment of the 72+[404] ground state of 10.5 h 175Ta

The magnetic hyperfine splitting ν_M = |gμ_NB_HF/h| of ${}^{175}\text{Ta}\text{(J}{}^{\mathrm{\pi }}\text{=}\text{7}\text{2}{}^{\mathrm{+}}$; $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 10.5}\text{h}\text{)}$ in Fe has been measured with the technique of nuclear magnetic resonance on oriented nuclei as 320.4(1) MHz. With the known hyperfine field $\text{B}{}_{\mathrm{<mtext>HF</mtext>}}\text{(}\text{Ta}\text{Fe}\text{) = ?648(13)}\text{kG}$ the magnetic moment of the $\text{7}\text{2}{}^{\mathrm{+}}\text{[404]}$ ground state of ¹⁷⁵Ta is deduced to be $\text{¦μ¦ = 2.27(5)μ}{}_{\mathrm{<mtext>N</mtext>}}$.     

Flavor changing neutral currents and multileptons in e+e- and vμN,vμN

New quarks and new flavor-changing neutral currents give multiple lepton plus hadron final states in e⁺e^-, $\text{v}{}_{\mathrm{\mu }}\text{N,}\text{v}{}_{\mathrm{\mu }}\text{N}$. We observe that (i) e⁺e^- is a favored place to search for their effects through inclusive ratios σ(e⁺e^-+x:σ (μ⁺μ^- +x): σ(e±μ±+x) and same sign leptons e±e±+x, μ±μ±+x,e±μ±+x. Above a new flavor threshold four charged lrpton final states may become important. (ii) Trilepton final states in $\text{v}{}_{\mathrm{\mu }}\text{N,}\text{v}{}_{\mathrm{\mu }}\text{N}$ are not sensitive to the presence of flavor-changing neutral currents. Much more sensitive are the processes $\text{v}{}_{\mathrm{\mu }}\text{N}$ are ⁺e^-+βand (for charm changing neutral currents) $\text{v}{}_{\mathrm{\mu }}\text{N→e}{}^{\mathrm{+}}\text{β}$.     

Nuclear magnetic resonance of 9Be atoms by charge exchange with optically pumped 9Be+ ions

NMR of free ${}^9\text{Be}\text{(I =}\text{3}\text{2}\text{)}{}^1\text{S}{}_0$ atoms is observed via resonant charge exchange with optically pumped ${}^9\text{Be}{}^{\mathrm{+}}{}^2\text{S}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}$ ions in He buffer gas, yielding $\text{μ(}{}^9\text{Be}\text{) = ?1.1778 (9) μ}{}_{\mathrm{<mtext>n</mtext>}}$. Applications of the method suitable for all group II elements and Yb include: precision measurements of nuclear moments, chemical shifts, hfs-anomalies, and investigation of charge exchange processes.     

The g-factor of the72+[404] ground state of 177Ta

With the technique of nuclear magnetic resonance on oriented nuclei the hyperfine splitting $\text{ν}{}_{\mathrm{<mtext>M</mtext>}}\text{= ¦gμ}{}_{\mathrm{<mtext>N</mtext>}}\text{B}{}_{\mathrm{<mtext>HF</mtext>}}\text{/h¦}\text{of}{}^{177}\text{Ta}\text{(j}{}^{\mathrm{\pi }}\text{7}\text{2}{}^{\mathrm{+}}\text{; T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 56.6h)}$ in Fe has been measured With the known hyperfine field $\text{B}{}_{\mathrm{<mtext>HF</mtext>}}\text{(}\text{Ta}\text{Fe}\text{) = ?648 (13)}\text{kG the}\text{g-}\text{factor of the}\text{7}\text{2}{}^{\mathrm{+}}\text{[404]}$ ground state of ¹⁷⁷Ta is deduced to be $\text{¦g¦ = 0.643 (13)}$.     

One- and three-quasiparticle states in 171Hf and high spin rotational bands

The $\text{1}\text{2}{}^{\mathrm{?}}\text{[521]}\text{and}\text{7}\text{2}{}^{\mathrm{+}}\text{[633]}$ one-quasiparticle bands in the N = 99 nucleus ¹⁷¹Hf have been identified to spins of about $\text{45}\text{2}$ using (heavy ion, xn) reactions. The moments of inertia of these bands are consistent with the absence of backbending in the N = 98 core nucleus. The half-life of the $\text{5}\text{2}{}^{\mathrm{?}}\text{[512]}$ intrinsic state was measured as 63.6 ns. The strength of the $\text{5}\text{2}{}^{\mathrm{?}}\text{[512] →}\text{7}\text{2}{}^{\mathrm{+}}\text{[633]}\text{E}\text{1}$ transition is discussed. Two three-quasiparticle isomers with spins and parities $\text{19}\text{2}{}^{\mathrm{+}}\text{and}\text{23}\text{2}{}^{\mathrm{?}}$ have been identified and their suggested configurations are a $\text{7}\text{2}{}^{\mathrm{+}}\text{[633]}$ neutron added to the 6⁺ and 8^? two-quasiproton states of the core. The moment of inertia of a rotational band based on the $\text{23}\text{2}{}^{\mathrm{?}}$ isomer supports this suggestion, and shows the effect of partial rotation alignment of the $\text{i}{}_{\mathrm{<mtext>13</mtext><mtext>2</mtext>}}$ neutron.     

Beta-decay asymmetry and nuclear magnetic moment of 24Nam(T12 = 20 ms)

Polarized isomeric ${}^{24}\text{Na}{}^{\mathrm{m}}\text{(T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 20}\text{ms}\text{, I}{}^{\mathrm{\pi }}\text{= 1}{}^{\mathrm{+}}\text{)}$ nuclei were produced by capture of polarized thermal neutrons in a NaF single crystal at room temperature. The asymmetric β-decay radition of ²⁴Na^m was used to detect nuclear magnetic resonance signals yielding the magnetic moment $\text{|μ(}{}^{24}\text{Na}{}^{\mathrm{m}}\text{)| = 1.930 (3)}\text{n.m.}$ (uncorrected).     

The magnetic moment of the 22 μs isometric state in 38K

The g-factor of the $\text{τ}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{=22 μ}\text{s}\text{, J}{}^{\mathrm{\pi }}\text{=(7}{}^{\mathrm{+}}\text{), T=0}$ isomeric state at 3.46 MeV in ³⁸K has been measured by the differential spin precession method with the ${}^{35}\text{Cl}\text{(α,}\text{n}\text{)}{}^{38}\text{K}$ reaction. The result of g=+0.548 (μ=+3.836± 0.014 n.m.) is consistent with a pure configuration.     

The decay properties of 3.25 min 169Hf and 2.05 min 167Hf

The decays of 3.25 min ¹⁶⁹Hf and 2.05 min ¹⁶⁷Hf have been studied with high-resolution Ge(Li) and Si(Li) detectors. The total decay energy of ¹⁶⁹Hf determined from our experimental $\text{K}\text{β}{}^{\mathrm{+}}$ ratio is 3.29^+0.05_?0.13 MeV. The allowed unhindered character of the main β-branches in the decay of both isotopes allows unique Nilsson model assignments.     

The quadrupole moments of the 5− states in 116Sn, 118Sn and 120Sn

The quadrupole interaction frequencies $\text{ω}{}_0\text{=}\text{3eQ}{}_1\text{V}{}_{\mathrm{zz}}\text{41(21-1)}\text{h}\text{?}$ in the 5^? state of ¹¹⁸Sn have been measured by time differential perturbed angular correlation technique in Sn, Sb and (95% Sn+5% Sb) environments. The ω₀ for ¹¹⁶Sn was determined in Sn environment only. With the help of the known electric field gradient ¹) of Sn in a Sn lattice the quadrupole moments have been deduced as $\text{Q(5}{}^{\mathrm{?}}\text{,}{}^{118}\text{Sn}\text{) = ±0.10(4) b}\text{and}\text{Q(5}{}^{\mathrm{?}}\text{,}{}^{116}\text{Sn}\text{) = ±0.165(60)}\text{b}$. These values together with the known²) quadrupole moment of the analogous 5^? state in ¹²⁰Sn are interpreted in terms of the pure single-particle model. The data exhibit the expected strong systematic variation of Q_I with the number of particles in the h_{$\text{11}\text{2}$}. subshell which is being filled with 1, 3 and 5 neutrons in ¹¹⁶Sn, ¹¹⁸Sn, and ¹²⁰Sn, respectively.     

Magnetic moments of Jπ = 192− mirror states in 43Ti and 43Sc

The time-differential perturbed angular distribution method was used to determine the g-factors of the $\text{(}\text{f}{}_{\mathrm{<mtext>7</mtext><mtext>2</mtext>}}\text{)}{}^3\text{19}\text{2}{}^{\mathrm{?}}$ states in ⁴³Ti and ⁴³Sc. The results for the mass 43 mirror pair are: ${}^{43}\text{Ti}\text{: g = 0.760 ± 0.001, T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{, = 560 ± 6}\text{ns}$, ${}^{43}\text{Sc}\text{: g = 0.3286± 0.0007, T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 473 ± 5}\text{ns}$. Considering in addition the magnetic moments in A = 41 and 42, it is suggested that the deformed states considered by Johnstone and Castel and by Erikson are responsible for the observed large deviations from the Schmidt values.     

Nuclear orientation study of the excited states of 129I populated in the decay of 129gTe and 129mTe

From the angular distributions of γ-rays emitted by oriented ^129gTe and ^129mTe nuclei implanted in iron by isotope separator, unique spin assignments could be made for the excited states of ¹²⁹I at 487.4 keV $\text{(}\text{5}\text{2}{}^{\mathrm{+}}\text{)}$, 696.0 keV $\text{(}\text{11}\text{2}{}^{\mathrm{+}}\text{)}$, 729.6 keV $\text{(}\text{9}\text{2}{}^{\mathrm{+}}\text{)}$, 768.9 keV $\text{(}\text{7}\text{2}{}^{\mathrm{+}}\text{)}$, 1050.4 keV $\text{(}\text{7}\text{2}{}^{\mathrm{+}}\text{)}$ and 1111.8 keV $\text{(}\text{5}\text{2}{}^{\mathrm{+}}\text{)}$. In addition, E2/M1 amplitude ratios for the following ¹²⁹I γ-rays (energies are in keV) are derived: δ(459.6) = ?(0.076^+0.037_?0.148); δ(487.4) = 0.50^+0.17_?0.10 or δ^? = 0.35^+0.15_?0.09; δ(556.7) = 0.06±0.02 or δ^? = ?(0.10±0.02); δ(624.4) = 0.10±0.26 or δ^? > 0.4; the 696.0 keV γ-ray is pure E2; δ(729.6) = ?(0.34±0.06) or δ^?1 = 0.55±0.05; δ(741.1) = ?(0.27±0.10) or δ^?1 = ?(0.43±0.12); δ(817.2) = 0.46±0.04 or δ^?1 =0.20±0.03 if $\text{I}{}^{\mathrm{\pi }}\text{(845}\text{keV}\text{) =}\text{7}\text{2}{}^{\mathrm{+}}$; δ(1022.6) = ?(0.02 ±0.02) or δ^?1 = ?(0.23±0.02); $\text{δ(1084) = 0.56}{}^{\mathrm{+0.04}}{}_{\mathrm{?0.14}}$; δ(1111.8) = 0.06±0.05 or δ^?1 = ?(0.08±0.05). The anisotropy of the 531.8 keV γ-ray excludes $\text{1}\text{2}{}^{\mathrm{+}}$ as a possible spin assignment for the 559.6 keV level, so that no $\text{1}\text{2}{}^{\mathrm{+}}$ level is fed in the decay from ¹²⁹Te. Anisotropies for the 209, 250.7, 278.4 and 281.1 keV γ-rays are also measured. Comparison of the level scheme is made with theoretical predictions from both the pairing-plus-quadrupole model and the intermediate coupling unified model.     

Magnetic moments of isomeric bandheads in transitional nuclei: 119I and 192Tl

Nuclear g-factors of isomeric bandheads in the transition nuclei ¹¹⁹I and ¹⁹²Tl have been measured to be $\text{g[}{}^{119}\text{I}\text{(}\text{9}\text{2}{}^{\mathrm{+}}\text{)] = 1.20(3)}$ and $\text{g[}{}^{192}\text{Tl}\text{(8}{}^{\mathrm{?}}\text{)] = 0.207(5)}$. These values are in agreement with a model of one or two quasiparticles coupled to a deformed core. This interpretation is also supported by a preliminary quadrupole moment determination of $\text{Q[}{}^{192}\text{Tl}\text{(8}{}^{\mathrm{?}}\text{)] = 45(9)}\text{fm}{}^2$. The lifetimes were remeasured to be $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 34.6(5)}\text{ns}$ and $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 296(5)}\text{ns}$ for the ¹¹⁹I and the ¹⁹²Tl isomers, respectively.