Measurement of multi-exponential optical decay processes by?phase-shift cavity ring-down

Multi-exponential decay waveforms are common occurrences in cavity ring-down spectroscopy and the respective ring-down times are typically obtained by fitting the ring-down waveform to the sum of exponential decay functions. In phase-shift cavity ring-down (CRD) spectroscopy the measurement of a single phase angle will not provide sufficient information and needs to be complemented by either intensity measurements or phase angle measurements at different modulation frequencies. Here, a formalism analogous to that developed for fluorescence lifetime spectroscopy is adapted to the phase-shift CRD technique and is tested for two types of waveguide CRD systems: (1) a single-mode fiber cavity in which light is confined by two identical Fiber Bragg Gratings and (2) a multimode fiber loop. By measuring the phase angle at different modulation frequencies, lifetimes for up to three different decay processes were obtained.     

Passive mode-locking in diode-pumped c-cut Nd:LuVO<Subscript>4</Subscript> laser with a semiconductor saturable-absorber mirror

We demonstrated a diode-pumped passively mode-locked c-cut Nd:LuVO₄ picosecond laser with a semiconductor saturable-absorber mirror (SESAM) at a wavelength of 1067.8 nm. Due to the wide bandwidth of 0.48 nm, stable mode-locking has been generated with a duration as short as 3.7 ps, which is shorter than for the a-cut Nd:LuVO₄ laser. A maximum output power of 1.67 W was achieved to give a highest peak power of 3.47 KW at 18 W absorbed pump power.     

Direct observation of the anomalous zeeman effect at the X → B transition of molecular iodine by the method of nonlinear laser spectroscopy

Direct observation of the magnetic structure of transitions in molecular iodine is first reported. Using the method of saturated absorption spectroscopy in an external cell with I₂ vapour located in a longitudinal magnetic field we resolved the magnetic structure of the components of the hyperfine structure of the transition

120 W high repetition rate Nd:YVO<Subscript>4</Subscript> MOPA laser with a Nd:YAG cavity-dumped seed laser

A master oscillator power amplifier (MOPA) system in which the output from an end-pumped Nd:YAG oscillator cavity dumped at 500 kHz is scaled up by a four-stage Nd:YVO₄ amplifier is reported. Decrease in extraction efficiency of the amplifier chain with crystals different from that in the oscillator was analyzed. With the 5.4 W seed output, 118 W of power was extracted from the amplifier chain at the pump power of 345 W, with an extraction efficiency of 34.2% and an overall optical–optical efficiency of 30.9% for the MOPA system. The beam quality factors were measured as M _x ²=1.45 and M _y ²=1.59 in two orthogonal directions, respectively.     

Modelocked quantum dot vertical external cavity surface emitting laser

We report the first successful modelocking of a vertical external cavity surface emitting laser (VECSEL) with a quantum dot (QD) gain region. The VECSEL has a total of 35 QD-layers with an emission wavelength of about 1060 nm. In SESAM modelocked operation, we obtain an average output power of 27.4 mW with 18-ps pulses at a repetition rate of 2.57 GHz. This QD-VECSEL is used as-grown on a 450 μm thick substrate, which limits the average output power.     

Multi-point abnormal-temperature warning sensor system with?different thresholds

We propose and experimentally demonstrate a time-division-multiplexing-based (TDM-based) multi-point abnormal-temperature warning sensor system with different thresholds. A multi-channel fiber Bragg grating (FBG) serving as the wavelength selector is employed in the fiber ring laser to generate a multi-wavelength pulsed light source. The sensor array is composed of multiple uniform sensing FBGs at different positions and with different nominal wavelengths. The warning signal is obtained by only monitoring the time slot between the injected pulse and the reflected pulse. The measurement range and resolution are theoretically discussed and experimentally demonstrated.     

Kinetic temperature and electron density measurement in?an?inductively coupled plasma torch using degenerate four-wave mixing

Laser wave mixing is presented as an effective technique for spatially resolved kinetic temperature measurements in an atmospheric-pressure radio-frequency inductively coupled plasma. Measurements are performed in a 1 kW, 27 MHz radio-frequency plasma using a continuous-wave, tunable 811.5 nm diode laser to excite the 4s³P₂→4p³D₃ argon transition. Kinetic temperature measurements are made at five radial steps from the center of the torch and at four different torch heights. The kinetic temperature is determined by measuring simultaneously the line shape of the sub-Doppler backward phase-conjugate degenerate four-wave mixing and the Doppler broadened forward-scattering degenerate four-wave mixing. The temperature measurements result in a range of 3,500 to 14,000±150 K. Electron densities measured range from 6.1 (±0.3)×10¹⁵ cm⁻³ to 10.1 (±0.3)×10¹⁵ cm⁻³. The experimental spectra are analyzed using a perturbative treatment of the backward phase-conjugate and forward-geometry wave-mixing theory. The Stark width is determined from the collisional broadening measured in the phase-conjugate geometry. Electron density measurements are made based on the Stark width. The kinetic temperature of the plasma was found to be more than halved by adding deionized water through the nebulizer.     

Wavelength-independent all-optical synchronization of a Q-switched 100-ps microchip laser to a femtosecond laser reference source

We present a Q-switched microchip laser emitting 1064-nm pulses as short as 100 ps synchronized to a cavity dumped femtosecond laser emitting 800-nm pulses as short as 80 fs. The synchronization is achieved by presaturating the saturable absorber of the microchip laser with femtosecond pulses even though both lasers emit at widely separated wavelengths. The mean timing jitter is 40 ps and thus considerably shorter than the pulse duration of the microchip laser.     

Self-trapping of weak optical beams in photorefractive materials

Intensity-independent self-trapping of optical beams in photorefractive crystals was found recently. But we show that due to the existence of dark conductivity in some photorefractive materials or coherent and non-coherent background irradiance, the self-trapping of weak optical beams in photorefractive materials, such as SBN, becomes intensity dependent. The threshold condition of the applied external de electric field for self-trapping is determined as function of the material parameters as well as the initial transverse sizes and relative intensities of the beams.     

Gain versus tuning issues to Q-switch with Yb<Superscript>3+</Superscript>:LSO and amplify broad-bandwidth pulses

We report on the development of Incoherent Broadband Cavity Enhanced Absorption Spectroscopy (IBBCEAS) using a blue light emitting diode (LED) for the detection of NO₂ in laboratory ambient air. Absorption of the oxygen collisional pair in the atmosphere was also detected in the same spectral range. The mirror reflectivity was determined using a standard gas sample mixture of NO₂, and calibrated with the help of the absorption spectrum of the oxygen collisional pair in pure oxygen at atmospheric pressure. Optimization of the experimental parameters was investigated and is discussed in detail. For the first time in IBBCEAS involving broadband absorption spectra, averaging time for signal-to-noise ratio enhancement has been optimized using Allan variance plot. 18.1 ppbv NO₂ in laboratory ambient air has been retrieved from the absorption spectra using differential fitting method over a 40 nm spectral region centered at 470 nm. A minimum detection sensitivity of about 2.2 ppbv (1σ) for NO₂ at atmospheric pressure has been achieved using the optimal averaging time of 100 s by means of a high finesse optical cavity formed with two moderate reflectivity (∼99.55%) mirrors. No purging of the cavity mirrors by high purity He or N₂ gas streams was necessary to prevent contamination of the mirror faces for the in situ measurements.     

Post-growth tailoring of quantum-dot saturable absorber mirrors by chemical etching

We have designed and grown a resonant, low-finesse quantum-dot saturable absorber mirror and subsequently modified the important parameters using chemical etching. The modulation depth and saturation fluence at the design wavelength of 1064 nm were modified by etching the sample to tune the cavity resonance. The device properties were characterised using normal incidence spectroscopic reflectivity measurements, intensity dependent reflectivity measurements and modelled using a transfer matrix approach. The saturable absorber mirror was used to facilitate self-starting, passively mode locked pulses in a neodymium vanadate laser operating at 1064 nm. The etching was found to affect the duration of the pulses, leading to temporal width tuning over a range of 94 ps. The shortest pulse duration of 84 ps was achieved for the cavity resonance close to 1064 nm, with an output power of 3 W. This method is an effective technique for post-growth engineering of the properties of semiconductor saturable absorber mirrors (SESAMs) with nanometre precision.     

Fast algorithms for ring recognition and electron identification in the CBM RICH detector

The algorithm for recognition of Cherenkov radiation rings based on the Hough Transform Method (HTM), as well as the innovations which allow one to considerably speed up the HTM algorithm, are described. An ellipse-fitting algorithm has been elaborated, because most of the CBM RICH rings have elliptic shapes; moreover, it helps improve the ring-track matching and electron identification procedures. An elaborated procedure of the radius correction is also presented. A detailed study of the procedure of fake ring elimination by artificial neural networks is given. The results of the primary electron identification are presented. All developed algorithms were tested on large statistics of simulated events and are included into the CBM software framework for common use.     

Scanning the laser beam for ultrafast pulse laser cleaning of paint

Aligned arrays of N₂-encapsulated multilevel branched carbon nanotubes were synthesized using a simple one step CVD method by pyrolysis of ferrocene and acetonitrile. Electron energy loss spectroscopy (EELS) and elemental mapping studies reveal that gaseous nitrogen was encapsulated in the carbon nanotubes. Batch-type pyrolysis of catalysts induced flow fluctuation of the reaction gases, resulting in the growth of branched junctions. Molecular nitrogen extruded rapidly along conical catalyst particles inducing N₂ encapsulation inside the branched nanotubes. PACS 07.78.+s; 61.46.+w; 81.07.De; 81.15.Gh     

Mode-locked diode-pumped vanadate lasers operated with PbS quantum dots

The use of glasses doped with PbS nanocrystals as intracavity saturable absorbers for passive Q-switching and mode locking of c-cut Nd:Gd_0.7Y_0.3VO₄, Nd:YVO₄, and Nd:GdVO₄ lasers is investigated. Q-switching yields pulses as short as 35 ns with an average output power of 435 mW at a repetition rate of 6–12 kHz at a pump power of 5–6 W. Mode locking through a combination of PbS nanocrystals and a Kerr lens results in 1.4 ps long pulses with an average output power of 255 mW at a repetition rate of 100 MHz.     

A linear optical method for measuring the carrier-envelope phase drift

The carrier-envelope offset frequency of a laser oscillator is determined from the visibility of spectrally resolved fringes in a combined two-path multiple-path interferometer. At maximum visibility the pulses have zero carrier-envelope phase drift, while the visibility becomes zero for uncorrelated pulses. The method is widely independent of bandwidth and pulse energy. The effects of carrier-envelope offset phase noise, finite detection time, and dispersion are also discussed. M. G?rbe and C. Grebing have equally contributed to this paper.     

Diode-pumped passively mode-locked Nd:CTGG disordered crystal laser

A diode-pumped passively mode-locked Nd: CTGG disordered crystal laser has been experimentally demonstrated for the first time to our knowledge. Mode locked with a semiconductor saturable absorber mirror, the laser generated 5.2 ps pulses at a repetition rate of 88 MHz. After intracavity dispersion compensation, the mode-locked pulses were shortened to 4.3 ps. Multiple emission wavelengths of the Nd:CTGG laser could be synchronously mode locked under dispersion compensation.     

Diode end pumped Nd:YAG laser at 946 nm with high pulse energy limited by thermal lensing

Diode lasers with peak powers in the kW range and pulse durations of micro- to milli-seconds have been available since several years. Pumping solid state lasers with such sources yield high output pulse energies in spiking or Q-switched operation. The output energy is limited by the thermal lens effects, which are measured and calculated. The time dependent heat conduction equation in the laser crystal is solved numerically to predict the overall temperature rise and thermal lensing. The thermally induced optical path difference is approximated by a quadratic distribution to obtain the focal length f of the thermal lens. The thermal lens coefficient K=1/(f⋅P _av), which depends only weakly on the heat transfer coefficient H of the laser crystal to the heat sink, decreases exponentially with increasing pump frequency until the steady state is reached. Experiments were done with a Nd:YAG crystal at different pump frequencies up to 100 Hz. The thermal lens coefficients obtained by the power maxima of asymmetric flat-flat resonators agree with our calculations.     

Ultrafast dynamic ellipsometry measurements of early time laser ablation of titanium thin films

The dynamics of laser ablated titanium thin films are investigated using a recently developed technique that measures time-resolved and one-dimensional spatially-resolved ablation dynamics in a single shot. Ultrafast dynamic ellipsometry, a technique based on space-shifted spectral interferometry, uses the time-dependent frequency of a chirped laser pulse to provide time encoding, allowing the picosecond probing of material dynamics in a single shot. With this technique, the sample is probed at two different incident angles with both s- and p-polarized light, which measures the motion of the material and any change in its complex refractive index. Ultrafast dynamic ellipsometry is applied to study the mechanism of initiation by laser-based optical detonators that employ the ablation of titanium thin films. The resulting data indicate that the titanium is ablated as a fragmented flyer and not as an expanding plasma.     

Sub-90 fs pulses from a passively mode-locked Yb:YAl<Subscript>3</Subscript>(BO<Subscript>3</Subscript>)<Subscript>4</Subscript> laser

Passive mode locking of the self-frequency doubling Yb:YAB crystal with a saturable absorber mirror is studied at the fundamental wavelength. This laser has a very low threshold, and pulses as short as 85 and 87 fs are obtained for Ti:sapphire and diode laser pumping, respectively.