1-mJ, sub-5-fs carrier–envelope phase-locked pulses

We report the routine generation of sub-5-fs laser pulses with 1-mJ energy and stable carrier–envelope phase at 1-kHz repetition rate, obtained by compressing the multi-mJ output from a phase-locked Ti:sapphire amplifier in a rare-gas-filled hollow fiber. The dual-stage amplifier features a hybrid transmission grating/chirped mirror compressor providing 2.2-mJ, 26-fs pulses at 1 kHz with standard phase deviation of 190 mrad rms. We demonstrate hour-long phase stability without feedback control of grating position or rigorous control of the laser environment, simply by using small pulse stretching factors in the amplifier, which minimize the beam pathway in the compressor. The amplifier also integrates a versatile AOPDF (acousto-optic programmable dispersive filter) for closed-loop spectral phase optimization. The various factors influencing the overall phase stability of the system are discussed in detail. Using the optimized output, 1-mJ, 4.5-fs pulses are generated by seeding the neon gas filled hollow fiber with a circularly polarized input beam. A standard phase deviation of 230 mrad after the HCF is obtained by direct f-to-2f detection and slow-loop feedback to the oscillator locking electronics without any additional spectral broadening.     

On the use of lenses to focus few-cycle pulses with controlled carrier–envelope phase

From a model of focusing with lenses that includes the effects of the lens variable thickness, material dispersion, aperture, spherical and chromatic aberrations, we characterize the conditions under which a lens can focus to few-cycle, transform-limited pulses propagating without distortion along the focal region. A lens also allows to control the carrier?Cenvelope phase shift along the focus. The carrier?Cenvelope phase shift is drastically reduced by focusing with specific focal lengths and input spot sizes, which are of the same order as those typically used in experiments involving focusing for phase-sensitive, light-matter interactions.     

Direct carrier–envelope phase stabilization of a soliton-effect compressed sub-two-cycle pulse source through nonlinear mixing of solitonic and dispersive waves

We present a carrier–envelope phase (CEP) stabilized sub-two-cycle 5.2 fs pulse source based on soliton-effect self-compression of femtosecond laser pulses in millimetre-long highly nonlinear photonic crystal fibres. We employ a simple and efficient scheme to generate a strong (40–60 dB, configuration dependent) CEP beat signal directly from the pulse source via f-to-2f interferometry where the second harmonic of the main soliton pulse is mixed with the isolated dispersive blue/green radiation peak that is also generated in the compression process, obviating the need for additional spectral broadening mechanisms.     

A fiber Mach–Zehnder interferometer for the unique phase retrieval of ultrafast pulses with a 1 THz gap

Unique phase retrieval of ultrashort pulses with well-separated frequency components was demonstrated using a cross-correlation technique with a conditioning filter. Here, this filter was designed as an unbalanced fiber Mach–Zehnder interferometer. A pulse-shaping apparatus was used to generate pulses with a 1 THz gap. A fast phase-retrieval algorithm was then employed to reconstruct these pulses. Ambiguities of relative-phase or other characteristics were not found under any circumstances.     

57 W, 27 fs pulses from a fiber laser system using nonlinear compression

We report on the generation of 27 fs pulses with an average output power of 57 W and a repetition rate of 78 MHz. The pulses are generated by combining a high average power fiber chirped pulse amplification (FCPA) system with a microstructured large-mode-area fiber for nonlinear compression. The FCPA system delivers 270 fs pulses in a linearly polarized beam with diffraction-limited quality. Nonlinear compression is achieved by launching the pulses into a short (few cm) piece of microstructured fiber and subsequent compression by a pair of chirped mirrors. PACS  42.55.Wd; 42.55.Xi, 42.65.Re     

Composition dependent phase transformation of Pt0.5−x Mn0.5+x from A1 to L10 phase

Pt_0.5−x Mn_0.5+x films were prepared by sputtering deposition of Pt foil and Mn target to study the order-disorder transition from a thermodynamic metastable fcc (A1) phase to L1₀ phase. Both Differential Scanning Calorimetry and High Temperature X-Ray Diffraction studies showed the phase transformation from fcc to the L1₀ structure for the Pt_0.50Mn_0.50 and Pt_0.40Mn_0.60 samples but along completely different kinetic paths. A composition dependent phase transformation was observed by comprehensive Differential Scanning Calorimetry studies on a series of Pt_0.5−x Mn_0.5+x samples. The changes of the lattice parameter and the cell volume of L1₀ Pt_0.5−x Mn_0.5+x as a function of composition suggest that the anti-site is not the dominant point defect for L1₀ Pt_0.5−x Mn_0.5+x .     

Suppression of forward dilepton production from an anisotropic quark–gluon plasma

We calculate the rapidity dependence of leading-order medium dilepton yields resulting from a quark–gluon plasma which has a local time-dependent anisotropy in momentum space. We present a phenomenological model which includes the temporal evolution of the plasma anisotropy parameter, ξ, and the hard momentum scale, p _hard. Our model interpolates between a 1+1 dimensional collisionally broadened expansion at early times and a 1+1 dimensional ideal hydrodynamic expansion at late times. Using our model, we find that at LHC energies, forward high-energy medium dilepton production would be suppressed by a factor of up to 3 if one assumes an isotropization/thermalization time of 2 fm/c. Therefore, it may be possible to use forward dilepton yields to experimentally determine the time of the onset of locally isotropic hydrodynamic expansion of the quark–gluon plasma as produced in ultrarelativistic heavy-ion collisions.     

Cleaning of artificially soiled paper using nanosecond, picosecond and femtosecond laser pulses

Cleaning of cultural assets, especially fragile organic materials like paper, is a part of the conservation process. Laser radiation as a non-contact tool offers prospects for that purpose. For the studies presented here, paper model samples were prepared using three different paper types (pure cellulose, rag paper, and wood-pulp paper). Pure cellulose serves as reference material. Rag and wood-pulp paper represent essential characteristics of the basic materials of real-world artworks. The papers were mechanically soiled employing pulverized charcoal. Pure and artificially soiled paper samples were treated with laser pulses of 28 fs (800 nm wavelength) and 8–12 ns (532 nm) duration in a multi pulse approach. Additionally, the cellulose reference material was processed with 30 ps (532 nm) laser pulses. Damage and cleaning thresholds of pure and soiled paper were determined for the different laser regimes. Laser working ranges allowing for removal of contamination and avoiding permanent modification to the substrate were found. The specimens prior and after laser illumination were characterized by light-optical microscopy (OM) and scanning electron microscopy (SEM) as well as multi spectral imaging analysis. The work extends previous nanosecond laser cleaning investigations on paper into the ultra-short pulse duration domain.     

Thermal,Raman and dielectric study of 0.5K0.5Bi0.5TiO3–0.5PbTiO3 ceramics

The 0.5K_0.5Bi_0.5TiO₃–0.5PbTiO₃ ceramics were prepared by following a standard solid-state method. The Raman, thermal and dielectric properties of these ceramics were investigated. The X-ray measurements showed that samples have single perovskite-type structure with tetragonal symmetry. Dielectric study revealed that the dielectric behaviour of the investigated ceramics is rather of normal ferroelectrics with large thermal hysteresis. The transition temperature observed by means of differential scanning calorimetry measurements is in good agreement with that obtained from dielectric study.     

Effect of annealing temperature on hardness, thickness and phase structure of carbonitrided 304 stainless steel

Carbonitriding of AISI 304 austenitic stainless steel was performed at a plasma-processing power of 450 W using inductively coupled radio frequency (rf) plasma in a gas mixture of 50% N₂ and 50% C₂H₂. The rate of carbonitriding, microhardness, phase structure of the compound layer, surface microstructure and cross-section morphology were studied before and after the annealing process. At the annealing temperature up to 800°C, the microhardness values of the compound zones decrease, while the associated values of the diffused zones increase. Little change was found in the thickness of the compound and diffused zones when the carbonitrided samples were annealed up to 400°C. However, at a higher annealing temperature, the thicknesses of both zones increase. The γ-Fe austenite is the main crystalline phase that can be detected by X-ray diffraction. As the annealing temperature increases up to 500°C, X-ray spectra show α-Fe and Fe₅C₂ phases. Nitrogen diffuses more deeply from the near surface to the interior of the treated sample as the annealing temperature increases up to 800°C and this might explain the extent of carbonitrided thickness and the enhanced microhardness of the diffused zone.     

Limits on a nucleon–nucleon monopole–dipole coupling from spin relaxation of polarized ultra-cold neutrons in traps

A new limit is presented on the axion-like monopole–dipole P, T-non-invariant interaction in a range (10⁻⁴–1) cm. The spin-dependent nucleon–nucleon potential between neutrons and nucleons of the walls of the cavity containing ultra-cold neutrons should affect the neutron depolarization probability at their reflection from the walls. The limit is obtained from existing data on the ultra-cold neutron depolarization probability per one collision with the walls.     

Nonparaxial propagation of linearly polarized modified Bessel–Gaussian beams and phase singularities of the electromagnetic field components

Based on an operator transformation technique and the nonparaxial propagation results of linearly polarized Gaussian beams, the nonparaxial propagation formulas of linearly polarized modified Bessel–Gaussian beams with optical vortices are constructed. Numerical investigations indicate that electromagnetic field components associated with the beams exhibit different phase singularities.     

Evolution of phase,texture, microstructure and magnetic properties of Fe–Cr–Co–Mo–Ti permanent magnets

Magnetic phase evolution, crystallographic texture, microstructure and magnetic properties of Fe–28Cr–15Co–3.5Mo–1.8Ti alloy have been investigated by X-ray diffractometry, scanning transmission electron microscopy and magnetometry techniques as a function of processing conditions. Heat treatment conditions for obtaining optimum textural, microstructural and magnetic properties have been established by the experimentations. The Goss {110}〈001〉 and cube type {001}〈010〉 textures have been developed in an optimal treated Fe–28Cr–15Co–3.5Mo–1.8Ti magnets. The coercive force in Fe–28Cr–15Co–3.5Mo–1.8Ti magnets depends critically on the shape anisotropy of rod-like Fe Co Ti-rich α₁ particles and remanence on the alignment and elongation of α₁ particles parallel to applied magnetic field 〈100〉 directions. The optimum magnetic properties obtained in Fe–28Cr–15Co–3.5Mo–1.8Ti alloy are intrinsic coercive force, _iH_c, of 78.8 kA/m (990 Oe), remanence, B_r of 1.12 T (11.2 kG) and energy product, (BH)_max of 52.5 kJ/m³ (6.5 MGOe). The development of Fe–28Cr–15Co–3.5Mo–1.8Ti magnets as well as characterization of texture, microstructural and magnetic properties in the current study would be helpful in designing the new Fe–Cr–Co–Mo based magnets suitable for scientific and technological applications.     

A thermoluminescence study of mineral silicates extracted from herbs in the dose range 0.5–5 Gy

The presence of silicates in many personal objects suggests their potential use at low dose as fortuitous dosimeter in an accidental radiological exposure, when conventional dosimetry is not available. The goal of the present work is the dosimetric characterization of mineral silicates extracted from the plant Hibiscus Sabdariffa L, known as Jamaica flower, in the dose range 0.5–5 Gy. By studying the radiation-induced signal in time, the temperature integration region between 210 °C and 250 °C was found to be the most stable and also reduced the effects of thermal fading in the dose reconstruction process; the dose response curve was linear between 0.5 Gy and 5 Gy. By checking the change in sensitivity after repeated exposures to ionizing radiations and to high temperature heating, no variation in the glow curve shape or peak intensities were detected. To eliminate a pre-existing background signal, all the characterization measurements were performed with aliquots “annealed” by a preliminary readout of the TL.     

Measurements of gas desorption from polyethylene-UHMWPE irradiated by 5 MeV electrons

Gas desorption in vacuum from electron irradiated ultra high molecular weight polyethylene (PE) is measured with a high sensible mass quadrupole spectrometer. Measurements are performed in thick PE irradiated with 5 MeV electron beams at doses of the order of tens of kGy. The irradiation modifies the PE molecules producing dehydrogenation, emission of different C _x –H _y groups, C-enrichment and carbon cross-linking processes. Results indicate that the radiation damage depends on the dose and that a significant change of chemical and physical polymer properties is reached for a critical dose of 18 kGy.     

Vapor–liquid–solid growth and Sb doping of Ge nanowires from a liquid Au-Sb-Ge ternary alloy

Single-crystalline Sb-doped Ge nanowires (NWs) with excellent structural properties and uniform composition have been synthesized with high yield by vapor–liquid–solid (VLS) growth by low-temperature thermal evaporation from a mixture of Ge and Sb powders. During deposition, both the Ge and the Sb dopant became incorporated in the VLS seed nanoparticle. In situ annealing experiments during transmission electron microscopy establish that a liquid ternary Au-Sb-Ge alloy constitutes the active phase of the VLS seed drop at high temperatures, which governs the growth of the one-dimensional Ge NW and its doping by Sb.     

Anisotropy of the solid–liquid interface properties of the Ni–Zr B33 phase from molecular dynamics simulation

Solid–liquid interface (SLI) properties of the Ni–Zr B33 phase were determined from molecular dynamics simulations. In order to perform these measurements, a new semi-empirical potential for Ni–Zr alloy was developed that well reproduces the material properties required to model SLIs in the Ni_50.0Zr_50.0 alloy. In particular, the developed potential is shown to provide that the solid phase emerging from the liquid Ni_50.0Zr_50.0 alloy is B33 (apart from a small fraction of point defects), in agreement with the experimental phase diagram. The SLI properties obtained using the developed potential exhibit an extraordinary degree of anisotropy. It is observed that anisotropies in both the interfacial free energy and mobility are an order of magnitude larger than those measured to date in any other metallic compound. Moreover, the [0 1 0] interface is shown to play a significant role in the observed anisotropy. Our data suggest that the [0 1 0] interface simultaneously corresponds to the lowest mobility, the lowest free energy and the highest stiffness of all inclinations in B33 Ni–Zr. This finding can be understood by taking into account a rather complicated crystal structure in this crystallographic direction.     

Impact of long-term relaxation on the phase composition of Pd–5.3 at % In–0.5 at % Ru alloy after hydrogenation

The structural state of a hydrogenated foil of Pd 5.3 at %–In 0.5 at % Ru alloy with a long relaxation time (55000 h) is studied via X-ray diffraction. Changes in the phase composition of the alloy during relaxation after hydrogen escapes from it are established. The quasi-stability of the distribution of the widths of areas of coherent scattering (ACS) is revealed by the concentration of indium atoms in directions ?100? and ?111?.