Energy levels of Tm

Fifty-one levels in Tm¹⁶⁸ have been observed up to an excitation energy of 1514 keV utilizing 12-MeV deuterons and the reaction Tm¹⁶⁹(d, t)Tm¹⁶⁸. The Q value of the lowest observed state was determined to be −1776 ± 15 keV. The spectrum below 700 keV has been interpreted in terms of the coupling of the [411↓] Nilsson proton orbital with the neutron orbitals prominent in the low-energy (d, t) spectrum of Er¹⁶⁷. This interpretation has resulted in the determination of relative energies due to the residual neutron-proton interaction for six different configurations. The observed singlet-triplet splitting energies for the [633↑], [521↓], and [512↑] neutron orbitals coupled to the [411↓] proton orbital were measured to be −157, +191, and −234 keV, respectively. Theoretical calculations of these energies made for a zero range spin-dependent central potential gave values of −87, +154, and −255 keV, respectively. The good agreement indicates that the spin-spin interaction can account for most of the singlet-triplet splitting energy.     

New157Lu isomer

The new low spin isomeric state of¹⁵⁷Lu (probably s_1/2) with T_1/2=9.6(8) s and E_±=4925(5) keV was found in experiments on YASNAPP-2 ISOL facility. The previously known isomer of¹⁵⁷Lu (T_1/2=4.75(10) s,_±=4998(5) keV) lies 32(2) keV higher than the new one.On leave from the M. Curie-Sklodowska University, Lublin, Poland     

The decays of 21.55 min 162gTm and 24.3 s 162Tm (a new isomer)

The decay of the 21.55 min ground state and of the 24.3 s isomeric state of ¹⁶²Tm was investigated with semiconductor detectors. The γ-ray spectrum was investigated with a Compton-suppression Ge(Li)-NaI(Tl) arrangement. A Si (Li) detector, mounted in an electron transport solenoid, was used to investigate the conversion electron spectrum. Three-dimensional coincidence measurements were performed with large-volume Ge(Li) detectors. The ¹⁶²Tm ground state has spin-parity 1^? and Nilsson assignment p[411]↓?n[521]↑. An allowed β-transition (log ft ≈ 6.4) was observed to a 2^?, 2 octupole vibrational level at 1572.84 keV. The Q-value determined from positon-gamma coincidence measurements is 4705 ± 70keV. The discrepancy of the experimental K /β⁺ ratio with theoretical predictions might possibly be explained by a large number of unobserved weak γ-rays besides the total of 315 stronger ones observed in this study. The average β-strength function was calculated to be 1.2 × 10^?5. Among the 50 levels observed in the decay, the 2⁺, 4⁺ and 6⁺ members of the ground-state band, the 2⁺, 3⁺ and 4⁺ members of the γ-band, several 0⁺ and 2⁺ members of the K = 0 β-bands and 1^?, 2^? and 3^? octupole vibrational levels were identified. Parameter values Z_γ(0) and Z_γ(2) determining the mixing between the γ-band and the ground-state band, allow no conclusive evidence about unequalness of the intrinsic quadrupole moments of the ground states and the γ-band. The Z(0) parameters, determining the mixing between the β-bands and the ground-state band, and X parameters determining the ratio of E0 to E2 transition probabilities, were deduced. A previously unreported 24.3 sec isomer in ¹⁶²Tm was observed to decay in 10% of the cases by an allowed unhindered (log ft = 4.7) β-ray transition to a level at 1712.20 keV in ¹⁶²Er. The Nilsson configurations assigned to the isomeric and 1712.20 keV levels are p[523]↑ + n[521]↑₅₊ and n[523]↓ + n[521]↑₄₊ respectively. The isomeric level decays in 90% of the cases by an E3 transition (E_IT < 125 keV) to a p[404]↓ ?n[521]↑_2? level at 66.90 keV in ¹⁶²Tm, which decays by an (M1+ < 40 % E2) to the 21.55 min ¹⁶²Tm 1^? ground state.     

The decay of 1.4 min173Er

A 1.4 ± 0.1 min activity which is assigned to β^?-decay of ₆₈ ¹⁷³ Er has been produced with 14–15 MeV neutrons through the reaction¹⁷⁶Yb(n, α)¹⁷³Er. Its decay has been studied with Ge(Li) detectors and several (γ)(γ) as well as (γ)(β) coincidence arrangements. Eight gamma rays with energies 94.2, 116.14, 118.6, 122.40, 192.8, 199.2, 800.8 and 895.2 keV were assigned to the decay of¹⁷³Er. The proposed level scheme of the daughter nuclide ₆₉ ¹⁷³ Tm contains levels at 0, 2.5, 118.6, 124.9, 317.7, 411.9 and 1212.8 keV. The 317.7 keV level is an isomeric state with a measured half-life of 10±3 μs. This 10 μs isomer and the 411.9 keV level are thought to be the band head and 9/2^? rotational member of 7/2^? [523] Nilsson state, respectively. The levels at 0, 2.5, 118.6 and 124.9 keV are interpreted as 1/2⁺, 3/2⁺, 5/2⁺ and 7/2⁺ members of the 1/2⁺ [411] band and the level at 1212.8 keV as the 9/2^? [514] Nilsson state. Some systematic considerations and theoretical transition probability calculations are also included.     

In-beam study of174Lu isomers

Levels in¹⁷⁴Lu have been investigated using the¹⁷⁶Yb(p,3n) reaction. Prompt and delayedγ-ray spectra have been observed with a 0.56-cm³ Ge(Li) detector by a multispectrum analysis method. The half-life and decay mode of two isomeric levels, one at 240.8keV (395±15ns) and the other at 365.1keV (145±3ns) have been firmly established. Hindrance factors are discussed. New delayed transitions in¹⁷⁵Lu are also noted.     

High-spin states in odd-odd 168Lu

High-spin states of odd-odd ¹⁶⁸Lu were observed up to 18ħ for the first time using the ¹⁵⁹Tb(¹³C, 4nγ)¹⁶⁸Lu reaction at E _13C= 58.5 MeV. γ-γ coincidence, E _γ singles, excitation function, and the DCO ratios were measured. Two rotational bands with signature splitting were populated, among which the lower-energy band is identified as π 7/2⁺[404] ⊗ν 5/2⁺[642] in view of alignment and energy systematics. Received: 27 October 1997     

The hyperfine magnetic field of172Yb in Fe and Ni

Time-differential perturbed angular correlation measurements have been performed on the 91–1095 keV -ray cascade emitted by¹⁷²Yb nuclei in the capture decay of¹⁷²Lu, using implanted sources of¹⁷²Lu in Fe and Ni. From these measurements hyperfine field valuesB(YbFe)=–1253±83 kG andB(YbNi)=–143±12 kG follow at room temperature. From the modulation amplitude of the spectra it follows that only about 20% of the ytterbium nuclei participate in the precession.     

The160Tb →160Dy decay

Gamma-ray spectra in the decay of¹⁶⁰Tb were measured with the aid of two coaxial Ge(Li) spectrometers. Absolute intensities and multipolarities were obtained. Three new transitions of 486·5 keV, 1069 keV, and 1102·5 keV were found and introduced into the decay scheme. The level scheme is discussed from the point of view of the generalized model of the nucleus. Experimental data show the 1264·4 keV level to be a two-quasi-particle state of the p p (411–523) type. The beta-transition from the ground state of¹⁶⁰Tb (p 411+n 521) to this two-quasi-particle state with logft=8·00 ± 0·05 is interpreted as -forbidden.The authors are indebted to Prof. K. E. Alexandrov, K. A. Gromov, and E. P. Grigoriev for useful remarks and interest concerning the work.     

Niederenergetische Gammalinien vom Neutroneneinfang in Lu 175 und Lu 176

The low energy gamma-rays from neutron-capture in Lu 175 and Lu 176 have been investigated by means of the bent crystal-spectrometer at the DR-3-reactor at Risø. From the transitions in Lu 177 3 rotational bands have been determined. The levels of the (404)K=7/2⁺ groundstate rotational band are: 121,62 keV (I=9/2), 268,79keV (I=11/2), 440,66 keV (I=13/2), 636,22 keV (I=15/2), 854,34 keV (I=17/2). The level-sequence of the (514)K=9/2^?-band is: 150,39 keV (I=9/2), 288,99 keV (I=11/2), 451,49 keV (I=13/2), 637,05 keV (I=15/2) and 844,88 keV (I=17/2). At 457,92 keV is the basis for the (402)K=5/2⁺-band the higher levels of which are 552,05 keV (I=7/2), 671,89 keV (I=9/2), 816,63 keV (I=11/2), 985,23 keV (I=13/2), 1176,73keV (I=15/2) and probably 1389,5 keV (I=17/2). The energies of the levels apart from the 1389 keV-level have an accuracy of 7×10^?5. The energy differences between the 3 bands agree very well with the values expected from the Bohr-Mottelson-formulaE=A·I(I+1)+B·I ²(I+1)². The calculated branching-ratios within the 3 bands are in fairly good agreement with the experimental values. Theg _K -factors have been determined for 2 bands: It was found that for the (514)-bandg _K =1,16±0,04 and for the (402)-bandg _K =1,33±0,07.     

Messung des Elektroneneinfangs am Kern176m Lu

The electron capture of^176m Lu to the ground state and to the first excited state of¹⁷⁶Yb has been observed by measuring the YbK x-rays and the 82,2 keV gamma-rays from the gamma decay of the first excited state in¹⁷⁶Yb. With the data of the 88,36 keV gammarays following the beta decay of^176m Lu to the first excited state of¹⁷⁶Hf the electron capture/beta decay ratio of^176m Lu was found to be (0,95±0,16)·10^?4. The electron capture branching ratio to the ground state and to the first excited state of¹⁷⁶Yb was found to be 40/60±30%. By analyzing the 88,36keV gamma-rays and the HfKx-rays the halflife of^176m Lu was evaluated to be 3,66±0,04 h. The value for theK-conversion coefficient of the 88,36keV transition was determined from the x-ray/gamma-ray ratio to be 1,19±0,09.     

Der Zerfall der Cäsiumisotope Cs129 und Cs130

Cs¹²⁹(T_1/2=32 h) and Cs¹³⁰(T_1/2=30 min) were produced by J¹²⁷(α,2n)Cs¹²⁹and J¹²⁷(α,n)Cs¹³⁰reactions, respectively. The γ-ray-spectra from the decays of Cs¹²⁹ and Cs¹³⁰ have been investigated using Li-drifted Ge-counters and scintillation spectrometers. In the decay of Cs¹²⁹15 γ-rays have been observed having the following energies and relative intensities: 95 keV (1.6), 177 keV (1.1), 267 keV (1.7), 278 keV (4.8), 317 keV (7.6), 371 keV (100), 410 keV (69), 511 keV (≦ 0.1), 548 keV (10.5), 587 keV (1.7), 623 keV (0.12), 660 keV (0.07), 864 keV (0.09), 907 keV (0.67) and 948 keV (0.2). The electron capture branching ratios to the ground state and excited states of Xe¹²⁹were determined; logft values for the various decay branches were derived from these ratios. In the decay of Cs¹³⁰twoγ-transitions with the following energies and intensities relative to the β⁺ emission have been found: 535 keV (11) and 585 keV (1.3). A new level at 1122 keV in Xe¹³⁰is proposed.     

The decay of Ag

The γ-radiation following the decay of ¹¹²Ag has been studied with a Ge(Li) detector. A total of 76 γ-rays was observed. The γ-γ coincidence and angular correlation relations involving the 617 keV 2⁺-0⁺ transition have been measured using Ge(Li)-NaI(Tl) and NaI(Tl)-NaI(Tl) detectors. These results have been used to confirm spins and parities of some levels of ¹¹²Cd in the proposed decay scheme. Cross sections for ¹¹²Ag production by ¹¹⁵In(n,α) and ¹¹²Cd(n, p) reactions have been measured; the ¹¹²Ag half-life has been determined as 3.14 ± 0.02 h.     

Beta-delayed proton emission from heavy nuclei: (I). The observation of coincidences between protons and γ-rays

Coincidences have been detected between γ-rays and β-delayed protons emitted after the decay of very neutron-deficient nuclei. In the three cases studied the decay proceeds to the ground state with branches to the first excited (2⁺) state of the even daughter nucleus of (58±7) % (¹¹⁵Xe to 709 keV in ¹¹⁴Te), (14±3) % (¹¹⁷Xe to 679 keV in ¹¹⁶Te), and (50±10) % (¹⁸¹Hg to 158 keV in ¹⁸⁰Pt). Upper limits of 2 and 6 % can be placed on the branches to the 4⁺ states of ¹¹⁴Te and ¹⁸⁰Pt. For the cases of ^115,117Xe, coincidences with annihilation radiation were also observed; the measured positon/proton ratio determines the difference Q—B_p, between the energy available for electron capture and the proton separation energy for the daughter. For ¹¹⁵Xe the result is 6.20±0.13 MeV, for ¹¹⁷Xe 4.10±0.20 MeV.     

Study of the 176Lu(n, γ)177Lu reaction using a gamma band-filter spectrometer

The γ-ray spectrum from the ¹⁷⁶Lu(n, γ)¹⁷⁷Lu reaction has been investigated in the energy range 450 to 1420 keV using a newly developed gamma band-filter spectrometer. A total of 153 transitions have been observed. Improvements to the ¹⁷⁷Lu scheme are suggested, and in particular the γ-decay of several levels of the $\text{1}\text{2}$^?[530↑] and $\text{3}\text{2}$^?[532↓] rotational bands is proposed. Special attention has been given to the Coriolis coupling between the two latter bands and the $\text{1}\text{2}$^?[541↓] band. Results on a complementary investigation of the ¹⁷⁵Lu(n, γ)¹⁷⁶Lu reaction are presented.     

The decay of 4 min 158Tm

The decay of 4 min ¹⁵⁸Tm has been investigated with on-line mass-separated samples obtained from the Orsay ISOCELE separator. Measurements of γ-rays, conversion electron lines and γ-γ bi-dimensional coincidences were performed. About 180 transitions were ascribed to the decay and two thirds of them were placed in a decay scheme. The β-band and the γ-band were identified with bandheads situated at 806.40 and 820.13 keV respectively. In addition, a number of other vibrational bands (β-γ, β-β, K^π = 0^? and 1^?) are proposed. The decay properties of those bands are discussed in the framework of current nuclear models. The log ft values suggest a 2^? assignment for ¹⁵⁸Tm with the possible configuration (p404J↓-n521↑).     

Levels in160Yb from the radioactive decay of160Lu

Theγ-rays following the radioactive decay of¹⁶⁰Lu into¹⁶⁰Yb have been studied. The Lu source was produced in the¹⁴⁴Sm(¹⁹F, 3n) reaction at 85 MeV. Excitation functions, half-lives,γ-γ andγ-X-ray coincidences and conversion electrons were measured. Twoβ ⁺ decaying states in¹⁶⁰Lu were found with half-lives of 36.2(3) s and 40(1) s.¹⁶⁰Yb levels deduced from the decay of¹⁶⁰Lu are presented.     

Multipole mixing ratios of transitions in168Er

Time-integral and time-differentialγ-γ directional correlation measurements were performed for cascades in¹⁶⁸Er populated from the electron-capture decay of¹⁶⁸Tm(87d). The¹⁶⁸Tm source was dissolved in HF acid to minimize extranuclear perturbations. The results of the time-differential experiment for the 448-99.3 keV and 448-198 keV cascades showed agreement with time dependent interaction and gaveλ ₂(1094)=(0.79±0.09) ×10⁷ sec^?1. The attenuation factors for the 80 keV level were determined asG ₂₂ (80)=0.90±0.01 and G₄₄(80)=0.94±0.01. OnlyI=4 spin value for the 1094 keV level is consistent with our measurements. The 632, 731, 741, and 816 keV transitions connecting theK=2⁺ andK = 0⁺ rotational bands were found to be of almost pureE2 character. The 99.3, 198, 547, 720, 830, and 1277 keV transitions are of practically pureE1 multipolarity. The 448 keVMl transition has (0.8 _?0.4 ^+2.0 )%E2 admixture. The results for the 1014?80keV cascade give (23±4)%E3 component in the 1014 keV transition.     

The decay schemes of Y and Y and γ-rays observed in the decay of Y

Active yttrium was separated from ²³⁵U fission products and the decay of ⁹⁴Y, ⁹⁵Y and ⁹⁶Y to the levels of ⁹⁴Zr, ⁹⁵Zr and ⁹⁶Zr, respectively, has been studied with the aid of a 17 cm³ Ge(Li) detector. Gamma-ray energies and intensities were accurately determined. In the decay of ⁹⁴Y four new transitions at 1232.78 ± 0.35, 1324.97 ± 0.35, 1363.48 ± 0.35 and 2467.00 ± 2.75 keV were observed. The data obtained support the level scheme proposed for ⁹⁴Zr by Knight et al. and that deduced from more recent reaction data. Evidence supporting the location of the 0⁺ excited state at 1300 keV is presented. Branching ratios are calculated and a modified level scheme for ⁹⁴Zr is proposed. In the decay of ⁹⁵Y the energies of 13 γ-rays, previously identified with the decay of this nuclide, have been accurately measured and are presented in a partial level scheme for ⁹⁵Zr. The data obtained in this work support the level structure deduced from reaction data by Cohen and Chubinsky and by other workers. New γ-transitions at 550.10 ± 0.23, 1723.30 ± 0.90 and 1805.0 ± 1.0 keV were measured in the decay of ⁹⁶Y.     

Evidence for dipole-quadrupole-octupole mixing in the 902 keV 2 → 2 transition in W

From known conversion coefficients and angular correlations combined with the γ-ray decay deduced from the ¹⁸¹Ta(p, 2n¹⁸⁰W reaction it is found that the 1007 → 104 keV (2⁻ → 2⁺) transition in ¹⁸⁰W has mixing parameters δ₁ = −0.16 ± 0.07 and δ₂ = −0.64 ± 0.17 for M2/E1 and E3/E1, respectively