Low-lying energy levels in 166Ho

The properties of some low-excited states of ¹⁶⁶Ho have been studied using thin, high resolution Ge detectors. The relative intensities of γ-lines were determined. The directional angular correlation measurements for the 28.23–54.24 keV cascade are in agreement with the 1^?(M1)2^?(E2)0^? spin sequence. The magnetic moment μ = 0.068 ± 0.010 μ_N of the 54.24 keV level was determined by integral perturbed angular correlation (IPAC) in an external magnetic field. This value can be explained by the configuration mixing due to the Coriolis interaction.     

Nuclear orientation of 160Tb in Tb metal

The decay of ¹⁶⁰Tb oriented at low temperatures in Tb metal has been investigated, and angular distributions of 19 γ-rays have been determined. The reduction in anisotropy in polycrystalline metal samples is discussed. Multipole mixing ratios have been determined for many of the γ-rays. A critical discussion is given of the previously reported $\text{M2}\text{E1}$ mixing ratios, and previous nuclear orientation studies are re-analyzed in a consistent manner so that their results can be compared. It is shown that the nuclear orientation and angular correlation results for the 1178 keV transition are consistent only if E3/E1 mixing is present. The El branching ratios and $\text{M2}\text{E1}$ mixing ratios are analyzed on the basis of Coriolis-mixed K = 0, 1 and 2 character for the negative-parity levels of ¹⁶⁰Dy.     

Levels in 156Gd studied in the (n, γ) reaction

Levels up to 2.3 MeV in ¹⁵⁶Gd have been studied using the (n, γ) reaction. Energies and intensities of low-energy γ-rays and electrons emitted after thermal neutron capture have been measured with a curved-crystal spectrometer, Ge(Li) detectors and a magnetic electron spectrometer. High-energy (primary) γ-rays and electrons have been measured with Ge(Li) detectors and a magnetic spectrometer. The high-energy γ-ray spectrum has also been measured in thermal neutron capture in 2 keV resonance neutron capture. The neutron separation energy in ¹⁵⁶Gd was measured as S_n = 8535.8 ± 0.5 keV.About 600 transitions were observed of which ~50% could be placed in a level scheme containing more than 50 levels up to 2.3 MeV excitation energy. 42 of these levels were grouped into 15 excited bands. In addition to the β-band at 1050 keV we observe 0⁺ bands at 1168, 1715 and 1851 keV. Other positive-parity bands are: 1⁺ bands at 1966, 2027 and 2187 keV; 2⁺ bands at 1154 (γ-band) and 1828 keV; and 4⁺ bands at 1511 and 1861 keV. Negative-parity bands are observed at 1243 keV (1^?), 1366 keV (0^?), 1780 keV (2^?) and 2045 keV (4^?). Reduced E2 and E0 transition probabilities have been derived for many transitions. The ground band, the β- and γ-bands and the 0⁺ band at 1168 keV have been included in a phenomenological four-band mixing calculation, which reproduces well the experimental energies and E2 transition probabilities.The lowest three negative-parity (octupole) bands of which the 0^? and the 1^? bands are very strongly mixed, were included in a Coriolis-coupling analysis, which reproduces well the observed energies. The E1 transition probabilities to the ground band are also well reproduced, while those from the higher-lying 0⁺ bands to the octupole bands are not reproduced. Absolute and relative transition probabilities have been compared with predictions of the IBA model and the pairingplus-quadrupole model. Both models reproduce well the E2 transitions from the γ-band, while strong disagreements are found for the E2 transitions from the β-band. The IBA model predicts part of the decay features of the higher lying 2⁺₂, 4⁺₁ and 2^?₁ bands.     

Multipole mixing ratios of γ-transltions in 182W

γ-γ directional correlation experiments were performed on 14 cascades in ¹⁸²W populated from the β^? decay of ¹⁸²Ta(115 d). Two Ge(Li) detectors were used in a coincidence arrangement, and the ¹⁸²Ta sources were dissolved in HF acid to minimize extranuclear perturbations. For the 1189keV, 2^? → 2⁺ transition, the measured directional correlation coefficients are consistent only with multipole mixing ratios $\text{δ}\text{(}\text{M}\text{2}\text{E}\text{1)}\text{= 0.45 ± 0.03}\text{and}\text{δ}\text{(E3}\text{E1)}\text{= ?0.67 ± 0.07}$. These mixing ratios are discussed and compared with the known conversion coefficients for the 1189keV transition. The E2/M1 multipole mixing ratios determined are (energy in keV): δ(66) = 0.15 ± 0.15, δ(85) = 0.31 ± 0.05, δ(114) = 0.31 ± 0.05, 0.56 ≦ δ(179) ≦ 1.36, δ(1121) = 12⁺²_?1, and δ(1231) = ?(32⁺¹⁴²_?15). The measured M2/E1 mixing ratios are: δ(68) = 0.03 ± 0.02, δ(152) = 0.014 ± 0.013 and δ(156) = ?0.13 ± 0.19.     

Collective and two-quasiparticle states in 158Gd observed through study of radiative neutron capture in 157Gd

The level structure of ¹⁵⁸Gd has been studied using the prompt γ-rays and conversion electrons emitted following neutron capture in ¹⁵⁷Gd. The γ-ray energy and intensity measurements were made using both Ge(Li) detectors and a curved-crystal spectrometer. Conversion-electron energy and intensity measurements were made using two separate magnetic spectrometers: one to measure the primary electron spectrum and the other to measure the lower energy secondary electron spectrum. Some γ-γ coincidence measurements were also made among the secondary γ-rays. From these data, a neutron separation energy of 7937.1 ± 0.5 keV has been determined for ¹⁵⁸Gd. A level scheme containing 59 excited states with energies < 2.25 MeV, for which de-excitation modes have been identified, is proposed for ¹⁵⁸Gd. Many of these states have been grouped into rotational bands. A total of thirteen excited rotational bands with band-head energies below 2.0 MeV are contained in the level scheme. Features of the proposed level scheme include: the K^π = 0^?, 1^? and 2^? octupole-vibrational bands with band-head energies of 1263, 977 and 1793 keV, respectively; the γ-vibrational band at 1187 keV; three excited K^π = 0⁺ bands with band-head energies of 1196, 1452 and 1743 keV; several two-quasiparticle bands with band-head energies in keV (and K^π assignments) of 1380 (4⁺), 1636 (4^?), 1847 (1⁺), 1856 (1^?), 1920 (4⁺) and 1930 (1⁺). An analysis of (d, p) reaction data is presented which permits definite two-quasiparticle configuration assignments to be made to most of these latter bands. Evidence is presented which suggests strong mixing of some two-neutron and two-proton bands. A phenomenological four-band mixing analysis is made of the energy and E2 transition-probability data for the ground-state band and the three lowest-lying excited collective positive-parity bands. Good agreement with experiment is obtained. A Coriolis-mixing analysis of the octupole bands has been carried out and good agreement with the data on level energies and E1 transition probabilities to the ground-state band has been achieved. Values of Z, the ratio of the E1 transition matrix element with ΔK = 1 to that with ΔK = 0, involving the octupole bands and the first four 0⁺ bands are derived. For three of these 0⁺ bands, absolute values of these matrix elements are deduced. An interesting alternation in the sign of Z is observed for these four 0⁺ bands.     

The decays of 21.55 min 162gTm and 24.3 s 162Tm (a new isomer)

The decay of the 21.55 min ground state and of the 24.3 s isomeric state of ¹⁶²Tm was investigated with semiconductor detectors. The γ-ray spectrum was investigated with a Compton-suppression Ge(Li)-NaI(Tl) arrangement. A Si (Li) detector, mounted in an electron transport solenoid, was used to investigate the conversion electron spectrum. Three-dimensional coincidence measurements were performed with large-volume Ge(Li) detectors. The ¹⁶²Tm ground state has spin-parity 1^? and Nilsson assignment p[411]↓?n[521]↑. An allowed β-transition (log ft ≈ 6.4) was observed to a 2^?, 2 octupole vibrational level at 1572.84 keV. The Q-value determined from positon-gamma coincidence measurements is 4705 ± 70keV. The discrepancy of the experimental K /β⁺ ratio with theoretical predictions might possibly be explained by a large number of unobserved weak γ-rays besides the total of 315 stronger ones observed in this study. The average β-strength function was calculated to be 1.2 × 10^?5. Among the 50 levels observed in the decay, the 2⁺, 4⁺ and 6⁺ members of the ground-state band, the 2⁺, 3⁺ and 4⁺ members of the γ-band, several 0⁺ and 2⁺ members of the K = 0 β-bands and 1^?, 2^? and 3^? octupole vibrational levels were identified. Parameter values Z_γ(0) and Z_γ(2) determining the mixing between the γ-band and the ground-state band, allow no conclusive evidence about unequalness of the intrinsic quadrupole moments of the ground states and the γ-band. The Z(0) parameters, determining the mixing between the β-bands and the ground-state band, and X parameters determining the ratio of E0 to E2 transition probabilities, were deduced. A previously unreported 24.3 sec isomer in ¹⁶²Tm was observed to decay in 10% of the cases by an allowed unhindered (log ft = 4.7) β-ray transition to a level at 1712.20 keV in ¹⁶²Er. The Nilsson configurations assigned to the isomeric and 1712.20 keV levels are p[523]↑ + n[521]↑₅₊ and n[523]↓ + n[521]↑₄₊ respectively. The isomeric level decays in 90% of the cases by an E3 transition (E_IT < 125 keV) to a p[404]↓ ?n[521]↑_2? level at 66.90 keV in ¹⁶²Tm, which decays by an (M1+ < 40 % E2) to the 21.55 min ¹⁶²Tm 1^? ground state.     

Coulomb excitation in 180Hf

Coulomb excitation studies have been performed to measure transition probabilities of collective quadrupole vibrational states in ¹⁸⁰Hf. The I = 2 level of the K^π = 2⁺ collective γ-band is established at 1200.5 keV with B(E2)_exc = (11.0 ± 1.1) × 10^?50e² · cm⁴ (3.6 ± 0.4 s.p.u.). The angular distribution of the de-exciting γ-rays from this level yields δ = 9.6⁺²²_?5.8 or, less likely, 0.7 ± 0.2 for the 1107.2 keV 2_γ⁺ → 2_g⁺ transition. The B(E2)_exc for any K^πI = 0⁺2 stateorother 2⁺ states up to 1500 keV is less than 5 × 10^?51e² · cm⁴ (< 0.2. s.p.u.).     

Electric monopole component in the 2+' → 2+ transition in 192Pt

Angular correlation measurements of K- and L-conversion electrons following the decay ¹⁹²Ir → ¹⁹²Pt have been made using a spectrometer with Ge(Li) and Si (Li) detectors. Absolute and relative internal conversion coefficients of transitions in ¹⁹²Pt were measured, using an ICC and prism β-spectrometers, to ≈ 2 % and values of δ_γ determined from the relative ICC. The experimental values measured in the study, A₂₂(K296γ316) = 0.138 ± 0.010, A₂₂(L296γ316) = 0.125 ± 0.013, α_K(296) = 0.0711 ± 0.0011, K/L_III = 9.65 ± 0.13. With δ_γ = + 5.4 ± 0.2, were employed for determining the E0/E2 amplitude ratios of conversion transitions, q(E0/E2), and the penetration parameter λ of the Ml component for the 2⁺' → 2⁺ (296 keV) transition in ¹⁹²Pt. The angular correlation measurements of L-conversion electrons enabled the elimination of one of two ranges of values of q and λ usually obtained. For the first time in our work, analysis of the e_Lγ angular correlation for the determination of the E0 component in the transition was carried out. As a result, q = +0.04 ± 0.05 with λ = ?4.5 ± 3.5 was obtained for the 296 keV transition. In this case, _ρ(E0) = 0.004 ± 0.005 agrees with _ρ(E0) = +0.006 determined theoretically by Kumar and Baranger for the 2⁺' → 2⁺ transition     

E0/E2 and E2/M1 multipole mixing amplitudes of γ-transitions in 192Pt

Angular correlation measurements of conversion electrons and γ-rays in ¹⁹²Pt following the decay of ¹⁹²Ir (74 d) have been made. In particular, the 296 keV e^?-316 keV γ correlation was measured in order that the electric monopole admixture in the 296 keV transition could be determined. The results of the angular correlation coefficients measured here and the ratio of K-shell to L_III shell conversion electrons measured by others are: ?0.09 < q < +0.26 as +62 < λ < +92 or ?0.29 < q < ?0.06 as ?5 < λ < +45. A possible explanation of the disagreement between two earlier measurements is suggested. The angular correlation coefficients for the measured e^?-γ and γ-γ cascades and the derived multipole mixing ratios are tabulated and compared with other recent measurements and with the predictions of the Kumar-Baranger nuclear model.     

g-factor of the 91.5 keV state in 151Sm

The g-factor of the 91.5 keV state in ¹⁵¹Sm has been measured by the TDPAC method using γγ cascades following the β-decay of 28 h ¹⁵¹Pm. The result is g = ?0.21±0.01. The anisotropy of the angular correlation for the 232.2-25.7 keV cascade is measured to be A = +0.058±0.006. From this an M1/E2 mixing ratio of δ² = 0.008±0.002 for the 232.3 keV transition is concluded. No attenuation of the anisotropy of the angular correlation is observed for aqueous solution sources of SmC1 in excess of hydrochloric acid. Spin and parity assignments for excited states in ¹⁵¹Sm are presented.     

Conversion-electron-gamma and gamma-gamma directional angular correlations in 160Dy

Gamma-gamma and conversion-electron-gamma angular correlations in ¹⁶⁰Dy have been measured for the 298 keV–966 keV and 298 keV–879 keV cascades. Particle parameters of the 966 keV E2 transition were determined to be b₂(E2; e_K) = +1.23±0.08 and b₂(E2; e_{ΣL + ΣM) = +1.27±0.23}. The multipole mixing ratio for the 298 keV radiation was determined to be δ(M2/E1) = +0.04±0.01 and we have confirmed the value δ(E2/M1) = ?13±2 for the 879 keV. The E0–E2 mixture parameter for the 879 keV transition was determined as q_K = ?0.03±0.09 assuming penetration effects to be negligible.     

Nuclear orientation of negative parity states of 131Xe

The anisotropies of the 177, 326, and 503 keV γ-transitions between negative parity states of ¹³¹Xe have been remeasured in the decay of oriented ¹³¹I nuclei. In addition the linear polarization of the 503 keV radiation has been determined with a Compton polarimeter consisting of two Ge(Li) detectors. A combined analysis of the reported experiment and earlier internal conversion and angular distribution data yields the unique assignments $\text{9}\text{2}{}^{\mathrm{?}}\text{and}\text{7}\text{2}{}^{\mathrm{?}}$ for the levels at 341 and 667 keV. The $\text{E2}\text{M1}$ mixing ratios of the 177 and 326 keV transitions are δ(177) = ?4.5 ± 1.5 and δ(326) = ?4.4 ± 1.6. The intensity of the L = 2 component in the first forbidden β-decay to the 667 keV level is at most 60 %.     

Analysis of the properties of excited states in 165Er

An analysis of ¹⁶⁵Tm decay has shown that precision measurements of the γ-ray and internal conversion electron intensities, in combination with angular correlation measurements, provide additional data useful for the determination of the mixing and intensity ratios of γ-transitions with a small energy difference. The spin of the 589.868 keV state is found to be $\text{I}{}^{\mathrm{\pi }}\text{=}\text{1}\text{2}{}^{\mathrm{?}}$. Doublet opposite-parity transitions from states at 1103.495, 920.632 and 745.968 keV to levels near 590 keV with an energy difference ΔE = 108 ± 22 eV are identified.     

Level structure of 184W from the 183W(n, γ) reaction

The level structure of ¹⁸⁴W has been studied from the prompt γ-rays emitted following the capture of both thermal and 2 keV neutrons by ¹⁸³W. Energies and intensities were measured for both the primary and the secondary (low-energy) prompt γ-rays. From these data, a level scheme is proposed for ¹⁸⁴W in which all the I^π = 0⁺, 1⁺ and 2⁺ states below ≈ 2.0 MeV are observed. Where possible, rotational-band assignments have been made to these and other levels. Additional evidence is presented which confirms the 1130 keV state as being the band head of a K^π = 2^? octupole vibrational band. Admixed K^π = 0⁺ and 2⁺ bands are established at 1322 and 1386 keV, respectively, with the I^π = 2⁺ states (at 1431 and 1386 keV) having a mutual admixture of ≈ 12%. In the energy region above 1.5 MeV, the following bands and band-head energies are identified: K^π = 1⁺, 1613 keV; K^π = 0⁺, 1614 keV; K^π = 1⁺, 1713 keV; K^π = 2⁺, 1877 keV. The neutron binding energy in ¹⁸⁴W has been determined to be 7411.1±0.6 keV. The band structure of the 1613 keV (1⁺) and 1614 keV (0⁺) bands is observed to be strongly distorted, the observed $\text{A (}\text{h}\text{?}{}^2\text{/2}\text{I}\text{)}$ values being ≈ 3.6 keV and ≈ 32 keV, respectively. This strong distortion is shown to be explainable in terms of Coriolis coupling of reasonable strength between the two bands. A similar explanation is shown to account for the somewhat less anomalous A-values (22.8 keV and 14.0 keV, respectively) of the 2⁺ band at 1386 keV and the 3⁺ band at 1425 keV. The results of a phenomenological fiveband-mixing analysis involving the K^π = 0⁺ and 2⁺ bands below ≈ 1.5 MeV are presented and discussed. These calculations indicate, among other things, that the direct E2 matrix element connecting the 1322 keV, K^π = 0⁺ band and the ground-state band is quite small, possibly zero. They also indicate that a nonzero E2 matrix element exists between this excited K^π = 0⁺ band and the γ-vibrational band and that the magnitude of this element is comparable with that between the γ-vibrational and ground-state bands. Arguments favoring and apparently refuting the interpretation of the 1322 keV, 0⁺ band as a “two-phonon γ-vibration” are presented.     

Properties of the 2' and 2” states in 106, 112, 114Cd

Angular correlations have been measured between γ-rays from the 2 → 2 → 0 cascades in ^106,112,114Cd and the beam of 11.0 MeV α particles effecting Coulomb excitation. Multipole admixtures for the 2 → 2 transitions, as deduced from these correlations, when combined with earlier results establish their B(E2) and B(M1) values. For the transitions from the 1312 and 1208 keV states in ^112,114Cd the B(E2) values in single-particle units are 18±4 and 24±7. These values are typical for transitions from “two-quadrupole-phonon” states in this mass region whereas that of the 1718 keV transition in ¹⁰⁶Cd has the smaller value of 7.0±2.3. The B(E2) values of the 2 → 2 transitions in ^112,114Cd from the 1468 and 1363 keV states are < 0.3 single-particle units. The B(M1) values of all five transitions are ≈ 10^?2$\text{(}\text{e}\text{h}\text{?}\text{2Mc}\text{)}{}^2$.     

Spins and mixing ratios in 138Ba

The spin assignments to the 1899 (4⁺), 2308 (3⁺ or 4⁺) and 2446 (3⁺) keV levels in ¹³⁸Ba have been confirmed by γ-γ directional correlation measurements. In addition, the multipolarity and $\text{E2}\text{M1}$ mixing parameters for a number of transitions have been established as follows: 409 keV (M1+E2, ?0.75 < δ < ?0.45 or ?0.85 < δ < ?0.05 depending on the choice of J^π = 3⁺ or 4⁺ for the initial state), 463 keV (E2, 0 < δ < 0.15 for $\text{M3}\text{E2}$ admixture), 547 keV (M1+E2, ?0.06 < δ < ?0.015), 872 keV (M1+E2, δ undefined) and 1010 keV (M1+E2, ?0.015 < δ < +0.020).     

Gamma transitions in 59Ni following the β+ decay of 59Cu

The γ-ray decay spectrum of 82 s ⁵⁹Cu produced by the ⁵⁸Ni(p, γ) ⁵⁹Cu reaction has been studied with a 40 cm³ Ge(Li) detector. The number of γ-rays now known for this decay has more than doubled. Additional direct β⁺ branches to the 1679.7($\text{5}\text{2}{}^{\mathrm{?}}$), 2414.8($\text{3}\text{2}{}^{\mathrm{?}}$) and 2681 keV states of ⁵⁹Ni have been identified with log ft values of 5.5, 5.5 and 6.0, respectively. A major change is the reassignment of the 1340.4 keV γ-ray to a 1679.7 → 339.3 keV transition. A limit of log $\text{ft ≧ 6.9}$ is given for the direct feeding of the 1337($\text{7}\text{2}{}^{\mathrm{?}}$) keV state, together with limits for direct population of other energetically available states. The new weak γ-ray branches found for the 878.0, 1301.5 and 1679.7 keV levels are in excellent agreement with the recent theoretical calculations of Glaudemans et al.     

Spins of levels in 194Pt

Selected cascades in the level scheme of the ¹⁹⁴Pt nucleus have been studied by the γ-γ directional correlation method and the spins of the 924, 1513, 1623, 1672 and 1798 keV levels determined to be 3, 2, 2, 2 and 1 respectively. The multipole mixing ratios of the 301, 594, 1184 and 1295 keV γ-transitions have been determined and a number of B(E2) ratios are compared with theory.     

Spectroscopic investigations of the decay 223Ra → 219Rn

Internal conversion electron spectra of the transitions 4.4 keV, 10.0 keV, 14.4 keV, and 324.1 keV in the decay ²²³Ra → ²¹⁹Rn were measured. E2/M1 mixing ratios of these γ-transitions were deduced from conversion electron intensity ratios: δ² = 3.8(4) · 10^?3, 2.35(18) · 10^?3, 12.85(36) · 10^?3, 0.23(3). The half-lives of the 4.4 keV and 14.4 keV levels were determined as $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 15.4(1.3)}$ nsec and 0.875(30) nsec. Reduced transition probabilities were calculated and compared to the Weisskopf estimates. αγ angular correlation measurements of the transitions 269.6 keV, 324.1 keV, and 338.6 keV and an αγ linear polarization measurement of the 269.6 keV transition were performed for spin determination. We assign $\text{I =}\text{7}\text{2}$ to the ²¹⁹Rn ground state and $\text{I =}\text{5}\text{2}$ or $\text{9}\text{2}$ to the 269.6 keV state. All other low excitations including the 338.6 keV level have spins $\text{I =}\text{5}\text{2}$, $\text{7}\text{2}$, or $\text{9}\text{2}$. The spins of the states 158.7 keV and 14.4 keV are equal. The ²²³Ra ground state spin is $\text{I =}\text{7}\text{2}$ or $\text{9}\text{2}$. The possibility of an interpretation of the transitional nucleus ²¹⁹Rn in the frame of the collective model is discussed.     

The level structure of 184W FROM THE β− decay of 184Ta

Levels of ¹⁸⁴W populated in the decay of 8.7 h ¹⁸⁴Ta have been studied by a variety of experimental techniques. As a result of β and γ-ray energy and intensity determinations and extensive β-γ and γ-γ coincidence measurements, a detailed ¹⁸⁴Ta decay scheme accommodating more than 99.5% of the decay intensity has been established. Intense β-ray groups of end-point energies 1165±26 and 1123±26 keV populate levels in ¹⁸⁴W at 1699 and 1746 keV, which de-excite predominantly to the 8.3 μs isomeric level at 1285 keV, recently identified as the $\text{1}\text{2}{}^{\mathrm{?}}\text{[510]ν?}\text{11}\text{2}{}^{\mathrm{+}}\text{[615]ν K}{}^{\mathrm{\pi }}\text{= 5}{}^{\mathrm{?}}$ band origin. The 1699 keV level also de-excites to members of a $\text{1}\text{2}{}^{\mathrm{?}}\text{[510]ν?}\text{7}\text{2}\text{[503]ν K}{}^{\mathrm{\pi }}\text{= 3}{}^{\mathrm{+}}$ band based at 1425 keV. New information about the properties of the γ-vibrational and K = 2 octupole bands in ¹⁸⁴W is presented and the possible configurations of the levels directly populated in the β^? decay are discussed. The configuration $\text{7}\text{2}{}^{\mathrm{+}}\text{[404]π ?}\text{3}\text{2}{}^{\mathrm{?}}\text{[512]ν K}{}^{\mathrm{\pi }}\text{= 5}{}^{\mathrm{?}}$ is indicated for the ¹⁸⁴Ta ground state.