Neutron emission in interactions of 1H, 2H, 4He, and 12C nuclei with lead nuclei at 1–2 GeV per nucleon

The double differential cross sections for neutron production that were measured by the time-of-flight method for interactions of 2-GeV p and d, 4-GeV ⁴He, and 24-GeV ¹²C with Pb nuclei are discussed. In the phenomenological model of four moving sources, the neutron energy distribution shape at emission angles above 30° is well reproduced with the temperature parameters for all sources that are almost independent of the type and the energy of incident nuclei. Using the developed model, we estimate the mean neutron multiplicity and the energy removed by neutron emission.     

Neutron ambient dose equivalent from 5 MeV/u 10,11B, 12,13C and 16,18O projectiles incident on a thick Al target

The neutron ambient dose equivalent has been measured from ¹⁰B, ¹¹B, ¹²C, ¹³C, ¹⁶O and ¹⁸O projectiles of energy 5 MeV/amu incident on a thick Al target at 0°, 30°, 60° and 90° with respect to the beam direction using a conventional dose equivalent meter. The calculated results obtained using previously reported empirical relations do not reproduce the experimental data. The results obtained from the PACE nuclear reaction code are closer to the experimental data as compared to the various empirical expressions. The ratio of the increase in the dose rates when the projectile is changed from the lighter to the heavier isotopes is fairly reproduced by most of the empirical formulations and the PACE code. A previously reported relation for the slope parameter is used to predict the directional distribution of the neutron dose for the projectiles used in this study. The calculated doses are lower than the experimental results in the forward directions but agree within the uncertainties at the backward directions. A new set of projectile-based parameters have been derived from the present experimental data which can be used in an empirical formulation.     

Observation of the ABC effect in the reaction n+p → d+(mm)0 with A 1.88 GeV/c neutron beam

A significant production of the ABC effect is observed in the free nucleon reaction n+p → d+(mm)°, using a 1.88 GeV/c neutron beam. The complete deuterón momentum spectra produced in this inclusive experiment are measured at 0°, 4.5°, 7.5° and 10.5° (lab). The double differential cross sections $\text{d}{}^2\text{σ/}\text{d}\text{Ω}\text{d}\text{p}$, are compared with the predictions of two exchange models.     

7Li(α,n)10B differential cross-section measurements from threshold to Eα = 5.1 MeV

Differential cross sections for the ⁷Li(α, n)¹⁰B reaction have been measured at lab angles of 0°, 20°, 31°, 50°, 60°, 70°, 80°, 90°, 100° and 114° for α-particle energies between 4.385 and 5.1 MeV. A thick natural lithium target was bombarded with a 5.2 MeV, nanosecond-pulsed ⁴He⁺ beam and neutron velocity spectra at each angle were measured by time-of-flight techniques. These data have been converted to cross sections at 10 keV intervals in α-particle energy. Angular distributions have been fitted with a series of Legendre polynomials. Angle-integrated cross sections, the 0° excitation function, and angular distributions are compared to past measurements and R-matrix calculations.     

An experimental study on cross-section ratio of coherent to incoherent scattering for 145 keV incident gamma photons

The coherent (Rayleigh) to incoherent (Compton) scattering cross-section ratio of elements, in the range 6 ≤ Z ≤ 82, are determined experimentally for 145 keV incident gamma photons. An HPGe (High purity germanium) semiconductor detector is employed, at scattering angle of 50°, 70° and 90°, to record the spectra originating from interactions of incident gamma photons with the target under investigation. The intensity ratio of Rayleigh to Compton scattered peaks observed in the recorded spectra, and corrected for photo-peak efficiency of gamma detector and absorption of photons in the target and air, along with the other required parameters provides the differential cross-section ratio. The measured values of cross-section ratio are found to agree with theoretical predictions (corresponding to 4.939, 6.704 and 8.264 Å⁻¹ photon momentum transfer) based upon non-relativistic form factor, relativistic form factor, modified form factor and S-matrix theory.     

Thermoluminescence and optically stimulated luminescence characteristics of Al2O3 doped with Tb

In the present work policrystals of α − Al₂O₃ doped with terbium were synthesized using the solvent evaporation method. The samples were prepared using Al(NO₃)₃·9H₂O and Tb(NO₃)₃·5H₂O reagents, with Tb concentrations between 1 and 5 mol% and thermally treated at high temperature above ∼1400 °C. X-ray diffraction measurements showed the α-phase formation of samples. TL glow curve presented an intense peak at ∼190 °C and two other with low intensity at 290 and 350 °C after gamma irradiation. The best doping concentration which presented high luminescence was the sample doped with 3 mol% of Tb. TL spectra and fluorescence measurements showed similar luminescence spectra with lines attribute to Tb³⁺ ions. A linear behavior to gamma dose between 1 and 20 Gy was observed in TL, using 190 °C peak as well as in OSL signal, this last carried out using 532 nm wavelength stimulation.     

The polarization and differential cross section of fast neutrons scattered from 6Li and an R-function analysis of the interaction below 4 MeV

The analyzing power of ⁶Li for the elastic scattering of polarized neutrons with energies between 2 and 4 MeV, has been measured at six angles ranging from 25° to 150°. The polarized neutrons were generated from the reactions Pb(γ, n) and ¹²C(n, $\text{n}$), and their polarization was measured using the double-scattering method. The neutron energies were determined with a nanosecond timeof-flight spectrometer. In addition, the differential cross section was measured at three angles in the same energy range; the cross section was determined relative to the well-known n-¹²C cross section. The present results have been combined with existing data for the neutron total, (n, α), and differential elastic cross sections, in a reduced R-function analysis. Clear evidence of a p-wave triplet of shellmodel states emerges from the analysis.     

Small-angle neutron scattering investigation of the nanostructure of ferritic-martensitic 12%-chromium steels

The nanostructure (nanoparticle distribution) of ferritic-martensitic 12%-chromium steels EK-181 (Fe-12Cr-2W-V-Ta-B) and ChS-139 (Fe-12Cr-2W-V-Ta-B-Nb-Mo) subjected to different modes of mechanical and heat treatments and neutron irradiation has been investigated using small-angle neutron scattering. The samples have been studied in the initial state and after neutron irradiation (IVV-2M reactor) at a temperature of 80°C with fluences of 10¹⁸, 10¹⁹, and 5 × 10¹⁹ cm^?2 (E ≥ 0.1 MeV). The nanostructure of the steels is characterized by precipitations of nanoparticles with two characteristic sizes of 1.0–1.5 and 7–8 nm. The dependence of the nanostructure parameters on the composition of the steels and on the conditions of heat treatment and irradiation has been discussed.     

Messung der Neutronenpolarisation bei der Reaktion12C(d,n 0)13N mit Hilfe der Mott-Schwinger-Streuung

The polarization of neutrons produced in the reaction¹²C(d, n ⁰)¹³N was measured. Deuterons from the Karlsruhe isochronous cyclotron were used to induce this reaction at 51,5 MeV laboratory energy. The degree of polarization was determined by using the special features of Mott-Schwinger scattering. With an uranium scatterer analysing efficiencies of up to 0.92 can be obtained at very small angles (0.23°). The analysing efficiency can be calculated if the differential cross section at 0° and the total cross section is known. These quantities were experimentally determined. The differential cross section for 49.4 MeV neutrons, scattered by uranium, was measured between 0.88° and 2.10°. By an extrapolation the value 43.4±2.6 b/sr was found for the nuclear differential cross section at zero degree. A total cross section ofσ _t=4.80±0.22 b was obtained. The neutron polarization was measured at a reaction angle of 24.5° and the result isP=?0.45±0.07. This value is fairly above the semiclassical 1/3 limit and can be only explained, if spin orbit forces are taken into account. For (d, n) reactions this is the first neutron-polarization measurement above an energy of 20 MeV.     

Neutron induced light-ion production from iron and bismuth at 175 MeV

We have measured light-ion (p, d, t, ³He and α) production in the interaction of 175 MeV neutrons with iron and bismuth with low-energy thresholds and for a wide angular range (from 20° to 160°, in steps of 20°). Measurements have been performed with the Medley setup, semi-permanently installed at the The Svedberg Laboratory, Uppsala (Sweden), where a quasi-monoenergetic neutron beam is available and well characterized. Medley is a conventional spectrometer system and consists of eight telescopes, each of them composed of two silicon surface barrier detectors, to perform particle identification, and a CsI(Tl) scintillator to fully measure the kinetic energy of the produced light-ions. We report preliminary double-differential cross sections for production of protons, deuterons and tritons in comparison with model calculations using TALYS-1.0 code. These show better agreement for the production of protons, while the theoretical calculations seem to overestimate the experimental production of deuterons and tritons.     

Dosimetry and spectrometry at accelerator based neutron source for boron neutron capture therapy

An innovative accelerator-based neutron source for boron neutron capture therapy has started operation at the Budker Institute of Nuclear Physics, Novosibirsk. This facility is based on a compact vacuum insulation tandem accelerator designed to produce proton current up to 10 mA. Epithermal neutrons are proposed to be generated by 1.915 MeV protons bombarding a lithium target using ⁷Li(p,n)⁷Be threshold reaction.In the article, techniques to detect neutron and gamma-rays at the facility are described. Gamma radiation is measured with NaI and BGO gamma-spectrometers. The total yield of neutrons is determined by measuring the 477 keV γ-quanta from beryllium decay. For the rough analysis of the generated neutron spectrum we used bubble detectors. As the epithermal neutrons are of interest for neutron capture therapy the NaI detector is used as activation detector. We plan to use a time-of-flight technique for neutron spectra measurement. To realize this technique a new solution of short time neutron generation is proposed.     

The energy dependence of Delbrück scattering investigated at Z = 73, 82 and 92

Using neutron capture γ-rays from a ¹⁴⁰CeO₂ source installed in the Grenoble high-flux reactor, differential cross sections for the elastic scattering of photons by Ta, Pb and U through θ = 120° have been measured for E = 4.291 and 4.767 MeV. These data have been supplemented by measuring elastic differential cross sections for U, θ = 120° and energies ranging from 0.279 to 1.332 MeV, using radioactive sources. The experimental differential cross sections below 1 MeV confirm the predicted Rayleigh amplitudes based on the second-order S-matrix within 3%. An excellent agreement between experiment and lowest-order Delbrück theory is observed between 1.0 and 1.4 MeV, showing that Coulomb corrections are small close to the threshold for pair production. At 4.291 and 4.767 MeV experiment and lowest-order Delbrück theory agree within ~12%     

Neutron,photon and proton energy spectra at high altitude measured using a phoswich-type neutron detector

Neutron energy spectrum from 7 to 180 MeV, photon energy spectrum from 4 to 50 MeV and proton energy spectrum from 94 to 145 MeV were measured simultaneously using a phoswich-type neutron detector with particle discrimination methods at atmospheric depth of 249 g/cm², a vertical cut-off rigidity of 10.2 GV and at a heliocentric potential of 312 MV. We compared our results with other measured and calculated particle energy spectra. Our measured results give a large, sharp neutron peak around 70 MeV, although Bonner balls show a broad peak around 100 MeV due to low energy resolution. The measured photon and proton spectra are between the calculated energy spectra. This onboard study provides the first experimental neutron energy spectrum over 10 MeV with a high-energy resolution.     

Neutron fluence spectrometry using disk activation

A simple and robust detector for spectrometry of environmental neutrons has been developed. The technique is based on neutron activation of a series of different metal disks followed by low-level gamma-ray spectrometry of the activated disks and subsequent neutron spectrum unfolding. The technique is similar to foil activation but here the applied neutron fluence rates are much lower than usually in the case of foil activation. The detector has been tested in quasi mono-energetic neutron fields with fluence rates in the order of 1000–10000 cm⁻² s⁻¹, where the obtained spectra showed good agreement with spectra measured using a Bonner sphere spectrometer. The detector has also been tested using an AmBe source and at a neutron fluence rate of about 40 cm⁻² s⁻¹, again, a good agreement with the assumed spectrum was achieved.     

Polarization of recoil neutrons from single-pion photoproduction off protons in the resonance region

The polarization of the recoil neutrons from the reaction γp→π⁺n was measured at a c.m. angle of 105° for incident photon energies between 675 and 1125 MeV. A scattered π⁺ meson and a recoil neutron were detected in coincidence with a magnetic spectrometer and a neutron polarimeter system using liquid hydrogen. Results are compared with recent phenomenological analyses and the other existing data measured by the double polarization measurement technique.     

Photoionization studies of the atmospherically important species N and OH at the Elettra synchrotron radiation source

In this paper angularly resolved photoelectron spectra (PES) and constant-ionic-state (CIS) spectra are presented for the atmospherically important species N and OH.The natural width Γ, line shape parameters q and ρ² and discrete oscillator strengths f have been measured for the members of the N*[2s2p³(⁵S), np] (⁴P) ← N(⁴S) autoionizing resonances for n = 5–10. The n = 5 parameters calculated in this work are in good agreement with the values obtained previously whereas for the resonances with n = 6–10 the values of these parameters are reported for the first time. The asymmetry parameter (β) for the first band of N atoms, the N⁺(³P) ← N(⁴S) ionization, has also been measured in the photon energy range of the above autoionizing resonances.For OH, CIS spectra have been recorded for the first photoelectron band corresponding to the ionization OH⁺(X³Σ⁻, v⁺ = 0) ← OH(X²Π, v″ = 0). In these spectra, rotationally partially resolved bands associated with OH*(a¹Δ3d, v′ = 0) ← OH(X²Π, v″ = 0) resonances have been observed. Suggestions for their assignment are made on the basis of their positions and band simulations which use rotational line strength calculations.     

Protonic conductivity of β″ and ion-rich β-alumina. II: Ammonium compounds

The conductivity and thermal stability of NH⁺₄, H⁺(H₂O)_nβ″ and ion-rich β-alumina single crystals have been measured by the complex impedance method in the 25–700°C temperature range. Both structures have similar properties, but ion-rich β-alumina shows a higher stability and a lower activation energy (β: 0.18 eV, β″ 0.24 eV below 400°C and 250°C respectively). The room temperature conductivity is about 3×10^-5ω^-1cm^-1. The conducting properties and mechanisms are discussed and compared to other protonic or ionic conductors.     

The 10,11B(n, p)10,11Be reactions at En=96 MeV

Double-differential cross sections of the ^10,11B(n, p)^10,11Be reactions have been measured at 96 MeV in the angular range 0°–30° for excitation energies up to 35 MeV. The spectra have been decomposed into different multipolarities using sample angular distributions calculated within the distorted-wave Born approximation. From the identified Gamow–Teller strength, S_β⁺ values were obtained for ¹⁰B and ¹¹B. At higher excitation energies, the spectra are dominated by L=1 strength in broad distributions with maxima around 22 and 12 MeV in ¹⁰B and ¹¹B, respectively.     

The simulated workplace field with a high-energy neutron component produced by irradiating a Fe-target with 200 MeV/u 12C-ions

Recent developments in accelerator physics have led to new challenges for radiation protection dosimetry. Doses have to be determined for workplace fields which are characterized by high-energy radiation, a dominant contribution from neutrons, high intensities and pulsed time structure This may present problems for active measuring devices. As is well known, the ambient dose equivalent is often underestimated by area monitors operating in high-energy neutron fields behind shielding. Therefore, it is desirable to calibrate survey monitors in a characterized neutron field with the type of spectral fluence distribution that is expected behind shielding, i.e. where the main dose from neutrons arises from two peaks with mean energies of about 1 MeV and 100 MeV, respectively. Such a neutron fluence distribution is produced by the irradiation of a Fe-target with 200 MeV/u ¹²C-ions. Measurements with the extended range Bonner sphere spectrometer NEMUS of PTB were performed at two positions inside the experimental area Cave A of the heavy-ion synchrotron SIS at GSI. The measured neutron spectra show different fluence contributions for the two peaks at the two positions. The results were compared to Monte Carlo Simulations with MCNPX and FLUKA.     

Inclusive neutron and proton energy spectra following the negative pion absorption at rest in 12C

The results of a measurement of the inclusive energy spectra of the neutrons and protons emitted following the absorption at rest of negative pions on ¹²C are presented. The spectra have been measured with the time-of-flight method with an overall resolution of 650 psec. From the neutron spectrum the rate of 1.7 × 10^?2 neutrons per stopped pion has been deduced for the single-neutron emission reaction ¹²C(π^?, n)¹¹ B. Comparisons are made with calculated spectra and other experimental spectra.