Interaction between magnetic agglomerates and an extended free radicals network studied by magnetic resonance

Solids containing an extended network of free radicals have been prepared and studied by magnetic resonance techniques in the 4–290 K temperature range. One solid contained additionally a small amount of magnetic γ-Fe₂O₃ in the form of nanoparticle agglomerates. The solid without agglomerates displayed only a narrow, single resonance line centered at g _eff = 2.0043. The magnetic resonance measurements of the solid with γ-Fe₂O₃ agglomerates gave a spectrum composed of two lines attributed to two different magnetic centers: a narrow line due to free radicals and a broad line arising from magnetic iron oxide agglomerates. In the high temperature range the integrated intensities of both lines decreased with decreasing temperature. The resonance field of the broad line shifted to lower magnetic fields upon lowering the temperature with the gradient ΔH _r /ΔT = 2.3 G/K, while the narrow line shifted towards higher magnetic fields. The linewidth of the broader line increased with decreasing temperature while for the narrow lines in both samples this change was small. The magnetic iron oxide clusters produce a magnetic field which acts on the free radicals network and its strength depends essentially on the concentration of clusters. The reorientation process in the free radicals network is more intense in the sample without magnetic clusters.     

Self-consistent structure of a dc discharge with a closed hall current in crossed electric and magnetic fields

A dc glow discharge with a closed Hall current in crossed electric and magnetic fields in helium is investigated. It is shown that the main features of an unmagnetized dc discharge [1] (such as the separation of the discharge into a space charge sheath and a quasineutral plasma, the formation of a cathode fall region and a negative glow, the appearance of a region with a reversed electric field producing a potential well for low-energy electrons and resulting in the formation of a Faraday dark space, and the formation of three pronounced groups of electrons in the electron distribution function) are also retained in a discharge in crossed fields. It is found that the sheath length is almost independent of the magnetic field, while the length of the negative glow region decreases appreciably with increasing magnetic field. The measured electron distribution function agrees well with the nonlocal theory, according to which the current in the Faraday dark space is carried by the intermediate electrons that are not trapped in the potential well and the energies of which are lower than the first excitation energy.     

Optical control of magnetic Feshbach resonances in Bose gases

We theoretically investigate optical control of magnetic Feshbach resonance in Bose gases with two optical fields. The two optical fields couple two ground states through an excited state. Compared with the usual single-optical scheme, two optical fields can greatly suppress the inelastic loss resulting from spontaneous emission by the destructive quantum interference. Using the mean field theory, the analytical formula of the scattering length is obtained. The results show that the scattering length can be modified in a large range by changing the Rabi frequency or the optical field frequency. The strong atom–molecule interaction has obvious effect on the scattering length.     

Bifurcations of the shape of a magnetic fluid droplet in a rotating magnetic field

An analysis is made of the behavior of a magnetic droplet suspended in a liquid in a high-frequency uniform, rotating magnetic field. In weak fields the droplet is spheroidal while in strong fields it is disk-shaped. The observed change in the shape of the droplet as the amplitude of the field increases depends on the magnetic permeability μ of the liquid and takes place according to three scenarios: (a) for small μ the spheroidal droplet is continuously converted into a disk; (b) for intermediate μ there is a range of fields in which the droplet becomes a triaxial ellipsoid with its major axis lying in the plane of the field, and spheroid-triaxial ellipsoid-disk transitions take place as a result of a soft bifurcation; (c) at high μ both transitions are hard. Theoretical calculations are made of the stability curve for the various droplet shapes. It is predicted that a change in the types of droplet shape bifurcations will occur in strong fields. A comparison is made with the experimental data.     

Effects of sweep rates of external magnetic fields on the labyrinthine instabilities of miscible magnetic fluids

The interfacial instability of miscible magnetic fluids in a Hele-Shaw Cell is studied experimentally, with different magnitudes and sweep rates of the external magnetic field. The initial circular oil-based magnetic fluid drop is surrounded by the miscible fluid, diesel. The external uniform magnetic fields induce small fingerings around the initial circular interface, so call labyrinthine fingering instability, and secondary waves. When the magnetic field is applied at a given sweep rate, the interfacial length grows significantly at the early stage. It then decreases when the magnetic field reaches the preset values, and finally approaches a certain asymptotic value. In addition, a dimensionless parameter, Pe, which includes the factors of diffusion and sweep rate of the external magnetic field, is found to correlate the experimental data. It is shown that the initial growth rate of the interfacial length is linearly proportional to Pe for the current experimental parameter range and is proportional to the square root of the sweep rate at the onset of labyrinthine instability.     

Magnetic Field Mapping Around Individual Magnetic Nanoparticle Agglomerates Using Nitrogen-Vacancy Centers in Diamond

A modified diamond–photonics based metrology is proposed to explore the magnetic fields created by agglomerates of magnetic nanoparticles (MNPs). MNPs are promising for environmental and medical applications; those proposed for cancer magnetic hyperthermia treatments are small superparamagnetic <20 nm iron oxide particles. Inside cells, they assemble in larger MNP agglomerates, reaching cross-sections of several micrometers. Here, these conditions are reproduced and MNP agglomerates immobilized. Optically detected magnetic resonance (ODMR) signals recorded without a bias field in a confocal microscope and scanning across a homogenous shallow layer of fluorescent nitrogen-vacancy centers in a bulk diamond sample placed in direct contact with the MNP agglomerates are used to determine magnetic fields with a spatial resolution of 500 nm in a lateral direction. This spatial resolution allows determining magnetic field maps around individual MNP agglomerates, for which magnetic fields with strengths ranging from 0.03 mT to maximal 1.2 mT in the direct vicinity of the agglomerates and with detectable fields up to 5 µm away from the agglomerates, are determined. Based on the findings, a pathway to non-invasively study the micro/nano topology of MNP agglomerates is proposed.     

Electrofluidized bed of silica nanoparticles

The behavior of a fluidized bed of electroneutral silica nanopowder under the influence of a cross-flow electric field is studied. Nanoparticle agglomerates experience an electrophoretic force as a consequence of being naturally charged, which leads to electrophoretic deposition at static and low frequency fields. In contrast, fluidization is enhanced at intermediate field frequencies, which can be attributed to agglomerate forced flow.     

Effect of magnetic field on Mott's variable-range hopping parameters in multiwall carbon nanotube mat

We report the temperature and magnetic field dependence of the conductivity of multiwall carbon nanotube mat in the temperature range 1.4-150 K and in magnetic fields up to 10 T. It is observed that charge transport in this system is governed by Mott’s variable-range hopping of three-dimensional type in the higher temperature range and two-dimensional type in the lower temperature range. Mott’s various parameters, such as localization length, hopping length, hopping energy and density of states at the Fermi level are deduced from the variable-range hopping fit. The resistance of the sample decreases with the magnetic field applied in the direction of tube axis of the nanotubes. The magnetic field gives rise to delocalization of states with the well-known consequence of a decrease in Mott’s T0 parameter in variable-range hopping. The application of magnetic field lowers the crossover temperature at which three-dimensional variable-range hopping turns to two-dimensional variable-range hopping. The conductivity on the lower temperature side is governed by the weak localization giving rise to positive magnetoconductance. Finally, a magnetic field-temperature diagram is proposed showing different regions for different kinds of transport mechanism.     

Nonlinear oscillation characteristics of magnetic microbubbles under acoustic and magnetic fields

Microbubbles loaded with magnetic nanoparticles (MMBs) have attracted increasing interests in multimode imaging and drug/gene delivery and targeted therapy. However, the dynamic behaviors generated in diagnostic and therapeutic applications are not clear. In the present work, a novel theoretical model of a single MMB was developed, and the dynamic responses in an infinite viscous fluid were investigated under simultaneous exposure to magnetic and acoustic fields. The results showed that the amplitude reduces and the resonant frequency increases with the strength of the applied steady magnetic field and the susceptibility of the magnetic shell. However, the magnetic field has a limited influence on the oscillating. It is also noticed that the responses of MMB to a time-varying magnetic field is different from a steady magnetic field. The subharmonic components increase firstly and then decrease with the frequency of the magnetic field and the enhanced effect is related to the acoustic driving frequency. It is indicated that there may be a coupling interaction effect between the acoustic and magnetic fields.     

Electrically induced luminescence in parabolic quantum wells in a magnetic field

Interband luminescence in a parabolic quantum well is studied in applied electric and magnetic fields. It is shown that the luminescence peak is displaced towards higher frequencies with increasing magnetic field strength, while an increase in the electric field strength causes a displacement of the emission peak towards the long-wave region and a decrease in its amplitude. The theoretical results are compared with the experimental data. The existence of a new electromagnetic-wave emission channel (electrically induced luminescence) associated with indirect optical transitions is predicted. The frequency dependence of the electrically induced radiation is computed, taking into account the interaction of an electron with acoustic and optical phonons. It is found that the half-width of the luminescence peak increases with the electric field strength.     

Effect of a change in the optical density of a magnetic emulsion in electric and magnetic fields

The change in the optical density of an emulsion of magnetic fluid drops suspended in a mineral oil under the action of electric and magnetic fields has been investigated. It is found that the sign of the change in transparency in an ac electric field depends on the field frequency. It is shown that, joint action of codirectional low-frequency electric and dc magnetic fields can compensate for the change in the optical density. Calculation of the change in the emulsion optical density within the anomalous diffraction approximation showed that this effect can be explained by small field-induced deformation of microdrops.     

Magnetotransport in a semconductor superlattice with transverse magnetic field

Magnetotransport in a semiconductor superlattice (SL) under transverse magnetic field has been investigated. It is shown that in weak magnetic and electric fields there is negative magnetoresistivity along the SL layers and positive magnetoresistivity along the SL axis. The Hall resistivity is much less than the usual semiconductor value. With an increase of electric field, there appears a negative differential conductivity (NDC) along the SL layers, and the Hall voltage depends nonlinearly on current density. In higher electric field, destroying the miniband structure, the magnetoresistivity along the SL axis is negative. The magnetoresistivity along the SL axis in strong magnetic field is positive for any current density. The Hall resistivity in strong magnetic (electric) field equals the classical value.     

Quasistationary magnetic field generated in a plasma by a whistler-mode radio pulse

It has been shown experimentally that a quasistationary magnetic field is generated in a weakly collisional magnetized plasma by a spatially nonuniform high-frequency whistler-mode field. The sources of the quasistationary magnetic field are nonlinear currents generated due to the longitudinal and transverse components of the ponderomotive force, acting on charged particles in the spatially localized high-frequency pump field. The dynamics of the excited magnetic fields has been analyzed. It was found that the settling time of the quasistationary magnetic field is determined by the switching-on time of the high-frequency field and the propagation of pulsed current and magnetic fields from the region of their generation occurs with the velocity of low-frequency whistler waves.     

Electron self-energy in a magnetic field

In the lowest order in the fine-structure constant, the electron self-energy in an external magnetic field can be written in the form of a double integral representation containing the exact information about the radiative shift and width of the energy levels, without approximation in the field strength. In the low-field expansion of the radiative shift, the leading term is conveniently interpreted in terms of the electron's anomalous magnetic moment, whilst in very strong fields the enhancement of the cyclotron motion makes the shift a positive, slowly increasing function of the field intensity. It follows that, even in superstrong magnetic fields, the electromagnetic interaction cannot give rise to an instability of the electron-positron vacuum.     

Investigation of airborne nanopowder agglomerate stability in an orifice under various differential pressure conditions

The stability of agglomerates is not only an important material parameter of powders but also of interest for estimating the particle size upon accidental release into the atmosphere. This is especially important when the size of primary particles is well below the agglomerate size, which is usually the case when the size of primary particles is below 100 nm. During production or airborne transportation in pipes, high particle concentrations lead to particle coagulation and the formation of agglomerates in a size range of up to some micrometers. Binding between the primary particles in the agglomerates is usually due to van der Waals forces. In the case of a leak in a pressurized vessel (e.g. reactor, transport pipe, etc.), these agglomerates can be emitted and shear forces within the leak can cause agglomerates to breakup. In order to simulate such shear forces and study their effect on agglomerate stability within the airborne state, a method was developed where agglomerate powders can be aerosolized and passed through an orifice under various differential pressure conditions. First results show that a higher differential pressure across the orifice causes a stronger fragmentation of the agglomerates, which furthermore seems to be material dependent.     

Photon-drag effect in a two-dimensional electron gas in high magnetic fields

We present the first measurements concerning the photon drag effect in a two-dimensional electron gas based on intersubband transitions in high magnetic fields. It is shown that the excitation mechanism of the drag voltage in a magnetic field differs obviously from the case of zero magnetic field. The longitudinal as well as the Hall drag voltage show strong oscillations around zero when the magnetic field is swept. Both consist of a B-symmetrical and an antisymmetrical part with the same periodicity in B as the magnetoresistanceR_xx. The drag voltage oscillations are strongly correlated to the relative position of Fermi energy and Landau levels and are independent of the photon energy in the range of usable laser lines.     

Oscillator strengths of optical transitions of a cylindrical shell: Crossed static electric and magnetic fields

The single-electron eigenstates of a cylindrical shell are determined as functions of the applied crossed electric and magnetic fields in the effective-mass approximation. The system considered consists of donor charges taken to be uniformly distributed within an inner core of infinitely long length. The core is concentrically enveloped by a semiconducting material of finite thickness; which is essentially the host material. This configuration of the donor charges sets up a spatially varying electric field nonetheless with only the radial component. In addition, a uniform magnetic field is applied parallel to the axis of symmetry of the inner core. As is well known, the axial applied magnetic field lifts the double degeneracies of the electron’s subbands characterized by the same azimuthal quantum numbers which differ only in sign. The main effect of increasing the external electric field is to elevate the various energy subbands, more or less to the same extent, to higher values. Further, evaluations of the oscillator strengths of optical transitions of the cylindrical shell are carried out within the dipole approximation. The radiation field is taken to be that of circularly polarized light incident along the axis of the core. The oscillator strengths of optical transitions are found to increase with an increase of the applied magnetic field, particularly in the regime of small magnetic fields. In contrast, the oscillator strengths of these optical interactions become suppressed as the donor charge density is increased.     

Electrically stimulated motion of dislocations in a constant magnetic field

This paper reports on the results of investigations into the dislocation mobility in n-Si single crystals (N _d =5×10²⁴ m^?3) upon simultaneous exposure to electric (j=3×10⁵ A/m²) and magnetic (B≤1 T) fields. It is found that the introduction of dislocations (≈10⁹ m^?2) into dislocation-free silicon doped with phosphorus leads to the appearance of the paramagnetic component of the magnetic susceptibility. The paramagnetic component increases with an increase in the dopant concentration. Similar transformations in silicon account for the formation of magnetically sensitive impurity stoppers that respond to external magnetic perturbations. An analysis of the behavior of dislocations in electric and magnetic fields has revealed a parabolic dependence of the dislocation path length on the magnetic induction B. The effective charges and mobilities of dislocations are numerically calculated from the results obtained. A model is proposed according to which the observed increase in the dislocation mobility is associated with the decrease in the retarding power of magnetically sensitive stoppers due to a local change in the magnetic characteristics of the material and the spin-dependent reactions stimulated by a magnetic field.     

Righi-Leduc effect in a quantizing magnetic field

The Righi-Leduc effect in semiconductors with a Kane dispersion law in the presence of strong, quantizing, magnetic fields is studied theoretically. The explicit form of the dependence on the magnetic field, temperature, and concentration in arbitrary quantizing magnetic fields is established for semiconductors with a nondegenerate electron gas in the approximation of small nonparabolicity. A simple formula that is applicable for all strong magnetic fields, including quantizing fields, is derived for the Righi-Leduc coefficient in the case of strongly degenerate semiconductors with an arbitrary nonparabolic band. It is shown that in order to determine the photon part of the thermal conductivity ,ph directly from experiment it is best to employ samples with a nondegenerate electron gas in strong, but nonquantizing, magnetic fields.Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 7, pp. 102–107, July, 1988.     

Dynamics of a dielectric droplet suspended in a magnetic fluid in electric and magnetic fields

The behavior of a microdrop of dielectric liquid suspended in a magnetic fluid and exposed to the action of electric and magnetic fields is studied experimentally. With increasing electric field, the deformation of droplets into oblate ellipsoid, toroid and curved toroid was observed. At the further increase in the electric field, the bursting of droplets was also revealed. The electrorotation of deformed droplets was observed and investigated. The influence of an additional magnetic field on the droplet dynamics was studied. The main features of the droplet dynamics were interpreted and theoretically examined.