Multi-wavelength generation based on cascaded Raman scattering and self-frequency-doubling in KTA

A multi-wavelength laser is developed based on cascaded stimulated Raman scattering (SRS) and self-frequency-doubling in an x-cut KTA crystal pumped by an A-O Q-switched Nd:YAG laser. The generation of 1178 nm from cascaded SRS of 234 and 671 cm⁻¹ Raman modes is observed. The six wavelengths, including the fundamental 1064 nm, four Stokes waves at 1091, 1120, 1146, 1178 nm, and the second harmonic generation (SHG) of 1146 nm, are tens to hundreds of millwatts for each at 10 kHz, corresponding to a total conversion efficiency of 8.72%.     

Visible supercontinuum generation controlled by intermodal four-wave mixing in microstructured fiber

We present an experimental and numerical study of supercontinuum generation extended in the visible part of the spectrum by using a selective optical coupling of the pump wave in the largely anomalous dispersion regime. The broadband frequency generation is induced by an initial four-wave mixing process that converts the pump wave at 1064 nm into 831 nm anti-Stokes and 1478 nm Stokes wavelengths. Phase matching is ensured on such a large frequency shift thanks to a microstructured multimodal fiber with a specific design. Continuum generation is therefore enhanced around the two generated sidebands.     

高功率,红光至中红外可调谐腔内和频光学参量振荡器

本文利用高重复频率,高平均功率大模场面积飞秒光纤激光器作为同步抽运源,抽运以多周期极化掺氧化镁铌酸锂为非线性晶体的单共振光学参量振荡器,获得了高功率可调谐红光至中红外光,信号光调谐范围为1450—2200 nm,闲频光调谐范围为2250—4000 nm,在2 W的抽运功率下,信号光输出波长为1502 nm时获得最大输出功率374 mW,转换效率为18.7%,脉冲宽度为144 fs,此时中红外输出中心波长为3.4μm,平均功率为166 mW.再利用BBO晶体对信号光进行腔内和频,获得和频光输出波长调谐范围为610—668 nm,在4.1 W抽运的情况下,最高平均功率为615 nm处的694 mW,转换效率达16.9%.     

All-solid-state low noise Yb:YAG/LBO green laser at 515 nm

We report the efficient compact green laser at 515 nm generation by intracavity frequency doubling of a continuous wave (CW) laser operation of a diode-pumped Yb:YAG laser on the transition at 1030 nm. An LBO crystal, cut for critical type I phase matching at room temperature is used for second harmonic generation (SHG) of the laser. With the incident pump power of 10 W, 270 mW of CW output power at 515 nm is achieved with 15-mm-long LBO. The optical-to-optical conversion efficiency is 2.7%, and the power stability in 8 h is better than 2.36% with low noise.     

Compact 498-nm light source based on intracavity sum-frequency Nd:GGG laser

We report a coherent cyan radiation at 498 nm by intracavity sum-frequency generation of the 937 and 1062 nm laser-lines of the Nd:GGG crystal. With a diode pump power of 18.2 W, the maximum cyan output power of 186 mW is obtained. The beam quality M² value is 1.22 in the horizontal plane. The output power stability over 30 min is better than 5%. To the best of our knowledge, this is first work on intracavity sum-frequency generation of a diode pumped Nd:GGG laser at 498 nm.     

激光二极管侧面泵浦高功率266 nm紫外激光器

 报道了一种半导体激光列阵侧面泵浦Nd：YAG四倍频266 nm全固态紫外激光器,采用Z型腔结构,Ⅰ类临界相位匹配LBO和BBO晶体分别作为二倍频晶体和四倍频晶体。在调制频率为5 kHz时,最终获得了2.1 W的266 nm紫外激光输出,单脉冲能量420 μJ, 绿光到紫外激光的转换率为13.13%,在相同的泵浦功率下利用V型腔结构仅获得305 mW的266 nm紫外激光输出。     

Influence of the metal electronic properties on the sum-frequency generation spectra of dodecanethiol self-assembled monolayers on Pt (111), Ag (111) and Au (111) single crystals

Infrared-visible sum-frequency generation (SFG) spectroscopy is performed at different visible wavelengths between 450 and 650 nm in order to investigate the interaction between metallic substrates (Pt, Ag and Au) and 1-dodecanethiol self-assembled monolayers. We show that such measurements provide a means to study the electronic properties of metals as well as the interference phenomena between the SFG signals from the adsorbate and the substrate. The common features of the three interfaces are the vibration modes of the terminal methyl groups. However, these resonances appear as peaks for Pt (111) and as dips in the case of Ag (111). Their shape is not modified when the visible wavelength is tuned between 450 and 650 nm. Moreover, the metal sum-frequency generation contribution is slightly modified in that spectral range. For Au (111) samples, the sum-frequency generation spectrum drastically evolves with the visible wavelength: the peak resonant sum-frequency generation signal at 450 nm becomes rather dip-shaped at 650 nm. The non-linear response of gold is also enhanced when the wavelength associated with the sum-frequency process is close to 480 nm. These results are interpreted on the basis of the metal electronic properties that are responsible for the non-resonant contribution to the SFG signal. Received: 15 October 2001 / Revised version: 27 March 2002 / Published online: 6 June 2002     

175 to 210 nm widely tunable deep-ultraviolet light generation based on KBBF crystal

We have developed a widely tunable deep-ultraviolet (DUV) laser in the wavelength range from 175 to 210 nm by the fourth harmonic generation of Ti:Sapphire laser. The fourth harmonic generation is performed by direct second-harmonic generation (SHG) of a frequency doubled Ti:Sapphire laser with KBBF crystal. The highest output power is 2.23 mW at 193 nm, and the power of the DUV laser is more than 1 mW from 182 nm to 210 nm. To our knowledge, it is the first demonstration of milliwatt-level widely tunable DUV all-solid-state laser below 200 nm by direct SHG technique.     

基于单块周期极化铌酸锂晶体级联三倍频的440 nm蓝光固体激光器

阐述了一种基于单块周期极化铌酸锂晶体级联三倍频实现440 nm蓝光输出的实验方案。根据周期极化铌酸锂晶体的Sellmeier方程以及倍频与和频的相位匹配条件,在一块周期极化铌酸锂晶体上设计了两段不同的极化周期,使其在同一工作温度下能分别实现倍频与和频,在先后经过倍频与和频后,实现级联三倍频输出。实验采用Nd: YAG产生的1319 nm光作为基频光,重频400 Hz,脉宽110 ns,横向和纵向光束质量因子分别为1.81和2.65。耦合进周期极化铌酸锂晶体后,出射光中检测到660 nm的红光和440 nm的蓝光。通过调整工作温度和入射基频光功率,得到2.4 mW的最大蓝光输出,此时工作温度55.5 ℃,基频光功率530 mW。实验结果验证了单块晶体实现级联三倍频440 nm蓝光输出的可行性。     

Continuous wave Nd:YAG-BiBO blue laser under direct 869 nm pumping

We report a blue laser at 473 nm generation by intracavity frequency doubling of a continuous wave (CW) laser operation of a 946 nm Nd:YAG laser under in-band diode pumping at 869 nm. An BiBO crystal, cut for critical type I phase matching at room temperature is used for second harmonic generation of the laser. At an incident pump power of 8.6 W, as high as 721 mW of CW output power at 473 nm is achieved. The optical-to-optical conversion efficiency is up to 8.4%, and the fluctuation of the blue output power was better than 3.5% in the given 30 min.     

色散平坦渐减光纤中超连续谱的产生

对双正交偏振光脉冲在色散平坦渐减光纤中传输时超连续谱的产生进行了计算和分析。结果表明，由于交叉相位调制效应的作用，双光脉冲可以产生比单光脉冲明显展宽且更为平坦的超连续谱。对于双基孤子脉冲，可以得到-20dB谱宽达388nm的平坦宽带超连续谱，比单基孤子脉冲产生的超连续谱谱宽增加72nm，交叉相位调制效应对超连续谱的产生起到增强的效果。当输入脉冲的抽运功率较低时，交叉相位调制效应对超连续谱的产生的增强效果更为显著，它极大地提高了超连续谱的产生的效率。数值计算的结果还表明，与其他高阶非线性效应相比，拉曼自频率移效应对超连续谱产生的影响更为明显。     

Synthesis of periodic femtosecond pulse trains in the ultraviolet by phase-locked Raman sideband generation

We demonstrate a new technique for femtosecond-pulse generation that employs ultrafast modulation of a laser field phase by impulsively excited molecular rotational or vibrational motion with subsequent temporal compression. An ultrashort pump pulse at 800 nm performs impulsive excitation of a molecular gas in a hollow waveguide, and a weak delayed probe pulse at 400 nm is scattered on the temporal oscillations of its dielectric index. The resultant sinusoidal phase modulation of the probe pulse permits probe pulse temporal compression by use of both positively and negatively dispersive elements. The potential of this new method is demonstrated by the generation of a periodic train of 5.8-fs pulses at 400 nm with positive group-delay dispersion compensation.     

High-energy Q-switched fiber laser based on the side-pumped active fiber

A relatively simple fiber-laser system that is based on a dual fiber, is pumped by a single CW source with an output power of 12 W (976 nm), and provides an output pulse energy of up to 110 μJ at a wavelength of 1080 nm is demonstrated for the first time. The output-pulse repetition rate and duration can be varied in the ranges 45–140 kHz and 0.28–1.80 μs, respectively, with a variation in the pumping power. The maximum output power is 5 W. It is demonstrated that the generation instability observed at an output power of greater than 5 W gives rise to giant pulses that can induce the supercontinuum generation in the range 530–1750 nm in a relatively short microstructured fiber.     

Generation of UV radiation at 335.5 nm based on frequency-quadrupling of a diode-pumped Nd:YVO4 laser

The generation of ultraviolet （UV） light at 335.5 nm based on frequency quadrupling of a diode-end- pumped Q-switched Nd：YVO4 laser at 1342 nm was demonstrated. KTP crystal was used for generation of wavelength of 671 nm by intracavity doubling and LBO （BBO） crystal was exploited for the subsequent external fourth harmonic generation （FHG）. With 6.3-W absorbed pump power and 10-kHz frequency repetition rate, the UV output power of 35 and 63 mW were obtained by using LBO and BBO as frequency quadrupling nonlinear crystals, respectively. The experimental results show that the conversion efficiency （red-UV） of 6.4% for BBO crystal is higher than that of 3.5% for LBO crystal, but the UV beam quality obtained by LBO crystal is better than by BBO crystal.     

All solid-state CW Nd:LuVO<Subscript>4</Subscript>-LBO yellow-green laser under direct 888 nm pumping

We report a yellow-green laser at 544.5 nm generation by intracavity frequency doubling of a continuous wave (CW) laser operation of a 1089 nm Nd:LuVO₄ laser under in-band diode pumping at 888 nm. An LBO crystal, cut for critical type I phase matching is used for second harmonic generation of the laser. At an incident pump power of 17.9 W, as high as 3.81 W of CW output power at 544.5 nm is achieved. The optical-to-optical conversion efficiency is up to 21.3%, and the fluctuation of the yellow-green output power was better than 3.7% in the given 4 h.     

Dispersion flattened photonic crystal fiber with high nonlinearity for supercontinuum generation at 1.55 μm

A robust design for a photonic crystal fiber (PCF) based on pure silica with small normal dispersion and high nonlinear coefficient for its dual concentric core structure is presented.This design is suitable for flat broadband supercontinuum (SC) generation in the 1.55-μm region.The numerical results show that the nonlinear coefficient of the proposed eight-ring PCF is 33.8 W -1 ·km -1 at 1550 nm.Ultraflat dispersion with a value between -1.65 and -0.335 ps/(nm·km) is obtained ranging from 1375 to 1625 nm.The 3-dB bandwidth of the SC is 125 nm (1496–1621 nm),with a fiber length of 80 m and a corresponding input peak power of 43.8 W.The amplitude noise is considered to be related to SC generation.For practical fabrication,the influence of the random imperfections of airhole diameters on dispersion and nonlinearity is discussed to verify the robustness of our design.     

555 nm laser sources based on intracavity frequency doubling of Nd:YGG laser

We report for the first time a yellow-green laser at 555 nm generation by intracavity frequency doubling of a continuous wave (CW) laser operation of a 1110 nm Nd-doped yttrium gallium garnet (Nd:YGG) laser under in-band diode pumping at 808 nm. An LBO crystal, cut for critical type I phase matching is used for second harmonic generation of the laser. At an incident pump power of 18.5 W, as high as 2.31 W of CW output power at 555 nm is achieved. The optical-to-optical conversion efficiency is up to 12.4%, and the fluctuation of the yellow-green output power was better than 2.8% in the given 4 h.     

Tunable microwave signal generation based on an Opto-DMD processor and a photonic crystal fiber

Frequency-tunable microwave signal generation is proposed and experimentally demonstrated with a dual-wavelength single-longitudinal-mode （SLM） erbium-doped fiber ring laser based on a digital Opto-DMD processor and four-wave mixing （FWM） in a high-nonlinear photonic crystal fiber （PCF）. The high-nonlinear PCF is employed for the generation of the FWM to obtain stable and uniform dual-wavelength oscillation. Two different short passive sub-ring cavities in the main ring cavity serve as mode filters to make SLM lasing. The two lasing wavelengths are electronically selected by loading different gratings on the Opto-DMD processor controlled with a computer. The wavelength spacing can be smartly adjusted from 0.165 nm to 1.08 nm within a tuning accuracy of 0.055 nm. Two microwave signals at 17.23 GHz and 27.47 GHz are achieved. The stability of the microwave signal is discussed. The system has the ability to generate a 137.36-GHz photonic millimeter signal at room temperature.     

Second-harmonic generation of light at 544 and 272 nm from an ytterbium-doped distributed-feedback fiber laser

We report external cavity second-harmonic generation of light at 544 and 272 nm based on an ytterbium-doped distributed-feedback fiber laser. The nonlinear crystal used to generate light at 544 nm is LiNbO3, and the maximum output of the cavity is 845 mW, corresponding to a conversion efficiency of 55%. In a second frequency-doubling step, using a beta-BaBa2O4 crystal, we generate up to 115 mW of light at 272 nm with a conversion efficiency of 14%.     

101 W of average green beam from diode-side-pumped Nd:YAG/LBO-based system in a relay imaged cavity

A 52-W green laser at 532 nm by extra-cavity second-harmonic generation in a coupled-cavity configuration is demonstrated. The fundamental laser is a diode-side-pumped acousto-optic (AO) Q-switched Nd:YAG rod laser producing 84 W of average power at 1064 nm at 8 kHz repetition rate. Type-II phase-matched polished KTP crystal is used as the nonlinear crystal for second-harmonic generation. The individual green pulse width is 50 ns and the fundamental to second harmonic conversion efficiency is 61.8%.