Multipole mixing ratios of γ-transltions in 182W

γ-γ directional correlation experiments were performed on 14 cascades in ¹⁸²W populated from the β^? decay of ¹⁸²Ta(115 d). Two Ge(Li) detectors were used in a coincidence arrangement, and the ¹⁸²Ta sources were dissolved in HF acid to minimize extranuclear perturbations. For the 1189keV, 2^? → 2⁺ transition, the measured directional correlation coefficients are consistent only with multipole mixing ratios $\text{δ}\text{(}\text{M}\text{2}\text{E}\text{1)}\text{= 0.45 ± 0.03}\text{and}\text{δ}\text{(E3}\text{E1)}\text{= ?0.67 ± 0.07}$. These mixing ratios are discussed and compared with the known conversion coefficients for the 1189keV transition. The E2/M1 multipole mixing ratios determined are (energy in keV): δ(66) = 0.15 ± 0.15, δ(85) = 0.31 ± 0.05, δ(114) = 0.31 ± 0.05, 0.56 ≦ δ(179) ≦ 1.36, δ(1121) = 12⁺²_?1, and δ(1231) = ?(32⁺¹⁴²_?15). The measured M2/E1 mixing ratios are: δ(68) = 0.03 ± 0.02, δ(152) = 0.014 ± 0.013 and δ(156) = ?0.13 ± 0.19.     

The electron capture decay of 131Ba

The decay of ¹³¹Ba has been investigated by means of a 4π internal source scintillation spectrometer and a Ge(Li) detector. The L/K. and M/L electron capture ratios of the allowed transitions to the 373, 620 and 1048 keV levels in ¹³¹Cs have been measured. From these electron capture ratios, the ifQ_EC value and the exchange and overlap corrections X^L/K and X^M/L have been derived.     

Spins of levels in 194Pt

Selected cascades in the level scheme of the ¹⁹⁴Pt nucleus have been studied by the γ-γ directional correlation method and the spins of the 924, 1513, 1623, 1672 and 1798 keV levels determined to be 3, 2, 2, 2 and 1 respectively. The multipole mixing ratios of the 301, 594, 1184 and 1295 keV γ-transitions have been determined and a number of B(E2) ratios are compared with theory.     

Spins of the levels and multipole mixing ratios of transitions in 125Sb determined from γ-γ directional correlation and polarization-directional correlation measurements

In order to resolve several discrepancies in spin assignments to levels in ¹²⁵Sb, directional correlations and polarization-directional correlations have been measured for several γ-γ cascades in ¹²⁵Sb populated from the decay of ¹²⁵Sn. Earlier results obtained from using NaI and Ge(Li) and NaI detectors were difficult to interpret due to the complex structure of the decay scheme. To improve the experimental situation, we have used two coaxial Ge(Li) detectors for the angular correlation measurements and a coaxial Ge(Li)-planar Ge(Li) combination for the polarization-directional correlations. Combination of the results of these measurements give unique spin assignments of $\text{11}\text{2}$^?, $\text{11}\text{2}$^?, $\text{9}\text{2}$⁺, $\text{11}\text{2}$⁺ and $\text{9}\text{2}$⁺ to the 1982 keV, 1890 keV, 1420 keV, 1089 keV and 1067 keV levels, respectively. The determined E2/M1 mixing ratios are : δ(470) = 0.010±0.027, δ(1067) = ?0.86±0.18, and δ(916) = ?0.02±0.01.     

The decay scheme of 127Ba and half-lives of some low-lying excited states in 123, 125, 127, 129Cs

Radioactive sources of ^{123, 125, 127, 129}Ba obtained in the spallation reaction have been studied with Ge(Li), Si(Li), NaI(Tl) and plastic detectors. On the basis of γ-ray energies, intensities, energy sums and coincidence information, the decay scheme has been proposed for ¹²⁷Ba. No high-spin isomer of ¹²⁷Ba has been observed. The lifetimes of $\text{5}\text{2}$⁺ → $\text{1}\text{2}$⁺ transitions in ^{123, 125, 127, 129}Cs have been measured. No evidence for the shape isomerism in ¹²⁷Cs has been found.     

The decay of 174Tm and mixing of the Kπ = 5− two-quasiparticle states in 174Yb

The decay of 5.4 min ¹⁷⁴Tm has been investigated using Ge(Li) spectrometers in singles and coincidence measurements. A total of 43 γ-ray transitions, 26 of them not reported before, have been observed following the decay of ¹⁷⁴Tm. All transitions could be placed in a level scheme comprising 19 excited states of ¹⁷⁴Yb. The Nilsson model has been used to interpret the level structure. The mixing of two-quasineutron and two-quasiproton states is studied and the experimental mixing matrix element is compared with the results of theoretical calculations.     

A study of the 138Ba(d,p)139Ba reaction at 19 MeV

The ¹³⁸Ba(d,p) reaction has been studied at an incident deuteron energy of 19 MeV, using the injector-tandem accelerator and the multichannel magnetic spectrograph of the University of Oxford. Deuteron and proton optical model parameters have been obtained from the analysis of elastic scattering experiments on a ¹³⁸Ba target. The parameters have been used to calculate theoretical (d, p) angular distributions on the basis of the DWBA. From the comparison of experimental and theoretical distributions, orbital angular momentum transfers have been deduced and spectroscopic factors determined for all the levels observed up to an excitation energy of 2.5 MeV in ¹³⁹Ba. The spectroscopic information thus obtained is more complete than that from previous studies, and is in satisfactory agreement with expected sum rule limits. A notable item of new information is the assignment of an l_n = 6 transition to the level at 1.54 MeV in ¹³⁹Ba.     

Decay of 48K, 49K and 50K

The ⁴⁸K, ⁴⁹K and ⁵⁰K nuclides have been produced in high energy fragmentation and analyzed by mass spectroscopy techniques. Their half-lives have been measured as 6 ± 1 s, 1.1 ± 0.3 s and and 0.7 ± 0.3 s, respectively. The γ-rays from their radioactive decay have been observed and the corresponding γ-intensities measured. The nuclide ⁵⁰K is shown to be a delayed neutron emitter. The antianalog states in the daughter Ca nuclei with a $\text{(1d}{}_{\mathrm{<mtext>3</mtext><mtext>2</mtext>}}\text{)}{}^{\mathrm{?}}$ neutron configuration, preferentially populated in the β-decay, have been located. The corresponding $\text{1d}{}_{\mathrm{<mtext>3</mtext><mtext>2</mtext>}}$ neutron single-particle energy is found to remain approximately constant for these neutron-rich Ca isotopes.     

Measurement of the parity non-conservation in nuclear forces in 75As, 171Tm,and 175Lu and of the polarized bremsstrahlung from 51Cr, 170Tm, 177Lu,and 198Au

The circular polarization P of γ-rays from unpolarized sources of ⁷⁵Se, ¹⁷¹Er, and ¹⁷⁵Yb of strengths ? 500 Ci has been measured with a Compton polarimeter of the radial transmission type. Eight NaI crystals and a four-fold current integration system were used to simultaneously record the data in four independent channels. The results are: P = ?(1.8 ± 6.0) × 10^?5 for the 401 keV transition in ⁷⁵As (the experimental error is ± 1.5 × 10^?5, the remaining part is due to the uncertainty in the decay scheme of ⁷⁵Se), P = (0.8 ± 1.5) × 10^?4 for the 296 keV and 308 keV transition in ¹⁷¹Tm, and P = (5.7 ± 0.8) × 10^?5 for the 396 keV transition in ¹⁷⁵Lu. The last value confirms the parity non-conservation in nuclear forces. The polarimeter was calibrated with bremsstrahlung from ¹⁷⁰Tm. The correction for polarized bremsstrahlung was given special attention. Correction factors are derived for ⁵¹Cr, ¹⁷⁷Lu, and ¹⁹⁸Au from a comparison of the measured and calculated bremsstrahlung yields.     

Beta decays of 25Na, 25Al and 29Al

The radioactivities ²⁵Na, ²⁵Al, and ²⁹Al were produced in the ²³Na(t, p)²⁵Na, ²⁴Mg(d, n)²⁵Al, and ²⁷Al(t, p)²⁹Al reactions using a 3.5 MV Van de Graaff. γ-radiations were measured by means of a target-transfer system and a Ge(Li) detector with or without Compton suppression. Decay schemes derived for ²⁵Na and ²⁹Al are in general agreement with earlier results, but with improved accuracy of branching ratios and much sharper limits on the intensities of certain unobserved β- and γ-ray transitions. Precision measurements of the energies of principal γ-rays gave results in keV for the listed decaying bodies as follows: ²⁵Na ? 1611.716(11); ²⁵Al ? 1611.708(11); and ²⁹Al ? 1273.361(9). The energy determinations of the ²⁵Mg 1612 keV γ-transition measured in the decays of ²⁵Na and ²⁵Al differ by 8 ± 9 eV.     

The quadrupole moments of the 5− states in 116Sn, 118Sn and 120Sn

The quadrupole interaction frequencies $\text{ω}{}_0\text{=}\text{3eQ}{}_1\text{V}{}_{\mathrm{zz}}\text{41(21-1)}\text{h}\text{?}$ in the 5^? state of ¹¹⁸Sn have been measured by time differential perturbed angular correlation technique in Sn, Sb and (95% Sn+5% Sb) environments. The ω₀ for ¹¹⁶Sn was determined in Sn environment only. With the help of the known electric field gradient ¹) of Sn in a Sn lattice the quadrupole moments have been deduced as $\text{Q(5}{}^{\mathrm{?}}\text{,}{}^{118}\text{Sn}\text{) = ±0.10(4) b}\text{and}\text{Q(5}{}^{\mathrm{?}}\text{,}{}^{116}\text{Sn}\text{) = ±0.165(60)}\text{b}$. These values together with the known²) quadrupole moment of the analogous 5^? state in ¹²⁰Sn are interpreted in terms of the pure single-particle model. The data exhibit the expected strong systematic variation of Q_I with the number of particles in the h_{$\text{11}\text{2}$}. subshell which is being filled with 1, 3 and 5 neutrons in ¹¹⁶Sn, ¹¹⁸Sn, and ¹²⁰Sn, respectively.     

The half-life of 207Bi and decays of 211At and 211Po

The half-life of ²⁰⁷Bi was obtained from the genetic relation between ²⁰⁷Po and ²⁰⁷Bi, and between ²¹¹At and ²⁰⁷Bi. The half-life was found to be 33.4 ± 0.8 y. The half-life of ²⁰⁷Po was determined to be 5.81 ± 0.04 h by following the decay of the characteristic γ-rays from ²⁰⁷Po. The half-life of ²¹¹ At was determined tobe 7.23 ± 0.02 h by following the decay of γ-rays and α-particles from ²¹¹At and ²¹¹Po. The half-lives determined in the present work for ²⁰⁷Po and ²¹¹At agree with the literature although the half-life of ²⁰⁷Bi differs considerably from the currently accepted value of 38 y. The branching ratio of ²¹¹ At decaying through EC and α-decay modes was determined together with the branching ratios of the three α-particles emitted from ²¹¹Po.     

Beta-decay of 32C1 and 40Sc

The β⁺ decays of ³²C1 and ⁴⁰Sc have been investigated with a rabbit system. New β-branches and γ-lines are reported. Branching ratios and log ft values are determined. The 6.66 MeV state of ³²S is shown to have J^π = 1⁺ or 2⁺.     

Beta decay studies in the vicinity of 13250Sn82: Excited states in 13051Sb, 13052Te and 13252Te

Using the OSIRIS on-line isotope separator facility, the decays of ¹³⁰Sn and ^{130, 132}Sb have been studied. On the basis of singles γ and γ-γ coincidence Ge(Li) spectra and conversion electron Si(Li) measurements, level schemes for ¹³⁰Sb, ¹³⁰Te and ¹³²Te have been constructed. The corresponding half-lives have been measured using multiscaling technique. The 3.8 min ground state of ¹³⁰Sn populates only positive parity states in the πν^?3 nucleus ¹³⁰Sb: the energetically lowest 5⁺ state with the $\text{(π1}\text{g}{}_{\mathrm{<mtext>7</mtext><mtext>2</mtext>}}\text{, ν2}\text{d}{}_{\mathrm{<mtext>3</mtext><mtext>2</mtext>}}\text{)}$ configuration assignment; the $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 3.6 ± 0.3}\text{ns}\text{4}{}^{\mathrm{+}}$ state at 70.0 keV; the 2⁺ state at 262.5 keV; the (0, 1)⁺ state at 697.2 keV; the 3⁺ state at 813.1 keV and the 1⁺ state at 1042.3 keV excitation energy. A 1.7 min isomeric state in ¹³⁰Sn, with the tentative spin assignment (7^?), populates several odd parity levels in ¹³⁰Sb. These arise from the $\text{(π1}\text{g}{}_{\mathrm{<mtext>7</mtext><mtext>2</mtext>}}\text{, ν1}\text{h}{}_{\mathrm{<mtext>11</mtext><mtext>2</mtext>}}{}^{-1}\text{)}$ and/or $\text{(π2}\text{d}{}_{\mathrm{<mtext>5</mtext><mtext>2</mtext>}}\text{, ν1}\text{h}{}_{\mathrm{<mtext>11</mtext><mtext>2</mtext>}}{}^{-1}\text{)}$ configurations and are located 84.7 keV (6^?), 144.9 keV (7^?), 688.5 keV and 1044.0 keV above the 40 min 8^? β- decaying state. No transitions between odd and even parity states have been observed.The most important excited states in ¹³⁰Te found in the β^? decay of the 6.6 min ¹³⁰Sb 5⁺ state are: 839.4 keV, 2⁺; 1632.8 keV, 4⁺; 1815.1 keV, 6⁺; 2100.8 keV, 5^?.Levels in the π²ν^?2 nucleus ¹³²Te were observed in the β^? decays of the 2.8 min ¹³²Sb (4⁺) and the 4.2 min ¹³²Sb (8^?) states. Unique spin and parity assignments have been given to the following states: 973.9 keV, 2⁺; 1670.7 keV, 4⁺; 1774.1 keV, 6⁺; 1924.7 keV, 7^?; 2053.0 keV, 5^?.     

Gamma transitions in 59Ni following the β+ decay of 59Cu

The γ-ray decay spectrum of 82 s ⁵⁹Cu produced by the ⁵⁸Ni(p, γ) ⁵⁹Cu reaction has been studied with a 40 cm³ Ge(Li) detector. The number of γ-rays now known for this decay has more than doubled. Additional direct β⁺ branches to the 1679.7($\text{5}\text{2}{}^{\mathrm{?}}$), 2414.8($\text{3}\text{2}{}^{\mathrm{?}}$) and 2681 keV states of ⁵⁹Ni have been identified with log ft values of 5.5, 5.5 and 6.0, respectively. A major change is the reassignment of the 1340.4 keV γ-ray to a 1679.7 → 339.3 keV transition. A limit of log $\text{ft ≧ 6.9}$ is given for the direct feeding of the 1337($\text{7}\text{2}{}^{\mathrm{?}}$) keV state, together with limits for direct population of other energetically available states. The new weak γ-ray branches found for the 878.0, 1301.5 and 1679.7 keV levels are in excellent agreement with the recent theoretical calculations of Glaudemans et al.     

A re-investigation of 19O(β−)19F

Gamma rays observed in¹⁹O(β^?)¹⁹F have been studied with Ge(Li) spectroscopy utilizing activity created via the ¹⁸O(d, p) ¹⁹O reaction. Precision measurements of γ-ray energies and intensities, in conjunction with previous work, define the following excitation energies (in keV) and β-branching ratios (in %) for states of ¹⁹F: 109.894(5), 0.055(13/38); 197.143(4), 45.4(1.5); 1345.67(13), 0.017(2); 1554.038(9), 54.4(1.2); 2779.849(34), < 0.002; 3908.17(20), 0.0081(5); 4377.700(42), 0.0984(30). The corresponding values of logft are 8.34(30/10); 5.384(14); 8.25(5); 4.625(10); > 8.17; 6.133(27); and 3.859(17), respectively. The β-branches to the 1346 and 3908 keV states had not been observed previously. The β-branch for the 4378 keV state is in significantly better accord with theoretical expectations than the previous value of 0.160(12) %.     

On the decay of 201Bi and 199Bi

Level schemes for ²⁰¹Pb and ¹⁹⁹Pb, studied from the radioactive decay of bismuth isobars, are proposed on the basis of γ-ray, electron spectra and γ-γ coincidence measurements. The experimental results are compared mainly with those of two theoretical approaches.     

Beta-delayed proton emission from 97Cd and 99Cd

Two new β-delayed proton precursors, ^97,99Cd, have been identified at the ISOLDE on-line isotope separator. The proton branching ratio for ⁹⁹Cd is (1.7^+1.1_?0.5) × 10^?3. The ⁹⁹Cd proton spectrum is discussed in terms of the statistical model with Porter-Thomas fluctuations. The half-life of ⁹⁹Cd was determined to be 16±3 sec. A search for ⁹⁸Cd was also performed and it was found to be a pure β-emitter with a probable half-life of ≈ 8 sec.     

Levels of 190Os populated in the decays of 3.3 h 190mRe and 12 d 190Ir and in the 189Os(d,p)190Os reaction

The level structure of ¹⁹⁰Os has been investigated by the techniques of radioactive decay and neutron transfer reaction spectroscopy. The existence of 3.3 h ^190mRe has been confirmed; it decays ≈ 49% by isomeric transitions and ≈ 51% by β^? decay to levels in ¹⁹⁰Os with spins $\text{\$}\text{?}\text{= 5}$. In a re-investigation of the 12 d ¹⁹⁰Ir decay, a virtually complete decay scheme has been established and discrepancies between the I^π values assigned to several ¹⁹⁰Os levels by earlier workers have been resolved. The reaction ¹⁸⁹Os(d, p)¹⁹⁰Os has been studied and information about the locations of two-quasiparticle states involving the $\text{3}\text{2}\text{[512]ν}$ orbital and about the microscopic compositions of collective excitations has been derived. Various aspects of the ¹⁹⁰Os level structure are discussed in the light of the combined radioactivity and transfer reaction results.     

g-factors of 2.7 h 93Tc, 4.9 h 94Tc and 20 h 95Tc

The hyperfine splitting frequencies gμ_NB_H.F./h of 2.7 h ⁹³Tc $\text{(J}{}^{\mathrm{\pi }}\text{=}\text{9}\text{2}{}^{\mathrm{+}}\text{)}$, 4.9 h ⁹⁴Tc (J^π = 7⁺) and 20 h ⁹⁵Tc $\text{(J}{}^{\mathrm{\pi }}\text{=}\text{9}\text{2}{}^{\mathrm{+}}\text{)}$ as dilute impurities in Fe have been measured with NMR on oriented nuclei as 336.36(5) MHz, 175.11(1) MHz and 315.97(2) MHz, respectively. From the resonance shifts with an external magnetic field B₀ the hyperfine field of Tc$\text{Fe}$ has been determined as -317(5) kG. Taking this into account the nuclear g-factors are deduced as $\text{g(}{}^{93}\text{Tc}\text{) = 1.392(22), g(}{}^{94}\text{Tc}\text{) = 0.725(11)}\text{and}\text{g(}{}^{95}\text{Tc}\text{) = 1.308(21)}$.