A theoretical study of low-energy position diffraction

In an exploratory study of the diffraction of slow positrons from atoms and single-crystal surfaces, theoretical intensity and spin polarization results from a W crystal-atom and a W(001) surface are compared to corresponding electron diffraction results obtained with and without an exchange potential. In contrast to e^- diffraction, significant spin polarization effects are found for e⁺ only at energies above about 100 eV. The computing time for e⁺ is about half of the time required for e^-.     

μ+ Knight shift in Be

A first principles calculation of the Knight shift of a ⁺ in beryllium was carried out using a cellular multiple scattering technique (Keller 1972, 1977). The main conclusion is that the ⁺ induces the segregation of one state (of each spin) from the conduction band to lower energies, a molecular orbital of the ⁺ and its nearest neighbours. This state is occupied (with two antiparallel spin electrons) but it has less than 35% of ⁺ character. The screening is then completed with the conduction electrons properly. The observed Knight shift is then the sum of a diamagnetic shielding and a typical enhanced spin susceptibility term of opposite sign and smaller value.     

Evidence for the coexistence of spherical and deformed states in38Ar

The³⁸Ar levels at E_x=5350, 7289 and 9341 keV have been investigated using the³⁵Cl(α,pγ) reaction at E_α=l4 and 14.5 MeV. From particle-γ-ray angular correlations the spin assignments J(5350)=4, J(7289)=6,4 and J(9341)=8,6,4 have been obtained. Life-time measurements using the Doppler-shift attenuation method yielded τ(9341)=106±25 fs and τ(7289)=77±30 fs, while the lifetime τ(5350)=200±50 fs was known previously. All levels have positive parity and decay by enhanced E2 transitions. Hence we propose that they are the J^π=4⁺, 6⁺ and 8⁺ members, respectively, of a K^π=0⁺ rotational band which has the E_x=3377keV, J^π=0⁺ and the 3937 keV, J^π=2⁺ levels as further members. The enhancement of inband E2 transitions is 30 _?6 ⁺¹⁰ W.u. (4→2), 35 _?14 ⁺³⁰ W.u. (6→4) and 20–36 W.u. (8 → 6), respectively, yielding an average intrinsic quadrupole moment Q₀=850 _?125 ⁺²⁰⁰ mb. The moment of inertia is given by h²2θ=92 keV. The present data are in good agreement with the predictions of a deformed state in³⁸Ar that coexists with the spherical states.     

Multiplicities for evaporative4He emission in heavy ion reactions: Relationships to spin and lifetime expectancy of the composite nucleus

Multiplicities are compared for⁴He evaporation in reactions of⁴⁰Ar and⁵⁶Fe projectiles (8.5 MeV/u) with with^natAg and²³⁸U targets. Coincidence requirements involving fusion-fission and projectile-like fragments have been used to select separate entrance-channel spin zones. Evaporation-like⁴He emission from the composite nuclei is shown to be large for mean spins ≦100?, and to decrease dramatically with increasing spin. Coincidence measurements between two⁴He particles have also been studied for⁴⁰Ar+^natAg. This requirement is shown to select reactions that lead to evaporation residues and therefore to a zone of relatively low spin. The shapes of the⁴He spectra provide an interesting probe of the mechanism and also of the thermodynamic properties of hot nuclei.     

Performance assessment of a new laser system for efficient spin exchange optical pumping in a spin maser measurement of <Superscript>129</Superscript>Xe EDM

We demonstrate spin-exchange optical pumping of ¹²⁹Xe atoms with our newly made laser system. The new laser system was prepared to provide higher laser power required for the stable operation of spin maser oscillations in the ¹²⁹Xe EDM experiment. We studied the optimum cell temperature and pumping laser power to improve the degree of ¹²⁹Xe spin polarization. The best performance was achieved at the cell temperature of 100 ^°C with the presently available laser power of 1 W. The results show that a more intense laser is required for further improvement of the spin polarization at higher cell temperatures in our experiment.     

Spin-Dependent Forces and Current Quark Masses

The J = (3/2) , J = 1/2 Nucleon mass difference shows the quark energies can be spin dependent. It is natural to expect that the quark wave functions also depend on spin. A spin-dependent quark force is fitted to the proton and neutron magnetic moments, axial charge, and spin content using a (1/2⁺)³ configuration for the quarks and assuming only zero mass u and d quarks are in the nucleon. In the octet, such spin-dependent forces lead to different wave functions for quarks with spin parallel or antiparallel to the nucleon spin. The eigen-energy of this potential is 0.15 GeV higher for quark spin parallel than for the quark spin antiparallel to the proton spin. This potential predicts a single quark energy of 0.37 GeV for mass-less quarks in the Delta. Assuming the quark forces are flavor independent, this potential predicts magnetic moments of a bound strange quark to be very close to those determined empirically from the octet magnetic moments.     

Novel electron spin resonance spectra of a tetrathiafulvalene salt of copper chloride, (TTF) 2CuCl2

An ESR study has been carried out on electrically conducting (TTF)₂CuCl₂ crystals. The peak-to-peak width W of the ESR spectrum exhibited an unusual angular dependence with respect to the angle θ between the TTF-stack direction and the external field: the W showed a sharp minimum (4.9 G at 300 K) at θ = 0°, a maximum (7.5 G) at 60° (corresponding to 3cos²θ ∼ 1), and another minimum (6.9 G) at 90°. This angular depence has been explained by assuming an anisotropic motional narrowing that may arise from a spin correlation in one-dimensional electroconductive lattices. The temperature dependence of the W showed no anomaly around the temperature of metal-semiconductor transition: the spin relaxation is substantially unchanged by the phase transition.     

Angular momentum dependence of 200Pb fission studied by comparison of 19F on 181Ta with 16O on 184W

The time development of fission in highly excited Pb nuclei has been studied by the crystal blocking technique. Thin Ta crystals were bombarded with ¹⁹F ions in the energy range 90–120 MeV and the yield of fission fragments was measured for emission directions close to a strong axis. The experimental blocking dips are compared with calculated dips containing a superposition of two components, corresponding to short- and long-lived compound nuclei. The information extracted is the energy dependence of the relative amount of fission which comes from compound nuclei with lifetimes of τ≳3 × 10⁻¹⁷s. The total fission cross section and angular distribution of fission fragments were also measured for ¹⁹F bombardment of ¹⁸¹Ta in the energy range 84.3–114.7 MeV and for ¹⁶O bombardment of ¹⁸⁴W in the energy range 83.4–107.9 MeV. The results of the three types of measurements have been interpreted through comparison with statistical model calculations that follow the spin and energy distribution of compound nuclei through the neutron evaporation cascade. The ¹⁹F + ¹⁸¹Ta measurements, when compared with the present ¹⁶O + ¹⁸⁴W cross section and angular distribution measurements and earlier lifetime measurements for ¹⁶O + W, yield information on the spin distribution for the compound nucleus and its influence on the fission process.     

A method for investigations of solid surfaces by nuclear spin relaxation

A method is presented which allows to investigate hot metal surfaces (1,000 K to 1,600 K) by use of nuclear spin polarized alkali atom beams (⁶Li,⁷Li,²³Na). At these temperatures the atoms are adsorbed for about 10^–4 s to 1 s. During the residence time on the surface the nuclear moments interact with the electromagnetic fields of their environment. The nuclear spin polarization of the ions desorbing from the surface is detected by beam foil spectroscopy. The depolarization gives information on electric field gradients and magnetic fields originating in the surface and on the electronic state of the absorbed alkali atoms.Supported partly by the Deutsche Forschungsgemeinschaft and the Bundesministerium für Forschung und Technologie, both Bonn, FRG     

Polarization of high spin nuclear levels via tilted multifoil interaction

It has been demonstrated that with suitably spaced carbon foils, tilted with respect to the particle momentum, a large polarization can be generated in high spin nuclei by the tilted foil atomic polarization. Two experiments have been carried out with such polarized high spin isomers: a measurement of the sign of the quadrupole moment of the 10⁺ isomer in⁵⁴Fe, and a new attempt of higher sensitivity at detecting a possible positive parity admixture to the 17/2^– isomer in⁹³Tc.On leave from the Hahn-Meitner Institut, Berlin, W. Germany.On leave from Physics Department, Brooklyn College of the City of New York, Brooklyn, New York.     

First Eigenvalue of the Dirac Operator for a Kähler Manifold of Even Complex Dimension: The Limiting Case

K. D. Kirchberg has given a minoration of the absolute value of the eigenvalues of the Dirac operator for a compact Kähler spin manifold (W,g) with positive scalar curvature and has introduced, in this context, the notion of Kähler twistor-spinor. We prove here that if dim_C W = p 4 is even, in the limiting case, (W, g) is the Kähler product of an odd-dimensional limiting case compact Kähler spin manifold of complex dimension (p-1), by a flat Kähler manifold which is a compact quotient of C.     

High-spin structure in 169W and 170W

High-spin states in ^{169, 170}W have been populated in ${}^{154}\text{Gd}\text{(}{}^{20}\text{Ne}\text{, x}\text{n}\text{)}$ reactions. In-beam γ-ray spectroscopic techniques with multi-detector set-ups, multiplicity filters and an anti-Compton shield have been used. Levels up to about spin 30 (tentatively up to 36) in ¹⁷⁰W and up to $\text{57}\text{2}$ (tentatively up to $\text{61}\text{2}$) in ¹⁶⁹W have been identified. The data are interpreted within the framework of a pairing-selfconsistent cranking model. The nuclear shape evolution with increasing spin is studied theoretically within a configuration-controlled shell correction approach and also pairing effects are studied. The behaviour of the yrast states around 28⁺ in ¹⁷⁰W can be related in a model-dependent way to a reduction of the neutron-pairing correlations.     

Transfer Matrix Spectrum and Bound States for Lattice Classical Ferromagnetic Spin Systems at High Temperature

We obtain new properties of general d-dimensional lattice ferromagnetic spin systems with nearest neighbor interactions in the high-temperature region (1). Each model is characterized by a single-site a priori spin distribution, taken to be even. We state our results in terms of the parameter =s ⁴–3s ²², where s ^k denotes the kth moment of the a priori distribution. Associated with the model is a lattice quantum field theory which is known to contain particles. We show that for >0, small, there exists a bound state with mass below the two-particle threshold. The existence of the bound state has implications for the decay of correlations, i.e., the 4-point functions decay at a slower rate than twice that of the 2-point function. These results are obtained using a lattice version of the Bethe–Salpeter equation. The existence results generalize to N-component models with rotationally invariant a priori spin distributions.     

Magnetic properties of high-T c superconductors from NQR and NMR measurements

NMR and NQR spectra and spin-lattice relaxation measurements carried out in LASCO and YBCO-type crystals are presented and analyzed in order to derive insights on the correlations and spin-dynamics of the Cu²⁺ ions and on the microscopic mechanisms of high-T _c superconductivity. As an illustrative example on how the magnetic correlation length and spin dynamics properties can be extracted from the relaxation rateW, the³⁵Cl NMR data in the two-dimensional Heisenberg system Sr₂CuCl₂O₂, around the paramagnetic-antiferromagnetic (PA-AF) transition are first considered. Then the¹³⁹La NQR relaxation measurements in La_2?xSr_xCuO₄ are briefly reviewed and it is shown how a simple picture of localized Cu²⁺ magnetic moments, whose spin fluctuation times are controlled by the charge defects induced by the doping, leads in a direct way to quantitative estimates for the progressive shift, on cooling, of the spectral density of the low-frequency spin excitations towards the high frequency range. This phenomenon can be described in terms of effective spin at the Cu²⁺ ions, and its similarities with the analogous effect of progressive delocalization in Heavy Fermions systems are pointed out. Thus, the superconducting transition appears to occur in an unconventional Fermi liquid with AF correlations among itinerant pseudoparticles, possibly involving a mechanism not directly related to the magnetic correlated dynamics. In fact, a universal behavior of the relaxation rates as a function of temperature is observed, regardless of the transition temperatureT _c. The independence ofT _c from the low frequency static and dynamical spin properties is also indicated by⁸⁹Y Knight shifts and from⁶³Cu relaxation rates in systems like YBa₂Cu₄O₈ (Y124), whereT _c can be changed by atomic substitutions and by controlling the oxygen stoichiometry. The effect of an external magnetic field on the correlated spin dynamics of the AF Fermi liquid is investigated and from a comparison of Cu NQR relaxation and NMR relaxation in oriented powder of YBCO and LASCO it is shown that the external field has the small but unambiguous effect of depressing the relaxation rates aboveT _c, besides strongly enhancing them in the superconducting phase. A maximum in the ratio \({{W\left( {NQR} \right)} \mathord{\left/ {\vphantom {{W\left( {NQR} \right)} {W\left( {\vec H\left\| {\vec c} \right.} \right)}}} \right. \kern-0em} {W\left( {\vec H\left\| {\vec c} \right.} \right)}}\) is thus observed around 80 K, either in LASCO or in YBCO, again indicating that the transition could be driven by a mechanism not directly involving the spin dynamic properties. To study the role of the fluxions belowT _c ⁸⁹Y NMR shifts and spectra in oriented powders of YBCO are analyzed. Information on the spin susceptibility and on the structure of the vortex lattice is obtained. In addition, from the temperature behavior of the linewidth a motional narrowing related to flux melting is evidenced. The effective correlation time for the vortex motion is derived and it is discussed why μ⁺SR cannot detect it in view of the different rigid-lattice line broadening.     

Fragmentation of the yrast band in186Os atI π =18+ and disappearance of the collective minimum

High-spin states in¹⁸⁶Os have been populated by the¹⁸⁶W(⁴He,4n)-reaction at 55MeV. The emittedγ-radiation was detected with the OSIRIS spectrometer. The yrast band, for which the nucleus has a prolate shape, was found to terminate atI ^π =18⁺. Theγ-ray intensity is then distributed between several irregular sequences. Different to other cases of band termination, the minimum in the total routhian surface corresponding to a collective shape is calculated to disappear in this spin region, although the available spin of the valence nucleons is far from being exhausted. A different structure, which is dominated by non-collective states becomes yrast.     

Evidence for deformed states in 75Br

The excited states in ⁷⁵Br have been studied via the reactions ⁷⁴Se(p, γ), ⁷⁴Se(d, n), ⁷⁴Se(³He, pn) and ⁷⁴Se(α, p2n) by using in-beam γ-ray spectroscopy. In addition to measurements of γ-γ coincidences, excitation functions and angular distributions of γ-rays, ns lifetime measurements have also been carried out. As a result 19 levels have been identified up to spin ($\text{17}\text{2}$) and excitation energies up to 2.6 MeV. The B(E2) value of 88 W.u. derived for the 88.4 keV γ-ray indicates strong collectivity within a positive-parity band. A comparison of the excitation energies of the unique-parity states in ⁷⁵Br and ⁷⁷Br with those in ¹⁵³Tb and ¹⁵⁵Tb reveals that the average deformation increases when going from ⁷⁷Br (N = 42) to ⁷⁵Br (N = 40).     

Creation of the nuclear alignment and theG-parity conservation law in weak nucleon currents

-ray angular distributions from nuclear spin aligned¹²B and¹²N were detected and the correlation coefficients were determined. From the comparison of these with the experimental weak magnetism term, it was concluded that the parity of the weak nucleon currents in the iso-spin space was strictly conserved.     

Temperature dependence of the spinS=1/2 fluctuation rate and the low-spin versus high-spin transition in native chloroperoxidase

We analyzed two preparations of native, low-spin ferric chloroperoxides as a function of temperature with the following results. (i) The spin lattice transition rateW(T) is relative slow, following a power lawW=0.035 (T/K)^4.98 (rad/s) for one of the samples. (ii) The quadrupole splitting is strongly temperature dependent, dropping from ¦E _Q¦ 2.94 mm/s at 100 K to 2 mm/s at 250 K. (iii) Starting at 190 K, the low-spin heme iron in frozen adqueous solution converts reversibly to a high-spin form, reaching 40% high-spin at 250 K. The two forms appear to be in thermal equilibrium, (iv) Optical data indicate that in a 70% glycerol glass, the conversion starts at lower temperature and reaches 50% highspin at 190 K.Supported in part by GM 49513 and GM 16406.