The 198Au βhalf-life in the metal Au⋆

For the β^--decay of ¹⁹⁸Au in a Au metallic environment the half-life was observed to be longer by 0.4±0.7% at room temperature (T = 293K) and by 4.0±0.7% when the metal was cooled to T = 12K, both compared to the literature value of T _1/2 = 2.6943±0.0008d.     

Alpha-decay half-life of <Superscript>221</Superscript>Fr in different environments

A possible dependence of the alpha decay process on the solid-state environment of the decaying nucleus has been investigated by measuring the alpha-decay half-life of ²²¹Fr at room temperature in different materials ( Au, W, Si and polyethylene). The change in half-life between the insulator Si and the metals Au/ W is found to be 0.30(17)% / 0.42(21)%, respectivly. Furthermore an improved value of 4.79(2)min was found for the absolute half-life of ²²¹Fr.     

1<Superscript>+</Superscript>(0<Superscript>+</Superscript>) state at 12.4 MeV in <Superscript>20</Superscript>Ne

Careful review of all the evidence makes it clear that at least three states are important at 12.4-MeV excitation in ²⁰Ne (four, if the broad (2⁺) at 12.5 MeV is included). The three states are 3 ^- , 0 ⁺ , and 1 ⁺ (0⁺). The latter, which is quite strong in ¹⁹F (³He, d) singles, is probably the state observed in coincidence with 6.13-MeV γ-rays in ¹⁹F(³He, dγ). Received: 19 August 2002 / Accepted: 28 October 2002 / Published online: 17 January 2003 RID="a" ID="a"e-mail: fortune@physics.upenn.edu Communicated by D. Guerreau     

Investigations into the alpha-decay of <Superscript>195</Superscript>At

The low-energy nuclear structure and decay properties of the neutron-deficient isotopes ¹⁹⁵At and ¹⁹¹Bi have been studied. ¹⁹⁵At was produced in the reaction ¹⁴²Nd(⁵⁶Fe,p2n)¹⁹⁵At and ¹⁹¹Bi as the daughter activity of ¹⁹⁵At. The activities were implanted in a position-sensitive silicon detector after being separated from the primary beam by a gas-filled recoil separator. The 1/2⁺ intruder state was determined to be the ground state in ¹⁹⁵At with an alpha-decay energy of E _α = 6953(3) keV and a half-life T _1/2 = 328(20) ms. Another state with an alpha-decay energy E _α = 7075(4) keV and a half-life T _1/2 = 147(5) ms was found to decay to a 148.7(5) keV excited state in ¹⁹¹Bi for which a spin and parity of 7/2^- were deduced. Consequently, the same 7/2^- character was assigned to the initial state at 32(7) keV in ¹⁹⁵At on the basis of unhindered alpha-decay. The 9/2^- state, being the ground state in heavier odd-mass astatine isotopes, was not observed. Received: 16 September 2002 / Accepted: 19 December 2002 / Published online: 25 March 2003 RID="a" ID="a"e-mail: heikki.kettunen@phys.jyu.fi RID="b" ID="b"Present address: Laboratory of Radiochemistry, P.O. Box 55, FIN-00014, University of Helsinki, Finland. RID="c" ID="c"Present address: Radiation and Nuclear Safety Authority, P.O. Box 14, FIN-00881 Helsinki, Finland. Communicated by W. Henning     

Inelastic excitation of <Superscript>187</Superscript>Re

Excited states in ¹⁸⁷Re populated by inelastic scattering of a 500 MeV ⁸²Se beam have been studied by means of in-beam γ-ray spectroscopy. Levels built on the 5/2⁺[402] and 9/2^-[514] one-quasiparticle states were measured up to I ^π = (21/2⁺) and (21/2^-), respectively. In addition, several new levels including an isomer at 1682 keV with a half-life of 114(23) ns have been found. Quasiparticle configurations of the levels and the transition rates are discussed. Received: 12 December 2002 / Accepted: 13 March 2003 / Published online: 13 May 2003     

On the unusual properties of the 282 keV state in <Superscript>135</Superscript>Sb

Recently the first excited state in ¹³⁵Sb has been observed at the unexpectedly low excitation energy of only 282keV and interpreted as mainly d _5/2 proton coupled to the ¹³⁴Sn core. Based on theoretical considerations it was suggested that its low excitation energy is related to a relative shift of the proton d _5/2 and g _7/2 orbits induced by the neutron excess. We have measured the lifetime of the 282keV state by the advanced time-delayed βγγ(t) method. The measured half-life, T _1/2 = 6.1(4)ns, yields exceptionally low limits of B(M1;5/2₁ ⁺→7/2₁ ⁺)≤3.0×10^-4 μ ² _N and B(E2;5/2₁ ⁺→7/2₁ ⁺)≤54e ² fm ⁴. These strongly hindered M1 and slow E2 transition rates are similar to those for the transition de-populating the first excited state at 405keV in ²¹¹Bi. Results of shell model calculations with realistic interactions are presented. The M1 decay rate was found to be extremely sensistive both to the wave function and to the M1 effective operator.     

The <Superscript>198</Superscript>Au <Emphasis Type="Italic">β</Emphasis><Superscript>−</Superscript> half-life in the metal Au revisited

The half-life of the β ⁻ -decay of ¹⁹⁸Au has been measured for room temperature and 12K. The resulting values of T _1/2 ^(RT) = 2.684±0.004 d and T _1/2 ^(12K) = 2.687±0.005 d agree well within statistical uncertainties. Evidence for the temperature dependence of the half-life was not observed.     

First hint on a change of the 210Po alpha-decay half-life in the metal Cu

In the metal Cu cooled to T = 12K the α-decay half-life of ²¹⁰Po nuclides, located inside the metal, was measured to be shorter by 6.3±1.4% compared to that at room temperature.     

First observation of medium-spin excitations in the <Superscript>138</Superscript>Cs nucleus

The Penning trap mass spectrometer JYFLTRAP, coupled to the Ion Guide Isotope Separator On-Line (IGISOL) facility at Jyv?skyl?, was employed to measure the atomic masses of neutron-rich ^70-73Ni and ^{73, 75}Cu isotopes with a typical accuracy less than 5keV. The mass of ⁷³Ni was measured for the first time. Comparisons with the previous data are discussed. Two-neutron separation energies show a weak subshell closure at ⁶⁸ ₂₈Ni₄₀ . A well established proton shell gap is observed at Z = 28 .     

Nuclear quadrupole moments of 5/2<Superscript>-</Superscript> and 9/2<Superscript>-</Superscript> states in <Superscript>169</Superscript>Ta

The nuclear spectroscopic quadrupole moments for the πh_9/25/2^-, 1/2^-[541] and the πh_11/29/2^-, 9/2^-[514] isomeric states in ¹⁶⁹Ta have been measured employing the time differential perturbed angular-distribution technique following the nuclear reaction ¹⁵⁹Tb(¹⁶O, 6nγ)¹⁶⁹Ta at beam energy 104 MeV. The ratio of the intrinsic quadrupole moments has been derived as 1.87(13) from the measured quadrupole precession frequencies of the corresponding states. The model-independent analysis of the equilibrium deformation indicates strong prolate- and oblate-driving nature of the 1/2^-[541] and 9/2^-[514] orbitals in ^169,171Ta isotopes, respectively.     

Investigation on phase and shape transitions in the hot rotating nucleus <Superscript>154</Superscript>Dy

A statistical theory for hot rotating nuclei incorporating deformation, collective and non-collective rotational degrees of freedom, shell effects and pairing correlations is used to investigate the occurrence of phase and shape transitions in the hot rotating deformed nucleus ¹⁵⁴Dy . The interplay of various degrees of freedom and their influence on the behavior of nuclei formed as fused compounds in heavy-ion reactions are studied. A phase transition from the superfluid to normal state in the nucleus with increasing temperature and angular momentum is observed. The effect of pairing on the level density parameter and nucleon separation energy has been analyzed and is found to be substantial. The neutron and proton separation energies extracted as a function of the angular momentum and temperature is found to decrease sharply for particular angular momentum states of the nucleus due to shape transitions from prolate collective to oblate non-collective at higher temperatures.     

Precision electron-gamma spectroscopic measurements in <Superscript>75</Superscript>As

The decay of ⁷⁵Se to levels of ⁷⁵As has been studied using an HPGe detector for gamma-ray and a mini-orange electron spectrometer for conversion electron measurements. We identify 38 transitions in this decay, including 18 gamma rays and 16 conversion electron lines reported for the first time. New results also include E2 multipolarity assignment for the 81 keV transition, M1 assignment to three newly observed transitions and M1 + E2 for the 617 keV transition. A revised ⁷⁵As level scheme is constructed using the Ritz combination principle through the computer code GTOL. While confirming the existence of 10 well-established levels, two levels at 587 and 859 keV are newly placed into the decay scheme of ⁷⁵Se. The interpretation of the observed levels in terms of various theoretical approaches is briefly discussed. The newly placed 586.8 keV 1/2^- and 859.9 keV 1/2⁺ levels are studied in the light of the Interacting Boson-Fermion Model.     

Measurement of quadrupole moment of the 134 keV level in <Superscript>131</Superscript>Cs

The time differential as well as time integral perturbed angular correlations of the 486-134 keV cascade in ¹³¹Cs have been studied in a polycrystalline BaSO₄ powder source using a HPGe-BaF₂ detector system. The fundamental quadrupole frequency for the 134 keV level has been found to be ω₀= (4.4 ± 0.4) × 10⁷ rad/s. From a comparison of the quadrupole frequencies of this level and that of the 81 keV level in ¹³³Cs, measured earlier in the same crystalline environment of the source, the absolute value of the quadrupole moment of the 134 keV level in ¹³¹Cs has been found to be 0.022 ± 0.002 b. This value of the quadrupole moment is reported for the first time and compared with the value predicted theoretically within the unified nuclear model with intermediate coupling. Received: 21 October 1999 / Revised version: 22 December 1999     

High-spin states in the <Superscript>97</Superscript>Tc nucleus

High-spin states in the ⁹⁷Tc nucleus have been studied by in-beam γ-ray spectroscopy with the reaction ⁸²Se(¹⁹F,4nγ) at 68 MeV incident energy. Excited states have been observed up to about 8 MeV excitation and spin 43/2. The observed level scheme is compared with results of shell model calculations. Received: 22 November 2002 / Accepted: 23 December 2002 / Published online: 18 March 2003 RID="a" ID="a"e-mail: bucurescu@tandem.nipne.ro RID="b" ID="b"Present address: INFN, Laboratori Nazionali di Legnaro, Legnaro, Italy. RID="b" ID="b"Present address: INFN, Laboratori Nazionali di Legnaro, Legnaro, Italy. RID="b" ID="b"Present address: INFN, Laboratori Nazionali di Legnaro, Legnaro, Italy. RID="c" ID="c"Present address: Università di Padova, Padova, Italy. Communicated by C. Signorini     

Super-allowed α decay above doubly-magic <Superscript>100</Superscript>Sn and properties of <Superscript>104</Superscript>Te = <Superscript>100</Superscript>Sn ⊗ α

α-decay half-lives for ^{104, 105, 106}Te and ^{108, 109, 110}Xe close above the doubly-magic ¹⁰⁰Sn are calculated from systematic double-folding potentials. The derived α preformation factors are compared to results for ^{212, 213, 214}Po and ^{216, 217, 218}Rn above the doubly-magic ²⁰⁸Pb. α-decay energies of Q _α = 5.42±0.07MeV and 4.65±0.15MeV are predicted for ¹⁰⁴Te and ¹⁰⁸Xe; the corresponding half-lives are T _1/2 ≈ 5ns for ¹⁰⁴Te and of the order of 60μs for ¹⁰⁸Xe. Additionally, the properties of rotational bands in ¹⁰⁴Te are analyzed, and the first excited 2⁺ state in ¹⁰⁴Te is predicted at E _x = 650±40keV; it decays preferentially by γ emission with a reduced transition strength of 10 Weisskopf units to the ground state of ¹⁰⁴Te and with a minor branch by α emission to the ground state of ¹⁰⁰Sn.     

Search for superheavy hydrogen isotopes <Superscript>6</Superscript>H and <Superscript>7</Superscript>H in stopped π-absorption reactions

Experimental search for superheavy hydrogen isotopes ⁶H and ⁷H was performed in the stopped pion absorption on ⁹Be and ¹¹B nuclei. The structures in the missing-mass spectra were observed in the reaction channels ⁹Be(π^-, pd )X and ¹¹B(π^-, p⁴He)X . Four states of ⁶H were proposed. Evidences for ⁷H formation were obtained in the reaction channels ⁹Be(π^-, pp)X and ¹¹B(π^-, p³He)X .     

Change of the 7Be electron capture half-life in metallic environments

For the electron capture of ⁷Be in the metallic environments Pd and In the ⁷Be half-life was observed to increase by 0.9±0.2 and 0.7±0.2%, respectively, while in the insulator Li₂O it was unchanged within experimental error (all samples cooled to T = 12K). The observations are consistent with the predictions of the Debye plasma model applied to the quasi-free electrons in the metals.     

Stable collective triaxial rotation in <Superscript>77</Superscript>Kr

Based on the γ -spectroscopic analysis of G.N. Sylvan et al., configuration-dependent cranked Nilsson-Strutinsky calculations have been performed. They describe the nucleus ⁷⁷Kr globally in good agreement with the experimental findings and the expectations derived from single-particle orbitals in a deformed potential. Within these calculations, the unambiguous assignment of a configuration with three protons and five neutrons in the g _9/2 shell to the high-spin Yrast states of negative parity indicates that the nucleus ⁷⁷Kr has stable triaxial deformation and rotates about the intermediate axis. This not only disproves the recent interpretation of an occupation of the d _5/2 orbital being responsible for the strong deformation in this band, but also represents one of the first examples in this mass region for such a rotation.     

First hints on a change of the 22Na βdecay half-life in the metal Pd

For the β⁺-decay of ²²Na in the metallic environment Pd cooled to T = 12 K the ²²Na half-life was observed to be shorter by 1.2±0.2%. The result is consistent with --but lower than-- the prediction of the Debye plasma model.     

Structure of low-lying <Superscript>12</Superscript>C resonances

The hyperspherical adiabatic expansion is combined with complex scaling and used to calculate low-lying nuclear resonances of ¹²C in the 3α model. We use Ali-Bodmer potentials and compare results for other potentials α-α with similar ⁸Be properties. A three-body potential is used to adjust the ¹²C resonance positions to desired values extending the applicability of the method to many-body systems decaying into three α-particles. For natural choices of three-body potentials we find 14 resonances below the proton separation threshold, i.e. two 0⁺, three 2⁺, two 4⁺, one of each of 1^±, 2^-, 3^±, 4^-, and 6⁺. The partial-wave decomposition of each resonance is calculated as a function of the hyperradius. Strong variation is found from small to large distance. The connection to previous experimental and theoretical results is discussed and agreements as well as disagreements are emphasized.