High efficiency long pulse FIR Raman conversion in ammonia

Generally the quantum efficiency of FIR Raman generation in molecular gases is below the theoretical value. This disagreement is particularly evident in Raman scattering from pulsed sources with short pulse length, when the vibrational saturation limits the power conversion. Other nonlinear processes can overcome this saturation, but they require a very intense pump power for too short a time to use the FIR radiation in high sensitive experiments with heterodyne detection. This is the case, for instance, of RFWM. In this work we describe the experimental conditions to achieve a high efficiency 90 micron Raman conversion in ammonia, with both short and long pulses.     

New CH2F2 FIR laser lines pumped by a tunable WG CO2 laser

8 new large offset FIR laser lines of CH₂F₂ have been discovered by pumping with a high tunability waveguide CW CO₂ laser. Optoacoustic measurements of CH₂F₂ have also been performed and the pump offsets of the new and of previously known lines have been measured and checked. Some assignments are proposed and a few assignments found in literature are checked     

Optically pumped NH3 laser using a continuously tunable CO2 laser

The use of a continuously tunable CO₂ laser to optically pump the NH₃ laser via previously inaccessible absorption lines is described. Efficient laser action has thus been achieved in the 11–13 μm region on transitions formerly only obtained in buffered mixtures.     

Tuning characteristics of a high pressure CO2 laser pumped CH3F Raman laser

Conclusion We described a CH₃F Raman laser pumped by a two stage 20 atmospheres CO₂ laser. The emission spectrum of the CH₃F laser at 11 Torr extends from 23 cm^–1 to 45 cm^–1 when the CO₂ laser is scanned over the 9R emission branch at a fixed pump power of 180 mJ. The emission spectrum shows a strong structure with large parts where the FIR energy decreases to zero. This fact makes the use of such a laser for spectroscopic scanning experiments in the FIR difficult. The laser is, however, very suited for working at fixed but adjustable FIR frequencies. The pulse energy in the maxima of the emission characteristics at a pump energy of 180 mJ exceeds 300 J, which corresponds a photon conversion coefficient of more than 6%.     

Compact, high power FIR NH3 laser pumped in a three mirror CO2 laser cavity

A compact CO₂–NH₃ FIR laser system where an NH₃ laser cavity was inserted in pump, three mirror CO₂ laser cavity was designed. The total length of this system was about 1.8 m. Output energy of about 1 mJ (10 KW pea power) was obtained at the 152 m and 90 m lines in NH₃. Power conversion efficiency of 1.7 percent was obtained at the 90 m line.     

Interaction of multi-raman-processes in miniature optically pumped NH3 fir laser

The principle of Raman gain superposition was introduced to the theory of multi-Raman- processes interaction. Spectral characteristics of Raman lines from miniature NH₃-optically pumped FiR lasers were studied and measured.supported by the National Nature Science Foundation of P.R.C. and the Special Research Foundation of Doctorate Stations of P.R.C.     

New cascade laser transitions in CH2F2 pumped with the 9R32 line of a cw CO2 laser

New cascade laser transitions of¹²CH₂F₂ at 172.50m, 208.83m, 220.44m, 223.99m and 250.61m are reported. A waveguide FIR laser was pumped with a quasi cw¹²C¹⁶O₂ laser operating on the 9R32 line. Together with the already known lines at 184.3m, 196.1m and 235.9m, the laser lines can be assigned to rotational transitions in the ₉ vibrational band of¹²CH₂F₂ and to refill transitions of the vibrational ground state ₀.     

Thermal dissipation effects of the entangled photon generated by four-wave mixing process in a nonlinear ring resonator

We firstly analyze the thermal dissipation effects of the entangled photons generated by a nonlinear optical ring resonator. To obtain the corresponding equation of motion of the entangled photons generated by a four-wave mixing process within the system, we propose the Markov approximation to repel the reservoir operators. The system master equation in the interaction picture for both degenerate and non-degenerate cases is analyzed and obtained. The established system can be used to characterize the optimum entangled photons in some cases where the thermal dissipation effects may be introduced noise into the system. In this work, the entangled photons can be generated into two forms, firstly, the two entangled photon states is generated, the other, the four entangled photon states can be easily obtained. Results obtained have shown that the optimum entangled photon in term of entangled photon visibility can be compensated (i.e. unchanged) under thermal dissipation effects.     

Spikes in raman spectrum of miniature optically pumped NH3 fir laser

In this paper, the semiclassical density matrix equation was solved to calculate the spectral characteristics of V₂:a--sR(0,0) transition in a miniature optically pumped NH₃ far infrared laser (mini-NH₃-OPFIRL), which was pumped by CO₂-10R(6) line. The results of theoretical calculation showed that the spikes in Raman spectrum of V₂:a--sR(0,0) would appear when the operating NH₃ gas pressure was higher than a certain critical value or pumping power density was lower than a certain critical value, which was caused by Raman processes interaction of AC-Stark splitting. In our experiment, 298 µm FIR spetral line of a--sR(0,0) pumped by a TEA-CO₂ laser with 10R(6) line was observed but the spikes could not be observed owing to the limitation of the resolution of the F-P interferometer.Supported by the National Natural Sciences Foundation of P.R.China.     

Assignments of fir laser emissions from CH3OH optically pumped by an intra-cavity etalon tuned TEA-CO2 laser

The author reports that TEA-CO₂ with an intra-cavity etalon is a useful pumping source which can deliver widely tunable beam (tunable range 1 GHz) with accurate oscillation frequencies and with high power compared to a tunable wave guide laser.The source is applied to the excitations of CH₃OH and the FIR emissions from it are well assigned for there absorption transitions and FIR emissions. This proves that the source display not only usefulness for development of new FIR emissions but also for molecular spectroscopy.     

Mixing effect in the NH3 absorption and MIR emission spectra pumped by a continuously tunable CO2 laser

By tuning a high pressure CO2 laser (HPL) around strong ammonia lines nearly coincident with CO2 lines an of-fresonant absorption is observed which can be confirmed by the superfluorescent MIR emission. This effect is related to a two frequency v₁, v₃ HPL emission in the regime of moderate pulling. Around a strong absorption line a mixed v₄=2v₁–v₃ frequency is produced that is strongly absorbed     

First-order layout of a two-lens varifocal objective focusing a CO2 laser beam in a post-objective three-axis scanner

In this paper we describe a procedure to work out the first-order layout of a two-lens varifocal objective for a post-objective three-axis scanner. In particular, the two lenses are considered thin, the laser beam is propagated paraxially (ABCD law) and the focal lengths of the two lenses and the maximum value of the distance between them are worked out in accordance with the specifications of the objective. Finally, the plots of the dimension and the position of the focused light spot versus the distance between the two lenses are evaluated.     

Processing of concretes with a high power CO2 laser

Laser material processing, being a non-contact process, minimizes many of the complexities involved in the decontamination and decommissioning of nuclear facilities. A high power laser beam incident on a concrete surface can produce spalling, glazing or vaporization, depending upon the laser power density and scan speed. This paper presents effect of various laser processing parameters on the efficiency of material removal by surface spalling and glazing. The size of laser beam at constant fluence or energy density had significantly different effect on the spalling process. In thick concrete block cutting the flow or removal of molten material limits the cutting depth. By employing repeated laser glazing followed by mechanical scrubbing process cutting of 150 mm thick concrete block was carried out. Gravitation force was utilized for molten materials to flow out while drilling holes on vertical concrete walls. The dependence of the incident laser beam angle on drilling time was experimentally studied.     

Optoacoustic Laser Stark spectroscopy and FIR laser action on CH3Br using a waveguide CO2 laser

The optoacoustic spectrum of CH₃Br around 10 m band lines of a tunable cw waveguide CO₂ laser is investigated. Several new infrared absorptions are observed and most of the correspond ing molecular transitions are assigned. Far infra red laser action is reported by pumping with the same CO₂ laser: pump offsets are given using the Transferred Lambs dip (TLD) technique. A new FIR laser emission is obtained and assigned. An optoacoustic Laser Stark spectroscopy technique is used to investigate off resonance infrared tran sitions.     

在固体透明材料中利用级联四波混频方法获得宽带多色飞秒激光脉冲的研究

飞秒激光光谱学实验研究的深入与拓展对飞秒激光脉冲的要求也越来越高.比如多色抽运探测实验需要同时用到多个不同频率的超短飞秒激光脉冲.本文设计了一个更加简单紧凑的实验装置,对两束不同中心频率的入射光引入相反啁啾,在厚度为0.5 mm的CaF2晶体中利用级联四波混频获得了光谱半高全宽近100nm,支持傅里叶转换极限脉宽小于10 fs的多色飞秒激光脉冲.这一结果将为拓展飞秒激光光谱学研究和应用发挥重要作用.     

Multiple four-wave mixing in optical fibers: 1.5-3.4-THz femtosecond pulse sources and real-time monitoring of a 20-GHz picosecond source

In this work, we report recent progress on the design of all-fibered ultra-high repetition-rate pulse sources for telecommunication applications around 1550 nm. The sources are based on the non-linear compression of an initial beat-signal through a multiple four-wave mixing process taking place into an optical fiber. We experimentally demonstrate real-time monitoring of a 20 GHz pulse source having an integrated phase noise 0.01 radian by phase locking the initial beat note against a reference RF oscillator. Based on this technique, we also experimentally demonstrate a well-separated high-quality 110 fs pulse source having a repetition rate of 2 THz. Finally, we show that with only 1.4 m of standard single mode fiber, we can achieve a twofold increase of the repetition rate, up to 3.4 THz, through the self-imaging Talbot effect. Experimental results are supported by numerical simulations based on the generalized non-linear Schrödinger equation.     

Measurement of the argon-gas-induced broadening and line shifting of the barium Rydberg level 6s24d 1D2 by two-photon resonant nondegenerate four-wave mixing

We apply two-photon resonant nondegenerate four-wave mixing with a resonant intermediate state to the obser-vation of the broadening and shifting of the barium Rydberg level 6s24d 1^D2 by collision with argon. The collision broadening and shifting cross sections are measured. This technique is purely optical, and can investigate the pressure dependence of the transverse relaxation rate-P21 between the Rydberg state and an intermediate state, as well as the transverse relaxation rate F20 between the Rydberg state and the ground state.     

Assignment of laser lines in an optically pumped submillimeter and near millimeter laser: (H2CO)3

A large number of emissions is obtained in the submillimeter and near millimeter range with the (H₂CO)₃ laser optically pumped by a CO₂ laser. A study of the microwave absorption spectrum of the molecule carried out simultaneously with the submm analysis allows us to assign six of the laser lines in thev ₅ excited state of the molecule and to determine the rotational constants and vibrational energy ofv ₅.     

A high-power far-infrared NH3 laser pumped in a three-mirror CO2 laser cavity with optically-switched cavity-dumping

Results are reported of cavity-dumping a submillimeter radiation high-Q, zig-zag optically-pumped resonator which utilizes a silicon optical switch photo-excited by a NdYAG laser. Peak powers at 152 m approaching 10 kW in temporally smooth pulses of 5 ns (FWHM) duration have been obtained at a pulse repetition rate of 12 Hz. The far-infrared laser radiation, as measured with a scanning metal-mesh Fabry-Perot interferometer and averaged over many pulses, is, upon deconvolution of the 125 MHz instrumental linewidth, found to oscillate in a predominantly single longitudinal mode of width 250 MHz. Theoretical investigations of the transient far-infrared reflectivity of the silicon optical switch predict a rise in the Brewster-angle reflectivity from 0% to nearly 80% in 1 ns, when activated by a Q-switched, frequency-doubled NdYAG laser providing an incident energy density of 50 mJ/cm² in a pulsewidth of 10 ns.