Phase Controlled Laser Interference for Tunable Phase Gratings in Dye-Doped Nematic Liquid Crystals

A phase controlled multi-beam interference is applied to excite the doped liquid crystals. Control of the phase difference between the exciting beams allows the external control of the interference pattern inside the liquid crystal. The dynamic variation of the grating is made possible with a time-dependent phase change to derive the nonlinear refractive index as well as the responding speed of the material. The induced grating structure is numerically modelled with reorientational phase gratings in the liquid crystal, and the diffraction dynamics is found to be in good agreement between theoretical and experimental results.     

High-resolution photorefractive gratings in nematic liquid crystals sandwiched with photoconductive polymer film

Photorefractive gratings with high grating resolution were observed in the 20 μm thick low-molar-mass nematic liquid crystal (NLC) cell with a separate photoconductive (PC) poly(N-vinylcarbazole) layer. An orientational grating with a grating spacing of 1.9 μm was produced. It is believed that a space–charge field with small fringe spacing forms in the PC layer and its evanescent component penetrates into the NLC layer. The penetrated evanescent field drives the NLC to reorient, and consequently the orientational grating forms. The model indicates that the modulated field exists in several hundred nanometers near the surface, and thus the orientational grating is not full of the NLC film, which is consistent with the observed phenomena of the multiple diffractions. Besides, asymmetric two-beam coupling of 11.2% was achieved for the grating with a grating spacing of 1.9 μm, and a net gain coefficient of larger than 62 cm⁻¹ was obtained.     

Development of narrow-linewidth diode lasers by use of volume holographic transmission gratings

We present two diode laser setups that employ volume holographic transmission gratings to provide optical feedback. The advantage of this kind of grating is high diffraction efficiency and the possibility to place optical elements on both sides of the grating. This allows for advanced external cavities and adjustable feedback efficiency. The first setup is a diode laser in the Littman configuration with the transmission grating replacing the conventional reflection grating. The second setup improves the frequency selectivity by substituting the feedback mirror with a passive resonator. This grating-enhanced external cavity diode laser (GECDL) achieves excellent frequency stability. A prototype of the GECDL setup demonstrates an intrinsic linewidth of 7 kHz and an operation range that covers the full amplification profile of the laser diode.     

Storage of laser-induced holographic gratings in discotic liquid crystals

We demonstrate that low molar mass discotic liquid crystals can be used for holographic storage. Grating structures are optically induced and stored in the glassy state of the investigated liquid crystal. The material is suitable for multiple storage processes since the stored information can be erased by heating the sample above the glass transition temperature.     

Detection of higher nonlinear harmonics of volume photorefractive gratings in reflection geometry

A comprehensive technique has been used to detect diffraction from the second and the third nonlinear spatial harmonic components, along with the fundamental harmonic of volume photorefractive gratings recorded in a channel waveguide in a LiNbO₃ substrate. For the first time to our knowledge, efficient diffraction from the higher spatial harmonic components of a photorefractive grating has been detected in reflection geometry. The dependence of a Bragg wavelength shift on the order of nonlinearity is also reported.     

Effects of recording wavelength on three-dimensional vector holograms in photoreactive liquid crystal composites

Effects of recording wavelength on the recently proposed (Sasaki, 2008) three-dimensional vector holograms, in which the optical anisotropy is three-dimensionally modulated, are presented experimentally and theoretically. The polarization states of the interference light are three-dimensionally modulated due to both the polarization interference and optical anisotropy in the recording medium. These spatial distributions of the polarization states and the resulting diffraction properties in the three-dimensional vector holograms are strongly dependent on the recording wavelength. Theoretical consideration based on the finite-difference time-domain (FDTD) method reveals the mechanism of the optical characteristics of the three-dimensional vector holograms recorded by various kinds of light sources with different wavelengths.     

Fast electrically switchable holographic optical elements in LiNbO3

We present here the realization of fast electrically switchable holographic optical elements based on electric field multiplexing of volume holograms in lithium niobate crystals. We demonstrate the electrical control of holographic lenses and holographic mirrors for fast switching of the focal length and the direction of the reconstructed light beam, respectively. The switching time in the range of few hundred microseconds has been demonstrated using this technique.     

Holographic recording mechanisms of gratings in indium oxide films using 325 nm helium–cadmium laser irradiation

UV (325 nm) holographic recording of gratings in indium oxide films fabricated by reactive pulsed laser deposition has been investigated as a function of growth temperature, oxygen pressure and angle of incidence of the plasma plume on the substrate. The influence of the ambient environment (air or vacuum) and the film temperature during recording has also been studied. Large steady state refractive index changes up to 6×10^-3 were observed in layers grown at an oblique angle of 75°. About 77% of the magnitude of these changes residues after thermal annealing and is attributed to UV-induced permanent structural rearrangements. In contrast, refractive index changes in films grown at normal incidence were smaller in magnitude and completely reversible. Received: 30 July 2001 / Accepted: 20 November 2001 / Published online: 23 January 2002     

Estimation of trap concentration in photorefractive crystals by a technique of adaptive holographic interferometry

12 GeO₂₀, Bi₁₂SiO₂₀, Bi₁₂TiO₂₀). Received: 17 June 1998/Revised version: 3 August 1998     

Fabrication of surface relief gratings on transparent dielectric materials by two-beam holographic method using infrared femtosecond laser pulses

Fabrication of surface relief-type gratings in transparent dielectrics, which are hard to machine, has been achieved by a holographic technique using two infrared femtosecond (fs) pulses from a mode-locked Ti:sapphire laser. The present method can be applied for a variety of transparent dielectrics, Al₂O₃ (sapphire), TiO₂, ZrO₂, LiNbO₃, SiC, ZnO, CdF₂, MgO, CaF₂ crystals, and SiO₂ glass. It is found that the grating formation is due primarily to laser ablation processes. Planar surface relief gratings can be fabricated by colliding two fs laser pulses on the surface of substrates which move at a constant speed, synchronized with the laser repetition rate. Received: 1 March 2000 / Published online: 7 June 2000     

Observation of superluminal and slowdown light propagation in doped lithium niobate crystals

We investigate the group velocity of light in a one-dimensional volume grating inside lithium niobate crystals doped with different impurities. The superluminal and slowdown light propagations are both observed in the crystals. The relationships between the group refractive index and the grating amplitude and phase shift are presented and discussed.     

Second-order grazing-angle scattering in uniform wide holographic gratings

Grazing-angle scattering (GAS) is a type of Bragg scattering in slanted wide periodic gratings. It occurs when the diffracted order satisfying the Bragg condition (scattered wave) propagates at a grazing angle to the grating boundaries. Previous research has been concerned only with first-order GAS, which has been shown to be a highly unusual type of scattering characterised by a strong resonant increase of amplitudes of the scattered and incident waves in the grating. In this paper, a rigorous numerical study of second-order GAS is presented for the case of bulk TE electromagnetic waves in planar holographic gratings. A highly unusual pattern of strong resonances in the grating, which is strongly different from that for first-order GAS, is predicted, described, and discussed. Physical interpretations of the predicted results are presented. In particular, a special new type of eigenmodes in a slanted wide periodic grating with large amplitude is predicted. These eigenmodes are shown to be guided by the grating alone without any conventional guiding effect in the structure. The typical field structure in such eigenmodes is investigated and discussed. Received: 16 September 2002 / Revised version: 4 November 2002 / Published online: 22 January 2003 RID="*" ID="*"Corresponding author. Fax: +61-7/3864-9079, E-mail: d.pile@osa.org     

Microphotometric investigations of thick refractive index gratings in photorefractive crystals

Transmission microphotometry is used as a new tool for the investigation of the holographic writing process of thick refractive index gratings. Theoretical results on the origin of the contrast formation are discussed. They are experimentally confirmed by rocking curves of thick refractive index gratings in doped LiNbO₃ crystals.     

Comparison of the effects of two bleaching agents on the recording of phase holograms in silver halide emulsions

Optical densities before bleaching and final Lin-curves of plane-wave phase holograms recorded in Agfa-Gevaert 8E75HD emulsions were determined for combinations of the AAC developer with a solvent bleach (R-9) and a (fixation-free) rehalogenating bleach (R-10). To characterize the processing, the square root of the diffraction efficiency of the processed holograms was related to the amplitude of the optical density modulation obtained at the development step. Sensitivity, linearity and dynamic range of the processes could thereby be compared directly.     

Photorefractive properties of Cr-doped Sr0.61Ba0.39Nb2O6 related to crystal purity and doping concentration

The purity and the concentrations of the constituents Sr, Ba, Nb and Cr were determined in single crystals of chromium-doped Sr_0.61Ba_0.39Nb₂O₆ (SBN) by instrumental neutron activation analysis (INAA) and X-ray fluorescence analysis (XRF). Experiments with different Cr concentrations C_Cr reveal constant Sr and Ba concentrations as well as a decreasing Nb concentration with an increasing C_Cr. Therefore, Cr is incorporated at Nb lattice sites. The distribution coefficient of Cr is 1.2 between 100 and about 7000 ppm Cr and 1 above. From measurements of the holographic two-beam coupling gain Γ for different C_Cr, we deduced response times for the buildup of holographic gratings. The saturation value of Γ depends in a nonlinear manner on C_Cr and reaches its maximum at about 6000 ppm Cr. The inverse photorefractive response time of the grating erasure depends linearly on the erasure intensity for all doping concentrations. Thus a one-center model can be assumed for the charge transport in SBN:Cr. Received: 8 December 2000 / Revised version: 23 January 2001 / Published online: 21 March 2001     

Nonlinear interactions and scattering of space charge waves in sillenites

For the first time the effects of overall doubling, spatial doubling, and overall rectification of space charge waves in a photorefractive crystal (Bi₁₂GeO₂₀, BGO) have been detected and theoretically studied. The effects of overall doubling and overall rectification resemble second-harmonic generation and rectification of light in nonlinear optics. A good agreement between theory and experiment is found for the effect of spatial doubling, while for overall doubling and overall rectification effects only a qualitative agreement between theory and experiment has been established until now. Received: 13 July 2001 / Published online: 10 October 2001     

Photofabrication of periodic microstructures in azodye-doped polymers by interference of laser beams

Volume holographic gratings and two-dimensional periodic microstructures in azodye-doped polymethylmethacrylate were fabricated, respectively, by interference of two coherent beams of a femtosecond laser and by interference of three coherent beams of a nanosecond laser. The dependence of the first-order Bragg diffraction efficiency and the photoinduced refractive-index modulation of the gratings on the intensity of the writing light was investigated. The measurements of the absorption spectra before and after irradiation with the writing light suggest that the photoinduced gratings were refractive-index-modulated gratings, which arose from a photoinduced decomposition reaction of the azodye molecules through multiphoton absorption. In the experiments involving the interference of three beams, the period of the two-dimensional periodic microstructures was changed by adjusting the angle between the three writing beams. Received: 10 July 2002 / Revised version: 5 September 2002 / Published online: 20 December 2002 RID="*" ID="*"Corresponding author. Fax: +81-774/955206, E-mail: jhsi@photon.jst.go.jp     

Photoinduced anisotropy in an azo-containing ionic liquid-crystalline polymer

Photoinduced anisotropy in an azobenzene ionic liquid-crystalline polymer was investigated through dichroism, birefringence and polarization holography. A dichroism degree of 1.58 and a birefringence value Δn ∼ 10⁻² were achieved in the polymer film at room temperature, and the polymer film was found to possess the characteristics of reversible and long-term optical storage. Particularly the stored birefringence could be enhanced to Δn ∼ 10⁻¹ by annealing the film, and it is attributed to the thermal self-organization of the molecules. Furthermore, linear- and circular-polarization holographic recordings were accomplished in the polymer film and pure polarization gratings were produced.     

Nonlinear diffraction in gratings based on polymer–dispersed TiO 2 nanoparticles

In this letter we report a simple technique to produce volume holographic gratings based on photopolymerizable composites containing TiO₂ nanoparticles. Diffraction gratings with high refractive index modulation amplitude (up to 1.25 × 10⁻²) have been formed due to the periodic distribution of high refractive index nanoparticles in a low refractive index polymer matrix. The diffraction efficiency increases strongly on increasing the nanoparticle concentration. Taking the mixture with 10 wt.% TiO₂ nanoparticles, gratings with high diffraction efficiency, low level of scattering and high transparency in the visible-wavelength range have been obtained. This will ultimately lead to different applications of diffractive optical elements based on nanocomposites. The dependence of the gratings’ diffraction efficiency on the intensity of probe laser pulses at 1064 nm has been explored. It is shown that the nonlinear response of the gratings is attributed mainly to the nonlinear properties of the TiO₂ nanoparticles embedded in the polymer matrix. The mechanism of the grating formation and the reasons for the nonlinear behavior of the diffraction efficiency are discussed.     

Extremely asymmetrical scattering in gratings with weak dissipation: some physical analogies

A detailed analysis of new effects related to extremely asymmetrical scattering (EAS) of bulk and guided weakly dissipating electromagnetic waves in oblique periodic gratings is presented. A very important role of the previously determined critical grating width is demonstrated for EAS in dissipative gratings. Incident and scattered wave amplitudes inside and outside the grating are analysed as functions of dissipation coefficient, grating width, grating amplitude, etc. Strong differences in the patterns of scattering in gratings that are narrower and wider than the critical width are demonstrated and discussed. Deep analogies between EAS and other resonant optical effects, such as attenuated total reflection, Fabry–Pérot interferometry, etc. are revealed and discussed. A physical interpretation of the obtained results is presented. Received: 19 February 2002 / Revised version: 28 June 2002 / Published online: 22 November 2002 RID="*" ID="*"Corresponding author. Fax: +61-7/3864-9079, E-mail: d.gramotnev@qut.edu.au