Spectroscopic quadrupole moments of high-spin isomers in 193 Pb

The quadrupole interaction of high-spin isomers in ¹⁹³Pb implanted into solid Hg cooled at a temperature T = 170 K has been investigated by the time-differential perturbed -ray angular-distribution method. Spectroscopic quadrupole moment values of eb and 0.45(4) eb have been deduced for the 21/2^- and 33/2 ⁺ three-neutron states, respectively. A much higher value eb has been determined for the 29/2^- isomer, the band head of a magnetic rotational band.Received: 4 November 2002, Published online: 2 March 2004PACS: 21.10.Ky Electromagnetic moments - 27.80. + w      

Nuclear polarization and signs of quadrupole moments of high-spin Gd isomers

Time-differential perturbed-angular-distribution (TDPAD) experiments have been performed on polarized intermediate- and high-spin isomers ${}^{144}\text{Gd}\text{(10}{}^{\mathrm{+}}\text{)}\text{and}{}^{147}\text{Gd}\text{(}\text{13}\text{2}{}^{\mathrm{+}}\text{,}\text{27}\text{2}{}^{\mathrm{?}}\text{,}\text{49}\text{2}{}^{\mathrm{+}}\text{)}$. Excited Gd nuclei populated by $\text{(}{}^{28}\text{Si}\text{, x}\text{n}\text{)}$ reactions were polarized by the tilted-multifoil technique and implanted in a Gd single-crystal host. Observation of the subsequent electric quadrupole interaction with the known electric field gradient yielded negative values of the sign of the deformation for all isomers studied. The magnitude of the induced nuclear polarization P_I was also determined from the TDPAD data and compared to model calculations in order to deduce the average atomic angular momentum and polarization of Gd ions at v/c ～ 0.018.     

Static electric quadrupole and hexadecapole moments of nuclei

Ground-state static electric quadrupole and hexadecapole moments of even nuclei are calculated microscopically. Rare-earth, actinide and neutron-deficient nuclei with 50 <Z, N < 82 and neutron-rich nuclei with 28 < Z < 50, 50 < N < 82 are studied. Fairly good agreement with experiment is found. In the actinide region, the electric moments of fission isomers are also examined.     

Calculations of electric quadrupole moments and charge radii for high-K isomers

Configuration-constrained potential-energy-surface calculations are performed to investigate high-K isomers in ⁹⁷Y, ¹³⁰Ba, ¹⁷⁶Yb, ¹⁷⁷Lu, and ¹⁷⁸Hf that were observed to have increased electric quadrupole moments but decreased charge radii relative to the states on which they are built. Taking into account the effects of deformation change and unpaired protons, our calculations can reproduce the enhancement of electric quadrupole moments for the isomers in ⁹⁷Y, ¹³⁰Ba, ¹⁷⁶Yb, ¹⁷⁷Lu and the K ^π = 8^? isomer in ¹⁷⁸Hf, and can reproduce the reduction of charge radii for the K ^π = 27/2^? isomer in ⁹⁷Y and the K ^π = 16⁺ isomer in ¹⁷⁸Hf.     

Electromagnetic moments of nuclei at high-spin

Choosing some of the current topics in the field of high-spin nuclear physics, I discuss what we learn from the study of electromagnetic moments of the high-spin states. Chosen topics are triaxial shape, superdeformed band, high-spin states with oblate shape, and g-factor before and after band-crossings.     

Measurement of transition quadrupole moments of high-spin states in the N=74 isotones Pr, Ce and La

The Doppler-Shift Attenuation Method has been used to extract transition quadrupole moments of high-spin bands in the N=74 isotones ¹³³Pr, ¹³²Ce and ¹³¹La, produced in the ³⁷Cl + ¹⁰⁰Mo reaction. The results appear to be configuration dependent and, for ¹³³Pr and ¹³²Ce, the involvement of Ω=1/2 νh_9/2 and νf_7/2 intruder orbitals appears to enhance the collectivity at high spin (I>25 ).     

Systematics of high-spin isomers in N = 83 isotones and a high-spin isomer beam

Isomers in N = 83 isotones of Z = 60-66, were studied systematically. Their spins and parities are 49/2⁺ and 27⁺ for odd and odd-odd nuclei, respectively. Nearly constant excitation energies of these isomers indicated a decrease of a Z = 64 shell gap energy as Z decreases from 64 to 60 within the framework of a deformed independent-particle model (DIPM). Their configurations are [ν(f _7/2 h _9/2 i _13/2),π(h _11/2)²]_49/2+ and [ν(f _7/2 h _9/2 i _13/2),π(h _11/2)²(d _5/2)^-1]₂₇₊ for odd and odd-odd nuclei, respectively. The shape of the yrast states changes suddenly at spin 49/2(odd) and 27(odd-odd) from a near spherical to an oblate shape. Transitions from isomers are highly hindered because of the shape changes. They may be categorized to be shape isomers. The development of a secondary beam produced by using these high-spin isomers is also described. Received: 1 May 2001 / Accepted: 4 December 2001     

New high-spin microsecond isomers in 131Sb

In this work we have identified and studied the decay of two new microsecond isomers 19/2^- and 23/2⁺ in ¹³¹Sb. This neutron-rich nucleus was produced by thermal neutron-induced fission of ²⁴¹Pu. The detection is based on time correlation between fission fragments selected by the LOHENGRIN spectrometer at ILL (Grenoble) and the γ-rays or conversion electrons from isomers. These new data on high-spin states complete the level scheme previously obtained from β-decay. A large fraction of the members of the πg _7/2ν(h _11/2 ^-1 d _3/2 ^-1) and πg _7/2νh _11/2 ^-2 multiplets are now known and were compared with a multi-particle shell model calculation. Received: 7 June 2000 / Accepted: 19 September 2000     

Microwave spectra,nuclear quadrupole coupling constants,dipole moments,and rotational isomers of propargylimine

The microwave spectra of the short-lived molecule, propargylimine (CHCCHNH), produced by the pyrolysis of dipropargylamine, have been observed. The spectra are analyzed with the aid of an ab initio MO calculation, and the rotational constants for the two isomers (Z- and E-propargylimines) have been determined as A = 54640.228 MHz, B = 4862.4191 MHz, and C = 4458.1986 MHz, and A = 63099.320 MHz, B = 4766.6104 MHz, and C = 4425.5144 MHz, respectively. The dipole moments, the quadrupole coupling constants, and the relative populations between the two isomers have also been obtained.     

Charge radii and quadrupole-deformation parameters of high-spin isomers

Experimental data on the differences of charge radii of nuclei in the ground and high-spin isomeric states are surveyed. High-resolution laser-spectroscopy methods were used for measurements. The results obtained for the differences of these radii by two methods—from measurements of isomeric shifts of the levels of atoms containing the nuclei being studied and from measurements of their quadrupole moments in both states under the assumption that the differences of the radii are determined by the difference in their quadrupole deformations—were compared. Two-particle isomers in odd—odd nuclei, isomers formed upon the break of one or several nucleon pairs, and isomers featuring the 1i _13/2 configuration of the odd neutron in mercury nuclei were considered. The observed distinctions between the aforementioned differences of charged radii are discussed for isomeric states of different nature.     

Nuclear quadrupole moments of bismuth

Multiconfiguration Dirac-Fock models have been employed to compute the electric field gradient in the ground state of the neutral bismuth atom. Combined with the experimental electric quadrupole hyperfine interaction constant, one obtains for (209)Bi the nuclear quadrupole moment Q = -516 (15) mb, which is almost 40% away from the previously accepted standard value [ -370 (26) mb], and narrows by over an order of magnitude the long-standing, extremely broad array of various results ranging from -370 to -710 mb. The recent Q values of (202-208,210(m)-213)Bi by Pearson et al. suffer a consequent change.     

Transitional quadrupole moments in83Y

Doppler shift attenuation lifetime measurements have been carried out for the 3qp and isomeric rotational bands in⁸³Y using the reaction⁵⁸Ni(²⁸Si,3p). While the transitional quadrupole moments in the 3qp bands are slightly lower than in the 1qp bands, we found evidence for a strong reduction in ¦Q_t¦ for the isomeric band.     

Description of high-spin isomers in theN=82 region

The high spin states and of those especially the yrast isomers are studied in the region near the rare earth nuclei. The deformation energy surface is calculated with a method modelled in principle according to a shape constrained cranked HF theory (CHF). In practice, the expectation value of the many-body Hamiltonian is calculated with cranked Nilsson functions. One finds rotation around a slightly deformed oblate or prolate symmetry axis in front or behind the rare earth region, respectively. Near the Hf isotopes strongly prolate deformed nuclei rotating around the symmetry axis are found in agreement with the knownK isomers in this region. These results are explained also qualitatively with the help of the MONA (Maximisation of theOverlap ofNucleonic wave functions byAlignment of single particle angular momenta) effect. In the second part high spin states and yrast isomers in theN=82 region are caluclated in the cranked Hartree-Fock-Bogoliubov approach with four and six quasi-particle excitations. For the excitation energies in¹⁴⁶Gd and¹⁵²Dy and a measuredg factor one finds satisfactory agreement.     

Description of high-spin isomers in theN=82 region

The high spin states and of those especially the yrast isomers are studied in the region near the rare earth nuclei. The deformation energy surface is calculated with a method modelled in principle according to a shape constrained cranked HF theory (CHF). In practice, the expectation value of the many-body Hamiltonian is calculated with cranked Nilsson functions. One finds rotation around a slightly deformed oblate or prolate symmetry axis in front or behind the rare earth region, respectively. Near the Hf isotopes strongly prolate deformed nuclei rotating around the symmetry axis are found in agreement with the knownK isomers in this region. These results are explained also qualitatively with the help of the MONA (Maximisation of theOverlap ofNucleonic wave functions byAlignment of single particle angular momenta) effect. In the second part high spin states and yrast isomers in theN=82 region are calculated in the cranked Hartree-Fock-Bogoliubov approach with four and six quasi-particle excitations. For the excitation energies in¹⁴⁶Gd and¹⁵²Dy and a measuredg factor one finds satisfactory agreement.     

Gamma-spectroscopy within the island of high-spin isomers nearN=82

A NaI sum-spectrometer combined with Ge-counters has been used to characterize the members of the island of high spin isomers nearN=82. On the basis of half lives, totalγ-decay energies and discreteγ-lines, assignments of 22 isomers are given or confirmed. The isomers are localized to the region 82≦N≦86 andZ≦68, and the excitation energies vary from 3 MeV to 12.2 MeV. An empirical relation between spin and excitation energy is presented and on this basis isomeric spin values up to (33±2)? are deduced. The isomers are thought to be due to strong alignment of 2 to 8 shell-model particles in a spherical or possibly weakly oblate potential.