碳纳米管锁模双包层光纤激光器的实验研究

本文采用双包层掺镱光纤作为增益介质,用单壁碳纳米管作为饱和吸收体,获得最高输出功率为336 mW的锁模脉冲激光.用飞秒激光诱导水击穿法直接在单模光纤上制备出D形区,通过在D形光纤上滴涂单壁碳纳米管溶液,成功制备出碳纳米管饱和吸收体,并对其饱和吸收特性进行测试,发现其调制深度为27％.利用该饱和吸收体作为锁模器件,制备出具有环形腔结构的锁模光纤激光器.当抽运功率为4W时,获得了脉宽为93.8 fs,中心波长为1083.8 nm,3 dB谱宽为8.6 nm,重复频率为5.59 MHz,平均功率为336 mW的飞秒脉冲激光输出.     

Systematical analysis of mode-locked fiber lasers using single-walled carbon nanotube saturable absorbers

The output characteristics of the Er-doped mode-locked fiber laser using a single-walled carbon nanotube saturable absorber are investigated theoretically with a nonlinear Schrtidinger equation and a saturable absorption equation using realistic parameters. Stable self-starting mode-locking pulses are achieved under net normal, net zero, and net anomalous cavity group velocity dispersion （GVD） respectively. A spectrum with a flat top is obtained from the net normal cavity GVD laser while a spectrum with Kelly side-bands is obtained from the net anomalous cavity GVD laser. The characteristics of the pulse duration changing with cavity GVD and modulation depth of the single-walled carbon nanotubes are discussed. The characteristics of the mode-locking pulses from net normal, net zero, and net anomalous cavity GVD mode-locked fiber lasers are compared. These systematical results are useful for designing mode-locked fiber lasers with saturable absorbers made by different kinds of carbon nano-materials.     

基于单壁碳纳米管调Q锁模低阈值Tm,Ho:LiLuF_4激光器

采用垂直生长法制作的单壁碳纳米管作为可饱和吸收体,结合特殊的低阈值谐振腔设计,首次在Tm,Ho:LiLuF_4全固态激光器中实现了低阈值自启动被动调Q锁模运转.以波长可调的掺钛蓝宝石固体激光器作为抽运源,选用1.5%,3%和5%的输出耦合镜,获得了出光阈值低至52,59和62mW的连续光输出.采用3%输出耦合镜,获得了阈值低至250mW的稳定调Q锁模脉冲输出,调Q包络的脉宽为2μs,调Q包络下锁模脉冲重复频率178.6MHz,最大输出功率154mW,最大的单脉冲能量为0.86nJ,调制深度接近100%.     

Bound states of solitons in a fiber laser mode locked with carbon nanotube saturable absorber

We report on the experimental observation of bound states of solitons in an erbium-doped fiber laser passively mode-locked by the carbon nanotube saturable absorber. Bound states of solitons with various pulse separations are obtained. While the tightly bound solitons always exhibit the same set of fixed discrete pulse separations with π or π/2 phase difference, the feature becomes less obvious for the loosely bound solitons. The result that various states of the bound solitons were obtained in the same fiber laser makes a systematic experimental study on them and a comparison of their properties possible. Our results once again show that the bound soliton emission is an intrinsic feature of the mode-locked soliton fiber lasers.     

147 fs碳纳米管倏逝场锁模全光纤掺铒光纤激光器

利用化学腐蚀法在光纤包层表面成功制备了调制深度为3.9%的单壁碳纳米管饱和吸收体.组建了环形腔结构的全光纤掺铒光纤激光器,以制备的单壁碳纳米管薄膜为锁模元件,利用倏逝场锁模实现了锁模输出.锁模脉冲的中心波长为1556 nm,3 dB光谱带宽为24 nm,脉冲宽度为147 fs,重复频率为150 MHz.在520mW抽运功率下,平均输出功率为21 mW,相应的单脉冲能量为0.14 nJ.     

Sequential generation of self-starting diverse operations in all-fiber laser based on thulium-doped fiber saturable absorber

Self-starting Q-switching, Q-switched mode-locking and mode-locking operation modes are achieved sequentially in an all-fiber erbium-doped fiber laser with thulium-doped fiber saturable absorber for the first time. The central wavelengths of Q-switching, Q-switched mode-locking and mode-locking operation modes are 1569.7 nm, 1570.9 nm, and 1572 nm, respectively. The mode-locking operation of the proposed fiber laser generates stable dark soliton with a repetition rate of 0.99 MHz and signal-to-noise ratio of 65 dB. The results validate the capability of generating soliton pulse by doped fiber saturable absorber. Furthermore, the proposed fiber laser is beneficial to the applications of optical communication and signal processing system.     

Flexible pulses from carbon nanotubes mode-locked fiber laser

We demonstrate a flexible erbium-doped pulsed fiber laser which achieves the wavelength and pulse width tuning by adjusting an intracavity filter. The intracavity filter is flexible to achieve any of the different wavelengths and bandwidths in the tuning range. The wavelength and width of pulse can be tuned in a range of ~ 20 nm and from ~0.8 ps to 87 ps,respectively. The flexible pulsed fiber laser can be accurately controlled, which is insensitive to environmental disturbance.     

Switchable single-longitudinal-mode dual-wavelength erbium-doped fiber ring laser based on one polarization-maintaining fiber Bragg grating incorporating saturable absorber and feedback fiber loop

Switchable single-longitudinal-mode (SLM) dual-wavelength erbium-doped fiber ring laser based on one polarization-maintaining fiber Bragg grating (PMFBG) is demonstrated. Due to the enhancement of the polarization hole burning (PHB) by the PMFBG, the laser can be designed to operate in stable dual-wavelength or wavelength-switching modes with a wavelength spacing of 0.336 nm at room temperature by adjusting a polarization controller (PC). The stable SLM operation is guaranteed by a compound-ring cavity and a saturable absorber (SA). The optical signal-to-noise ratio (OSNR) is over 45 dB. The amplitude variation in nearly one and half an hour is less than 0.2 dB.     

高效循环电弧放电法制备大量单壁纳米碳管的研究

介绍一种利用电弧放电法高效率制备大量单壁纳米碳管的新方法.以钨代替传统的石墨棒作为放电阴极，采取循环式往返放电法.同时利用高分辨透射电子显微镜及拉曼光谱对制备的单壁纳米碳管进行了观察、表征.实验证明：以钨为阴极的循环电弧放电法可以初步实现单壁纳米碳管的高效率、大批量生产. 关键词： 单壁纳米碳管 钨电极 拉曼光谱     

氧化石墨烯被动锁模掺镱光纤激光器多脉冲现象的实验研究

利用氧化石墨烯作为可饱和吸收体,在被动锁模全正常色散掺镱光纤激光器中研究了多脉冲的现象,在同一抽运功率不同偏振态下,实验获得了矩形脉冲谐波锁模、耗散孤子谐波锁模、准谐波锁模,脉冲峰值周期性调制,脉冲簇、脉冲束、混沌多重脉冲的多脉冲现象,插入激光腔内的2nm窄带滤波器具有限制增益带宽、对脉冲塑形、诱导多脉冲产生的作用,调节偏振控制器相当于改变腔内增益,是实现不同类型多脉冲现象的主要原因,本实验研究有利于加深对多脉冲动力学行为在正常色散区域氧化石墨烯锁模掺镱光纤激光器中的理解。     

A study on interaction of DNA molecules and carbon nanotubes for an effective ejection of the molecules

The ejection of DNA molecules from carbon nanotubes is reported from interaction energy perspectives by molecular dynamics simulations. The critical ejection energy, which is to be applied to a DNA molecule for a successful ejection from a carbon nanotube, is investigated based on a study on the friction and binding energy between the DNA molecule and the tube. An effective ejection is realized by subjecting a kinetic energy on the DNA molecule that is larger than the solved critical ejection energy. In addition, the relationship between ejection energies and sizes of DNA molecules and carbon nanotubes is investigated.     

High catalytic performance of Pt nanoparticles on plasma treated carbon nanotubes for electrooxidation of ethanol in a basic solution

Nanosized Pt particles deposited on plasma treated multi-walled carbon nanotubes have been used in electrocatalytic oxidation of ethanol in a basic solution. These Pt nanoparticles have very narrow size distribution and exhibit significant higher catalytic activities, higher Pt utilization efficiency (93.77%) and improved durability in comparison to the commercial available Johnson Matthey Pt/C catalyst.